DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Dynamical electron vortices in attosecond double photoionization of H2

Journal Article · · Physical Review A
 [1];  [2];  [2];  [3];  [4];  [5]
  1. Univ. of Nebraska, Lincoln, NE (United States); DOE/OSTI
  2. Voronezh State Univ. (Russia)
  3. Aarhus Univ. (Denmark)
  4. Univ. of Rochester, NY (United States)
  5. Univ. of Nebraska, Lincoln, NE (United States)

We study electron momentum vortices in single-photon double ionization of H2 by time-delayed, counter-rotating, elliptically polarized attosecond pulses propagating along kˆ either parallel or perpendicular to the molecular axis R. For ˆk∥R, kinematical vortices occur similar to those found for He. For kˆ⊥R, we find dynamical vortex structures originating from an ellipticity-dependent interplay of 1Σ$$^{+}_{u}$$ and 1Π$$^{+}_{u}$$ continuum amplitudes. Furthermore, we propose a complete experiment to determine the magnitudes and relative phase of these amplitudes by varying pulse ellipticities and time delays.

Research Organization:
Univ. of Nebraska, Lincoln, NE (United States); Univ. of Rochester, NY (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA)
Grant/Contract Number:
FG03-96ER14646; NA0001944
OSTI ID:
1614597
Journal Information:
Physical Review A, Journal Name: Physical Review A Journal Issue: 6 Vol. 98; ISSN 2469-9926
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (32)

Potential-energy curves for molecular hydrogen and its ions journal December 1970
High precision variational calculations for the Born-Oppenheimer energies of the ground state of the hydrogen molecule journal March 2006
A helium-like description of molecular hydrogen photo-double ionization journal September 1998
Solving the three-body Coulomb breakup problem using exterior complex scaling journal August 2004
Photoionization of triatomic molecular ions ${{\rm{H}}}_{3}^{2+}$ by intense bichromatic circularly polarized attosecond UV laser pulses journal May 2017
Classical two-slit interference effects in double photoionization of molecular hydrogen at high energies journal November 2009
Doubly-excited state effects on two-photon double ionization of helium by time-delayed, oppositely circularly-polarized attosecond pulses journal October 2017
A Molecular Beam Resonance Method with Separated Oscillating Fields journal June 1950
Double photoionization of aligned molecular hydrogen journal November 2006
Solving the m -mixing problem for the three-dimensional time-dependent Schrödinger equation by rotations: Application to strong-field ionization of H 2 + journal June 2007
Extracting continuum information from Ψ ( t ) in time-dependent wave-packet calculations journal December 2007
Grid-based methods for diatomic quantum scattering problems. III. Double photoionization of molecular hydrogen in prolate spheroidal coordinates journal August 2010
Breakup of the aligned H 2 molecule by xuv laser pulses: A time-dependent treatment in prolate spheroidal coordinates journal April 2011
Time-dependent calculations of double photoionization of the aligned H 2 molecule journal January 2012
One-photon double ionization of H 2 with arbitrary orientation journal December 2013
Photoelectron momentum distributions of molecules in bichromatic circularly polarized attosecond UV laser fields journal May 2016
Multistart spiral electron vortices in ionization by circularly polarized UV pulses journal July 2016
Kinematical vortices in double photoionization of helium by attosecond pulses journal July 2017
Control of three-dimensional electron vortices from femtosecond multiphoton ionization journal October 2017
Momentum Vortices on Pairs Production by Two Counter-Rotating Fields journal October 2017
Optimizing the FEDVR-TDCC code for exploring the quantum dynamics of two-electron systems in intense laser pulses journal May 2010
Physical Interpretation of the “Kinetic Energy Release” Effect in the Double Photoionization of H 2 journal May 2008
Classical Two-Slit Interference Effects in Double Photoionization of Molecular Hydrogen at High Energies journal October 2008
Nonlinear Dichroism in Back-to-Back Double Ionization of He by an Intense Elliptically Polarized Few-Cycle Extreme Ultraviolet Pulse journal November 2014
Electron Vortices in Photoionization by Circularly Polarized Attosecond Pulses journal September 2015
Electron Vortices in Femtosecond Multiphoton Ionization journal February 2017
Role of Nuclear Motion in Double Ionization of Molecular Hydrogen by a Single Photon journal February 2007
Triple Differential Cross Sections for the Double Photoionization of H 2 journal April 2007
Complete Photo-Induced Breakup of the H2 Molecule as a Probe of Molecular Electron Correlation journal December 2005
Odd-fold-symmetric spiral momentum distributions and their Stark distortions in hydrogen journal January 2018
Dynamic Stark induced vortex momentum of hydrogen in circular fields journal January 2018
Electron vortices in photoionization by a pair of elliptically polarized attosecond pulses [Electron vortices in photoionization by a pair of elliptically polarized attosecond pulses] journal January 2017

Cited By (6)

Two-photon laser-assisted electron scattering on hydrogen atom journal March 2019
Asymmetry of molecular frame photoelectron angular distributions in ${{\rm{H}}}_{2}^{+}$ by intense two-color attosecond pulses: coherent excitation and charge migration effects journal February 2020
Two-photon laser-assisted electron scattering on Hydrogen atom journal January 2020
Modeling tomographic measurements of photoelectron vortices in counter-rotating circularly polarized laser pulses journal December 2019
Molecular Symmetry-Mixed Dichroism in Double Photoionization of H 2 journal October 2019
Modeling tomographic measurements of photoelectron vortices in counter-rotating circularly polarized laser pulses text January 2019