Adaptive strong-field control of vibrational population in NO2+

Voznyuk, O.; Jochim, Bethany; Zohrabi, M.; Broin, Adam; Averin, R.; Carnes, K. D.; Ben-Itzhak, I.; Wells, E.

doi:10.1063/1.5115504

Title: Adaptive strong-field control of vibrational population in NO²⁺

Journal Article · 27 September 2019 · Journal of Chemical Physics

DOI: https://doi.org/10.1063/1.5115504 · OSTI ID:1610039

Voznyuk, O. ^[1];

^[2];

^[3]; Broin, Adam ^[4]; Averin, R. ^[4];

^[3];

^[4]

Augustana College, Sioux Falls, SD (United States); DOE/OSTI
Augustana College, Sioux Falls, SD (United States); Kansas State Univ., Manhattan, KS (United States)
Kansas State Univ., Manhattan, KS (United States)
Augustana College, Sioux Falls, SD (United States)

An adaptive closed-loop system employing coincidence time-of-flight feedback is used to determine the optimal pulse shapes for manipulating the branching ratio of NO dications following double ionization by an intense laser pulse. Selection between the long-lived NO²⁺ and the dissociative N⁺ + O⁺ final states requires control of the vibrational population distribution in the transient NO²⁺. The ability to both suppress and enhance NO²⁺ relative to N⁺ + O⁺ is observed, with the effectiveness of shaped pulses surpassing near Fourier transform-limited pulses by about an order of magnitude in each direction, depending on the pulse energy. The control is subsequently investigated using velocity map imaging, identifying plausible dissociation pathways leading to N⁺ + O⁺. Combining the information about the N⁺ + O⁺ dissociation with a well-defined control objective supports the conclusion that the primary control mechanism involves selectively populating long-lived NO²⁺ vibrational states.

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Research Organization:: Kansas State Univ., Manhattan, KS (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: FG02-86ER13491

OSTI ID:: 1610039

Journal Information:: Journal of Chemical Physics, Journal Name: Journal of Chemical Physics Journal Issue: 12 Vol. 151; ISSN 0021-9606

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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