High harmonic generation spectroscopy via orbital angular momentum

Troß, Jan; Trallero-Herrero, Carlos A.

doi:10.1063/1.5115152

Title: High harmonic generation spectroscopy via orbital angular momentum

Journal Article · 28 August 2019 · Journal of Chemical Physics

DOI: https://doi.org/10.1063/1.5115152 · OSTI ID:1610056

^[1];

^[2]

Kansas State Univ., Manhattan, KS (United States)
Univ. of Connecticut, Storrs, CT (United States)

We present an experimental technique using orbital angular momentum (OAM) in a fundamental laser field to drive high harmonic generation (HHG). The mixing of beams with different OAM allows us to generate two laser foci tightly spaced which generate harmonics that interfere in the far field. Thus, this technique is an OAM based in situ HHG interferometric spectroscopic method. With this tool, we measure the phase and amplitude of the angle dependent multiorbital HHG emission in molecular nitrogen

View Accepted Manuscript (DOE)

View Accepted Manuscript (Publisher)

Cite

Export

Save

Research Organization:: Kansas State Univ., Manhattan, KS (United States); Univ. of Connecticut, Storrs, CT (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: FG02-86ER13491; SC0019098

OSTI ID:: 1610056

Alternate ID(s):: OSTI ID: 1559370

Journal Information:: Journal of Chemical Physics, Vol. 151, Issue 8; ISSN 0021-9606

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 10 works

Citation information provided by
Web of Science

References (55)

