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Title: Core–shell structured catalysts for thermocatalytic, photocatalytic, and electrocatalytic conversion of CO 2

Abstract

Catalytic conversion of CO2 to produce fuels and chemicals is attractive in prospect because it provides an alternative to fossil feedstocks and the benefit of converting and cycling the greenhouse gas CO2 on a large scale. In today's technology, CO2 is converted into hydrocarbon fuels in Fischer–Tropsch synthesis via the water gas shift reaction, but processes for direct conversion of CO2 to fuels and chemicals such as methane, methanol, and C2+ hydrocarbons or syngas are still far from large-scale applications because of processing challenges that may be best addressed by the discovery of improved catalysts—those with enhanced activity, selectivity, and stability. Core–shell structured catalysts are a relatively new class of nanomaterials that allow a controlled integration of the functions of complementary materials with optimised compositions and morphologies. For CO2 conversion, core–shell catalysts can provide distinctive advantages by addressing challenges such as catalyst sintering and activity loss in CO2 reforming processes, insufficient product selectivity in thermocatalytic CO2 hydrogenation, and low efficiency and selectivity in photocatalytic and electrocatalytic CO2 hydrogenation. In the preceding decade, substantial progress has been made in the synthesis, characterization, and evaluation of core–shell catalysts for such potential applications. Nonetheless, challenges remain in the discovery of inexpensive, robust, regenerablemore » catalysts in this class. This review provides an in-depth assessment of these materials for the thermocatalytic, photocatalytic, and electrocatalytic conversion of CO2 into synthesis gas and valuable hydrocarbons.« less

Authors:
ORCiD logo [1]; ORCiD logo [2]; ORCiD logo [3];  [1];  [1]; ORCiD logo [4]; ORCiD logo [1]
+ Show Author Affiliations
  1. Department of Chemical and Biomolecular Engineering, National University of Singapore, Singapore
  2. Department of Chemical and Biomolecular Engineering, National University of Singapore, Singapore, Institute of Chemical and Bioengineering, Department of Chemistry and Applied Biosciences
  3. Key Laboratory for Green Chemical Technology of Ministry of Education, School of Chemical Engineering & Technology, Collaborative Innovation Center for Chemical Science & Engineering, Tianjin University, Tianjin
  4. Department of Chemical Engineering, University of California, Davis, USA
Publication Date:
Research Org.:
Univ. of California, Davis, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1618782
Alternate Identifier(s):
OSTI ID: 1800146
Grant/Contract Number:  
FG02-04ER15513
Resource Type:
Published Article
Journal Name:
Chemical Society Reviews
Additional Journal Information:
Journal Name: Chemical Society Reviews Journal Volume: 49 Journal Issue: 10; Journal ID: ISSN 0306-0012
Publisher:
Royal Society of Chemistry (RSC)
Country of Publication:
United Kingdom
Language:
English
Subject:
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY

Citation Formats

Das, Sonali, Pérez-Ramírez, Javier, Gong, Jinlong, Dewangan, Nikita, Hidajat, Kus, Gates, Bruce C., and Kawi, Sibudjing. Core–shell structured catalysts for thermocatalytic, photocatalytic, and electrocatalytic conversion of CO 2. United Kingdom: N. p., 2020. Web. doi:10.1039/C9CS00713J.
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Das, Sonali, Pérez-Ramírez, Javier, Gong, Jinlong, Dewangan, Nikita, Hidajat, Kus, Gates, Bruce C., & Kawi, Sibudjing. Core–shell structured catalysts for thermocatalytic, photocatalytic, and electrocatalytic conversion of CO 2. United Kingdom. https://doi.org/10.1039/C9CS00713J
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Das, Sonali, Pérez-Ramírez, Javier, Gong, Jinlong, Dewangan, Nikita, Hidajat, Kus, Gates, Bruce C., and Kawi, Sibudjing. Tue . "Core–shell structured catalysts for thermocatalytic, photocatalytic, and electrocatalytic conversion of CO 2". United Kingdom. https://doi.org/10.1039/C9CS00713J.
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@article{osti_1618782,
title = {Core–shell structured catalysts for thermocatalytic, photocatalytic, and electrocatalytic conversion of CO 2},
author = {Das, Sonali and Pérez-Ramírez, Javier and Gong, Jinlong and Dewangan, Nikita and Hidajat, Kus and Gates, Bruce C. and Kawi, Sibudjing},
abstractNote = {Catalytic conversion of CO2 to produce fuels and chemicals is attractive in prospect because it provides an alternative to fossil feedstocks and the benefit of converting and cycling the greenhouse gas CO2 on a large scale. In today's technology, CO2 is converted into hydrocarbon fuels in Fischer–Tropsch synthesis via the water gas shift reaction, but processes for direct conversion of CO2 to fuels and chemicals such as methane, methanol, and C2+ hydrocarbons or syngas are still far from large-scale applications because of processing challenges that may be best addressed by the discovery of improved catalysts—those with enhanced activity, selectivity, and stability. Core–shell structured catalysts are a relatively new class of nanomaterials that allow a controlled integration of the functions of complementary materials with optimised compositions and morphologies. For CO2 conversion, core–shell catalysts can provide distinctive advantages by addressing challenges such as catalyst sintering and activity loss in CO2 reforming processes, insufficient product selectivity in thermocatalytic CO2 hydrogenation, and low efficiency and selectivity in photocatalytic and electrocatalytic CO2 hydrogenation. In the preceding decade, substantial progress has been made in the synthesis, characterization, and evaluation of core–shell catalysts for such potential applications. Nonetheless, challenges remain in the discovery of inexpensive, robust, regenerable catalysts in this class. This review provides an in-depth assessment of these materials for the thermocatalytic, photocatalytic, and electrocatalytic conversion of CO2 into synthesis gas and valuable hydrocarbons.},
doi = {10.1039/C9CS00713J},
journal = {Chemical Society Reviews},
number = 10,
volume = 49,
place = {United Kingdom},
year = {Tue May 26 00:00:00 EDT 2020},
month = {Tue May 26 00:00:00 EDT 2020}
}
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Ultra-Small Platinum Nanoparticles Encapsulated in Sub-50 nm Hollow Titania Nanospheres for Low-Temperature Water–Gas Shift Reaction
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Metal–Organic Frameworks and Their Derived Materials as Electrocatalysts and Photocatalysts for CO 2 Reduction: Progress, Challenges, and Perspectives
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Hydrogenation of CO 2 to Methanol on CeO x /Cu(111) and ZnO/Cu(111) Catalysts: Role of the Metal–Oxide Interface and Importance of Ce 3+ Sites
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Preparation of CdS@CeO2 core/shell composite for photocatalytic reduction of CO2 under visible-light irradiation
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Insight into the effects of the oxygen species over Ni/ZrO2 catalyst surface on methane reforming with carbon dioxide
journal, May 2019

Confinement Effect and Synergistic Function of H-ZSM-5/Cu-ZnO-Al 2 O 3 Capsule Catalyst for One-Step Controlled Synthesis
journal, June 2010

  • Yang, Guohui; Tsubaki, Noritatsu; Shamoto, Jun
  • Journal of the American Chemical Society, Vol. 132, Issue 23
  • DOI: 10.1021/ja101882a

Incorporation of Nitrogen Defects for Efficient Reduction of CO 2 via Two-Electron Pathway on Three-Dimensional Graphene Foam
journal, December 2015

Synthesis of Dispersible Pd@CeO 2 Core−Shell Nanostructures by Self-Assembly
journal, February 2010

  • Cargnello, Matteo; Wieder, Noah L.; Montini, Tiziano
  • Journal of the American Chemical Society, Vol. 132, Issue 4
  • DOI: 10.1021/ja909131k

Bimetallic IrNi core platinum monolayer shell electrocatalysts for the oxygen reduction reaction
journal, January 2012

  • Kuttiyiel, Kurian A.; Sasaki, Kotaro; Choi, YongMan
  • Energy Environ. Sci., Vol. 5, Issue 1
  • DOI: 10.1039/C1EE02067F

Mono and Bifunctional Pathways of CO2/CH4Reforming over Pt and Rh Based Catalysts
journal, May 1998

  • Bitter, J. H.; Seshan, K.; Lercher, J. A.
  • Journal of Catalysis, Vol. 176, Issue 1
  • DOI: 10.1006/jcat.1998.2022

(Ni/MgAl2O4)@SiO2 core–shell catalyst with high coke-resistance for the dry reforming of methane
journal, March 2018

  • Wang, Yousen; Fang, Qiong; Shen, Weihua
  • Reaction Kinetics, Mechanisms and Catalysis, Vol. 125, Issue 1
  • DOI: 10.1007/s11144-018-1404-2

The Tunable and Highly Selective Reduction Products on Ag@Cu Bimetallic Catalysts Toward CO 2 Electrochemical Reduction Reaction
journal, May 2017

