DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Nematic transitions in iron pnictide superconductors imaged with a quantum gas

Abstract

The Scanning Quantum Cryogenic Atom Microscope (SQCRAMscope) uses an atomic Bose–Einstein condensate to measure magnetic fields emanating from solid-state samples. The quantum sensor does so with unprecedented d.c. sensitivity at micrometre resolution, from room to cryogenic temperatures. An additional advantage of the SQCRAMscope is the preservation of optical access to the sample so that magnetometry imaging of, for example, electron transport may be performed in concert with other imaging techniques. Here, we apply this multimodal imaging capability to the study of nematicity in iron pnictide high-temperature superconductors, where the relationship between electronic and structural symmetry breaking resulting in a nematic phase is under debate. We combine the SQCRAMscope with an in situ microscope that measures optical birefringence near the surface. This enables simultaneous and spatially resolved detection of both bulk and near-surface manifestations of nematicity via transport and structural deformation channels, respectively. By performing local measurements of emergent resistivity anisotropy in iron pnictides, we observe sharp, nearly concurrent transport and structural transitions. More broadly, these measurements demonstrate the SQCRAMscope’s ability to reveal important insights into the physics of complex quantum materials.

Authors:
 [1]; ORCiD logo [1];  [1];  [2];  [2]; ORCiD logo [1]
  1. Stanford Univ., CA (United States)
  2. Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials; SLAC National Accelerator Lab., Menlo Park, CA (United States)
Publication Date:
Research Org.:
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1616847
Grant/Contract Number:  
DGE-114747; AC02-76SF00515; SC0019174; N00014- 17-1-2248; GBMF3502; W911NF1910392
Resource Type:
Accepted Manuscript
Journal Name:
Nature Physics
Additional Journal Information:
Journal Volume: 16; Journal Issue: 5; Journal ID: ISSN 1745-2473
Publisher:
Nature Publishing Group (NPG)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats

Yang, Fan, Taylor, Stephen F., Edkins, Stephen D., Palmstrom, Johanna C., Fisher, Ian R., and Lev, Benjamin L. Nematic transitions in iron pnictide superconductors imaged with a quantum gas. United States: N. p., 2020. Web. doi:10.1038/s41567-020-0826-8.
Yang, Fan, Taylor, Stephen F., Edkins, Stephen D., Palmstrom, Johanna C., Fisher, Ian R., & Lev, Benjamin L. Nematic transitions in iron pnictide superconductors imaged with a quantum gas. United States. https://doi.org/10.1038/s41567-020-0826-8
Yang, Fan, Taylor, Stephen F., Edkins, Stephen D., Palmstrom, Johanna C., Fisher, Ian R., and Lev, Benjamin L. Mon . "Nematic transitions in iron pnictide superconductors imaged with a quantum gas". United States. https://doi.org/10.1038/s41567-020-0826-8. https://www.osti.gov/servlets/purl/1616847.
@article{osti_1616847,
title = {Nematic transitions in iron pnictide superconductors imaged with a quantum gas},
author = {Yang, Fan and Taylor, Stephen F. and Edkins, Stephen D. and Palmstrom, Johanna C. and Fisher, Ian R. and Lev, Benjamin L.},
abstractNote = {The Scanning Quantum Cryogenic Atom Microscope (SQCRAMscope) uses an atomic Bose–Einstein condensate to measure magnetic fields emanating from solid-state samples. The quantum sensor does so with unprecedented d.c. sensitivity at micrometre resolution, from room to cryogenic temperatures. An additional advantage of the SQCRAMscope is the preservation of optical access to the sample so that magnetometry imaging of, for example, electron transport may be performed in concert with other imaging techniques. Here, we apply this multimodal imaging capability to the study of nematicity in iron pnictide high-temperature superconductors, where the relationship between electronic and structural symmetry breaking resulting in a nematic phase is under debate. We combine the SQCRAMscope with an in situ microscope that measures optical birefringence near the surface. This enables simultaneous and spatially resolved detection of both bulk and near-surface manifestations of nematicity via transport and structural deformation channels, respectively. By performing local measurements of emergent resistivity anisotropy in iron pnictides, we observe sharp, nearly concurrent transport and structural transitions. More broadly, these measurements demonstrate the SQCRAMscope’s ability to reveal important insights into the physics of complex quantum materials.},
doi = {10.1038/s41567-020-0826-8},
journal = {Nature Physics},
number = 5,
volume = 16,
place = {United States},
year = {Mon Mar 30 00:00:00 EDT 2020},
month = {Mon Mar 30 00:00:00 EDT 2020}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record

