Nanocrystal synthesis, μfluidic sample dilution and direct extraction of single emission linewidths in continuous flow
Abstract
We present a flow-based system coupled with an optical interferometry setup for the extraction of single nanocrystal properties.
- Authors:
-
[1];
[2];
[2];
[3]
- Department of Chemical Engineering, Massachusetts Institute of Technology, Cambridge, USA, Department of Chemistry
- Department of Chemistry, Massachusetts Institute of Technology, Cambridge, USA
- Department of Chemical Engineering, Massachusetts Institute of Technology, Cambridge, USA
- Publication Date:
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1616630
- Grant/Contract Number:
- FG02-07ER46456
- Resource Type:
- Published Article
- Journal Name:
- Lab on a chip (Print)
- Additional Journal Information:
- Journal Name: Lab on a chip (Print) Journal Volume: 20 Journal Issue: 11; Journal ID: ISSN 1473-0197
- Publisher:
- Royal Society of Chemistry (RSC)
- Country of Publication:
- France
- Language:
- English
Citation Formats
Lignos, Ioannis, Utzat, Hendrik, Bawendi, Moungi G., and Jensen, Klavs F. Nanocrystal synthesis, μfluidic sample dilution and direct extraction of single emission linewidths in continuous flow. France: N. p., 2020.
Web. doi:10.1039/D0LC00213E.
Lignos, Ioannis, Utzat, Hendrik, Bawendi, Moungi G., & Jensen, Klavs F. Nanocrystal synthesis, μfluidic sample dilution and direct extraction of single emission linewidths in continuous flow. France. doi:https://doi.org/10.1039/D0LC00213E
Lignos, Ioannis, Utzat, Hendrik, Bawendi, Moungi G., and Jensen, Klavs F. Tue .
"Nanocrystal synthesis, μfluidic sample dilution and direct extraction of single emission linewidths in continuous flow". France. doi:https://doi.org/10.1039/D0LC00213E.
@article{osti_1616630,
title = {Nanocrystal synthesis, μfluidic sample dilution and direct extraction of single emission linewidths in continuous flow},
author = {Lignos, Ioannis and Utzat, Hendrik and Bawendi, Moungi G. and Jensen, Klavs F.},
abstractNote = {We present a flow-based system coupled with an optical interferometry setup for the extraction of single nanocrystal properties.},
doi = {10.1039/D0LC00213E},
journal = {Lab on a chip (Print)},
number = 11,
volume = 20,
place = {France},
year = {2020},
month = {6}
}
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DOI: https://doi.org/10.1039/D0LC00213E
DOI: https://doi.org/10.1039/D0LC00213E
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Works referenced in this record:
Oscillatory Microprocessor for Growth and in Situ Characterization of Semiconductor Nanocrystals
journal, August 2015
- Abolhasani, Milad; Coley, Connor W.; Xie, Lisi
- Chemistry of Materials, Vol. 27, Issue 17
A stable droplet reactor for high temperature nanocrystal synthesis
journal, January 2011
- Nightingale, A. M.; Krishnadasan, S. H.; Berhanu, D.
- Lab Chip, Vol. 11, Issue 7
Fluorescence correlation spectroscopy with high count rate and low background: analysis of translational diffusion
journal, August 1993
- Rigler, R.; Mets, �.; Widengren, J.
- European Biophysics Journal, Vol. 22, Issue 3
Synthesis of silver nanoparticles in a microfluidic coaxial flow reactor
journal, January 2015
- Baber, Razwan; Mazzei, Luca; Thanh, Nguyen T. K.
- RSC Advances, Vol. 5, Issue 116
Fluorescence Correlation Spectroscopy: Past, Present, Future
journal, December 2011
- Elson, Elliot L.
- Biophysical Journal, Vol. 101, Issue 12
On-line analysis of CdSe nanoparticle formation in a continuous flow chip-based microreactor
journal, January 2004
- Krishnadasan, S.; Tovilla, J.; Vilar, R.
- Journal of Materials Chemistry, Vol. 14, Issue 17
Building devices from colloidal quantum dots
journal, August 2016
- Kagan, C. R.; Lifshitz, E.; Sargent, E. H.
- Science, Vol. 353, Issue 6302
Evolution of the Single-Nanocrystal Photoluminescence Linewidth with Size and Shell: Implications for Exciton–Phonon Coupling and the Optimization of Spectral Linewidths
journal, December 2015
- Cui, Jian; Beyler, Andrew P.; Coropceanu, Igor
- Nano Letters, Vol. 16, Issue 1
Fluorescence correlation spectroscopy for flow rate imaging and monitoring—optimization, limitations and artifacts
journal, January 2005
- Brister, Paul C.; Kuricheti, Kalyan K.; Buschmann, Volker
- Lab Chip, Vol. 5, Issue 7
Hydrodynamic Flow Profiling in Microchannel Structures by Single Molecule Fluorescence Correlation Spectroscopy
journal, July 2000
- Gösch, Michael; Blom, Hans; Holm, Johan
- Analytical Chemistry, Vol. 72, Issue 14
Nanocrystal synthesis in microfluidic reactors: where next?
journal, January 2014
- Phillips, Thomas W.; Lignos, Ioannis G.; Maceiczyk, Richard M.
