Optically pumped colloidal-quantum-dot lasing in LED-like devices with an integrated optical cavity

Roh, Jeongkyun; Park, Young-Shin; Lim, Jaehoon; Klimov, Victor Ivanovich

doi:10.1038/s41467-019-14014-3

Title: Optically pumped colloidal-quantum-dot lasing in LED-like devices with an integrated optical cavity

Journal Article · 14 January 2020 · Nature Communications

DOI: https://doi.org/10.1038/s41467-019-14014-3 · OSTI ID:1619766

^[1];

^[2]; Lim, Jaehoon ^[3];

^[4]

Pusan National Univ., Busan (Korea); Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Univ. of New Mexico, Albuquerque, NM (United States)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Ajou Univ., Suwon (Korea)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

Realization of electrically pumped lasing with solution processable materials will have a revolutionary impact on many disciplines including photonics, chemical sensing, and medical diagnostics. Due to readily tunable, size-controlled emission wavelengths, colloidal semiconductor quantum dots (QDs) are attractive materials for attaining this goal. Here we use specially engineered QDs to demonstrate devices that operate as both a light emitting diode (LED) and an optically pumped laser. These structures feature a distributed feedback resonator integrated into a bottom LED electrode. By carefully engineering a refractive-index profile across the device, we are able to obtain good confinement of a waveguided mode within the QD medium, which allows for demonstrating low-threshold lasing even with an ultrathin (about three QD monolayers) active layer. These devices also exhibit strong electroluminescence (EL) under electrical pumping. The conducted studies suggest that the demonstrated dual-function (lasing/EL) structures represent a promising device platform for realizing colloidal QD laser diodes.

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Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE Laboratory Directed Research and Development (LDRD) Program

