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Title: Electronic and Optical Properties of 2D Transition Metal Carbides and Nitrides (MXenes)

Abstract

2D transition metal carbides, carbonitrides, and nitrides, known as MXenes, are a rapidly growing family of 2D materials with close to 30 members experimentally synthesized, and dozens more studied theoretically. They exhibit outstanding electronic, optical, mechanical, and thermal properties with versatile transition metal and surface chemistries. They have shown promise in many applications, such as energy storage, electromagnetic interference shielding, transparent electrodes, sensors, catalysis, photothermal therapy, etc. The high electronic conductivity and wide range of optical absorption properties of MXenes are the key to their success in the aforementioned applications. However, relatively little is currently known about their fundamental electronic and optical properties, limiting their use to their full potential. In this review, MXenes' electronic and optical properties from both theoretical and experimental perspectives, as well as applications related to those properties, are discussed, providing a guide for researchers who are exploring those properties of MXenes.

Authors:
ORCiD logo [1]; ORCiD logo [1]
  1. Drexel Univ., Philadelphia, PA (United States)
Publication Date:
Research Org.:
Drexel Univ., Philadelphia, PA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1612996
Alternate Identifier(s):
OSTI ID: 1482743
Grant/Contract Number:  
SC0018618
Resource Type:
Accepted Manuscript
Journal Name:
Advanced Materials
Additional Journal Information:
Journal Volume: 30; Journal Issue: 52; Journal ID: ISSN 0935-9648
Publisher:
Wiley
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; chemistry; science & technology - other topics; materials science; physics; 2D transition metal carbides; 2D transition metal nitrides; electronic properties; MXenes; optical properties; optoelectronics

Citation Formats

Hantanasirisakul, Kanit, and Gogotsi, Yury. Electronic and Optical Properties of 2D Transition Metal Carbides and Nitrides (MXenes). United States: N. p., 2018. Web. doi:10.1002/adma.201804779.
Hantanasirisakul, Kanit, & Gogotsi, Yury. Electronic and Optical Properties of 2D Transition Metal Carbides and Nitrides (MXenes). United States. doi:10.1002/adma.201804779.
Hantanasirisakul, Kanit, and Gogotsi, Yury. Mon . "Electronic and Optical Properties of 2D Transition Metal Carbides and Nitrides (MXenes)". United States. doi:10.1002/adma.201804779. https://www.osti.gov/servlets/purl/1612996.
@article{osti_1612996,
title = {Electronic and Optical Properties of 2D Transition Metal Carbides and Nitrides (MXenes)},
author = {Hantanasirisakul, Kanit and Gogotsi, Yury},
abstractNote = {2D transition metal carbides, carbonitrides, and nitrides, known as MXenes, are a rapidly growing family of 2D materials with close to 30 members experimentally synthesized, and dozens more studied theoretically. They exhibit outstanding electronic, optical, mechanical, and thermal properties with versatile transition metal and surface chemistries. They have shown promise in many applications, such as energy storage, electromagnetic interference shielding, transparent electrodes, sensors, catalysis, photothermal therapy, etc. The high electronic conductivity and wide range of optical absorption properties of MXenes are the key to their success in the aforementioned applications. However, relatively little is currently known about their fundamental electronic and optical properties, limiting their use to their full potential. In this review, MXenes' electronic and optical properties from both theoretical and experimental perspectives, as well as applications related to those properties, are discussed, providing a guide for researchers who are exploring those properties of MXenes.},
doi = {10.1002/adma.201804779},
journal = {Advanced Materials},
number = 52,
volume = 30,
place = {United States},
year = {2018},
month = {11}
}

