Plasmon–emitter interactions at the nanoscale

Gonçalves, P. A.  D.; Christensen, Thomas; Rivera, Nicholas; Jauho, Antti-Pekka; Mortensen, N. Asger; Soljačić, Marin

doi:10.1038/s41467-019-13820-z

Title: Plasmon–emitter interactions at the nanoscale

Journal Article · 16 January 2020 · Nature Communications

DOI: https://doi.org/10.1038/s41467-019-13820-z · OSTI ID:1624230

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Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States). Dept. of Physics, Massachusetts Institute of Technology; Technical University of Denmark, Lyngby (Denmark). Dept. of Photonics Engineering; Technical University of Denmark, Lyngby (Denmark). Center for Nanostructured Graphene; University of Southern Denmark, Odense M (Denmark). Center for Nano Optics; DOE/OSTI
Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States). Dept. of Physics, Massachusetts Institute of Technology
Technical University of Denmark, Lyngby (Denmark). Center for Nanostructured Graphene; Technical University of Denmark, Lyngby (Denmark). Dept. of Physics
Technical University of Denmark, Lyngby (Denmark). Center for Nanostructured Graphene; University of Southern Denmark, Odense M (Denmark). Center for Nano Optics; University of Southern Denmark, Odense M (Denmark). Danish Institute for Advanced Study

Plasmon–emitter interactions are of central importance in modern nanoplasmonics and are generally maximal at short emitter–surface separations. However, when the separation falls below 10–20 nm, the classical theory deteriorates progressively due to its neglect of quantum effects such as nonlocality, electronic spill-out, and Landau damping. Here we show how this neglect can be remedied in a unified theoretical treatment of mesoscopic electrodynamics incorporating Feibelman d-parameters. Our approach incorporates nonclassical resonance shifts and surface-enabled Landau damping—a nonlocal damping effect—which have a dramatic impact on the amplitude and spectral distribution of plasmon–emitter interactions. We consider a broad array of plasmon–emitter interactions ranging from dipolar and multipolar spontaneous emission enhancement, to plasmon-assisted energy transfer and enhancement of two-photon transitions. The formalism gives a complete account of both plasmons and plasmon–emitter interactions at the nanoscale, constituting a simple yet rigorous platform to include nonclassical effects in plasmon-enabled nanophotonic phenomena.

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Research Organization:: Krell Institute, Ames, IA (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: FG02-97ER25308

OSTI ID:: 1624230

Journal Information:: Nature Communications, Journal Name: Nature Communications Journal Issue: 1 Vol. 11; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Strong light-matter coupling in quantum chemistry and quantum photonics Flick, Johannes; Rivera, Nicholas; Narang, Prineha Nanophotonics, Vol. 7, Issue 9 https://doi.org/10.1515/nanoph-2018-0067	journal	September 2018
Research data supporting “Single-molecule optomechanics in "picocavities"” Benz, Felix; Schmidt, Mikolaj K.; Dreismann, Alexander Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.1675	dataset	January 2016
Single-molecule optomechanics in "picocavities" Benz, Felix; Schmidt, Mk; Dreismann, Alexander Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.6641	text	January 2016
Macroscopic quantum electrodynamics - Concepts and applications Scheel, Stefan; Buhmann, Stefan Acta Physica Slovaca. Reviews and Tutorials, Vol. 58, Issue 5 https://doi.org/10.2478/v10155-010-0092-x	journal	October 2008
On the use of Purcell factors for plasmon antennas Koenderink, A. F. arXiv https://doi.org/10.48550/arxiv.1007.1074	text	January 2010
Spontaneous emission from large quantum dots in nanostructures: exciton-photon interaction beyond the dipole approximation Stobbe, Søren; Kristensen, Philip T.; Mortensen, Jakob E. arXiv https://doi.org/10.48550/arxiv.1112.1835	text	January 2011
Nanophotonic control of the Forster resonance energy transfer efficiency Blum, Christian; Zijlstra, Niels; Lagendijk, Ad arXiv https://doi.org/10.48550/arxiv.1207.2272	text	January 2012
Ab-initio nanoplasmonics: The impact of atomic structure Zhang, Pu; Feist, Johannes; Rubio, Angel arXiv https://doi.org/10.48550/arxiv.1403.8016	text	January 2014
Multipole plasmons and their disappearance in few-nanometer silver nanoparticles Raza, Søren; Kadkhodazadeh, Shima; Christensen, Thomas arXiv https://doi.org/10.48550/arxiv.1505.00594	text	January 2015
Quantum corrections in nanoplasmonics: shape, scale, and material Christensen, Thomas; Yan, Wei; Jauho, Antti-Pekka arXiv https://doi.org/10.48550/arxiv.1608.05421	text	January 2016
Simultaneously giant enhancement of Forster resonance energy transfer rate and efficiency based on plasmonic excitations Ren, Jun; Wu, Tong; Yang, Bing arXiv https://doi.org/10.48550/arxiv.1712.09573	text	January 2017
Coherent and Collective Quantum Optical Effects in Mesoscopic Systems Brandes, Tobias arXiv https://doi.org/10.48550/arxiv.cond-mat/0409771	text	January 2004

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