Aggregation and morphology control enables multiple cases of high-efficiency polymer solar cells
Abstract
Although the field of polymer solar cell has seen much progress in device performance in the past few years, several limitations are holding back its further development. For instance, current high-efficiency (>9.0%) cells are restricted to material combinations that are based on limited donor polymers and only one specific fullerene acceptor. Here we report the achievement of high-performance (efficiencies up to 10.8%, fill factors up to 77%) thick-film polymer solar cells for multiple polymer:fullerene combinations via the formation of a near-ideal polymer:fullerene morphology that contains highly crystalline yet reasonably small polymer domains. This morphology is controlled by the temperature-dependent aggregation behaviour of the donor polymers and is insensitive to the choice of fullerenes. The uncovered aggregation and design rules yield three high-efficiency (>10%) donor polymers and will allow further synthetic advances and matching of both the polymer and fullerene materials, potentially leading to significantly improved performance and increased design flexibility.
- Authors:
-
- Hong Kong Univ.Science and Technology, Clear Water Bay (Hong Kong). Dept.of Chemistry
- North Carolina State Univ., Raleigh, NC (United States). Dept. of Physics and ORaCEL
- North Carolina State Univ., Raleigh, NC (United States). Dept. of Physics and ORaCEL
- Hong Kong Univ.Science and Technology, Clear Water Bay (Hong Kong). Dept.of Chemistry; HKUST-Shenzhen Research Institute, Shenzhen (China)
- Publication Date:
- Research Org.:
- North Carolina State University, Raleigh, NC (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1623961
- Grant/Contract Number:
- FG02-98ER45737
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 5; Journal Issue: 1; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- Science & Technology - Other Topics
Citation Formats
Liu, Yuhang, Zhao, Jingbo, Li, Zhengke, Mu, Cheng, Ma, Wei, Hu, Huawei, Jiang, Kui, Lin, Haoran, Ade, Harald, and Yan, He. Aggregation and morphology control enables multiple cases of high-efficiency polymer solar cells. United States: N. p., 2014.
Web. doi:10.1038/ncomms6293.
Liu, Yuhang, Zhao, Jingbo, Li, Zhengke, Mu, Cheng, Ma, Wei, Hu, Huawei, Jiang, Kui, Lin, Haoran, Ade, Harald, & Yan, He. Aggregation and morphology control enables multiple cases of high-efficiency polymer solar cells. United States. https://doi.org/10.1038/ncomms6293
Liu, Yuhang, Zhao, Jingbo, Li, Zhengke, Mu, Cheng, Ma, Wei, Hu, Huawei, Jiang, Kui, Lin, Haoran, Ade, Harald, and Yan, He. Mon .
"Aggregation and morphology control enables multiple cases of high-efficiency polymer solar cells". United States. https://doi.org/10.1038/ncomms6293. https://www.osti.gov/servlets/purl/1623961.
@article{osti_1623961,
title = {Aggregation and morphology control enables multiple cases of high-efficiency polymer solar cells},
author = {Liu, Yuhang and Zhao, Jingbo and Li, Zhengke and Mu, Cheng and Ma, Wei and Hu, Huawei and Jiang, Kui and Lin, Haoran and Ade, Harald and Yan, He},
abstractNote = {Although the field of polymer solar cell has seen much progress in device performance in the past few years, several limitations are holding back its further development. For instance, current high-efficiency (>9.0%) cells are restricted to material combinations that are based on limited donor polymers and only one specific fullerene acceptor. Here we report the achievement of high-performance (efficiencies up to 10.8%, fill factors up to 77%) thick-film polymer solar cells for multiple polymer:fullerene combinations via the formation of a near-ideal polymer:fullerene morphology that contains highly crystalline yet reasonably small polymer domains. This morphology is controlled by the temperature-dependent aggregation behaviour of the donor polymers and is insensitive to the choice of fullerenes. The uncovered aggregation and design rules yield three high-efficiency (>10%) donor polymers and will allow further synthetic advances and matching of both the polymer and fullerene materials, potentially leading to significantly improved performance and increased design flexibility.},
doi = {10.1038/ncomms6293},
journal = {Nature Communications},
number = 1,
volume = 5,
place = {United States},
year = {Mon Nov 10 00:00:00 EST 2014},
month = {Mon Nov 10 00:00:00 EST 2014}
}
Web of Science
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Binary Solvent Additives Treatment Boosts the Efficiency of PTB7:PCBM Polymer Solar Cells to Over 9.5%
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Introduction of Fluorine Into spiro[fluorene‐9,9′‐xanthene]‐Based Hole Transport Material to Obtain Sensitive‐Dopant‐Free, High Efficient and Stable Perovskite Solar Cells
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High‐Efficiency Polymer Solar Cells Over 13.9% With a High V OC Beyond 1.0 V by Synergistic Effect of Fluorine and Sulfur
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Core–shell super-structures via smart deposition of naphthothiadiazole and benzodithiophene-possessing polymer backbones onto carbon nanotubes and photovoltaic applications thereof
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Facile synthesis of naphthalene diimide (NDI) derivatives: aggregation-induced emission, photophysical and transport properties
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Enhanced open-circuit voltage in methoxyl substituted benzodithiophene-based polymer solar cells
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Towards a bright future: polymer solar cells with power conversion efficiencies over 10%
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New 2D-Conjugated Polymer for Non-Halogenated and Halogenated Solvents Processed Organic Solar Cells
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Competition between recombination and extraction of free charges determines the fill factor of organic solar cells