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Effects of Different Surface Functionalization and Doping on the Electronic Transport Properties of M 2 CT x –M 2 CO 2 Heterojunction Devices
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Organic-Base-Driven Intercalation and Delamination for the Production of Functionalized Titanium Carbide Nanosheets with Superior Photothermal Therapeutic Performance
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Fabrication of urchin-like ZnO-MXene nanocomposites for high-performance electromagnetic absorption
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Ti 3 C 2 MXenes with Modified Surface for High-Performance Electromagnetic Absorption and Shielding in the X-Band
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High and anisotropic carrier mobility in experimentally possible Ti 2 CO 2 (MXene) monolayers and nanoribbons
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Synthesis of two-dimensional titanium nitride Ti 4 N 3 (MXene)
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X-ray photoelectron spectroscopy of select multi-layered transition metal carbides (MXenes)
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Electronic properties and applications of MXenes: a theoretical review
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Refractory Plasmonics with Titanium Nitride: Broadband Metamaterial Absorber
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A highly flexible and sensitive piezoresistive sensor based on MXene with greatly changed interlayer distances
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Machine-Learning-Assisted Accurate Band Gap Predictions of Functionalized MXene
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Enhanced Terahertz Shielding of MXenes with Nano-Metamaterials
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On the organization and thermal behavior of functional groups on Ti 3 C 2 MXene surfaces in vacuum
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Highly Broadband Absorber Using Plasmonic Titanium Carbide (MXene)
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Heterostructures of MXenes and N-doped graphene as highly active bifunctional electrocatalysts
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Solution-processed titanium carbide MXene films examined as highly transparent conductors
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Exploration and prediction of topological electronic materials based on first-principles calculations
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Chemical Origin of Termination-Functionalized MXenes: Ti 3 C 2 T 2 as a Case Study
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2D Superparamagnetic Tantalum Carbide Composite MXenes for Efficient Breast-Cancer Theranostics
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Ti 3 C 2 MXenes modified with in situ grown carbon nanotubes for enhanced electromagnetic wave absorption properties
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Synthesis and Electrochemical Properties of Two-Dimensional Hafnium Carbide
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Graphene-like transition-metal nanocarbides and nanonitrides
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2D Ultrathin MXene-Based Drug-Delivery Nanoplatform for Synergistic Photothermal Ablation and Chemotherapy of Cancer
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Flexible and conductive MXene films and nanocomposites with high capacitance
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MXene-Silicon Van Der Waals Heterostructures for High-Speed Self-Driven Photodetectors
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MoS 2 /MX 2 heterobilayers: bandgap engineering via tensile strain or external electrical field
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Synthesis and characterization of two-dimensional Nb 4 C 3 (MXene)
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Rational Design of Two-Dimensional Metallic and Semiconducting Spintronic Materials Based on Ordered Double-Transition-Metal MXenes
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MXenes: Reusable materials for NH3 sensor or capturer by controlling the charge injection
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Ion Intercalation into Two-Dimensional Transition-Metal Carbides: Global Screening for New High-Capacity Battery Materials
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Two-Dimensional Titanium Carbide for Efficiently Reductive Removal of Highly Toxic Chromium(VI) from Water
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First-principles study of a MXene terahertz detector
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W-Based Atomic Laminates and Their 2D Derivative W 1.33 C MXene with Vacancy Ordering
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MXene: an emerging two-dimensional material for future energy conversion and storage applications
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Synthesis of two-dimensional Ti3C2Tx MXene using HCl+LiF etchant: Enhanced exfoliation and delamination
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Predicting stable phase monolayer Mo 2 C (MXene), a superconductor with chemically-tunable critical temperature
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MXene Ti 3 C 2 : An Effective 2D Light-to-Heat Conversion Material
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High-Capacitance Mechanism for Ti 3 C 2 T x MXene by in Situ Electrochemical Raman Spectroscopy Investigation
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Electronic and Transport Properties of Ti 2 CO 2 MXene Nanoribbons
journal, July 2016

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Effect of surface functionalization on the electronic transport properties of Ti 3 C 2 MXene
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Conductive transparent V 2 CT x (MXene) films
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Large-scale delamination of multi-layers transition metal carbides and carbonitrides “MXenes”
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Preparation and methane adsorption of two-dimensional carbide Ti2C
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Structure of Nanocrystalline Ti 3 C 2 MXene Using Atomic Pair Distribution Function
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A Nanolaminated Magnetic Phase: Mn 2 GaC
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Cation Intercalation and High Volumetric Capacitance of Two-Dimensional Titanium Carbide
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Two-Dimensional Transition Metal Carbides
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Dispersions of Two-Dimensional Titanium Carbide MXene in Organic Solvents
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A Two-Dimensional Biodegradable Niobium Carbide (MXene) for Photothermal Tumor Eradication in NIR-I and NIR-II Biowindows
journal, November 2017

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Synthesis of Two-Dimensional Materials by Selective Extraction
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Fabrication of Ti 3 C 2 T x MXene Transparent Thin Films with Tunable Optoelectronic Properties
journal, April 2016