Grant/Contract Number:: 89233218CNA000001

OSTI ID:: 1619766

Alternate ID(s):: OSTI ID: 1593117

Report Number(s):: LA-UR-19-29883

Journal Information:: Nature Communications, Vol. 11, Issue 1; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Integration of a Rib Waveguide Distributed Feedback Structure into a Light-Emitting Polymer Field-Effect Transistor Gwinner, Michael C.; Khodabakhsh, Saghar; Song, Myoung Hoon Advanced Functional Materials, Vol. 19, Issue 9 https://doi.org/10.1002/adfm.200801897	journal	May 2009
Inverted Polymer Solar Cells Integrated with a Low-Temperature-Annealed Sol-Gel-Derived ZnO Film as an Electron Transport Layer Sun, Yanming; Seo, Jung Hwa; Takacs, Christopher J. Advanced Materials, Vol. 23, Issue 14, p. 1679-1683 https://doi.org/10.1002/adma.201004301	journal	February 2011
Graphene as Transparent Electrode Material for Organic Electronics Pang, Shuping; Hernandez, Yenny; Feng, Xinliang Advanced Materials, Vol. 23, Issue 25 https://doi.org/10.1002/adma.201100304	journal	April 2011
Extremely Vivid, Highly Transparent, and Ultrathin Quantum Dot Light-Emitting Diodes Choi, Moon Kee; Yang, Jiwoong; Kim, Dong Chan Advanced Materials, Vol. 30, Issue 1 https://doi.org/10.1002/adma.201703279	journal	October 2017
Organic Semiconductor Lasers Samuel, I. D. W.; Turnbull, G. A. ChemInform, Vol. 38, Issue 31 https://doi.org/10.1002/chin.200731219	journal	July 2007
Organic solid-state integrated amplifiers and lasers Grivas, C.; Pollnau, M. Laser & Photonics Reviews, Vol. 6, Issue 4 https://doi.org/10.1002/lpor.201100034	journal	May 2012
Spectroscopic and Device Aspects of Nanocrystal Quantum Dots Pietryga, Jeffrey M.; Park, Young-Shin; Lim, Jaehoon Chemical Reviews, Vol. 116, Issue 18 https://doi.org/10.1021/acs.chemrev.6b00169	journal	September 2016
Organic Lasers: Recent Developments on Materials, Device Geometries, and Fabrication Techniques Kuehne, Alexander J. C.; Gather, Malte C. Chemical Reviews, Vol. 116, Issue 21 https://doi.org/10.1021/acs.chemrev.6b00172	journal	August 2016
Effect of Auger Recombination on Lasing in Heterostructured Quantum Dots with Engineered Core/Shell Interfaces Park, Young-Shin; Bae, Wan Ki; Baker, Thomas Nano Letters, Vol. 15, Issue 11 https://doi.org/10.1021/acs.nanolett.5b02595	journal	October 2015
Colloidal-Quantum-Dot Ring Lasers with Active Color Control le Feber, Boris; Prins, Ferry; De Leo, Eva Nano Letters, Vol. 18, Issue 2 https://doi.org/10.1021/acs.nanolett.7b04495	journal	January 2018
Droop-Free Colloidal Quantum Dot Light-Emitting Diodes Lim, Jaehoon; Park, Young-Shin; Wu, Kaifeng Nano Letters, Vol. 18, Issue 10 https://doi.org/10.1021/acs.nanolett.8b03457	journal	September 2018
Fully Transparent Quantum Dot Light-Emitting Diode with a Laminated Top Graphene Anode Yao, Li; Fang, Xin; Gu, Wei ACS Applied Materials & Interfaces, Vol. 9, Issue 28 https://doi.org/10.1021/acsami.7b02026	journal	July 2017
Red, Yellow, Green, and Blue Amplified Spontaneous Emission and Lasing Using Colloidal CdSe Nanoplatelets She, Chunxing; Fedin, Igor; Dolzhnikov, Dmitriy S. ACS Nano, Vol. 9, Issue 10 https://doi.org/10.1021/acsnano.5b02509	journal	September 2015
Colloidal Spherical Quantum Wells with Near-Unity Photoluminescence Quantum Yield and Suppressed Blinking Jeong, Byeong Guk; Park, Young-Shin; Chang, Jun Hyuk ACS Nano, Vol. 10, Issue 10 https://doi.org/10.1021/acsnano.6b03704	journal	October 2016
Lasing Supraparticles Self-Assembled from Nanocrystals Montanarella, Federico; Urbonas, Darius; Chadwick, Luke ACS Nano, Vol. 12, Issue 12 https://doi.org/10.1021/acsnano.8b07896	journal	November 2018
Violet-to-Blue Gain and Lasing from Colloidal CdS Nanoplatelets: Low-Threshold Stimulated Emission Despite Low Photoluminescence Quantum Yield Diroll, Benjamin T.; Talapin, Dmitri V.; Schaller, Richard D. ACS Photonics, Vol. 4, Issue 3 https://doi.org/10.1021/acsphotonics.6b00890	journal	February 2017
Bright and Efficient Full-Color Colloidal Quantum Dot Light-Emitting Diodes Using an Inverted Device Structure Kwak, Jeonghun; Bae, Wan Ki; Lee, Donggu Nano Letters, Vol. 12, Issue 5 https://doi.org/10.1021/nl3003254	journal	April 2012
Nonradiative Auger Recombination in Semiconductor Nanocrystals Vaxenburg, Roman; Rodina, Anna; Shabaev, Andrew Nano Letters, Vol. 15, Issue 3 https://doi.org/10.1021/nl504987h	journal	February 2015
Quantum Dot Light-Emitting Devices with Electroluminescence Tunable over the Entire Visible Spectrum Anikeeva, Polina O.; Halpert, Jonathan E.; Bawendi, Moungi G. Nano Letters, Vol. 9, Issue 7 https://doi.org/10.1021/nl9002969	journal	July 2009
Suppression of Auger Processes in Confined Structures Cragg, George E.; Efros, Alexander L. Nano Letters, Vol. 10, Issue 1 https://doi.org/10.1021/nl903592h	journal	January 2010
Amplified Spontaneous Emission and Lasing in Colloidal Nanoplatelets Guzelturk, Burak; Kelestemur, Yusuf; Olutas, Murat ACS Nano, Vol. 8, Issue 7 https://doi.org/10.1021/nn5022296	journal	June 2014
