Prospects and applications of plasmon-exciton interactions in the near-field regime

Kholmicheva, Natalia; Royo Romero, Luis; Cassidy, James; Zamkov, Mikhail

doi:10.1515/nanoph-2018-0143

Title: Prospects and applications of plasmon-exciton interactions in the near-field regime

Journal Article · 19 November 2018 · Nanophotonics (Online)

DOI: https://doi.org/10.1515/nanoph-2018-0143 · OSTI ID:1612692

Kholmicheva, Natalia ^[1]; Royo Romero, Luis ^[2]; Cassidy, James ^[2];

^[2]

Bowling Green State Univ., OH (United States); DOE/OSTI
Bowling Green State Univ., OH (United States)

Plasmonics is a rapidly developing field at the boundary of fundamental sciences and device engineering, which exploits the ability of metal nanostructures to concentrate electromagnetic radiation. The principal challenge lies in achieving an efficient conversion of the plasmon-concentrated field into some form of useful energy. To date, a substantial progress has been made within the scientific community in identifying the major pathways of the plasmon energy conversion. Strategies based on the hot electron injection and the near-field energy transfer have already shown promise in a number of proof-of-principle plasmonic architectures. Nevertheless, there are several fundamental questions that need to be addressed in the future to facilitate the transition of plasmonics to a variety of applications in both light amplification and optical detection. Of particular interest is a plasmon-induced resonance energy transfer (PIRET) process that couples the plasmon evanescent field to a semiconductor absorber via dipole-dipole interaction. This relatively unexplored mechanism has emerged as a promising light conversion strategy in the areas of photovoltaics and photocatalysis and represents the main focus of the present minireview. Along these lines, we highlight the key advances in this area and review some of the challenges associated with applications of the PIRET mechanism in nanostructured systems.

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Research Organization:: Bowling Green State Univ., OH (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Office of Science (SC)

Grant/Contract Number:: SC0016872

OSTI ID:: 1612692

Journal Information:: Nanophotonics (Online), Journal Name: Nanophotonics (Online) Journal Issue: 4 Vol. 8; ISSN 2192-8614

Publisher:: de GruyterCopyright Statement

Country of Publication:: United States

Language:: English

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Colloidal semiconductor nanocrystals in energy transfer reactions Moroz, Pavel; Royo Romero, Luis; Zamkov, Mikhail Chemical Communications, Vol. 55, Issue 21 https://doi.org/10.1039/c9cc00162j	journal	January 2019

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