High harmonic generation spectroscopy via orbital angular momentum
Abstract
We present an experimental technique using orbital angular momentum (OAM) in a fundamental laser field to drive high harmonic generation (HHG). The mixing of beams with different OAM allows us to generate two laser foci tightly spaced which generate harmonics that interfere in the far field. Thus, this technique is an OAM based in situ HHG interferometric spectroscopic method. With this tool, we measure the phase and amplitude of the angle dependent multiorbital HHG emission in molecular nitrogen
- Authors:
-
[1];
[2]
- Kansas State Univ., Manhattan, KS (United States)
- Univ. of Connecticut, Storrs, CT (United States)
- Publication Date:
- Research Org.:
- Kansas State Univ., Manhattan, KS (United States); Univ. of Connecticut, Storrs, CT (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1610056
- Alternate Identifier(s):
- OSTI ID: 1559370
- Grant/Contract Number:
- FG02-86ER13491; SC0019098
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Chemical Physics
- Additional Journal Information:
- Journal Volume: 151; Journal Issue: 8; Journal ID: ISSN 0021-9606
- Publisher:
- American Institute of Physics (AIP)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; Chemistry; Physics; Optical devices; Lasers; Geometrical optics; Gas jet; Photoionization; Interferometry; Spectroscopy
Citation Formats
Troß, Jan, and Trallero-Herrero, Carlos A. High harmonic generation spectroscopy via orbital angular momentum. United States: N. p., 2019.
Web. doi:10.1063/1.5115152.
Troß, Jan, & Trallero-Herrero, Carlos A. High harmonic generation spectroscopy via orbital angular momentum. United States. https://doi.org/10.1063/1.5115152
Troß, Jan, and Trallero-Herrero, Carlos A. Wed .
"High harmonic generation spectroscopy via orbital angular momentum". United States. https://doi.org/10.1063/1.5115152. https://www.osti.gov/servlets/purl/1610056.
@article{osti_1610056,
title = {High harmonic generation spectroscopy via orbital angular momentum},
author = {Troß, Jan and Trallero-Herrero, Carlos A.},
abstractNote = {We present an experimental technique using orbital angular momentum (OAM) in a fundamental laser field to drive high harmonic generation (HHG). The mixing of beams with different OAM allows us to generate two laser foci tightly spaced which generate harmonics that interfere in the far field. Thus, this technique is an OAM based in situ HHG interferometric spectroscopic method. With this tool, we measure the phase and amplitude of the angle dependent multiorbital HHG emission in molecular nitrogen},
doi = {10.1063/1.5115152},
journal = {Journal of Chemical Physics},
number = 8,
volume = 151,
place = {United States},
year = {2019},
month = {8}
}
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Works referenced in this record:
Atomic transient recorder
journal, February 2004
- Kienberger, R.; Goulielmakis, E.; Uiberacker, M.
- Nature, Vol. 427, Issue 6977
Information Content of High Harmonics Generated from Aligned Molecules
journal, September 2007
- Ramakrishna, S.; Seideman, Tamar
- Physical Review Letters, Vol. 99, Issue 11
Uncovering multiple orbitals influence in high harmonic generation from aligned N 2
journal, October 2009
- Le, Anh-Thu; Lucchese, R. R.; Lin, C. D.
- Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 42, Issue 21
A Molecular Orbital Theory of Reactivity in Aromatic Hydrocarbons
journal, April 1952
- Fukui, Kenichi; Yonezawa, Teijiro; Shingu, Haruo
- The Journal of Chemical Physics, Vol. 20, Issue 4
Direct Measurement of the Angular Dependence of Ionization for , , and in Intense Laser Fields
journal, June 2007
- Pavičić, Domagoj; Lee, Kevin F.; Rayner, D. M.
- Physical Review Letters, Vol. 98, Issue 24
High Harmonic Generation from Multiple Orbitals in N2
journal, November 2008
- McFarland, B. K.; Farrell, J. P.; Bucksbaum, P. H.
- Science, Vol. 322, Issue 5905
Methods for the measurement of the duration of high-harmonic pulses
journal, November 1997
- Constant, Eric; Taranukhin, Vladimir D.; Stolow, Albert
- Physical Review A, Vol. 56, Issue 5
High harmonic generation with a spatially filtered optical parametric amplifier
journal, December 2008
- Bandulet, H-C; Comtois, D.; Shiner, A. D.
- Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 41, Issue 24
Atomic photoionization experiment by harmonic-generation spectroscopy
journal, March 2016
- Frolov, M. V.; Sarantseva, T. S.; Manakov, N. L.
