Nematic transitions in iron pnictide superconductors imaged with a quantum gas
Abstract
The Scanning Quantum Cryogenic Atom Microscope (SQCRAMscope) uses an atomic Bose–Einstein condensate to measure magnetic fields emanating from solid-state samples. The quantum sensor does so with unprecedented d.c. sensitivity at micrometre resolution, from room to cryogenic temperatures. An additional advantage of the SQCRAMscope is the preservation of optical access to the sample so that magnetometry imaging of, for example, electron transport may be performed in concert with other imaging techniques. Here, we apply this multimodal imaging capability to the study of nematicity in iron pnictide high-temperature superconductors, where the relationship between electronic and structural symmetry breaking resulting in a nematic phase is under debate. We combine the SQCRAMscope with an in situ microscope that measures optical birefringence near the surface. This enables simultaneous and spatially resolved detection of both bulk and near-surface manifestations of nematicity via transport and structural deformation channels, respectively. By performing local measurements of emergent resistivity anisotropy in iron pnictides, we observe sharp, nearly concurrent transport and structural transitions. More broadly, these measurements demonstrate the SQCRAMscope’s ability to reveal important insights into the physics of complex quantum materials.
- Authors:
-
- Stanford Univ., CA (United States)
- Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials; SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Publication Date:
- Research Org.:
- SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1616847
- Grant/Contract Number:
- DGE-114747; AC02-76SF00515; SC0019174; N00014- 17-1-2248; GBMF3502; W911NF1910392
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Physics
- Additional Journal Information:
- Journal Volume: 16; Journal Issue: 5; Journal ID: ISSN 1745-2473
- Publisher:
- Nature Publishing Group (NPG)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Citation Formats
Yang, Fan, Taylor, Stephen F., Edkins, Stephen D., Palmstrom, Johanna C., Fisher, Ian R., and Lev, Benjamin L. Nematic transitions in iron pnictide superconductors imaged with a quantum gas. United States: N. p., 2020.
Web. doi:10.1038/s41567-020-0826-8.
Yang, Fan, Taylor, Stephen F., Edkins, Stephen D., Palmstrom, Johanna C., Fisher, Ian R., & Lev, Benjamin L. Nematic transitions in iron pnictide superconductors imaged with a quantum gas. United States. https://doi.org/10.1038/s41567-020-0826-8
Yang, Fan, Taylor, Stephen F., Edkins, Stephen D., Palmstrom, Johanna C., Fisher, Ian R., and Lev, Benjamin L. Mon .
"Nematic transitions in iron pnictide superconductors imaged with a quantum gas". United States. https://doi.org/10.1038/s41567-020-0826-8. https://www.osti.gov/servlets/purl/1616847.
@article{osti_1616847,
title = {Nematic transitions in iron pnictide superconductors imaged with a quantum gas},
author = {Yang, Fan and Taylor, Stephen F. and Edkins, Stephen D. and Palmstrom, Johanna C. and Fisher, Ian R. and Lev, Benjamin L.},
abstractNote = {The Scanning Quantum Cryogenic Atom Microscope (SQCRAMscope) uses an atomic Bose–Einstein condensate to measure magnetic fields emanating from solid-state samples. The quantum sensor does so with unprecedented d.c. sensitivity at micrometre resolution, from room to cryogenic temperatures. An additional advantage of the SQCRAMscope is the preservation of optical access to the sample so that magnetometry imaging of, for example, electron transport may be performed in concert with other imaging techniques. Here, we apply this multimodal imaging capability to the study of nematicity in iron pnictide high-temperature superconductors, where the relationship between electronic and structural symmetry breaking resulting in a nematic phase is under debate. We combine the SQCRAMscope with an in situ microscope that measures optical birefringence near the surface. This enables simultaneous and spatially resolved detection of both bulk and near-surface manifestations of nematicity via transport and structural deformation channels, respectively. By performing local measurements of emergent resistivity anisotropy in iron pnictides, we observe sharp, nearly concurrent transport and structural transitions. More broadly, these measurements demonstrate the SQCRAMscope’s ability to reveal important insights into the physics of complex quantum materials.},
doi = {10.1038/s41567-020-0826-8},
journal = {Nature Physics},
number = 5,
volume = 16,
place = {United States},
year = {Mon Mar 30 00:00:00 EDT 2020},
month = {Mon Mar 30 00:00:00 EDT 2020}
}
Web of Science
Works referenced in this record:
Symmetry-breaking orbital anisotropy observed for detwinned Ba(Fe1-xCox)2As2 above the spin density wave transition
journal, April 2011
- Yi, M.; Lu, D.; Chu, J. -H.
- Proceedings of the National Academy of Sciences, Vol. 108, Issue 17
Determination of the phase diagram of the electron-doped superconductor
journal, January 2009
- Chu, Jiun-Haw; Analytis, James G.; Kucharczyk, Chris
- Physical Review B, Vol. 79, Issue 1
Neutron-Diffraction Measurements of Magnetic Order and a Structural Transition in the Parent Compound of FeAs-Based High-Temperature Superconductors
journal, December 2008
- Huang, Q.; Qiu, Y.; Bao, Wei
- Physical Review Letters, Vol. 101, Issue 25
Broken rotational symmetry in the pseudogap phase of a high-Tc superconductor
journal, January 2010
- Daou, R.; Chang, J.; LeBoeuf, David
- Nature, Vol. 463, Issue 7280
Critical phenomena at surfaces
journal, February 1990
- Binder, K.; Landau, D. P.
