High-throughput investigation of crystal-to-glass transformation of Ti–Ni–Cu ternary alloy

Hui, Jian; Ma, Haiqian; Wu, Zheyu; Zhang, Zhan; Ren, Yang; Zhang, Hengrui; Zhang, Lanting; Wang, Hong

doi:10.1038/s41598-019-56129-z

Title: High-throughput investigation of crystal-to-glass transformation of Ti–Ni–Cu ternary alloy

Journal Article · 27 December 2019 · Scientific Reports

DOI: https://doi.org/10.1038/s41598-019-56129-z · OSTI ID:1614756

Hui, Jian ^[1]; Ma, Haiqian ^[1]; Wu, Zheyu ^[1]; Zhang, Zhan ^[2]; Ren, Yang ^[2];

^[1];

^[1]; Wang, Hong ^[1]

Shanghai Jiao Tong Univ. (China)
Argonne National Lab. (ANL), Argonne, IL (United States)

A high-throughput investigation of metallic glass formation via solid-state reaction was reported in this paper. Combinatorial multilayered thin-film chips covering the entire Ti-Ni-Cu ternary system were prepared using ion beam sputtering technique. Microbeam synchrotron X-ray diffraction (XRD) and X-ray fluorescence (XRF) measurements were conducted, with 1,325 data points collected from each chip, to map out the composition and the phase constitution before and after annealing at 373 K for 110 hours. The composition dependence of the crystal-to-glass transition by solid-state reaction was surveyed using this approach. The resulting composition-phase map is consistent with previously reported results. Time-of-flight secondary ion mass spectroscopy (ToF-SIMS) was performed on the representative compositions to determine the inter-diffusion between layers, the result shows that the diffusion of Ti is the key factor for the crystal-to-glass transition. In addition, both layer thickness and layer sequence play important roles as well. This work demonstrates that combinatorial chip technique is an efficient way for systematic and rapid study of crystal-to-glass transition for multi-component alloy systems.

View Accepted Manuscript (DOE)

Cite

Export

Save

Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: National Key Research and Development Program of China

Grant/Contract Number:: AC02-06CH11357; 2017YF0701900)

OSTI ID:: 1614756

Journal Information:: Scientific Reports, Vol. 9, Issue 1; ISSN 2045-2322

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 8 works

Citation information provided by
Web of Science

References (52)

