Phase stabilization by electronic entropy in plutonium

Harrison, N.; Betts, J. B.; Wartenbe, M. R.; Balakirev, F. F.; Richmond, S.; Jaime, M.; Tobash, P. H.

doi:10.1038/s41467-019-11166-0

Title: Phase stabilization by electronic entropy in plutonium

Authors:

Harrison, N.; Betts, J. B.; Wartenbe, M. R.;

;

; Jaime, M.; Tobash, P. H.

Publication Date:: 2019-07-18

Sponsoring Org.:: USDOE

OSTI Identifier:: 1619833

Resource Type:: Published Article

Journal Name:: Nature Communications

Additional Journal Information:: Journal Name: Nature Communications Journal Volume: 10 Journal Issue: 1; Journal ID: ISSN 2041-1723

Publisher:: Nature Publishing Group

Country of Publication:: United Kingdom

Language:: English

Citation Formats


                    Harrison, N., Betts, J. B., Wartenbe, M. R., Balakirev, F. F., Richmond, S., Jaime, M., and Tobash, P. H. Phase stabilization by electronic entropy in plutonium.  United Kingdom: N. p., 2019. 
Web.  https://doi.org/10.1038/s41467-019-11166-0.

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                    Harrison, N., Betts, J. B., Wartenbe, M. R., Balakirev, F. F., Richmond, S., Jaime, M., & Tobash, P. H. Phase stabilization by electronic entropy in plutonium.  United Kingdom.  https://doi.org/10.1038/s41467-019-11166-0

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                    Harrison, N., Betts, J. B., Wartenbe, M. R., Balakirev, F. F., Richmond, S., Jaime, M., and Tobash, P. H. Thu .  
"Phase stabilization by electronic entropy in plutonium".  United Kingdom.  https://doi.org/10.1038/s41467-019-11166-0.

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@article{osti_1619833,

  title        = {Phase stabilization by electronic entropy in plutonium},

  author       = {Harrison, N. and Betts, J. B. and Wartenbe, M. R. and Balakirev, F. F. and Richmond, S. and Jaime, M. and Tobash, P. H.},

  abstractNote = {},

  doi          = {10.1038/s41467-019-11166-0},

  journal      = {Nature Communications},

  number       = 1,

  volume       = 10,

  place        = {United Kingdom},

  year         = {2019},

  month        = {7}

}

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Title: Phase stabilization by electronic entropy in plutonium

Citation Formats

Magnetic-field, pressure, and temperature scaling of the first-order valence transition in pure and doped YbInCu 4 journal, July 1997

Equilibrium properties of delta-Pu: LDA+ U calculations (LDAequiv local density approximation) journal, February 2000

Valence fluctuation phenomena journal, January 1981

Electronic and phonon properties of six crystalline phases of Pu metal journal, December 1998

Fiber Bragg Grating Dilatometry in Extreme Magnetic Field and Cryogenic Conditions journal, November 2017

Melting of the light actinides journal, January 2000

Self-interaction-corrected local spin density theory of 5 f electron localization in actinides journal, September 2007

Electronic properties of f -electron metals using the generalized gradient approximation journal, September 1994

Suppression of the γ–α structural phase transition in Ce 0.8 La 0.1 Th 0.1 by large magnetic fields journal, February 2005

First-principles calculations of the electronic structure and spectra of strongly correlated systems: the LDA + U method journal, January 1997

Piezomagnetism and magnetoelastic memory in uranium dioxide journal, July 2017

Volume magnetostriction of intermediate valence systems journal, February 1985

Volume magnetostriction of rare-earth metals with unstable 4f shells journal, January 1986

Multiconfigurational nature of 5f orbitals in uranium and plutonium intermetallics journal, June 2012

Magnetic and magnetoelastic properties of PrNi 5 single crystal journal, February 1988

Dual nature of 5 f electrons: Effect of intra-atomic correlations on hopping anisotropies journal, March 2004

Magnetostriction in metals journal, November 1971

Correlated electrons in δ-plutonium within a dynamical mean-field picture journal, April 2001

