Single-Walled Carbon Nanotube Network Electrodes for the Detection of Fentanyl Citrate

Wester, Niklas; Mynttinen, Elsi; Etula, Jarkko; Lilius, Tuomas; Kalso, Eija; Mikladal, Bjørn F.; Zhang, Qiang; Jiang, Hua; Sainio, Sami; Nordlund, Dennis; Kauppinen, Esko I.; Laurila, Tomi; Koskinen, Jari

doi:10.1021/acsanm.9b01951

Title: Single-Walled Carbon Nanotube Network Electrodes for the Detection of Fentanyl Citrate

Journal Article · 09 January 2020 · ACS Applied Nano Materials

DOI: https://doi.org/10.1021/acsanm.9b01951 · OSTI ID:1617140

^[1]; Mynttinen, Elsi ^[1];

^[1]; Lilius, Tuomas ^[2]; Kalso, Eija ^[2]; Mikladal, Bjørn F. ^[3]; Zhang, Qiang ^[1]; Jiang, Hua ^[1];

^[4]; Nordlund, Dennis ^[4]; Kauppinen, Esko I. ^[1];

^[1]; Koskinen, Jari ^[1]

Aalto Univ., Otaniemi (Finland)
Univ. of Helsinki (Finland)
Canatu Oy, Helsinki (Finland)
SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Synchrotron Radiation Lightsource (SSRL)

Here, we prepare disposable single-walled carbon nanotube network electrodes for the detection of the potent opioid fentanyl, currently a leading cause for opioid overdose deaths in the USA. We show repeatable dry transfer of single-walled carbon nanotube (SWCNT) networks to produce robust electrodes. This process directly produces highly conductive SWCNT electrodes without the need for any further modifications required for conventional carbon electrodes. The realized electrode showed low background currents combined with spontaneous enrichment of fentanyl, resulting in a high signal-to-noise ratio. With this electrode, a detection limit of 11 nM and a linear range of 0.01–1 μM were found for fentanyl. Furthermore, selectivity is demonstrated in the presence of several common interferents.

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Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 1617140

Journal Information:: ACS Applied Nano Materials, Journal Name: ACS Applied Nano Materials Journal Issue: 2 Vol. 3; ISSN 2574-0970

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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