- Physical Review A, Vol. 93, Issue 3
Measurement of field-free alignment of jet-cooled molecules by nonresonant femtosecond degenerate four-wave mixing
journal, March 2012
- Ren, Xiaoming; Makhija, Varun; Kumarappan, Vinod
- Physical Review A, Vol. 85, Issue 3
Simple interferometric technique for generation of a radially polarized light beam
journal, January 2005
- Passilly, Nicolas; Treussart, François; Hierle, Rolland
- Journal of the Optical Society of America A, Vol. 22, Issue 5
Alignment-assisted field-free orientation of rotationally cold CO molecules
journal, July 2014
- Ren, Xiaoming; Makhija, Varun; Li, Hui
- Physical Review A, Vol. 90, Issue 1
Molecular Recollision Interferometry in High Harmonic Generation
journal, February 2008
- Zhou, Xibin; Lock, Robynne; Li, Wen
- Physical Review Letters, Vol. 100, Issue 7
Field-free alignment in repetitively kicked nitrogen gas
journal, December 2009
- Cryan, James P.; Bucksbaum, Philip H.; Coffee, Ryan N.
- Physical Review A, Vol. 80, Issue 6
Attosecond control of electronic processes by intense light fields
journal, February 2003
- Baltuška, A.; Udem, Th.; Uiberacker, M.
- Nature, Vol. 421, Issue 6923, p. 611-615
Attosecond Streak Camera
journal, April 2002
- Itatani, J.; Quéré, F.; Yudin, G. L.
- Physical Review Letters, Vol. 88, Issue 17
Linked attosecond phase interferometry for molecular frame measurements
journal, February 2013
- Bertrand, J. B.; Wörner, H. J.; Salières, P.
- Nature Physics, Vol. 9, Issue 3
A high frequency optical trap for atoms using Hermite-Gaussian beams
journal, January 2005
- Meyrath, T. P.; Schreck, F.; Hanssen, J. L.
- Optics Express, Vol. 13, Issue 8
High-Order Harmonic Generation in Aligned Molecules
text, January 2001
- Castillejo, M.; Hay, N.; Marangos, J. P.
- The American Physical Society
Measuring the intensity and phase of high-order harmonic emission from aligned molecules
journal, December 2009
- Lock, Robynne M.; Zhou, Xibin; Li, Wen
- Chemical Physics, Vol. 366, Issue 1-3
Observation of Enhanced Field-Free Molecular Alignment by Two Laser Pulses
journal, April 2004
- Bisgaard, Christer Z.; Poulsen, Mikael D.; Péronne, Emmanuel
- Physical Review Letters, Vol. 92, Issue 17
All-Optical Measurement of High-Harmonic Amplitudes and Phases in Aligned Molecules
journal, January 2012
- Rupenyan, A.; Bertrand, J. B.; Villeneuve, D. M.
- Physical Review Letters, Vol. 108, Issue 3
High-order harmonic generation from atoms and ions in the high intensity regime
journal, June 1992
- Krause, Jeffrey L.; Schafer, Kenneth J.; Kulander, Kenneth C.
- Physical Review Letters, Vol. 68, Issue 24
Quantum interference during high-order harmonic generation from aligned molecules
journal, May 2005
- Kanai, Tsuneto; Minemoto, Shinichirou; Sakai, Hirofumi
- Nature, Vol. 435, Issue 7041
Analytic Description of the High-Energy Plateau in Harmonic Generation by Atoms: Can the Harmonic Power Increase with Increasing Laser Wavelengths?
journal, June 2009
- Frolov, M. V.; Manakov, N. L.; Sarantseva, T. S.
- Physical Review Letters, Vol. 102, Issue 24
Intensity dependence of multiple orbital contributions and shape resonance in high-order harmonic generation of aligned N molecules
journal, January 2012
- Jin, Cheng; Bertrand, Julien B.; Lucchese, R. R.
- Physical Review A, Vol. 85, Issue 1
Probing Single-Photon Ionization on the Attosecond Time Scale
journal, April 2011
- Klünder, K.; Dahlström, J. M.; Gisselbrecht, M.
- Physical Review Letters, Vol. 106, Issue 14
Reconstruction of attosecond harmonic beating by interference of two-photon transitions
journal, June 2002
- Muller, H. G.
- Applied Physics B, Vol. 74, Issue S1
High-order harmonic generation in rare gases with a 1-ps 1053-nm laser
journal, February 1993
- L’Huillier, Anne; Balcou, Ph.
