Unusual behavior of cuprates explained by heterogeneous charge localization

Pelc, D.; Popčević, P.; Požek, M.; Greven, M.; Barišić, N.

doi:10.1126/sciadv.aau4538

Title: Unusual behavior of cuprates explained by heterogeneous charge localization

Journal Article · 25 January 2019 · Science Advances

DOI: https://doi.org/10.1126/sciadv.aau4538 · OSTI ID:1612522

Pelc, D. ^[1];

^[2];

^[3]; Greven, M. ^[4];

^[5]

Univ. of Zagreb (Croatia); Univ. of Minnesota, Minneapolis, MN (United States); DOE/OSTI
Technische Univ. Wien (Austria). Inst. of Solid State Physics; Inst. of Physics, Zagreb (Croatia)
Univ. of Zagreb (Croatia)
Univ. of Minnesota, Minneapolis, MN (United States)
Univ. of Zagreb (Croatia); Univ. of Minnesota, Minneapolis, MN (United States); Technische Univ. Wien (Austria). Inst. of Solid State Physics

The discovery of high-temperature superconductivity in cuprates ranks among the major scientific milestones of the past half century, yet pivotal questions regarding the complex phase diagram of these materials remain unanswered. Generally thought of as doped charge-transfer insulators, these complex oxides exhibit pseudogap, strange-metal, superconducting, and Fermi liquid behavior with increasing hole-dopant concentration. Motivated by recent experimental observations, here we introduce a phenomenological model wherein exactly one hole per planar copper-oxygen unit is delocalized with increasing doping and temperature. The model is percolative in nature, with parameters that are highly consistent with experiments. It comprehensively captures key unconventional experimental results, including the temperature and the doping dependence of the pseudogap phenomenon, the strange-metal linear temperature dependence of the planar resistivity, and the doping dependence of the superfluid density. The success and simplicity of the model greatly demystify the cuprate phase diagram and point to a local superconducting pairing mechanism.

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Research Organization:: Univ. of Minnesota, Minneapolis, MN (United States)

Sponsoring Organization:: Croatian Science Foundation; European Research Council (ERC); USDOE Office of Science (SC)

Grant/Contract Number:: SC0016371

OSTI ID:: 1612522

Journal Information:: Science Advances, Journal Name: Science Advances Journal Issue: 1 Vol. 5; ISSN 2375-2548

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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Direct relation between the low-energy spin excitations and superconductivity of overdoped high-$T_c$ superconductors Wakimoto, S.; Zhang, H.; Yamada, K. arXiv https://doi.org/10.48550/arxiv.cond-mat/0312648	text	January 2003
Evolution of the Hall Coefficient and the Peculiar Electronic Structure of the Cuprate Superconductors Ando, Yoichi; Kurita, Y.; Komiya, Seiki arXiv https://doi.org/10.48550/arxiv.cond-mat/0401034	text	January 2004
Scaling of the superfluid density in high-temperature superconductors Homes, C. C.; Dordevic, S. V.; Valla, T. arXiv https://doi.org/10.48550/arxiv.cond-mat/0410719	text	January 2004
Complexity in Strongly Correlated Electronic Systems Dagotto, Elbio arXiv https://doi.org/10.48550/arxiv.cond-mat/0509041	text	January 2005

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High-Temperature Superconductors as Ionic Metals Sunko, D. K. Journal of Superconductivity and Novel Magnetism, Vol. 33, Issue 1 https://doi.org/10.1007/s10948-019-05280-9	journal	October 2019
Universal superconducting precursor in three classes of unconventional superconductors Pelc, D.; Anderson, Z.; Yu, B. Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-10635-w	journal	June 2019
Diagonal nematicity in the pseudogap phase of HgBa2CuO4+δ Murayama, H.; Sato, Y.; Kurihara, R. Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-11200-1	journal	July 2019
Crossover of Charge Fluctuations across the Strange Metal Phase Diagram Husain, Ali A.; Mitrano, Matteo; Rak, Melinda S. Physical Review X, Vol. 9, Issue 4 https://doi.org/10.1103/physrevx.9.041062	journal	December 2019
Crossover of Charge Fluctuations across the Strange Metal Phase Diagram Husain, A. A.; Mitrano, M.; Rak, M. S. arXiv https://doi.org/10.48550/arxiv.1903.04038	text	January 2019

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