High harmonic generation spectroscopy via orbital angular momentum

Troß, Jan; Trallero-Herrero, Carlos A.

doi:10.1063/1.5115152

Title: High harmonic generation spectroscopy via orbital angular momentum

Journal Article · 27 August 2019 · Journal of Chemical Physics

DOI: https://doi.org/10.1063/1.5115152 · OSTI ID:1610056

^[1];

^[2]

Kansas State Univ., Manhattan, KS (United States); DOE/OSTI
Univ. of Connecticut, Storrs, CT (United States)

We present an experimental technique using orbital angular momentum (OAM) in a fundamental laser field to drive high harmonic generation (HHG). The mixing of beams with different OAM allows us to generate two laser foci tightly spaced which generate harmonics that interfere in the far field. Thus, this technique is an OAM based in situ HHG interferometric spectroscopic method. With this tool, we measure the phase and amplitude of the angle dependent multiorbital HHG emission in molecular nitrogen

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Research Organization:: Kansas State Univ., Manhattan, KS (United States); Univ. of Connecticut, Storrs, CT (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: FG02-86ER13491; SC0019098

OSTI ID:: 1610056

Journal Information:: Journal of Chemical Physics, Journal Name: Journal of Chemical Physics Journal Issue: 8 Vol. 151; ISSN 0021-9606

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Title: High harmonic generation spectroscopy via orbital angular momentum

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