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Efficient inverted polymer solar cells employing favourable molecular orientation
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Thienyl-BOPHY dyes as promising templates for bulk heterojunction solar cells
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Optimization of charge carrier transport balance for performance improvement of PDPP3T-based polymer solar cells prepared using a hot solution
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Rational selection of solvents and fine tuning of morphologies toward highly efficient polymer solar cells fabricated using green solvents
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Beyond PCBM: methoxylated 1,4-bisbenzyl[60]fullerene adducts for efficient organic solar cells
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Linear-scaling density functional simulations of the effect of crystallographic structure on the electronic and optical properties of fullerene solvates
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Synthesis of benzothiadiazole-based molecules via direct arylation: an eco-friendly way of obtaining small semi-conducting organic molecules
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9-Fluorenone and 9,10-anthraquinone potential fused aromatic building blocks to synthesize electron acceptors for organic solar cells
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Colorful semitransparent polymer solar cells employing a bottom periodic one-dimensional photonic crystal and a top conductive PEDOT:PSS layer
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Novel wide band gap copolymers featuring excellent comprehensive performance towards the practical application for organic solar cells
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Design, synthesis, and structural characterization of the first dithienocyclopentacarbazole-based n-type organic semiconductor and its application in non-fullerene polymer solar cells
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Alkylthienyl substituted asymmetric 2D BDT and DTBT-based polymer solar cells with a power conversion efficiency of 9.2%
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Textile-based washable polymer solar cells for optoelectronic modules: toward self-powered smart clothing
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Systematically investigating the influence of inserting alkylthiophene spacers on the aggregation, photo-stability and optoelectronic properties of copolymers from dithieno[2,3- d :2′,3′- d ′]benzo[1,2- b :4,5- b ′]dithiophene and benzothiadiazole derivatives
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Non-halogenated diphenyl-chalcogenide solvent processing additives for high-performance polymer bulk-heterojunction solar cells
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Polymer semiconductors incorporating head-to-head linked 4-alkoxy-5-(3-alkylthiophen-2-yl)thiazole
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Recent advances in electron acceptors with ladder-type backbone for organic solar cells
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Semi-transparent low-donor content organic solar cells employing cyclopentadithiophene-based conjugated molecules
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High face-on ratio isoindigo copolymers with extended nano-fibrillar networks in fullerene-based thick (>300 nm) photovoltaics achieving a high efficiency of 10.7%
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Simultaneous improvement of three parameters using a binary processing solvent system approach in as-cast non-fullerene solar cells
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A perylene diimide electron acceptor with a triphenylamine core: promoting photovoltaic performance via hot spin-coating
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Simulation of time-resolved x-ray absorption spectroscopy of ultrafast dynamics in particle-hole-excited 4‐(2-thienyl)-2,1,3-benzothiadiazole
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An Analytical Solution to Lumped Parameter Equivalent Circuit Model of Organic Solar Cells
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A Terminally Tetrafluorinated Nonfullerene Acceptor for Well‐Performing Alloy Ternary Solar Cells
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A Difluorobenzoxadiazole Building Block for Efficient Polymer Solar Cells
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Reduced Intramolecular Twisting Improves the Performance of 3D Molecular Acceptors in Non-Fullerene Organic Solar Cells
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Highly Efficient Fullerene-Free Polymer Solar Cells Fabricated with Polythiophene Derivative
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Alkyl Side-Chain Engineering in Wide-Bandgap Copolymers Leading to Power Conversion Efficiencies over 10%
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Artificial Muscles: Mechanisms, Applications, and Challenges
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An Unfused-Core-Based Nonfullerene Acceptor Enables High-Efficiency Organic Solar Cells with Excellent Morphological Stability at High Temperatures
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High-Performance Organic Bulk-Heterojunction Solar Cells Based on Multiple-Donor or Multiple-Acceptor Components
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Stirring Up Acceptor Phase and Controlling Morphology via Choosing Appropriate Rigid Aryl Rings as Lever Arms in Symmetry-Breaking Benzodithiophene for High-Performance Fullerene and Fullerene-Free Polymer Solar Cells
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Highly Efficient Nonfullerene Polymer Solar Cells Enabled by a Copper(I) Coordination Strategy Employing a 1,3,4-Oxadiazole-Containing Wide-Bandgap Copolymer Donor
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Over 14% Efficiency in Polymer Solar Cells Enabled by a Chlorinated Polymer Donor