- Physical Review Letters, Vol. 70, Issue 6
Linked attosecond phase interferometry for molecular frame measurements
text, January 2013
- Bertrand, Julien B.; Wörner, Hans Jakob; Salières, Pascal
- ETH Zurich
Materials processing with superposed Bessel beams
journal, January 2016
- Yu, Xiaoming; Trallero-Herrero, Carlos A.; Lei, Shuting
- Applied Surface Science, Vol. 360
Interferometric Autocorrelation of an Attosecond Pulse Train in the Single-Cycle Regime
journal, October 2006
- Nabekawa, Yasuo; Shimizu, Toshihiko; Okino, Tomoya
- Physical Review Letters, Vol. 97, Issue 15
High-Order Harmonic Generation in Aligned Molecules
journal, October 2001
- Velotta, R.; Hay, N.; Mason, M. B.
- Physical Review Letters, Vol. 87, Issue 18
Quasi-2D confinement of a BEC in a combined optical and magnetic potential
journal, January 2005
- Smith, N. L.; Heathcote, W. H.; Hechenblaikner, G.
- Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 38, Issue 3
Measurement and laser control of attosecond charge migration in ionized iodoacetylene
journal, October 2015
- Kraus, P. M.; Mignolet, B.; Baykusheva, D.
- Science, Vol. 350, Issue 6262
Theory of high-harmonic generation by low-frequency laser fields
journal, March 1994
- Lewenstein, M.; Balcou, Ph.; Ivanov, M. Yu.
- Physical Review A, Vol. 49, Issue 3
Optimization of the Gaussian beam flattening using a phase-plate
journal, July 1997
- Bourouis, R.; Ameur, K. Ait; Ladjouze, H.
- Journal of Modern Optics, Vol. 44, Issue 7
Near-Threshold High-Order Harmonic Spectroscopy with Aligned Molecules
journal, September 2010
- Soifer, H.; Botheron, P.; Shafir, D.
- Physical Review Letters, Vol. 105, Issue 14
Two-Pulse Field-Free Orientation Reveals Anisotropy of Molecular Shape Resonance
journal, July 2014
- Kraus, P. M.; Baykusheva, D.; Wörner, H. J.
- Physical Review Letters, Vol. 113, Issue 2
Quantum interference during high-order harmonic generation from aligned molecules
journal, January 2006
- Kanai, Tsuneto; Minemoto, Shinichirou; Sakai, Hirofumi
- The Review of Laser Engineering, Vol. 34, Issue Supplement
A Simplification of the Hartree-Fock Method
journal, February 1951
- Slater, J. C.
- Physical Review, Vol. 81, Issue 3
Direct observation of attosecond light bunching
journal, November 2003
- Tzallas, P.; Charalambidis, D.; Papadogiannis, N. A.
- Nature, Vol. 426, Issue 6964
Controlling the Interference of Multiple Molecular Orbitals in High-Harmonic Generation
journal, June 2010
- Wörner, H. J.; Bertrand, J. B.; Hockett, P.
- Physical Review Letters, Vol. 104, Issue 23
Isolated Single-Cycle Attosecond Pulses
journal, October 2006
- Sansone, G.; Benedetti, E.; Calegari, F.
- Science, Vol. 314, Issue 5798
Attosecond correlation dynamics
journal, November 2016
- Ossiander, M.; Siegrist, F.; Shirvanyan, V.
- Nature Physics, Vol. 13, Issue 3
Tomographic imaging of molecular orbitals
journal, December 2004
- Itatani, J.; Levesque, J.; Zeidler, D.
- Nature, Vol. 432, Issue 7019
HOMO-1 orbital cross section revealed through high-order-harmonic generation
journal, March 2017
- Troß, Jan; Ren, Xiaoming; Makhija, Varun
- Physical Review A, Vol. 95, Issue 3
Phase-Locked High-Order Harmonic Sources
journal, August 1997
- Zerne, Raoul; Altucci, Carlo; Bellini, Marco
- Physical Review Letters, Vol. 79, Issue 6
Fringe-pattern analysis using a 2-D Fourier transform
journal, January 1986
- Bone, Donald J.; Bachor, H. -A.; Sandeman, R. John
- Applied Optics, Vol. 25, Issue 10
High-Brightness High-Order Harmonic Generation by Truncated Bessel Beams in the Sub-10-fs Regime
journal, January 2002
- Nisoli, M.; Priori, E.; Sansone, G.
- Physical Review Letters, Vol. 88, Issue 3
Delay in Photoemission
journal, June 2010
- Schultze, M.; Fiess, M.; Karpowicz, N.