Atomic transient recorder Kienberger, R.; Goulielmakis, E.; Uiberacker, M. Nature, Vol. 427, Issue 6977 https://doi.org/10.1038/nature02277	journal	February 2004
Information Content of High Harmonics Generated from Aligned Molecules Ramakrishna, S.; Seideman, Tamar Physical Review Letters, Vol. 99, Issue 11 https://doi.org/10.1103/physrevlett.99.113901	journal	September 2007
Uncovering multiple orbitals influence in high harmonic generation from aligned N ₂ Le, Anh-Thu; Lucchese, R. R.; Lin, C. D. Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 42, Issue 21 https://doi.org/10.1088/0953-4075/42/21/211001	journal	October 2009
A Molecular Orbital Theory of Reactivity in Aromatic Hydrocarbons Fukui, Kenichi; Yonezawa, Teijiro; Shingu, Haruo The Journal of Chemical Physics, Vol. 20, Issue 4 https://doi.org/10.1063/1.1700523	journal	April 1952
High Harmonic Generation from Multiple Orbitals in N2 McFarland, B. K.; Farrell, J. P.; Bucksbaum, P. H. Science, Vol. 322, Issue 5905 https://doi.org/10.1126/science.1162780	journal	November 2008
High harmonic generation with a spatially filtered optical parametric amplifier Bandulet, H-C; Comtois, D.; Shiner, A. D. Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 41, Issue 24 https://doi.org/10.1088/0953-4075/41/24/245602	journal	December 2008
Simple interferometric technique for generation of a radially polarized light beam Passilly, Nicolas; Treussart, François; Hierle, Rolland Journal of the Optical Society of America A, Vol. 22, Issue 5 https://doi.org/10.1364/josaa.22.000984	journal	January 2005
Attosecond science Corkum, P. B.; Krausz, Ferenc Nature Physics, Vol. 3, Issue 6 https://doi.org/10.1038/nphys620	journal	June 2007
Alignment-assisted field-free orientation of rotationally cold CO molecules Ren, Xiaoming; Makhija, Varun; Li, Hui Physical Review A, Vol. 90, Issue 1 https://doi.org/10.1103/physreva.90.013419	journal	July 2014
Molecular Recollision Interferometry in High Harmonic Generation Zhou, Xibin; Lock, Robynne; Li, Wen Physical Review Letters, Vol. 100, Issue 7 https://doi.org/10.1103/physrevlett.100.073902	journal	February 2008
Attosecond control of electronic processes by intense light fields Baltuška, A.; Udem, Th.; Uiberacker, M. Nature, Vol. 421, Issue 6923, p. 611-615 https://doi.org/10.1038/nature01414	journal	February 2003
Linked attosecond phase interferometry for molecular frame measurements Bertrand, J. B.; Wörner, H. J.; Salières, P. Nature Physics, Vol. 9, Issue 3 https://doi.org/10.1038/nphys2540	journal	February 2013
High-Order Harmonic Generation in Aligned Molecules Castillejo, M.; Hay, N.; Marangos, J. P. The American Physical Society https://doi.org/10.17877/de290r-12358	text	January 2001
Measuring the intensity and phase of high-order harmonic emission from aligned molecules Lock, Robynne M.; Zhou, Xibin; Li, Wen Chemical Physics, Vol. 366, Issue 1-3 https://doi.org/10.1016/j.chemphys.2009.09.020	journal	December 2009
Quantum interference during high-order harmonic generation from aligned molecules Kanai, Tsuneto; Minemoto, Shinichirou; Sakai, Hirofumi Nature, Vol. 435, Issue 7041 https://doi.org/10.1038/nature03577	journal	May 2005
Analytic Description of the High-Energy Plateau in Harmonic Generation by Atoms: Can the Harmonic Power Increase with Increasing Laser Wavelengths? Frolov, M. V.; Manakov, N. L.; Sarantseva, T. S. Physical Review Letters, Vol. 102, Issue 24 https://doi.org/10.1103/physrevlett.102.243901	journal	June 2009
Reconstruction of attosecond harmonic beating by interference of two-photon transitions Muller, H. G. Applied Physics B, Vol. 74, Issue S1 https://doi.org/10.1007/s00340-002-0894-8	journal	June 2002
Linked attosecond phase interferometry for molecular frame measurements Bertrand, Julien B.; Wörner, Hans Jakob; Salières, Pascal ETH Zurich https://doi.org/10.3929/ethz-a-010781904	text	January 2013
Materials processing with superposed Bessel beams Yu, Xiaoming; Trallero-Herrero, Carlos A.; Lei, Shuting Applied Surface Science, Vol. 360 https://doi.org/10.1016/j.apsusc.2015.11.074	journal	January 2016
Quasi-2D confinement of a BEC in a combined optical and magnetic potential Smith, N. L.; Heathcote, W. H.; Hechenblaikner, G. Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 38, Issue 3 https://doi.org/10.1088/0953-4075/38/3/007	journal	January 2005