- Physica A: Statistical Mechanics and its Applications, Vol. 163, Issue 1
Manifestations of nematic degrees of freedom in the magnetic, elastic, and superconducting properties of the iron pnictides
journal, July 2012
- Fernandes, Rafael M.; Schmalian, Jörg
- Superconductor Science and Technology, Vol. 25, Issue 8
Pseudogap formation above the superconducting dome in iron pnictides
journal, January 2014
- Shimojima, T.; Sonobe, T.; Malaeb, W.
- Physical Review B, Vol. 89, Issue 4
Intrinsic pinning on structural domains in underdoped single crystals of
journal, November 2009
- Prozorov, R.; Tanatar, M. A.; Ni, N.
- Physical Review B, Vol. 80, Issue 17
Microstructure and tetragonal-to-orthorhombic phase transition of as seen via transmission electron microscopy
journal, February 2009
- Ma, C.; Yang, H. X.; Tian, H. F.
- Physical Review B, Vol. 79, Issue 6
Surface pinning of fluctuating charge order: An extraordinary surface phase transition
journal, June 2005
- Brown, Stuart E.; Fradkin, Eduardo; Kivelson, Steven A.
- Physical Review B, Vol. 71, Issue 22
Scanning Quantum Cryogenic Atom Microscope
journal, March 2017
- Yang, Fan; Kollár, Alicia J.; Taylor, Stephen F.
- Physical Review Applied, Vol. 7, Issue 3
Electronic liquid-crystal phases of a doped Mott insulator
journal, June 1998
- Kivelson, S. A.; Fradkin, E.; Emery, V. J.
- Nature, Vol. 393, Issue 6685
Divergent Nematic Susceptibility in an Iron Arsenide Superconductor
journal, August 2012
- Chu, J. -H.; Kuo, H. -H.; Analytis, J. G.
- Science, Vol. 337, Issue 6095
Direct imaging of the structural domains in the iron pnictides
journal, May 2009
- Tanatar, M. A.; Kreyssig, A.; Nandi, S.
- Physical Review B, Vol. 79, Issue 18
Electronic nematicity above the structural and superconducting transition in BaFe2(As1−xP x )2
journal, June 2012
- Kasahara, S.; Shi, H. J.; Hashimoto, K.
- Nature, Vol. 486, Issue 7403
Surface nematic order in iron pnictides
journal, September 2016
- Song, Kok Wee; Koshelev, Alexei E.
- Physical Review B, Vol. 94, Issue 9
What drives nematic order in iron-based superconductors?
journal, January 2014
- Fernandes, R. M.; Chubukov, A. V.; Schmalian, J.
- Nature Physics, Vol. 10, Issue 2
Imaging Anomalous Nematic Order and Strain in Optimally Doped
journal, July 2018
- Thewalt, Eric; Hayes, Ian M.; Hinton, James P.
- Physical Review Letters, Vol. 121, Issue 2
In-Plane Resistivity Anisotropy in an Underdoped Iron Arsenide Superconductor
journal, August 2010
- Chu, J. -H.; Analytis, J. G.; De Greve, K.
- Science, Vol. 329, Issue 5993
Nematic Fermi Fluids in Condensed Matter Physics
journal, August 2010
- Fradkin, Eduardo; Kivelson, Steven A.; Lawler, Michael J.
- Annual Review of Condensed Matter Physics, Vol. 1, Issue 1
Ubiquitous signatures of nematic quantum criticality in optimally doped Fe-based superconductors
journal, May 2016
- Kuo, H. -H.; Chu, J. -H.; Palmstrom, J. C.
- Science, Vol. 352, Issue 6288
Intra-unit-cell electronic nematicity of the high-Tc copper-oxide pseudogap states
journal, July 2010
- Lawler, M. J.; Fujita, K.; Lee, Jhinhwan
- Nature, Vol. 466, Issue 7304
Character of the structural and magnetic phase transitions in the parent and electron-doped BaFe As compounds
journal, April 2011
- Kim, M. G.; Fernandes, R. M.; Kreyssig, A.
- Physical Review B, Vol. 83, Issue 13
Orbital-anisotropic electronic structure in the nonmagnetic state of BaFe2(As1−xP x )2 superconductors
journal, February 2018
- Sonobe, T.; Shimojima, T.; Nakamura, A.
- Scientific Reports, Vol. 8, Issue 1
Formation of a Nematic Fluid at High Fields in Sr3Ru2O7
journal, January 2007
- Borzi, R. A.; Grigera, S. A.; Farrell, J.
- Science, Vol. 315, Issue 5809
Doping dependence of femtosecond quasiparticle relaxation dynamics in Ba(Fe,Co) As single crystals: Evidence for normal-state nematic fluctuations
journal, July 2012
- Stojchevska, L.; Mertelj, T.; Chu, Jiun-Haw
- Physical Review B, Vol. 86, Issue 2
Manifestations of nematic degrees of freedom in the magnetic, elastic, and superconducting properties of the iron pnictides
text, January 2012
- Fernandes, Rafael M.; Schmalian, Jörg
- arXiv
Pseudogap formation above the superconducting dome in iron-pnictides
text, January 2013
- Shimojima, T.; Sonobe, T.; Malaeb, W.
- arXiv
Scanning Quantum Cryogenic Atom Microscope
text, January 2016
- Yang, Fan; Kollár, Alicia J.; Taylor, Stephen F.
- arXiv