  • Chang, Zhiyuan; Huo, Shengjuan; Zhang, Wei
  • The Journal of Physical Chemistry C, Vol. 121, Issue 21
  • DOI: 10.1021/acs.jpcc.7b01586

Carbon-Supported Single Atom Catalysts for Electrochemical Energy Conversion and Storage
journal, August 2018

LaNiO3@SiO2 core–shell nano-particles for the dry reforming of CH4 in the dielectric barrier discharge plasma
journal, July 2014

Electrochemical Carbon Dioxide Splitting
journal, February 2019

Synergistic effect in plasmonic Au/Ag alloy NPs co-coated TiO2 NWs toward visible-light enhanced CO2 photoreduction to fuels
journal, May 2017

Direct synthesis of dimethyl ether from CO 2 hydrogenation over Cu–ZnO–ZrO 2 /SO 4 2− –ZrO 2 hybrid catalysts: effects of sulfur-to-zirconia ratios
journal, January 2015

  • Witoon, Thongthai; Permsirivanich, Tinnavat; Kanjanasoontorn, Nawapon
  • Catalysis Science & Technology, Vol. 5, Issue 4
  • DOI: 10.1039/C4CY01568A

Selective carbon dioxide electroreduction to ethylene and ethanol by core-shell copper/cuprous oxide
journal, September 2019

Controlled Synthesis of Monodisperse SiO 2 TiO 2 Microspheres with a Yolk-Shell Structure as Effective Photocatalysts
journal, November 2012

Synthesis of multi-shelled ZnO hollow microspheres and their improved photocatalytic activity
journal, January 2014

Poly(l-lysine)-modified silica nanoparticles for the delivery of antisense oligonucleotides
journal, April 2004

  • Zhu, Shi-Guo; Xiang, Juan-Juan; Li, Xiao-Ling
  • Biotechnology and Applied Biochemistry, Vol. 39, Issue 2
  • DOI: 10.1042/BA20030077

Design of Ni-ZrO2@SiO2 catalyst with ultra-high sintering and coking resistance for dry reforming of methane to prepare syngas
journal, October 2018

Encapsulation of Iron Nitride by Fe–N–C Shell Enabling Highly Efficient Electroreduction of CO 2 to CO
journal, April 2018

Highly Active and Stable Bimetallic Nickel-Copper Core-Ceria Shell Catalyst for High-Temperature Water-Gas Shift Reaction
journal, August 2015

Engineering Metal–Organic Frameworks for the Electrochemical Reduction of CO 2 : A Minireview
journal, July 2019

  • Wang, Riming; Kapteijn, Freek; Gascon, Jorge
  • Chemistry – An Asian Journal, Vol. 14, Issue 20
  • DOI: 10.1002/asia.201900710

Cu/Zn/Al/Zr catalysts via phase-pure hydrotalcite-like compounds for methanol synthesis from carbon dioxide
journal, September 2015

(Gold core)/(titania shell) nanostructures for plasmon-enhanced photon harvesting and generation of reactive oxygen species
journal, January 2014

  • Fang, Caihong; Jia, Henglei; Chang, Shuai
  • Energy Environ. Sci., Vol. 7, Issue 10
  • DOI: 10.1039/C4EE01787K

Pd/CNT-promoted CuZrO2/HZSM-5 hybrid catalysts for direct synthesis of DME from CO2/H2
journal, January 2013

Towards full one-pass conversion of carbon dioxide to methanol and methanol-derived products
journal, January 2014

Transition-Metal Nanoparticles in Hollow Zeolite Single Crystals as Bifunctional and Size-Selective Hydrogenation Catalysts
journal, December 2014

  • Li, Shiwen; Tuel, Alain; Laprune, David
  • Chemistry of Materials, Vol. 27, Issue 1
  • DOI: 10.1021/cm503921f

Photoreduction of CO2 on ZIF-8/TiO2 nanocomposites in a gaseous photoreactor under pressure swing
journal, December 2017

Recent developments on heterogeneous catalytic CO2 reduction to methanol
journal, December 2019

Bimetallic Fe–Co catalysts for CO2 hydrogenation to higher hydrocarbons
journal, December 2013

Hybrid carbon@TiO 2 hollow spheres with enhanced photocatalytic CO 2 reduction activity
journal, January 2017

  • Wang, Weikang; Xu, Difa; Cheng, Bei
  • Journal of Materials Chemistry A, Vol. 5, Issue 10
  • DOI: 10.1039/C6TA11121A

Au@Cu2O core@shell nanocrystals as dual-functional catalysts for sustainable environmental applications
journal, March 2019