Measurement and laser control of attosecond charge migration in ionized iodoacetylene Kraus, P. M.; Mignolet, B.; Baykusheva, D. Science, Vol. 350, Issue 6262 https://doi.org/10.1126/science.aab2160	journal	October 2015
Optimization of the Gaussian beam flattening using a phase-plate Bourouis, R.; Ameur, K. Ait; Ladjouze, H. Journal of Modern Optics, Vol. 44, Issue 7 https://doi.org/10.1080/09500349708230746	journal	July 1997
Quantum interference during high-order harmonic generation from aligned molecules Kanai, Tsuneto; Minemoto, Shinichirou; Sakai, Hirofumi The Review of Laser Engineering, Vol. 34, Issue Supplement https://doi.org/10.2184/lsj.34.86	journal	January 2006
Direct observation of attosecond light bunching Tzallas, P.; Charalambidis, D.; Papadogiannis, N. A. Nature, Vol. 426, Issue 6964 https://doi.org/10.1038/nature02091	journal	November 2003
Isolated Single-Cycle Attosecond Pulses Sansone, G.; Benedetti, E.; Calegari, F. Science, Vol. 314, Issue 5798 https://doi.org/10.1126/science.1132838	journal	October 2006
Attosecond correlation dynamics Ossiander, M.; Siegrist, F.; Shirvanyan, V. Nature Physics, Vol. 13, Issue 3 https://doi.org/10.1038/nphys3941	journal	November 2016
Tomographic imaging of molecular orbitals Itatani, J.; Levesque, J.; Zeidler, D. Nature, Vol. 432, Issue 7019 https://doi.org/10.1038/nature03183	journal	December 2004
Delay in Photoemission Schultze, M.; Fiess, M.; Karpowicz, N. Science, Vol. 328, Issue 5986 https://doi.org/10.1126/science.1189401	journal	June 2010
Self referencing attosecond interferometer with zeptosecond precision Tross, Jan; Kolliopoulos, Georgios; Trallero-Herrero, Carlos A. Optics Express, Vol. 27, Issue 16 https://doi.org/10.1364/oe.27.022960	journal	January 2019
Transverse Electromagnetic Mode Conversion for High-Harmonic Self-Probing Spectroscopy Camper, Antoine; Ferré, Amélie; Lin, Nan Photonics, Vol. 2, Issue 1 https://doi.org/10.3390/photonics2010184	journal	February 2015
A short pulse (7 μs FWHM) and high repetition rate (dc-5kHz) cantilever piezovalve for pulsed atomic and molecular beams Irimia, Daniel; Dobrikov, Dimitar; Kortekaas, Rob Review of Scientific Instruments, Vol. 80, Issue 11 https://doi.org/10.1063/1.3263912	journal	November 2009
Production of Doubly Charged Helium Ions by Two-Photon Absorption of an Intense Sub-10-fs Soft X-Ray Pulse at 42 eV Photon Energy Nabekawa, Yasuo; Hasegawa, Hirokazu; Takahashi, Eiji J. Physical Review Letters, Vol. 94, Issue 4 https://doi.org/10.1103/physrevlett.94.043001	journal	January 2005
High-order harmonic phase in molecular nitrogen McFarland, B. K.; Farrell, J. P.; Bucksbaum, P. H. Physical Review A, Vol. 80, Issue 3 https://doi.org/10.1103/physreva.80.033412	journal	September 2009
Creating high-harmonic beams with controlled orbital angular momentum Gariepy, Genevieve; Leach, Jonathan; Kim, Kyung Taec Frontiers in Optics 2014 https://doi.org/10.1364/fio.2014.fth2a.1	conference	January 2014
Orbital angular momentum of light and the transformation of Laguerre?Gaussian laser modes Allen, L.; Beijersbergen, M. W.; Spreeuw, R. J. C. Optical Angular Momentum https://doi.org/10.1887/0750309016/b1142c6	book	July 1992
Multiple-harmonic conversion of 1064 nm radiation in rare gases Ferray, M.; L'Huillier, A.; Li, X. F. Journal of Physics B: Atomic, Molecular and Optical Physics, Vol. 21, Issue 3 https://doi.org/10.1088/0953-4075/21/3/001	journal	February 1988
Probing Proton Dynamics in Molecules on an Attosecond Time Scale Baker, S.; Robinson, J. S.; Haworth, C. A. Science, Vol. 312, Issue 5772 https://doi.org/10.1126/science.1123904	journal	March 2006
Observation of a Train of Attosecond Pulses from High Harmonic Generation Paul, P. M. Science, Vol. 292, Issue 5522 https://doi.org/10.1126/science.1059413	journal	June 2001
Attosecond metrology Hentschel, M.; Kienberger, R.; Spielmann, Ch. Nature, Vol. 414, Issue 6863, p. 509-513 https://doi.org/10.1038/35107000	journal	November 2001
Phase-Matched Generation of Coherent Soft X-rays Rundquist, A. Science, Vol. 280, Issue 5368 https://doi.org/10.1126/science.280.5368.1412	journal	May 1998
