Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells

Shen, Gurong; Liu, Jing; Wu, Hao Bin; Xu, Pengcheng; Liu, Fang; Tongsh, Chasen; Jiao, Kui; Li, Jinlai; Liu, Meilin; Cai, Mei; Lemmon, John P.; Soloveichik, Grigorii; Li, Hexing; Zhu, Jian; Lu, Yunfeng

doi:10.1038/s41467-020-14822-y

Title: Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells

Abstract

Abstract Proton exchange membrane fuel cells have been regarded as the most promising candidate for fuel cell vehicles and tools. Their broader adaption, however, has been impeded by cost and lifetime. By integrating a thin layer of tungsten oxide within the anode, which serves as a rapid-response hydrogen reservoir, oxygen scavenger, sensor for power demand, and regulator for hydrogen-disassociation reaction, we herein report proton exchange membrane fuel cells with significantly enhanced power performance for transient operation and low humidified conditions, as well as improved durability against adverse operating conditions. Meanwhile, the enhanced power performance minimizes the use of auxiliary energy-storage systems and reduces costs. Scale fabrication of such devices can be readily achieved based on the current fabrication techniques with negligible extra expense. This work provides proton exchange membrane fuel cells with enhanced power performance, improved durability, prolonged lifetime, and reduced cost for automotive and other applications.

Authors:

Shen, Gurong;

;

; Xu, Pengcheng; Liu, Fang; Tongsh, Chasen; Jiao, Kui; Li, Jinlai;

;

; Lemmon, John P.; Soloveichik, Grigorii; Li, Hexing; Zhu, Jian; Lu, Yunfeng

Publication Date:: 2020-03-04

Research Org.:: Advanced Research Projects Agency-Energy (ARPA-E), Washington, DC (United States)

Sponsoring Org.:: USDOE Office of Science (SC)

OSTI Identifier:: 1619556

Alternate Identifier(s):: OSTI ID: 1629657

Grant/Contract Number:: AR0001256

Resource Type:: Published Article

Journal Name:: Nature Communications

Additional Journal Information:: Journal Name: Nature Communications Journal Volume: 11 Journal Issue: 1; Journal ID: ISSN 2041-1723

Publisher:: Nature Publishing Group

Country of Publication:: United Kingdom

Language:: English

Subject:: 24 POWER TRANSMISSION AND DISTRIBUTION; 25 ENERGY STORAGE

Citation Formats


                    Shen, Gurong, Liu, Jing, Wu, Hao Bin, Xu, Pengcheng, Liu, Fang, Tongsh, Chasen, Jiao, Kui, Li, Jinlai, Liu, Meilin, Cai, Mei, Lemmon, John P., Soloveichik, Grigorii, Li, Hexing, Zhu, Jian, and Lu, Yunfeng. Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells.  United Kingdom: N. p., 2020. 
Web.  doi:10.1038/s41467-020-14822-y.

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                    Shen, Gurong, Liu, Jing, Wu, Hao Bin, Xu, Pengcheng, Liu, Fang, Tongsh, Chasen, Jiao, Kui, Li, Jinlai, Liu, Meilin, Cai, Mei, Lemmon, John P., Soloveichik, Grigorii, Li, Hexing, Zhu, Jian, & Lu, Yunfeng. Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells.  United Kingdom.  https://doi.org/10.1038/s41467-020-14822-y

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                    Shen, Gurong, Liu, Jing, Wu, Hao Bin, Xu, Pengcheng, Liu, Fang, Tongsh, Chasen, Jiao, Kui, Li, Jinlai, Liu, Meilin, Cai, Mei, Lemmon, John P., Soloveichik, Grigorii, Li, Hexing, Zhu, Jian, and Lu, Yunfeng. Wed .  
"Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells".  United Kingdom.  https://doi.org/10.1038/s41467-020-14822-y.