Combinatorial solid-state chemistry of inorganic materials Koinuma, Hideomi; Takeuchi, Ichiro Nature Materials, Vol. 3, Issue 7 https://doi.org/10.1038/nmat1157	journal	July 2004
Transformation-mediated ductility in CuZr-based bulk metallic glasses Pauly, S.; Gorantla, S.; Wang, G. Nature Materials, Vol. 9, Issue 6 https://doi.org/10.1038/nmat2767	journal	May 2010
Amorphisation in solid metallic systems Samwer, K. Physics Reports, Vol. 161, Issue 1 https://doi.org/10.1016/0370-1573(88)90006-3	journal	April 1988
Preparation of ‘‘amorphous’’ Ni ₆ ₀ Nb ₄ ₀ by mechanical alloying Koch, C. C.; Cavin, O. B.; McKamey, C. G. Applied Physics Letters, Vol. 43, Issue 11 https://doi.org/10.1063/1.94213	journal	December 1983
COMBINATORIAL MATERIALS SYNTHESIS AND SCREENING: An Integrated Materials Chip Approach to Discovery and Optimization of Functional Materials Xiang, X. -D. Annual Review of Materials Science, Vol. 29, Issue 1 https://doi.org/10.1146/annurev.matsci.29.1.149	journal	August 1999
Determination of the thermodynamic functions and calculation of phase diagrams for metastable phases Bormann, R.; Zöltzer, K. Physica Status Solidi (a), Vol. 131, Issue 2 https://doi.org/10.1002/pssa.2211310238	journal	June 1992
Combinatorial Strategies for Synthesis and Characterization of Alloy Microstructures over Large Compositional Ranges Li, Yanglin; Jensen, Katharine E.; Liu, Yanhui ACS Combinatorial Science, Vol. 18, Issue 10 https://doi.org/10.1021/acscombsci.6b00040	journal	September 2016
High-temperature bulk metallic glasses developed by combinatorial methods Li, Ming-Xing; Zhao, Shao-Fan; Lu, Zhen Nature, Vol. 569, Issue 7754 https://doi.org/10.1038/s41586-019-1145-z	journal	May 2019
Non-crystalline Structure in Solidified Gold–Silicon Alloys Klement, W.; Willens, R. H.; Duwez, Pol Nature, Vol. 187, Issue 4740 https://doi.org/10.1038/187869b0	journal	September 1960
Solid-state reaction and structure in compositionally modulated zirconium-nickel and titanium-nickel films Clemens, Bruce M. Physical Review B, Vol. 33, Issue 11 https://doi.org/10.1103/PhysRevB.33.7615	journal	June 1986
A combinatorial thin film sputtering approach for synthesizing and characterizing ternary ZrCuAl metallic glasses Deng, Y. P.; Guan, Y. F.; Fowlkes, J. D. Intermetallics, Vol. 15, Issue 9 https://doi.org/10.1016/j.intermet.2007.02.011	journal	September 2007
Stabilization of metallic supercooled liquid and bulk amorphous alloys Inoue, Akihisa Acta Materialia, Vol. 48, Issue 1 https://doi.org/10.1016/S1359-6454(99)00300-6	journal	January 2000
Thermodynamic and kinetic aspects of the crystal to glass transformation in metallic materials Johnson, W. Progress in Materials Science, Vol. 30, Issue 2 https://doi.org/10.1016/0079-6425(86)90005-8	journal	January 1986
Crystal-Glass Transition in Zr-Co Multilayers Observed by in situ X-Ray Diffraction Measurements Krebs, H. U.; Samwer, K. Europhysics Letters (EPL), Vol. 2, Issue 2 https://doi.org/10.1209/0295-5075/2/2/012	journal	July 1986
A damage-tolerant glass Demetriou, Marios D.; Launey, Maximilien E.; Garrett, Glenn Nature Materials, Vol. 10, Issue 2 https://doi.org/10.1038/nmat2930	journal	January 2011
Combinatorial and High-Throughput Screening of Materials Libraries: Review of State of the Art Potyrailo, Radislav; Rajan, Krishna; Stoewe, Klaus ACS Combinatorial Science, Vol. 13, Issue 6 https://doi.org/10.1021/co200007w	journal	August 2011
Nanomoulding with amorphous metals Kumar, Golden; Tang, Hong X.; Schroers, Jan Nature, Vol. 457, Issue 7231 https://doi.org/10.1038/nature07718	journal	February 2009
Mapping Quantum Yield for (Fe–Zn–Sn–Ti)O _x Photoabsorbers Using a High Throughput Photoelectrochemical Screening System Xiang, Chengxiang; Haber, Joel; Marcin, Martin ACS Combinatorial Science, Vol. 16, Issue 3 https://doi.org/10.1021/co400081w	journal	February 2014
Calculations of Mixing Enthalpy and Mismatch Entropy for Ternary Amorphous Alloys Takeuchi, Akira; Inoue, Akihisa Materials Transactions, JIM, Vol. 41, Issue 11 https://doi.org/10.2320/matertrans1989.41.1372	journal	January 2000