Spin-polarized relativistic linear-muffin-tin-orbital method: Volume-dependent electronic structure and magnetic moment of plutonium journal, June 1991

Cancellation of spin and orbital magnetic moments in δ-Pu: Theory journal, October 2007

Density-functional investigation of magnetism in δ -Pu journal, November 2002

A unified and efficient theory for the structural properties of actinides and phases of plutonium journal, September 2018

Phase stability and phase transformations in Pu–Ga alloys journal, January 2004

Gallium stabilization of δ − Pu : Density-functional calculations journal, November 2005

Heat capacity measurements on a thin ribbon sample of Zr0.55Al0.10Ni0.05Cu0.30 glassy alloy and Apiezon N high vacuum grease using a Quantum Design Physical Property Measurement System journal, May 2009

Density-Functional Calculations of α , β , γ , δ , δ ′ , and ϵ Plutonium journal, May 2004

Phonon density of states of α - and δ -plutonium by inelastic x-ray scattering journal, February 2009

Hidden disorder in the α ′ → δ transformation of Pu-1.9 at. % Ga journal, June 2012

Influence of point defects and impurities on the dynamical stability of δ -plutonium journal, May 2017

Absence of magnetic moments in plutonium journal, August 2005

Magnetism or bonding: A nearly periodic table of transition elements journal, March 1983

Simple Scaling Approach to the Volume Magnetostriction in Unstable-Moment Systems journal, April 1986

Fluctuating valence in a correlated solid and the anomalous properties of δ-plutonium journal, March 2007

First-order valence transition in YbInCu 4 in the ( B , T )-plane journal, November 2000

Coulomb- U and magnetic-moment collapse in δ-Pu journal, February 2005

Phase stability and phase transformations in plutonium and plutonium-gallium alloys journal, August 2004

Phonon Dispersions of fcc -Plutonium-Gallium by Inelastic X-ray Scattering journal, August 2003

Giant magnetic Grüneisen parameters in nearly ferromagnetic and heavy-fermion systems journal, April 1988

Spectral properties of δ -plutonium: Sensitivity to 5 f occupancy journal, December 2007

The valence-fluctuating ground state of plutonium journal, July 2015

The dual nature of 5f electrons and the origin of heavy fermions in U compounds journal, July 2003

The mixed valence energy parameters of some Ce and Yb systems journal, February 1985

Nature of the 5 f states in actinide metals journal, February 2009

Experimental Electronic Heat Capacities of α - and δ -Plutonium: Heavy-Fermion Physics in an Element journal, November 2003

A novel electronic configuration of the 5f states in δ-plutonium as revealed by the photo-electron spectra journal, April 2004

Calculated Phonon Spectra of Plutonium at High Temperatures journal, May 2003

Dynamical mean-field theory of strongly correlated fermion systems and the limit of infinite dimensions journal, January 1996

The α − γ Transition of Cerium Is Entropy Driven journal, February 2006

Origin of the multiple configurations that drive the response of δ-plutonium’s elastic moduli to temperature journal, September 2016

Novel electronic configuration in ∂−Pu journal, June 1999

Invar model for δ-phase Pu: thermal expansion, elastic and magnetic properties journal, June 2006

Magnetic-field, pressure, and temperature scaling of the first-order valence transition in pure and doped YbInCu 4
journal, July 1997

Equilibrium properties of delta-Pu: LDA+ U calculations (LDAequiv local density approximation)
journal, February 2000

Valence fluctuation phenomena
journal, January 1981

Electronic and phonon properties of six crystalline phases of Pu metal
journal, December 1998

Fiber Bragg Grating Dilatometry in Extreme Magnetic Field and Cryogenic Conditions
journal, November 2017

Melting of the light actinides
journal, January 2000

Self-interaction-corrected local spin density theory of $5 f$ electron localization in actinides
journal, September 2007

Electronic properties of f -electron metals using the generalized gradient approximation
journal, September 1994

Suppression of the γ–α structural phase transition in Ce _0.8 La _0.1 Th _0.1 by large magnetic fields
journal, February 2005

First-principles calculations of the electronic structure and spectra of strongly correlated systems: the LDA + U method
journal, January 1997