- Lab on a Chip, Vol. 14, Issue 17
Direct probe of spectral inhomogeneity reveals synthetic tunability of single-nanocrystal spectral linewidths
journal, June 2013
- Cui, Jian; Beyler, Andrew P.; Marshall, Lisa F.
- Nature Chemistry, Vol. 5, Issue 7
Continuous microfluidic synthesis of colloidal ultrasmall gold nanoparticles: in situ study of the early reaction stages and application for catalysis
journal, January 2017
- Tofighi, Ghazal; Lichtenberg, Henning; Pesek, Jan
- Reaction Chemistry & Engineering, Vol. 2, Issue 6
Microfluidic Technology: Uncovering the Mechanisms of Nanocrystal Nucleation and Growth
journal, April 2017
- Lignos, Ioannis; Maceiczyk, Richard; deMello, Andrew J.
- Accounts of Chemical Research, Vol. 50, Issue 5
Toward continuous and scalable production of colloidal nanocrystals by switching from batch to droplet reactors
journal, January 2015
- Niu, Guangda; Ruditskiy, Aleksey; Vara, Madeline
- Chemical Society Reviews, Vol. 44, Issue 16
Opportunities and challenges for quantum dot photovoltaics
journal, December 2015
- Kovalenko, Maksym V.
- Nature Nanotechnology, Vol. 10, Issue 12
Synthesis of Cesium Lead Halide Perovskite Nanocrystals in a Droplet-Based Microfluidic Platform: Fast Parametric Space Mapping
journal, February 2016
- Lignos, Ioannis; Stavrakis, Stavros; Nedelcu, Georgian
- Nano Letters, Vol. 16, Issue 3
Nucleation and Growth of Gold Nanoparticles Studied via in situ Small Angle X-ray Scattering at Millisecond Time Resolution
journal, January 2010
- Polte, Jörg; Erler, Robert; Thünemann, Andreas F.
- ACS Nano, Vol. 4, Issue 2
Probing Linewidths and Biexciton Quantum Yields of Single Cesium Lead Halide Nanocrystals in Solution
journal, October 2017
- Utzat, Hendrik; Shulenberger, Katherine E.; Achorn, Odin B.
- Nano Letters, Vol. 17, Issue 11
High-Temperature Microfluidic Synthesis of CdSe Nanocrystals in Nanoliter Droplets
journal, October 2005
- Chan, Emory M.; Alivisatos, A. Paul; Mathies, Richard A.
- Journal of the American Chemical Society, Vol. 127, Issue 40
Deconstructing the photon stream from single nanocrystals: from binning to correlation
journal, January 2014
- Cui, Jian; Beyler, Andrew P.; Bischof, Thomas S.
- Chem. Soc. Rev., Vol. 43, Issue 4
Facile Room‐Temperature Anion Exchange Reactions of Inorganic Perovskite Quantum Dots Enabled by a Modular Microfluidic Platform
journal, March 2019
- Abdel‐Latif, Kameel; Epps, Robert W.; Kerr, Corwin B.
- Advanced Functional Materials, Vol. 29, Issue 23
Single-Nanocrystal Spectroscopy of White-Light-Emitting CdSe Nanocrystals
journal, April 2011
- Dukes, Albert D.; Samson, Philip C.; Keene, Joseph D.
- The Journal of Physical Chemistry A, Vol. 115, Issue 16
Synthesis and Characterization of Monodisperse Nanocrystals and Close-Packed Nanocrystal Assemblies
journal, August 2000
- Murray, C. B.; Kagan, C. R.; Bawendi, M. G.
- Annual Review of Materials Science, Vol. 30, Issue 1, p. 545-610
Controllable synthesis of nanocrystals in droplet reactors
journal, January 2018
- Pan, Liang-Jun; Tu, Jia-Wei; Ma, Hao-Tian
- Lab on a Chip, Vol. 18, Issue 1
Unveiling the Shape Evolution and Halide-Ion-Segregation in Blue-Emitting Formamidinium Lead Halide Perovskite Nanocrystals Using an Automated Microfluidic Platform
journal, January 2018
- Lignos, Ioannis; Protesescu, Loredana; Emiroglu, Dilara Börte
- Nano Letters, Vol. 18, Issue 2
Mechanistic Insights and Controlled Synthesis of Radioluminescent ZnSe Quantum Dots Using a Microfluidic Reactor
journal, November 2018
- Guidelli, Eder Jose; Lignos, Ioannis; Yoo, Jason Jungwan
- Chemistry of Materials, Vol. 30, Issue 23
Thermodynamic Fluctuations in a Reacting System—Measurement by Fluorescence Correlation Spectroscopy
journal, September 1972
- Magde, Douglas; Elson, Elliot; Webb, W. W.