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@article{osti_1619556,

  title        = {Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells},

  author       = {Shen, Gurong and Liu, Jing and Wu, Hao Bin and Xu, Pengcheng and Liu, Fang and Tongsh, Chasen and Jiao, Kui and Li, Jinlai and Liu, Meilin and Cai, Mei and Lemmon, John P. and Soloveichik, Grigorii and Li, Hexing and Zhu, Jian and Lu, Yunfeng},

  abstractNote = {Abstract Proton exchange membrane fuel cells have been regarded as the most promising candidate for fuel cell vehicles and tools. Their broader adaption, however, has been impeded by cost and lifetime. By integrating a thin layer of tungsten oxide within the anode, which serves as a rapid-response hydrogen reservoir, oxygen scavenger, sensor for power demand, and regulator for hydrogen-disassociation reaction, we herein report proton exchange membrane fuel cells with significantly enhanced power performance for transient operation and low humidified conditions, as well as improved durability against adverse operating conditions. Meanwhile, the enhanced power performance minimizes the use of auxiliary energy-storage systems and reduces costs. Scale fabrication of such devices can be readily achieved based on the current fabrication techniques with negligible extra expense. This work provides proton exchange membrane fuel cells with enhanced power performance, improved durability, prolonged lifetime, and reduced cost for automotive and other applications.},

  doi          = {10.1038/s41467-020-14822-y},

  journal      = {Nature Communications},

  number       = 1,

  volume       = 11,

  place        = {United Kingdom},

  year         = {2020},

  month        = {3}

}

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Similar Records

Title: Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells

Abstract

Citation Formats

Fuel cell electric vehicles and hydrogen infrastructure: status 2012 journal, January 2012

Humidity and Temperature Cycling Effects on Cracks and Delaminations in PEMFCs journal, February 2015

Effects of humidity and temperature on a proton exchange membrane fuel cell (PEMFC) stack journal, May 2008

Main factors affecting the lifetime of Proton Exchange Membrane fuel cells in vehicle applications: A review journal, July 2014

Transient analysis of polymer electrolyte fuel cells journal, January 2005

Statistic analysis of operational influences on the cold start behaviour of PEM fuel cells journal, August 2005

Humidification strategy for polymer electrolyte membrane fuel cells – A review journal, November 2018

Analysis of the behavior and degradation in proton exchange membrane fuel cells with a dead-ended anode journal, January 2014

Hexagonal single crystal growth of WO3 nanorods along a [110] axis with enhanced adsorption capacity journal, January 2011

Hierarchical Nanostructured WO 3 with Biomimetic Proton Channels and Mixed Ionic-Electronic Conductivity for Electrochemical Energy Storage journal, September 2015

A Reverse-Current Decay Mechanism for Fuel Cells journal, January 2005

A review of PEM fuel cell durability: materials degradation, local heterogeneities of aging and possible mitigation strategies: A review of PEM fuel cell durability journal, March 2014

The voltage characteristics of proton exchange membrane fuel cell (PEMFC) under steady and transient states journal, April 2008

PEM fuel cell cathode carbon corrosion due to the formation of air/fuel boundary at the anode journal, August 2006

Transport phenomena effect on the performance of proton exchange membrane fuel cell (PEMFC) journal, July 2013

PEMFC operation failure under severe dehydration journal, April 2012

Electrocatalyst Stability In PEMFCs And The Role Of Fuel Starvation And Cell Reversal Tolerant Anodes journal, July 2006

Experimental analysis of Hybridised Energy Storage Systems for automotive applications journal, August 2016

Behavior of PEMFC in starvation journal, June 2006

Nafion-sulfonated silica composite membrane for proton exchange membrane fuel cells under operating low humidity condition journal, August 2019

Optimal power management of an experimental fuel cell/supercapacitor-powered hybrid vehicle journal, January 2005

A review on performance degradation of proton exchange membrane fuel cells during startup and shutdown processes: Causes, consequences, and mitigation strategies journal, May 2012

Electrocatalyst approaches and challenges for automotive fuel cells journal, June 2012

Energy: Reimagine fuel cells journal, September 2015

Unique CO-tolerance of Pt–WOx materials journal, March 2009

High Surface Area Tunnels in Hexagonal WO 3 journal, June 2015

Analysis of equilibrium potentials of hydrogen tungsten bronzes journal, December 1977

Dynamic modeling, design and simulation of a PEM fuel cell/ultra-capacitor hybrid system for vehicular applications journal, May 2007

Tungsten-based materials for fuel cell applications journal, June 2010

Hydrogen Oxidation and Evolution Reaction Kinetics on Platinum: Acid vs Alkaline Electrolytes journal, January 2010

Mitigation strategies for hydrogen starvation under dynamic loading in proton exchange membrane fuel cells journal, May 2017