Formation of an Amorphous Alloy by Solid-State Reaction of the Pure Polycrystalline Metals Schwarz, R. B.; Johnson, W. L. Physical Review Letters, Vol. 51, Issue 5 https://doi.org/10.1103/PhysRevLett.51.415	journal	August 1983
Microstructural properties of (Ba, Sr)TiO3 films fabricated from BaF2/SrF2/TiO2 amorphous multilayers using the combinatorial precursor method Takeuchi, I.; Chang, K.; Sharma, R. P. Journal of Applied Physics, Vol. 90, Issue 5 https://doi.org/10.1063/1.1388563	journal	September 2001
Rapid Construction of Fe–Co–Ni Composition-Phase Map by Combinatorial Materials Chip Approach Xing, Hui; Zhao, Bingbing; Wang, Yujie ACS Combinatorial Science, Vol. 20, Issue 3 https://doi.org/10.1021/acscombsci.7b00171	journal	January 2018
Maximum thickness of amorphous NiZr interlayers formed by a solid‐state reaction technique Meng, W. J.; Nieh, C. W.; Johnson, W. L. Applied Physics Letters, Vol. 51, Issue 21 https://doi.org/10.1063/1.98546	journal	November 1987
Solid‐state interdiffusion reactions in Ni/Ti and Ni/Zr multilayered thin films Meng, W. J.; Fultz, B.; Ma, E. Applied Physics Letters, Vol. 51, Issue 9 https://doi.org/10.1063/1.98326	journal	August 1987
Controlling solid-state reaction mechanisms using diffusion length in ultrathin-film superlattice composites Fister, Loreli; Johnson, David C. Journal of the American Chemical Society, Vol. 114, Issue 12 https://doi.org/10.1021/ja00038a029	journal	June 1992
Cobalt-based bulk glassy alloy with ultrahigh strength and soft magnetic properties Inoue, Akihisa; Shen, Baolong; Koshiba, Hisato Nature Materials, Vol. 2, Issue 10 https://doi.org/10.1038/nmat982	journal	September 2003
Roles of minor additions in formation and properties of bulk metallic glasses Wang, W. Progress in Materials Science, Vol. 52, Issue 4 https://doi.org/10.1016/j.pmatsci.2006.07.003	journal	May 2007
High-Throughput Bubble Screening Method for Combinatorial Discovery of Electrocatalysts for Water Splitting Xiang, Chengxiang; Suram, Santosh K.; Haber, Joel A. ACS Combinatorial Science, Vol. 16, Issue 2 https://doi.org/10.1021/co400151h	journal	January 2014
Hydrogen absorption in various zirconium- and hafnium-based intermetallic compounds Van Essen, R. M.; Buschow, K. H. J. Journal of the Less Common Metals, Vol. 64, Issue 2 https://doi.org/10.1016/0022-5088(79)90178-4	journal	April 1979
Under what conditions can a glass be formed? Turnbull, David Contemporary Physics, Vol. 10, Issue 5 https://doi.org/10.1080/00107516908204405	journal	September 1969
Combinatorial search of thermoelastic shape-memory alloys with extremely small hysteresis width Cui, Jun; Chu, Yong S.; Famodu, Olugbenga O. Nature Materials, Vol. 5, Issue 4 https://doi.org/10.1038/nmat1593	journal	March 2006
On the layer sequence and morphology in solid-state displacement reactions van Loo, F. J. J.; van Beek, J. A.; Bastin, G. F. Oxidation of Metals, Vol. 22, Issue 3-4 https://doi.org/10.1007/bf00656903	journal	October 1984
Hydrogen absorption in various zirconium- and hafnium-based intermetallic compounds Van Essen, R. M.; Buschow, K. H. J. Journal of the Less Common Metals, Vol. 64, Issue 2 https://doi.org/10.1016/0022-5088(79)90178-4	journal	April 1979
Amorphisation in solid metallic systems Samwer, K. Physics Reports, Vol. 161, Issue 1 https://doi.org/10.1016/0370-1573(88)90006-3	journal	April 1988
Rapid Construction of Fe–Co–Ni Composition-Phase Map by Combinatorial Materials Chip Approach Xing, Hui; Zhao, Bingbing; Wang, Yujie ACS Combinatorial Science, Vol. 20, Issue 3 https://doi.org/10.1021/acscombsci.7b00171	journal	January 2018
High-Throughput Bubble Screening Method for Combinatorial Discovery of Electrocatalysts for Water Splitting Xiang, Chengxiang; Suram, Santosh K.; Haber, Joel A. ACS Combinatorial Science, Vol. 16, Issue 2 https://doi.org/10.1021/co400151h	journal	January 2014
Controlling solid-state reaction mechanisms using diffusion length in ultrathin-film superlattice composites Fister, Loreli; Johnson, David C. Journal of the American Chemical Society, Vol. 114, Issue 12 https://doi.org/10.1021/ja00038a029	journal	June 1992