Continuous-wave lasing in colloidal quantum dot solids enabled by facet-selective epitaxy Fan, Fengjia; Voznyy, Oleksandr; Sabatini, Randy P. Nature, Vol. 544, Issue 7648 https://doi.org/10.1038/nature21424	journal	March 2017
Low-threshold amplified spontaneous emission and lasing from colloidal nanocrystals of caesium lead halide perovskites Yakunin, Sergii; Protesescu, Loredana; Krieg, Franziska Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms9056	journal	August 2015
Microsecond-sustained lasing from colloidal quantum dot solids Adachi, Michael M.; Fan, Fengjia; Sellan, Daniel P. Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms9694	journal	October 2015
Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors Zhu, Haiming; Fu, Yongping; Meng, Fei Nature Materials, Vol. 14, Issue 6 https://doi.org/10.1038/nmat4271	journal	April 2015
Optical gain in colloidal quantum dots achieved with direct-current electrical pumping Lim, Jaehoon; Park, Young-Shin; Klimov, Victor I. Nature Materials, Vol. 17, Issue 1 https://doi.org/10.1038/nmat5011	journal	November 2017
Whispering-gallery-mode biosensing: label-free detection down to single molecules Vollmer, Frank; Arnold, Stephen Nature Methods, Vol. 5, Issue 7 https://doi.org/10.1038/nmeth.1221	journal	June 2008
Red, green and blue lasing enabled by single-exciton gain in colloidal quantum dot films Dang, Cuong; Lee, Joonhee; Breen, Craig Nature Nanotechnology, Vol. 7, Issue 5 https://doi.org/10.1038/nnano.2012.61	journal	April 2012
Hybrid perovskite light emitting diodes under intense electrical excitation Kim, Hoyeon; Zhao, Lianfeng; Price, Jared S. Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-07383-8	journal	November 2018
Full-color laser displays based on organic printed microlaser arrays Zhao, Jinyang; Yan, Yongli; Gao, Zhenhua Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-08834-6	journal	February 2019
High-efficiency colloidal quantum dot infrared light-emitting diodes via engineering at the supra-nanocrystalline level Pradhan, Santanu; Di Stasio, Francesco; Bi, Yu Nature Nanotechnology, Vol. 14, Issue 1 https://doi.org/10.1038/s41565-018-0312-y	journal	December 2018
Visible quantum dot light-emitting diodes with simultaneous high brightness and efficiency Shen, Huaibin; Gao, Qiang; Zhang, Yanbin Nature Photonics, Vol. 13, Issue 3 https://doi.org/10.1038/s41566-019-0364-z	journal	February 2019
Photonic band structure and emission characteristics of a metal-backed polymeric distributed feedback laser Andrew, Piers; Turnbull, Graham A.; Samuel, Ifor D. W. Applied Physics Letters, Vol. 81, Issue 6 https://doi.org/10.1063/1.1496497	journal	August 2002
Low-threshold polymeric distributed feedback lasers with metallic contacts Reufer, M.; Riechel, S.; Lupton, J. M. Applied Physics Letters, Vol. 84, Issue 17 https://doi.org/10.1063/1.1712029	journal	April 2004
Amplified spontaneous emission in an organic semiconductor multilayer waveguide structure including a highly conductive transparent electrode Reufer, M.; Feldmann, J.; Rudati, P. Applied Physics Letters, Vol. 86, Issue 22 https://doi.org/10.1063/1.1938001	journal	May 2005
Electroluminescence from heterostructures of poly(phenylene vinylene) and inorganic CdSe nanocrystals Mattoussi, Hedi; Radzilowski, Leonard H.; Dabbousi, Bashir O. Journal of Applied Physics, Vol. 83, Issue 12 https://doi.org/10.1063/1.367978	journal	June 1998
Flexible and Ultra-Lightweight Polymer Membrane Lasers Karl, Markus; Glackin, James M. E.; Schubert, Marcel 2019 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC) https://doi.org/10.1109/cleoe-eqec.2019.8872266	conference	June 2019
Toward continuous-wave operation of organic semiconductor lasers Sandanayaka, Atula S. D.; Matsushima, Toshinori; Bencheikh, Fatima Science Advances, Vol. 3, Issue 4 https://doi.org/10.1126/sciadv.1602570	journal	April 2017
Optical Gain and Stimulated Emission in Nanocrystal Quantum Dots Klimov, V. I.; Mikhailovsky, A. A.; Xu, Su Science, Vol. 290, Issue 5490, p. 314-317 https://doi.org/10.1126/science.290.5490.314	journal	October 2000
Sub–single-exciton lasing using charged quantum dots coupled to a distributed feedback cavity Kozlov, Oleg V.; Park, Young-Shin; Roh, Jeongkyun Science, Vol. 365, Issue 6454 https://doi.org/10.1126/science.aax3489	journal	August 2019
Vertical Cavity Biexciton Lasing in 2D Dodecylammonium Lead Iodide Perovskites Booker, Ep; Price, Mb; Budden, Pj Wiley https://doi.org/10.17863/cam.27007	journalarticle	January 2018
On-Chip Integrated Quantum-Dot Silicon-Nitride Microdisk Lasers Xie, Weiqiang; Stöferle, Thilo; Rainò, Gabriele arXiv https://doi.org/10.48550/arxiv.1901.06227	text	January 2019
Plastic lab-on-a-chip for fluorescence excitation with integrated organic semiconductor lasers Vannahme, C.; Klinkhammer, S.; Lemmer, U. Karlsruhe https://doi.org/10.5445/ir/1000025944	text	January 2011

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