Piezomagnetism and magnetoelastic memory in uranium dioxide
journal, July 2017

Volume magnetostriction of intermediate valence systems
journal, February 1985

Volume magnetostriction of rare-earth metals with unstable 4f shells
journal, January 1986

Multiconfigurational nature of 5f orbitals in uranium and plutonium intermetallics
journal, June 2012

Magnetic and magnetoelastic properties of ${PrNi}_{5}$ single crystal
journal, February 1988

Dual nature of $5 f$ electrons: Effect of intra-atomic correlations on hopping anisotropies
journal, March 2004

Magnetostriction in metals
journal, November 1971

Correlated electrons in δ-plutonium within a dynamical mean-field picture
journal, April 2001

Spin-polarized relativistic linear-muffin-tin-orbital method: Volume-dependent electronic structure and magnetic moment of plutonium
journal, June 1991

Cancellation of spin and orbital magnetic moments in δ-Pu: Theory
journal, October 2007

Density-functional investigation of magnetism in $δ$ -Pu
journal, November 2002

A unified and efficient theory for the structural properties of actinides and phases of plutonium
journal, September 2018

Phase stability and phase transformations in Pu–Ga alloys
journal, January 2004

Gallium stabilization of $δ − Pu$ : Density-functional calculations
journal, November 2005

Heat capacity measurements on a thin ribbon sample of Zr0.55Al0.10Ni0.05Cu0.30 glassy alloy and Apiezon N high vacuum grease using a Quantum Design Physical Property Measurement System
journal, May 2009

Density-Functional Calculations of $α$ , $β$ , $γ$ , $δ$ , $δ^{'}$ , and $ϵ$ Plutonium
journal, May 2004

Phonon density of states of $α$ - and $δ$ -plutonium by inelastic x-ray scattering
journal, February 2009

Hidden disorder in the $α^{'} \to δ$ transformation of Pu-1.9 at. $%$ Ga
journal, June 2012

Influence of point defects and impurities on the dynamical stability of δ -plutonium
journal, May 2017

Absence of magnetic moments in plutonium
journal, August 2005

Magnetism or bonding: A nearly periodic table of transition elements
journal, March 1983

Simple Scaling Approach to the Volume Magnetostriction in Unstable-Moment Systems
journal, April 1986

Fluctuating valence in a correlated solid and the anomalous properties of δ-plutonium
journal, March 2007

First-order valence transition in YbInCu 4 in the ( B , T )-plane
journal, November 2000

Coulomb- U and magnetic-moment collapse in δ-Pu
journal, February 2005

Phase stability and phase transformations in plutonium and plutonium-gallium alloys
journal, August 2004

Phonon Dispersions of fcc -Plutonium-Gallium by Inelastic X-ray Scattering
journal, August 2003

Giant magnetic Grüneisen parameters in nearly ferromagnetic and heavy-fermion systems
journal, April 1988

Spectral properties of $δ$ -plutonium: Sensitivity to $5 f$ occupancy
journal, December 2007

The valence-fluctuating ground state of plutonium
journal, July 2015

The dual nature of 5f electrons and the origin of heavy fermions in U compounds
journal, July 2003

The mixed valence energy parameters of some Ce and Yb systems
journal, February 1985

Nature of the $5 f$ states in actinide metals
journal, February 2009

Experimental Electronic Heat Capacities of $α$ - and $δ$ -Plutonium: Heavy-Fermion Physics in an Element
journal, November 2003

A novel electronic configuration of the 5f states in δ-plutonium as revealed by the photo-electron spectra
journal, April 2004

Calculated Phonon Spectra of Plutonium at High Temperatures
journal, May 2003

Dynamical mean-field theory of strongly correlated fermion systems and the limit of infinite dimensions
journal, January 1996

The $α − γ$ Transition of Cerium Is Entropy Driven
journal, February 2006

Origin of the multiple configurations that drive the response of δ-plutonium’s elastic moduli to temperature
journal, September 2016

Novel electronic configuration in ∂−Pu
journal, June 1999

Invar model for δ-phase Pu: thermal expansion, elastic and magnetic properties
journal, June 2006