Non-crystalline Structure in Solidified Gold–Silicon Alloys Klement, W.; Willens, R. H.; Duwez, Pol Nature, Vol. 187, Issue 4740 https://doi.org/10.1038/187869b0	journal	September 1960
Nanomoulding with amorphous metals Kumar, Golden; Tang, Hong X.; Schroers, Jan Nature, Vol. 457, Issue 7231 https://doi.org/10.1038/nature07718	journal	February 2009
Combinatorial solid-state chemistry of inorganic materials Koinuma, Hideomi; Takeuchi, Ichiro Nature Materials, Vol. 3, Issue 7 https://doi.org/10.1038/nmat1157	journal	July 2004
Combinatorial search of thermoelastic shape-memory alloys with extremely small hysteresis width Cui, Jun; Chu, Yong S.; Famodu, Olugbenga O. Nature Materials, Vol. 5, Issue 4 https://doi.org/10.1038/nmat1593	journal	March 2006
A damage-tolerant glass Demetriou, Marios D.; Launey, Maximilien E.; Garrett, Glenn Nature Materials, Vol. 10, Issue 2 https://doi.org/10.1038/nmat2930	journal	January 2011
Cobalt-based bulk glassy alloy with ultrahigh strength and soft magnetic properties Inoue, Akihisa; Shen, Baolong; Koshiba, Hisato Nature Materials, Vol. 2, Issue 10 https://doi.org/10.1038/nmat982	journal	September 2003
High-temperature bulk metallic glasses developed by combinatorial methods Li, Ming-Xing; Zhao, Shao-Fan; Lu, Zhen Nature, Vol. 569, Issue 7754 https://doi.org/10.1038/s41586-019-1145-z	journal	May 2019
Preparation of ‘‘amorphous’’ Ni ₆ ₀ Nb ₄ ₀ by mechanical alloying Koch, C. C.; Cavin, O. B.; McKamey, C. G. Applied Physics Letters, Vol. 43, Issue 11 https://doi.org/10.1063/1.94213	journal	December 1983
Solid‐state interdiffusion reactions in Ni/Ti and Ni/Zr multilayered thin films Meng, W. J.; Fultz, B.; Ma, E. Applied Physics Letters, Vol. 51, Issue 9 https://doi.org/10.1063/1.98326	journal	August 1987
Maximum thickness of amorphous NiZr interlayers formed by a solid‐state reaction technique Meng, W. J.; Nieh, C. W.; Johnson, W. L. Applied Physics Letters, Vol. 51, Issue 21 https://doi.org/10.1063/1.98546	journal	November 1987
Micromechanism for Metallic-Glass Formation by Solid-State Reactions Schröder, H.; Samwer, K.; Köster, U. Physical Review Letters, Vol. 54, Issue 3 https://doi.org/10.1103/physrevlett.54.197	journal	January 1985
COMBINATORIAL MATERIALS SYNTHESIS AND SCREENING: An Integrated Materials Chip Approach to Discovery and Optimization of Functional Materials Xiang, X. -D. Annual Review of Materials Science, Vol. 29, Issue 1 https://doi.org/10.1146/annurev.matsci.29.1.149	journal	August 1999
Crystal-Glass Transition in Zr-Co Multilayers Observed by in situ X-Ray Diffraction Measurements Krebs, H. U.; Samwer, K. Europhysics Letters (EPL), Vol. 2, Issue 2 https://doi.org/10.1209/0295-5075/2/2/012	journal	July 1986
Individualized Pixel Synthesis and Characterization of Combinatorial Materials Chips Xiang, Xiao-Dong; Wang, Gang; Zhang, Xiaokun Engineering, Vol. 1, Issue 2 https://doi.org/10.15302/j-eng-2015041	journal	June 2015
Calculations of Mixing Enthalpy and Mismatch Entropy for Ternary Amorphous Alloys Takeuchi, Akira; Inoue, Akihisa Materials Transactions, JIM, Vol. 41, Issue 11 https://doi.org/10.2320/matertrans1989.41.1372	journal	January 2000

Similar Records

High-throughput investigation of structural evolution upon solid-state in Cu–Cr–Co combinatorial multilayer thin-film

Journal Article · 2022 · Materials & Design · OSTI ID:1885799

Hui, Jian; Hu, Qingyun; Zhang, Hengrui; +5 more

Toward an Understanding of Surface Layer Formation, Growth, and Transformation at the Glass–Fluid Interface

Journal Article · 2018 · Geochimica et Cosmochimica Acta · OSTI ID:1423113

Hopf, Juliane; Eskelsen, Jeremy R.; Chiu, Michelle Y.; +4 more

Ternary titanium transition metal bismuthides Ti{sub 4}TBi{sub 2} with T = Cr, Mn, Fe, Co, and Ni

Journal Article · 1997 · Journal of Solid State Chemistry · OSTI ID:613703

Richter, C G; Jeitschko, W; Kuennen, B; +1 more

Related Subjects

36 MATERIALS SCIENCE
metals and alloys
synthesis and processing

Title: High-throughput investigation of crystal-to-glass transformation of Ti–Ni–Cu ternary alloy

Citation Formats

References (52)

Similar Records

Related Subjects