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Interfacial Materials for Organic Solar Cells: Recent Advances and Perspectives
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Real-Time Photoluminescence Studies of Structure Evolution in Organic Solar Cells
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Ternary Organic Solar Cells Based on Two Highly Efficient Polymer Donors with Enhanced Power Conversion Efficiency
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Reducing Voltage Losses in Cascade Organic Solar Cells while Maintaining High External Quantum Efficiencies
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Rational Strategy to Stabilize an Unstable High‐Efficiency Binary Nonfullerene Organic Solar Cells with a Third Component
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Quantifying and Understanding Voltage Losses Due to Nonradiative Recombination in Bulk Heterojunction Organic Solar Cells with Low Energetic Offsets
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Sequential Blade‐Coated Acceptor and Donor Enables Simultaneous Enhancement of Efficiency, Stability, and Mechanical Properties for Organic Solar Cells
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Hybrid Silver Mesh Electrode for ITO-Free Flexible Polymer Solar Cells with Good Mechanical Stability
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Efficient Large Area Organic Solar Cells Processed by Blade-Coating With Single-Component Green Solvent
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Photoelectrochemical water splitting in an organic artificial leaf
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Tuning the performance of the non-fullerene organic solar cells by the polarizability
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Systematic investigation of self-organization behavior in supramolecular π-conjugated polymer for multi-color electroluminescence
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Vinylene spacer effects of benzothiadiazole–quarterthiophene based conjugated polymers on transistor mobilities
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Efficient long-range electron transfer processes in polyfluorene–perylene diimide blends
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Highly efficient polymer solar cells with a thienopyrroledione and benzodithiophene containing planar random copolymer
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Synthesis and photophysical properties of water-soluble fluorinated poly(aryleneethynylene)s
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Fluorescent polycatecholamine nanostructures as a versatile probe for multiphase systems
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A new copolymer based on a D–π–A or D–A–π repeat unit for polymer solar cells employing non-halogenated solvents
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Improving the exciton dissociation of polymer/fullerene interfaces with a minimal loading amount of energy cascading molecular dopant
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Push–pull architecture eliminates chain length effects on exciton dissociation
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Polyelectrolyte interlayers with a broad processing window for high efficiency inverted organic solar cells towards mass production
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Design of asymmetric benzodithiophene based wide band-gap conjugated polymers toward efficient polymer solar cells promoted by a low boiling point additive
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Efficient design and structural modifications for tuning the photoelectric properties of small-molecule acceptors in organic solar cells
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Evolution of molecular aggregation in bar-coated non-fullerene organic solar cells
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Efficiency enhancement of organic photovoltaics by introducing high-mobility curved small-molecule semiconductors as additives
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Graphene and Carbon Quantum Dot-Based Materials in Photovoltaic Devices: From Synthesis to Applications
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Polymer Solar Cells Exceeding 10% Efficiency Enabled via a Facile Star-Shaped Molecular Cathode Interlayer with Variable Counterions
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A Vinylene-Bridged Perylenediimide-Based Polymeric Acceptor Enabling Efficient All-Polymer Solar Cells Processed under Ambient Conditions
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Graphene and Carbon Quantum Dot-Based Materials in Photovoltaic Devices: From Synthesis to Applications
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Enhancing Photoluminescence Quenching in Donor–Acceptor PCE11:PPCBMB Films through the Optimization of Film Microstructure
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Improving the Performances of Random Copolymer Based Organic Solar Cells by Adjusting the Film Features of Active Layers Using Mixed Solvents
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Bulk Heterojunction Solar Cells Based on Blends of Conjugated Polymers with II–VI and IV–VI Inorganic Semiconductor Quantum Dots
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- Polymers, Vol. 9, Issue 12
Control of Molecular Ordering, Alignment, and Charge Transport in Solution-Processed Conjugated Polymer Thin Films
journal, June 2017
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Long Lived Photoexcitation Dynamics in π-Conjugated Polymer/PbS Quantum Dot Blended Films for Photovoltaic Application
journal, August 2017
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High-resolution noncontact AFM and Kelvin probe force microscopy investigations of self-assembled photovoltaic donor–acceptor dyads
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Synthesis and characterization of fluorinated azadipyrromethene complexes as acceptors for organic photovoltaics
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