Origin of Enhancing the Photocatalytic Performance of TiO 2 for Artificial Photoreduction of CO 2 through a SiO 2 Coating Strategy
journal, December 2015

  • Yuan, Lan; Han, Chuang; Pagliaro, Mario
  • The Journal of Physical Chemistry C, Vol. 120, Issue 1
  • DOI: 10.1021/acs.jpcc.5b08893

Sodium-Containing Spinel Zinc Ferrite as a Catalyst Precursor for the Selective Synthesis of Liquid Hydrocarbon Fuels
journal, October 2017

TiO 2 /NiO hybrid shells: p–n junction photocatalysts with enhanced activity under visible light
journal, January 2015

  • Wang, Minggui; Hu, Yimin; Han, Jie
  • Journal of Materials Chemistry A, Vol. 3, Issue 41
  • DOI: 10.1039/C5TA05839B

Fe 2 O 3 @La x Sr 1− x FeO 3 Core-Shell Redox Catalyst for Methane Partial Oxidation
journal, February 2014

New and revisited insights into the promotion of methanol synthesis catalysts by CO2
journal, January 2013

  • Martin, Oliver; Pérez-Ramírez, Javier
  • Catalysis Science & Technology, Vol. 3, Issue 12
  • DOI: 10.1039/c3cy00573a

Cu–Sn Bimetallic Catalyst for Selective Aqueous Electroreduction of CO 2 to CO
journal, April 2016

  • Sarfraz, Saad; Garcia-Esparza, Angel T.; Jedidi, Abdesslem
  • ACS Catalysis, Vol. 6, Issue 5
  • DOI: 10.1021/acscatal.6b00269

Stabilization of Pt at the inner wall of hollow spherical SiO2 generated from Pt/hollow spherical SiC for sulfuric acid decomposition
journal, September 2018

Amine-Functionalized Titanate Nanosheet-Assembled Yolk@Shell Microspheres for Efficient Cocatalyst-Free Visible-Light Photocatalytic CO 2 Reduction
journal, April 2015

  • Liu, Shengwei; Xia, Jiaqiu; Yu, Jiaguo
  • ACS Applied Materials & Interfaces, Vol. 7, Issue 15
  • DOI: 10.1021/acsami.5b00982

Enhanced electrocatalytic activity of Au@Cu core@shell nanoparticles towards CO 2 reduction
journal, January 2015

  • Monzó, J.; Malewski, Y.; Kortlever, R.
  • Journal of Materials Chemistry A, Vol. 3, Issue 47
  • DOI: 10.1039/C5TA06804E

A novel Core–Shell structured CuIn@SiO 2 catalyst for CO 2 hydrogenation to methanol
journal, December 2018

  • Shi, Zhisheng; Tan, Qingqing; Wu, Dongfang
  • AIChE Journal, Vol. 65, Issue 3
  • DOI: 10.1002/aic.16490

Fabrication of cubic Zn 2 SnO 4 /SnO 2 complex hollow structures and their sunlight-driven photocatalytic activity
journal, January 2016

  • Sun, Linqiang; Han, Xiao; Jiang, Zhe
  • Nanoscale, Vol. 8, Issue 26
  • DOI: 10.1039/C5NR08004E

Size-dependent activity and selectivity of carbon dioxide photocatalytic reduction over platinum nanoparticles
journal, March 2018

Enhancing catalytic activity and stability for CO 2 methanation on Ni@MOF-5 via control of active species dispersion
journal, January 2015

  • Zhen, Wenlong; Li, Bo; Lu, Gongxuan
  • Chemical Communications, Vol. 51, Issue 9
  • DOI: 10.1039/C4CC08733J

1D carbon nanofibers@TiO2 core-shell nanocomposites with enhanced photocatalytic activity toward CO2 reduction
journal, May 2018

Crystal-plane effect of nanoscale CeO 2 on the catalytic performance of Ni/CeO 2 catalysts for methane dry reforming
journal, January 2016

  • Wang, Ning; Qian, Weizhong; Chu, Wei
  • Catalysis Science & Technology, Vol. 6, Issue 10
  • DOI: 10.1039/C5CY01790D

Highly selective plasma-activated copper catalysts for carbon dioxide reduction to ethylene
journal, June 2016

  • Mistry, Hemma; Varela, Ana Sofia; Bonifacio, Cecile S.
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms12123

Effect of metal particle size on coking during CO2 reforming of CH4 over Ni–alumina aerogel catalysts
journal, May 2000

Critical Aspects and Recent Advances in Structural Engineering of Photocatalysts for Sunlight‐Driven Photocatalytic Reduction of CO 2 into Fuels
journal, April 2019

