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Title: Molecular origins of bulk viscosity in liquid water

Abstract

The shear viscous response of water is closely associated with changes in network connectivity on the sub ps timescale. The bulk viscous response is shown here to be associated with local density fluctuations and rotational motion around 1–3 ps.

Authors:
 [1];  [1];  [2]; ORCiD logo [3];  [3];  [3];  [4]; ORCiD logo [1]
  1. Department of Chemical and Environmental Engineering, University of Cincinnati, Cincinnati, USA
  2. Shull Wollan Center—a Joint Institute for Neutron Sciences, Oak Ridge National Laboratory, Oak Ridge, USA
  3. Neutron Scattering Division, Oak Ridge National Laboratory, Oak Ridge, USA
  4. Neutron Technologies Division, Oak Ridge National Laboratory, Oak Ridge, USA
Publication Date:
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1615548
Grant/Contract Number:  
DEAC0500OR22725
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Physical Chemistry Chemical Physics. PCCP
Additional Journal Information:
Journal Name: Physical Chemistry Chemical Physics. PCCP Journal Volume: 22 Journal Issue: 17; Journal ID: ISSN 1463-9076
Publisher:
Royal Society of Chemistry (RSC)
Country of Publication:
United Kingdom
Language:
English

Citation Formats

Yahya, Ahmad, Tan, Luoxi, Perticaroli, Stefania, Mamontov, Eugene, Pajerowski, Daniel, Neuefeind, Joerg, Ehlers, Georg, and Nickels, Jonathan D. Molecular origins of bulk viscosity in liquid water. United Kingdom: N. p., 2020. Web. doi:10.1039/D0CP01560A.
Yahya, Ahmad, Tan, Luoxi, Perticaroli, Stefania, Mamontov, Eugene, Pajerowski, Daniel, Neuefeind, Joerg, Ehlers, Georg, & Nickels, Jonathan D. Molecular origins of bulk viscosity in liquid water. United Kingdom. doi:https://doi.org/10.1039/D0CP01560A
Yahya, Ahmad, Tan, Luoxi, Perticaroli, Stefania, Mamontov, Eugene, Pajerowski, Daniel, Neuefeind, Joerg, Ehlers, Georg, and Nickels, Jonathan D. Wed . "Molecular origins of bulk viscosity in liquid water". United Kingdom. doi:https://doi.org/10.1039/D0CP01560A.
@article{osti_1615548,
title = {Molecular origins of bulk viscosity in liquid water},
author = {Yahya, Ahmad and Tan, Luoxi and Perticaroli, Stefania and Mamontov, Eugene and Pajerowski, Daniel and Neuefeind, Joerg and Ehlers, Georg and Nickels, Jonathan D.},
abstractNote = {The shear viscous response of water is closely associated with changes in network connectivity on the sub ps timescale. The bulk viscous response is shown here to be associated with local density fluctuations and rotational motion around 1–3 ps.},
doi = {10.1039/D0CP01560A},
journal = {Physical Chemistry Chemical Physics. PCCP},
number = 17,
volume = 22,
place = {United Kingdom},
year = {2020},
month = {5}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
DOI: https://doi.org/10.1039/D0CP01560A

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