Probing collective multi-electron dynamics in xenon with high-harmonic spectroscopy Shiner, A. D.; Schmidt, B. E.; Trallero-Herrero, C. Nature Physics, Vol. 7, Issue 6 https://doi.org/10.1038/nphys1940	journal	March 2011
Multi-channel electronic and vibrational dynamics in polyatomic resonant high-order harmonic generation Ferré, A.; Boguslavskiy, A. E.; Dagan, M. Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms6952	journal	January 2015
High harmonic interferometry of multi-electron dynamics in molecules Smirnova, Olga; Mairesse, Yann; Patchkovskii, Serguei Nature, Vol. 460, Issue 7258 https://doi.org/10.1038/nature08253	journal	July 2009
Measurement and laser control of attosecond charge migration in ionized iodoacetylene Kraus, Peter M.; Mignolet, Benoît; Baykusheva, Denitsa ETH Zurich https://doi.org/10.3929/ethz-a-010782069	text	January 2015
Temporal Coherence of Ultrashort High-Order Harmonic Pulses Bellini, M.; Lynga, C.; Tozzi, A. CLEO/Europe Conference on Lasers and Electro-Optics https://doi.org/10.1109/cleoe.1998.719518	conference	January 1998
Near-Threshold High-Order Harmonic Spectroscopy with Aligned Molecules Soifer, Hadas; Bruner, Barry D.; Botheron, Pierre High Intensity Lasers and High Field Phenomena, Advances in Optical Materials https://doi.org/10.1364/hilas.2011.hfa3	conference	January 2011
All-optical measurement of high-harmonic amplitudes and phases in aligned molecules Rupenyan-Vasileva, Alisa Bohos; Bertrand, Julien B.; Villeneuve, David M. ETH Zurich https://doi.org/10.3929/ethz-a-010780589	text	January 2012
Molecular recollision interferometry in high harmonic generation Lock, Robynne; Zhou, Xibin; Wagner, Nick 2008 Conference on Lasers and Electro-Optics (CLEO) https://doi.org/10.1109/cleo.2008.4551950	conference	May 2008
Accurate retrieval of structural information from laser-induced photoelectron and high-harmonic spectra by few-cycle laser pulses Morishita, Toru; Le, Anh-Thu; Chen, Zhangjin arXiv https://doi.org/10.48550/arxiv.0707.3157	text	January 2007
Quantitative Rescattering Theory for high-order harmonic generation from molecules Le, Anh-Thu; Lucchese, R. R.; Tonzani, S. arXiv https://doi.org/10.48550/arxiv.0903.5354	text	January 2009
Near-threshold high-order harmonic spectroscopy with aligned molecules Soifer, H.; Botheron, P.; Shafir, D. arXiv https://doi.org/10.48550/arxiv.1009.2224	text	January 2010
Two-pulse field-free orientation reveals anisotropy of molecular shape resonance Kraus, P. M.; Baykusheva, D.; Wörner, H. J. arXiv https://doi.org/10.48550/arxiv.1311.3923	text	January 2013
A self referencing attosecond interferometer with zeptosecond precision Troß, Jan; Kolliopoulos, Georgios; Trallero-Herrero, Carlos A. arXiv https://doi.org/10.48550/arxiv.1905.04371	text	January 2019
Quasi-2D Confinement of a BEC in a Combined Optical and Magnetic Potential Smith, N. L.; Heathcote, W. H.; Hechenblaikner, G. arXiv https://doi.org/10.48550/arxiv.cond-mat/0410101	text	January 2004
A high frequency optical trap for atoms using Hermite-Gaussian beams Meyrath, T. P.; Schreck, F.; Hanssen, J. L. arXiv https://doi.org/10.48550/arxiv.cond-mat/0503349	text	January 2005

Similar Records

Self referencing attosecond interferometer with zeptosecond precision

Journal Article · 2019 · Optics Express · OSTI ID:1545179

Tross, Jan; Kolliopoulos, Georgios; Trallero-Herrero, Carlos A.

Real-Time Observation of Molecular Spinning with Angular High-Harmonic Spectroscopy

Journal Article · 2018 · Physical Review Letters · OSTI ID:1610049

He, Lixin; Lan, Pengfei; Le, Anh-Thu; +5 more

Phase-matching analysis in high-order harmonic generation with nonzero orbital angular momentum Laguerre-Gaussian beams

Journal Article · 2020 · Physical Review A · OSTI ID:1800614

Jin, Cheng; Li, Baochang; Wang, Kan; +4 more

Related Subjects

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
71 CLASSICAL AND QUANTUM MECHANICS
GENERAL PHYSICS
Chemistry
Physics
Optical devices
Lasers
Geometrical optics
Gas jet
Photoionization
Interferometry
Spectroscopy

Title: High harmonic generation spectroscopy via orbital angular momentum

Citation Formats

References (55)

Similar Records

Related Subjects