A review of automotive proton exchange membrane fuel cell degradation under start-stop operating condition journal, August 2018

Steady state and dynamic performance of proton exchange membrane fuel cells (PEMFCs) under various operating conditions and load changes journal, October 2006

Analysis of electrocatalyst degradation in PEMFC caused by cell reversal during fuel starvation journal, May 2004

Dynamic Models and Model Validation for PEM Fuel Cells Using Electrical Circuits journal, June 2005

Effects of operation temperature and reactant gas humidity levels on performance of PEM fuel cells journal, June 2016

Fuel cell electric vehicles and hydrogen infrastructure: status 2012
journal, January 2012

Humidity and Temperature Cycling Effects on Cracks and Delaminations in PEMFCs
journal, February 2015

Effects of humidity and temperature on a proton exchange membrane fuel cell (PEMFC) stack
journal, May 2008

Main factors affecting the lifetime of Proton Exchange Membrane fuel cells in vehicle applications: A review
journal, July 2014

Transient analysis of polymer electrolyte fuel cells
journal, January 2005

Statistic analysis of operational influences on the cold start behaviour of PEM fuel cells
journal, August 2005

Humidification strategy for polymer electrolyte membrane fuel cells – A review
journal, November 2018

Analysis of the behavior and degradation in proton exchange membrane fuel cells with a dead-ended anode
journal, January 2014

Hexagonal single crystal growth of WO3 nanorods along a [110] axis with enhanced adsorption capacity
journal, January 2011

Hierarchical Nanostructured WO ₃ with Biomimetic Proton Channels and Mixed Ionic-Electronic Conductivity for Electrochemical Energy Storage
journal, September 2015

A Reverse-Current Decay Mechanism for Fuel Cells
journal, January 2005

A review of PEM fuel cell durability: materials degradation, local heterogeneities of aging and possible mitigation strategies: A review of PEM fuel cell durability
journal, March 2014

The voltage characteristics of proton exchange membrane fuel cell (PEMFC) under steady and transient states
journal, April 2008

PEM fuel cell cathode carbon corrosion due to the formation of air/fuel boundary at the anode
journal, August 2006

Transport phenomena effect on the performance of proton exchange membrane fuel cell (PEMFC)
journal, July 2013

PEMFC operation failure under severe dehydration
journal, April 2012

Electrocatalyst Stability In PEMFCs And The Role Of Fuel Starvation And Cell Reversal Tolerant Anodes
journal, July 2006

Experimental analysis of Hybridised Energy Storage Systems for automotive applications
journal, August 2016

Behavior of PEMFC in starvation
journal, June 2006

Nafion-sulfonated silica composite membrane for proton exchange membrane fuel cells under operating low humidity condition
journal, August 2019

Optimal power management of an experimental fuel cell/supercapacitor-powered hybrid vehicle
journal, January 2005

A review on performance degradation of proton exchange membrane fuel cells during startup and shutdown processes: Causes, consequences, and mitigation strategies
journal, May 2012

Electrocatalyst approaches and challenges for automotive fuel cells
journal, June 2012

Energy: Reimagine fuel cells
journal, September 2015

Unique CO-tolerance of Pt–WOx materials
journal, March 2009

High Surface Area Tunnels in Hexagonal WO ₃
journal, June 2015

Analysis of equilibrium potentials of hydrogen tungsten bronzes
journal, December 1977

Dynamic modeling, design and simulation of a PEM fuel cell/ultra-capacitor hybrid system for vehicular applications
journal, May 2007

Tungsten-based materials for fuel cell applications
journal, June 2010

Hydrogen Oxidation and Evolution Reaction Kinetics on Platinum: Acid vs Alkaline Electrolytes
journal, January 2010

Mitigation strategies for hydrogen starvation under dynamic loading in proton exchange membrane fuel cells
journal, May 2017

A review of automotive proton exchange membrane fuel cell degradation under start-stop operating condition
journal, August 2018

Steady state and dynamic performance of proton exchange membrane fuel cells (PEMFCs) under various operating conditions and load changes
journal, October 2006

Analysis of electrocatalyst degradation in PEMFC caused by cell reversal during fuel starvation
journal, May 2004

Dynamic Models and Model Validation for PEM Fuel Cells Using Electrical Circuits
journal, June 2005

Effects of operation temperature and reactant gas humidity levels on performance of PEM fuel cells
journal, June 2016