- Physical Review Letters, Vol. 29, Issue 11
Automated microfluidic platform for systematic studies of colloidal perovskite nanocrystals: towards continuous nano-manufacturing
journal, January 2017
- Epps, Robert W.; Felton, Kobi C.; Coley, Connor W.
- Lab on a Chip, Vol. 17, Issue 23
Multistage Microfluidic Platform for the Continuous Synthesis of III-V Core/Shell Quantum Dots
journal, July 2018
- Baek, Jinyoung; Shen, Yi; Lignos, Ioannis
- Angewandte Chemie International Edition, Vol. 57, Issue 34
Extracting Spectral Dynamics from Single Chromophores in Solution
journal, July 2010
- Marshall, Lisa F.; Cui, Jian; Brokmann, Xavier
- Physical Review Letters, Vol. 105, Issue 5
Facile Droplet-based Microfluidic Synthesis of Monodisperse IV–VI Semiconductor Nanocrystals with Coupled In-Line NIR Fluorescence Detection
journal, April 2014
- Lignos, Ioannis; Protesescu, Loredana; Stavrakis, Stavros
- Chemistry of Materials, Vol. 26, Issue 9
Flow Synthesis of Biocompatible Fe 3 O 4 Nanoparticles: Insight into the Effects of Residence Time, Fluid Velocity, and Tube Reactor Dimension on Particle Size Distribution
journal, February 2015
- Jiao, Mingxia; Zeng, Jianfeng; Jing, Lihong
- Chemistry of Materials, Vol. 27, Issue 4
Reconceptualizing Fluorescence Correlation Spectroscopy for Monitoring and Analyzing Periodically Passing Objects
journal, October 2017
- Zamir, Eli; Frey, Christoph; Weiss, Marian
- Analytical Chemistry, Vol. 89, Issue 21
Colloidal nanoparticles as advanced biological sensors
journal, October 2014
- Howes, Philip D.; Chandrawati, Rona; Stevens, Molly M.
- Science, Vol. 346, Issue 6205
A serial dilution microfluidic device using a ladder network generating logarithmic or linear concentrations
journal, January 2008
- Kim, Choong; Lee, Kangsun; Kim, Jong Hyun
- Lab on a Chip, Vol. 8, Issue 3
Prospects of Colloidal Nanocrystals for Electronic and Optoelectronic Applications
journal, January 2010
- Talapin, Dmitri V.; Lee, Jong-Soo; Kovalenko, Maksym V.
- Chemical Reviews, Vol. 110, Issue 1
Tracking the Fluorescence Lifetimes of Cesium Lead Halide Perovskite Nanocrystals During Their Synthesis Using a Fully Automated Optofluidic Platform
journal, November 2019
- Lignos, Ioannis; Maceiczyk, Richard M.; Kovalenko, Maksym V.
- Chemistry of Materials, Vol. 32, Issue 1
Synthesis of 1 nm Pd Nanoparticles in a Microfluidic Reactor: Insights from in Situ X-ray Absorption Fine Structure Spectroscopy and Small-Angle X-ray Scattering
journal, May 2015
- Karim, Ayman M.; Al Hasan, Naila; Ivanov, Sergei
- The Journal of Physical Chemistry C, Vol. 119, Issue 23
Millisecond-Timescale Monitoring of PbS Nanoparticle Nucleation and Growth Using Droplet-Based Microfluidics
journal, May 2015
- Lignos, Ioannis; Stavrakis, Stavros; Kilaj, Ardita
- Small, Vol. 11, Issue 32
In-Situ Microfluidic Study of Biphasic Nanocrystal Ligand-Exchange Reactions Using an Oscillatory Flow Reactor
journal, November 2017
- Shen, Yi; Abolhasani, Milad; Chen, Yue
- Angewandte Chemie International Edition, Vol. 56, Issue 51
Photon-correlation Fourier spectroscopy
journal, January 2006
- Brokmann, Xavier; Bawendi, Moungi; Coolen, Laurent
- Optics Express, Vol. 14, Issue 13
Real-Time Sizing of Nanoparticles in Microfluidic Channels Using Confocal Correlation Spectroscopy
journal, January 2006
- Kuyper, Christopher L.; Budzinski, Kristi L.; Lorenz, Robert M.
- Journal of the American Chemical Society, Vol. 128, Issue 3
PbS Nanocrystal Emission Is Governed by Multiple Emissive States
journal, September 2016
- Caram, Justin R.; Bertram, Sophie N.; Utzat, Hendrik
- Nano Letters, Vol. 16, Issue 10
Differential detection photothermal spectroscopy: towards ultra-fast and sensitive label-free detection in picoliter & femtoliter droplets
journal, January 2017
- Maceiczyk, Richard M.; Hess, David; Chiu, Flora W. Y.
- Lab Chip, Vol. 17, Issue 21
The “Surface Optical” Phonon in CdSe Nanocrystals
journal, March 2014
- Lin, Chen; Kelley, David F.; Rico, Mikaela
- ACS Nano, Vol. 8, Issue 4