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Theoretical Prediction of the Intrinsic Half-Metallicity in Surface-Oxygen-Passivated Cr 2 N MXene
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An Organ-Like Titanium Carbide Material (MXene) with Multilayer Structure Encapsulating Hemoglobin for a Mediator-Free Biosensor
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Enhanced and tunable surface plasmons in two-dimensional Ti 3 C 2 stacks: Electronic structure versus boundary effects
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Oxide Thin-Film Electronics using All-MXene Electrical Contacts
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Rheological Characteristics of 2D Titanium Carbide (MXene) Dispersions: A Guide for Processing MXenes
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Studying of 2D Titanium Carbide Structure by Raman Spectroscopy after Heat Treatment in Argon and Hydrogen Atmospheres
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MXenes/graphene heterostructures for Li battery applications: a first principles study
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Role of the surface effect on the structural, electronic and mechanical properties of the carbide MXenes
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Selective Etching of Silicon from Ti 3 SiC 2 (MAX) To Obtain 2D Titanium Carbide (MXene)
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Large-Area Highly Conductive Transparent Two-Dimensional Ti 2 CT x Film
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Transition metal carbides go 2D
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3D Synergistical MXene/Reduced Graphene Oxide Aerogel for a Piezoresistive Sensor
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Room Temperature Gas Sensing of Two-Dimensional Titanium Carbide (MXene)
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Half-Metallic Ferromagnetism and Surface Functionalization-Induced Metal–Insulator Transition in Graphene-like Two-Dimensional Cr 2 C Crystals
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A novel nitrite biosensor based on the direct electrochemistry of hemoglobin immobilized on MXene-Ti3C2
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Theoretical prediction of two-dimensional functionalized MXene nitrides as topological insulators
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Two-dimensional molybdenum carbides: potential thermoelectric materials of the MXene family
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Control of electronic properties of 2D carbides (MXenes) by manipulating their transition metal layers
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Tunable Indirect to Direct Band Gap Transition of Monolayer Sc 2 CO 2 by the Strain Effect
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Large-gap two-dimensional topological insulator in oxygen functionalized MXene
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In situ atomistic insight into the growth mechanisms of single layer 2D transition metal carbides
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Two-Dimensional Molybdenum Carbide (MXene) as an Efficient Electrocatalyst for Hydrogen Evolution
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Tunable Multipolar Surface Plasmons in 2D Ti 3 C 2 T x MXene Flakes
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A graphene-based physiometer array for the analysis of single biological cells
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MXene as a novel intercalation-type pseudocapacitive cathode and anode for capacitive deionization
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Tuning the Basal Plane Functionalization of Two-Dimensional Metal Carbides (MXenes) To Control Hydrogen Evolution Activity
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Large-area high-quality 2D ultrathin Mo2C superconducting crystals
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Synthesis of nanoporous carbide-derived carbon by chlorination of titanium silicon carbide
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Achieving Type I, II, and III Heterojunctions Using Functionalized MXene
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Fluorine-Free Synthesis of High-Purity Ti 3 C 2 T x (T=OH, O) via Alkali Treatment
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Atomic Defects in Monolayer Titanium Carbide (Ti 3 C 2 T x ) MXene
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Strain-mediated type-I/type-II transition in MXene/Blue phosphorene van der Waals heterostructures for flexible optical/electronic devices
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Theranostic 2D Tantalum Carbide (MXene)
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New Two-Dimensional Niobium and Vanadium Carbides as Promising Materials for Li-Ion Batteries
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Charge transfer induced polymerization of EDOT confined between 2D titanium carbide layers
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Electronic properties of freestanding Ti 3 C 2 T x MXene monolayers
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Two-Dimensional Titanium Carbide (MXene) as Surface-Enhanced Raman Scattering Substrate
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Transparent and conductive Ti3C2Tx (MXene) thin film fabrication by electrohydrodynamic atomization technique
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Dirac points with giant spin-orbit splitting in the electronic structure of two-dimensional transition-metal carbides
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Optoelectronic and spectroscopic characterization of vapour-transport grown Cu 2 ZnSnS 4 single crystals
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Electronic and optical properties of 2D graphene-like compounds titanium carbides and nitrides: DFT calculations
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    Works referencing / citing this record:

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