- Science, Vol. 328, Issue 5986
Self referencing attosecond interferometer with zeptosecond precision
journal, January 2019
- Tross, Jan; Kolliopoulos, Georgios; Trallero-Herrero, Carlos A.
- Optics Express, Vol. 27, Issue 16
Transverse Electromagnetic Mode Conversion for High-Harmonic Self-Probing Spectroscopy
journal, February 2015
- Camper, Antoine; Ferré, Amélie; Lin, Nan
- Photonics, Vol. 2, Issue 1
A short pulse (7 μs FWHM) and high repetition rate (dc-5kHz) cantilever piezovalve for pulsed atomic and molecular beams
journal, November 2009
- Irimia, Daniel; Dobrikov, Dimitar; Kortekaas, Rob
- Review of Scientific Instruments, Vol. 80, Issue 11
Production of Doubly Charged Helium Ions by Two-Photon Absorption of an Intense Sub-10-fs Soft X-Ray Pulse at 42 eV Photon Energy
journal, January 2005
- Nabekawa, Yasuo; Hasegawa, Hirokazu; Takahashi, Eiji J.
- Physical Review Letters, Vol. 94, Issue 4
Measuring the angle-dependent photoionization cross section of nitrogen using high-harmonic generation
journal, October 2013
- Ren, Xiaoming; Makhija, Varun; Le, Anh-Thu
- Physical Review A, Vol. 88, Issue 4
High-order harmonic phase in molecular nitrogen
journal, September 2009
- McFarland, B. K.; Farrell, J. P.; Bucksbaum, P. H.
- Physical Review A, Vol. 80, Issue 3
Temporal Coherence of Ultrashort High-Order Harmonic Pulses
journal, July 1998
- Bellini, M.; Lyngå, C.; Tozzi, A.
- Physical Review Letters, Vol. 81, Issue 2
Frequency-resolved optical gating for complete reconstruction of attosecond bursts
journal, January 2005
- Mairesse, Y.; Quéré, F.
- Physical Review A, Vol. 71, Issue 1
Creating High-Harmonic Beams with Controlled Orbital Angular Momentum
journal, October 2014
- Gariepy, Genevieve; Leach, Jonathan; Kim, Kyung Taec
- Physical Review Letters, Vol. 113, Issue 15
Creating high-harmonic beams with controlled orbital angular momentum
conference, January 2014
- Gariepy, Genevieve; Leach, Jonathan; Kim, Kyung Taec
- Frontiers in Optics 2014
Interference effects in high-order harmonic generation with molecules
journal, August 2002
- Lein, M.; Hay, N.; Velotta, R.
- Physical Review A, Vol. 66, Issue 2
Multiple-harmonic conversion of 1064 nm radiation in rare gases
journal, February 1988
- Ferray, M.; L'Huillier, A.; Li, X. F.
- Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 21, Issue 3
Probing Proton Dynamics in Molecules on an Attosecond Time Scale
journal, March 2006
- Baker, S.; Robinson, J. S.; Haworth, C. A.
- Science, Vol. 312, Issue 5772
Observation of a Train of Attosecond Pulses from High Harmonic Generation
journal, June 2001
- Paul, P. M.
- Science, Vol. 292, Issue 5522
Alignment-Dependent Strong Field Ionization of Molecules
journal, June 2003
- Litvinyuk, I. V.; Lee, Kevin F.; Dooley, P. W.
- Physical Review Letters, Vol. 90, Issue 23
Revealing the Cooper minimum of by Molecular Frame High-Harmonic Spectroscopy
journal, October 2012
- Bertrand, J. B.; Wörner, H. J.; Hockett, P.
- Physical Review Letters, Vol. 109, Issue 14
Quantitative rescattering theory for high-order harmonic generation from molecules
journal, July 2009
- Le, Anh-Thu; Lucchese, R. R.; Tonzani, S.
- Physical Review A, Vol. 80, Issue 1
Studies of multiphoton production of vacuum-ultraviolet radiation in the rare gases
journal, January 1987
- McPherson, A.; Gibson, G.; Jara, H.
- Journal of the Optical Society of America B, Vol. 4, Issue 4
Attosecond Pulse Trains Generated Using Two Color Laser Fields
journal, July 2006
- Mauritsson, J.; Johnsson, P.; Gustafsson, E.
- Physical Review Letters, Vol. 97, Issue 1
Carrier-envelope-phase stabilized terawatt class laser at 1 kHz with a wavelength tunable option
journal, January 2015
- Langdon, Benjamin; Garlick, Jonathan; Ren, Xiaoming
- Optics Express, Vol. 23, Issue 4
Attosecond Pulse Trains Using High–Order Harmonics
journal, August 1996
- Antoine, Philippe; L'Huillier, Anne; Lewenstein, Maciej
- Physical Review Letters, Vol. 77, Issue 7
Role of the Intramolecular Phase in High-Harmonic Generation
journal, April 2002
- Lein, M.; Hay, N.; Velotta, R.