  • Vu, Nhu‐Nang; Kaliaguine, Serge; Do, Trong‐On
  • Advanced Functional Materials, Vol. 29, Issue 31
  • DOI: 10.1002/adfm.201901825

3D ordered macroporous TiO 2 -supported Pt@CdS core–shell nanoparticles: design, synthesis and efficient photocatalytic conversion of CO 2 with water to methane
journal, January 2015

  • Wei, Yuechang; Jiao, Jinqing; Zhao, Zhen
  • Journal of Materials Chemistry A, Vol. 3, Issue 20
  • DOI: 10.1039/C5TA00444F

Influence of preparation method on activity and stability of Ni catalysts supported on Gd doped ceria in dry reforming of methane
journal, July 2017

Ni-SiO2 Catalysts for the Carbon Dioxide Reforming of Methane: Varying Support Properties by Flame Spray Pyrolysis
journal, March 2015

A review of the catalytic hydrogenation of carbon dioxide into value-added hydrocarbons
journal, January 2017

  • Yang, Haiyan; Zhang, Chen; Gao, Peng
  • Catalysis Science & Technology, Vol. 7, Issue 20
  • DOI: 10.1039/C7CY01403A

A review on photochemical, biochemical and electrochemical transformation of CO2 into value-added products
journal, October 2019

Photocatalytic reduction of carbon dioxide with water using InNbO4 catalyst with NiO and Co3O4 cocatalysts
journal, May 2012

  • Lee, Der-Shing; Chen, Hsin-Ju; Chen, Yu-Wen
  • Journal of Physics and Chemistry of Solids, Vol. 73, Issue 5
  • DOI: 10.1016/j.jpcs.2012.01.005

The changing nature of the active site of Cu-Zn-Zr catalysts for the CO2 hydrogenation reaction to methanol
journal, June 2014

Controlling upconversion nanocrystals for emerging applications
journal, November 2015

Selective photocatalytic carbon dioxide conversion with Pt@Ag-TiO2 nanoparticles
journal, April 2018

Synthesis of isoalkanes over a core (Fe–Zn–Zr)–shell (zeolite) catalyst by CO 2 hydrogenation
journal, January 2016

  • Wang, Xiaoxing; Yang, Guohui; Zhang, Junfeng
  • Chemical Communications, Vol. 52, Issue 46
  • DOI: 10.1039/C6CC01965J

A Rational Design of Cu 2 O−SnO 2 Core‐Shell Catalyst for Highly Selective CO 2 ‐to‐CO Conversion
journal, May 2019

Tin Oxide Dependence of the CO 2 Reduction Efficiency on Tin Electrodes and Enhanced Activity for Tin/Tin Oxide Thin-Film Catalysts
journal, January 2012

  • Chen, Yihong; Kanan, Matthew W.
  • Journal of the American Chemical Society, Vol. 134, Issue 4
  • DOI: 10.1021/ja2108799

Effective nonmetal incorporation in black titania with enhanced solar energy utilization
journal, January 2014

  • Lin, Tianquan; Yang, Chongyin; Wang, Zhou
  • Energy & Environmental Science, Vol. 7, Issue 3
  • DOI: 10.1039/c3ee42708k

Palladium nanoparticle's surface structure and morphology effect on the catalytic activity for dry reforming of methane
journal, May 2014

A review of dry (CO 2 ) reforming of methane over noble metal catalysts
journal, January 2014

  • Pakhare, Devendra; Spivey, James
  • Chem. Soc. Rev., Vol. 43, Issue 22
  • DOI: 10.1039/C3CS60395D

Overcoating the Surface of Fe-Based Catalyst with ZnO and Nitrogen-Doped Carbon toward High Selectivity of Light Olefins in CO 2 Hydrogenation
journal, February 2019

  • Liu, Junhui; Zhang, Anfeng; Jiang, Xiao
  • Industrial & Engineering Chemistry Research, Vol. 58, Issue 10
  • DOI: 10.1021/acs.iecr.8b05478

Catalysts and Reaction Pathways for the Electrochemical Reduction of Carbon Dioxide
journal, September 2015

  • Kortlever, Ruud; Shen, Jing; Schouten, Klaas Jan P.
  • The Journal of Physical Chemistry Letters, Vol. 6, Issue 20
  • DOI: 10.1021/acs.jpclett.5b01559

CO 2 reforming with methane over small-sized Ni@SiO 2 catalysts with unique features of sintering-free and low carbon
journal, November 2018

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