Citation Metrics:
Cited by: 5 works
Citation information provided by
Web of Science

Save / Share:

Works referenced in this record:

Symmetry-breaking orbital anisotropy observed for detwinned Ba(Fe1-xCox)2As2 above the spin density wave transition
journal, April 2011

  • Yi, M.; Lu, D.; Chu, J. -H.
  • Proceedings of the National Academy of Sciences, Vol. 108, Issue 17
  • DOI: 10.1073/pnas.1015572108

Determination of the phase diagram of the electron-doped superconductor Ba ( Fe 1 x Co x ) 2 As 2
journal, January 2009


Broken rotational symmetry in the pseudogap phase of a high-Tc superconductor
journal, January 2010


Critical phenomena at surfaces
journal, February 1990


Manifestations of nematic degrees of freedom in the magnetic, elastic, and superconducting properties of the iron pnictides
journal, July 2012


Pseudogap formation above the superconducting dome in iron pnictides
journal, January 2014


Intrinsic pinning on structural domains in underdoped single crystals of Ba ( Fe 1 x Co x ) 2 As 2
journal, November 2009


Surface pinning of fluctuating charge order: An extraordinary surface phase transition
journal, June 2005


Scanning Quantum Cryogenic Atom Microscope
journal, March 2017


Electronic liquid-crystal phases of a doped Mott insulator
journal, June 1998

  • Kivelson, S. A.; Fradkin, E.; Emery, V. J.
  • Nature, Vol. 393, Issue 6685
  • DOI: 10.1038/31177

Divergent Nematic Susceptibility in an Iron Arsenide Superconductor
journal, August 2012


Direct imaging of the structural domains in the iron pnictides A Fe 2 As 2 ( A = Ca , Sr , Ba )
journal, May 2009


Electronic nematicity above the structural and superconducting transition in BaFe2(As1−xP x )2
journal, June 2012

  • Kasahara, S.; Shi, H. J.; Hashimoto, K.
  • Nature, Vol. 486, Issue 7403
  • DOI: 10.1038/nature11178

Surface nematic order in iron pnictides
journal, September 2016


What drives nematic order in iron-based superconductors?
journal, January 2014

  • Fernandes, R. M.; Chubukov, A. V.; Schmalian, J.
  • Nature Physics, Vol. 10, Issue 2
  • DOI: 10.1038/nphys2877

Imaging Anomalous Nematic Order and Strain in Optimally Doped BaFe 2 ( As , P ) 2
journal, July 2018


In-Plane Resistivity Anisotropy in an Underdoped Iron Arsenide Superconductor
journal, August 2010


Nematic Fermi Fluids in Condensed Matter Physics
journal, August 2010


Ubiquitous signatures of nematic quantum criticality in optimally doped Fe-based superconductors
journal, May 2016


Intra-unit-cell electronic nematicity of the high-Tc copper-oxide pseudogap states
journal, July 2010

  • Lawler, M. J.; Fujita, K.; Lee, Jhinhwan
  • Nature, Vol. 466, Issue 7304
  • DOI: 10.1038/nature09169

Character of the structural and magnetic phase transitions in the parent and electron-doped BaFe 2 As 2 compounds
journal, April 2011


Orbital-anisotropic electronic structure in the nonmagnetic state of BaFe2(As1−xP x )2 superconductors
journal, February 2018


Formation of a Nematic Fluid at High Fields in Sr3Ru2O7
journal, January 2007


Pseudogap formation above the superconducting dome in iron-pnictides
text, January 2013


Scanning Quantum Cryogenic Atom Microscope
text, January 2016