- Physical Review Letters, Vol. 88, Issue 18
Orbital angular momentum of light and the transformation of Laguerre-Gaussian laser modes
journal, June 1992
- Allen, L.; Beijersbergen, M. W.; Spreeuw, R. J. C.
- Physical Review A, Vol. 45, Issue 11
Attosecond metrology
journal, November 2001
- Hentschel, M.; Kienberger, R.; Spielmann, Ch.
- Nature, Vol. 414, Issue 6863, p. 509-513
Phase-Matched Generation of Coherent Soft X-rays
journal, May 1998
- Rundquist, A.
- Science, Vol. 280, Issue 5368
Probing collective multi-electron dynamics in xenon with high-harmonic spectroscopy
journal, March 2011
- Shiner, A. D.; Schmidt, B. E.; Trallero-Herrero, C.
- Nature Physics, Vol. 7, Issue 6
Multi-channel electronic and vibrational dynamics in polyatomic resonant high-order harmonic generation
journal, January 2015
- Ferré, A.; Boguslavskiy, A. E.; Dagan, M.
- Nature Communications, Vol. 6, Issue 1
High harmonic interferometry of multi-electron dynamics in molecules
journal, July 2009
- Smirnova, Olga; Mairesse, Yann; Patchkovskii, Serguei
- Nature, Vol. 460, Issue 7258
Plasma perspective on strong field multiphoton ionization
journal, September 1993
- Corkum, P. B.
- Physical Review Letters, Vol. 71, Issue 13
Accurate Retrieval of Structural Information from Laser-Induced Photoelectron and High-Order Harmonic Spectra by Few-Cycle Laser Pulses
journal, January 2008
- Morishita, Toru; Le, Anh-Thu; Chen, Zhangjin
- Physical Review Letters, Vol. 100, Issue 1
Measurement and laser control of attosecond charge migration in ionized iodoacetylene
text, January 2015
- Kraus, Peter M.; Mignolet, Benoît; Baykusheva, Denitsa
- ETH Zurich
Temporal Coherence of Ultrashort High-Order Harmonic Pulses
conference, January 1998
- Bellini, M.; Lynga, C.; Tozzi, A.
- CLEO/Europe Conference on Lasers and Electro-Optics
Near-Threshold High-Order Harmonic Spectroscopy with Aligned Molecules
conference, January 2011
- Soifer, Hadas; Bruner, Barry D.; Botheron, Pierre
- High Intensity Lasers and High Field Phenomena, Advances in Optical Materials
All-optical measurement of high-harmonic amplitudes and phases in aligned molecules
text, January 2012
- Rupenyan-Vasileva, Alisa Bohos; Bertrand, Julien B.; Villeneuve, David M.
- ETH Zurich
Molecular recollision interferometry in high harmonic generation
conference, May 2008
- Lock, Robynne; Zhou, Xibin; Wagner, Nick
- 2008 Conference on Lasers and Electro-Optics (CLEO)
Accurate retrieval of structural information from laser-induced photoelectron and high-harmonic spectra by few-cycle laser pulses
text, January 2007
- Morishita, Toru; Le, Anh-Thu; Chen, Zhangjin
- arXiv
Quantitative Rescattering Theory for high-order harmonic generation from molecules
text, January 2009
- Le, Anh-Thu; Lucchese, R. R.; Tonzani, S.
- arXiv
Near-threshold high-order harmonic spectroscopy with aligned molecules
text, January 2010
- Soifer, H.; Botheron, P.; Shafir, D.
- arXiv
Two-pulse field-free orientation reveals anisotropy of molecular shape resonance
text, January 2013
- Kraus, P. M.; Baykusheva, D.; Wörner, H. J.
- arXiv
A self referencing attosecond interferometer with zeptosecond precision
text, January 2019
- Troß, Jan; Kolliopoulos, Georgios; Trallero-Herrero, Carlos A.
- arXiv
Quasi-2D Confinement of a BEC in a Combined Optical and Magnetic Potential
text, January 2004
- Smith, N. L.; Heathcote, W. H.; Hechenblaikner, G.
- arXiv
A high frequency optical trap for atoms using Hermite-Gaussian beams
text, January 2005
- Meyrath, T. P.; Schreck, F.; Hanssen, J. L.
- arXiv