Discovery of topological Weyl fermion lines and drumhead surface states in a room temperature magnet
Abstract
Topological matter is known to exhibit unconventional surface states and anomalous transport owing to unusual bulk electronic topology. In this study, we use photoemission spectroscopy and quantum transport to elucidate the topology of the room temperature magnet Co2MnGa. We observe sharp bulk Weyl fermion line dispersions indicative of nontrivial topological invariants present in the magnetic phase. On the surface of the magnet, we observe electronic wave functions that take the form of drumheads, enabling us to directly visualize the crucial components of the bulk-boundary topological correspondence. By considering the Berry curvature field associated with the observed topological Weyl fermion lines, we quantitatively account for the giant anomalous Hall response observed in this magnet. Our experimental results suggest a rich interplay of strongly interacting electrons and topology in quantum matter.
- Authors:
-
more »
- Princeton Univ., NJ (United States). Lab. for Topological Quantum Matter and Advanced Spectroscopy (B7)
- Max Planck Inst. for Chemical Physics of Solids, Dresden (Germany)
- Shenzhen Univ., Shenzhen (China). SZU-NUS Collaborative Center and International Collaborative Lab. of 2D Materials for Optoelectronic Science and Technology, College of Optoelectronic Engineering
- Univ. of Missouri, Columbia, MO (United States)
- National Cheng Kung Univ., Tainan (Taiwan)
- National Sun Yat-Sen Univ., Kaohsiung (Taiwan)
- Northeastern Univ., Boston, MA (United States)
- Academia Sinica, Taipei (Taiwan)
- Princeton Univ., NJ (United States). Lab. for Topological Quantum Matter and Advanced Spectroscopy (B7), and Princeton Inst. for Science and Technology of Materials; Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Publication Date:
- Research Org.:
- SLAC National Accelerator Lab., Menlo Park, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); Gordon and Betty Moore Foundation (GBMF)
- OSTI Identifier:
- 1608973
- Alternate Identifier(s):
- OSTI ID: 1632129
- Grant/Contract Number:
- AC02-76SF00515; FG02-05ER46200; FG02-07ER46352; AC02-05CH11231; 291472; 742068
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Science
- Additional Journal Information:
- Journal Volume: 365; Journal Issue: 6459; Journal ID: ISSN 0036-8075
- Publisher:
- AAAS
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS
Citation Formats
Belopolski, Ilya, Manna, Kaustuv, Sanchez, Daniel S., Chang, Guoqing, Ernst, Benedikt, Yin, Jiaxin, Zhang, Songtian S., Cochran, Tyler, Shumiya, Nana, Zheng, Hao, Singh, Bahadur, Bian, Guang, Multer, Daniel, Litskevich, Maksim, Zhou, Xiaoting, Huang, Shin-Ming, Wang, Baokai, Chang, Tay-Rong, Xu, Su-Yang, Bansil, Arun, Felser, Claudia, Lin, Hsin, and Hasan, M. Zahid. Discovery of topological Weyl fermion lines and drumhead surface states in a room temperature magnet. United States: N. p., 2019.
Web. doi:10.1126/science.aav2327.
Belopolski, Ilya, Manna, Kaustuv, Sanchez, Daniel S., Chang, Guoqing, Ernst, Benedikt, Yin, Jiaxin, Zhang, Songtian S., Cochran, Tyler, Shumiya, Nana, Zheng, Hao, Singh, Bahadur, Bian, Guang, Multer, Daniel, Litskevich, Maksim, Zhou, Xiaoting, Huang, Shin-Ming, Wang, Baokai, Chang, Tay-Rong, Xu, Su-Yang, Bansil, Arun, Felser, Claudia, Lin, Hsin, & Hasan, M. Zahid. Discovery of topological Weyl fermion lines and drumhead surface states in a room temperature magnet. United States. https://doi.org/10.1126/science.aav2327
Belopolski, Ilya, Manna, Kaustuv, Sanchez, Daniel S., Chang, Guoqing, Ernst, Benedikt, Yin, Jiaxin, Zhang, Songtian S., Cochran, Tyler, Shumiya, Nana, Zheng, Hao, Singh, Bahadur, Bian, Guang, Multer, Daniel, Litskevich, Maksim, Zhou, Xiaoting, Huang, Shin-Ming, Wang, Baokai, Chang, Tay-Rong, Xu, Su-Yang, Bansil, Arun, Felser, Claudia, Lin, Hsin, and Hasan, M. Zahid. Thu .
"Discovery of topological Weyl fermion lines and drumhead surface states in a room temperature magnet". United States. https://doi.org/10.1126/science.aav2327. https://www.osti.gov/servlets/purl/1608973.
@article{osti_1608973,
title = {Discovery of topological Weyl fermion lines and drumhead surface states in a room temperature magnet},
author = {Belopolski, Ilya and Manna, Kaustuv and Sanchez, Daniel S. and Chang, Guoqing and Ernst, Benedikt and Yin, Jiaxin and Zhang, Songtian S. and Cochran, Tyler and Shumiya, Nana and Zheng, Hao and Singh, Bahadur and Bian, Guang and Multer, Daniel and Litskevich, Maksim and Zhou, Xiaoting and Huang, Shin-Ming and Wang, Baokai and Chang, Tay-Rong and Xu, Su-Yang and Bansil, Arun and Felser, Claudia and Lin, Hsin and Hasan, M. Zahid},
abstractNote = {Topological matter is known to exhibit unconventional surface states and anomalous transport owing to unusual bulk electronic topology. In this study, we use photoemission spectroscopy and quantum transport to elucidate the topology of the room temperature magnet Co2MnGa. We observe sharp bulk Weyl fermion line dispersions indicative of nontrivial topological invariants present in the magnetic phase. On the surface of the magnet, we observe electronic wave functions that take the form of drumheads, enabling us to directly visualize the crucial components of the bulk-boundary topological correspondence. By considering the Berry curvature field associated with the observed topological Weyl fermion lines, we quantitatively account for the giant anomalous Hall response observed in this magnet. Our experimental results suggest a rich interplay of strongly interacting electrons and topology in quantum matter.},
doi = {10.1126/science.aav2327},
journal = {Science},
number = 6459,
volume = 365,
place = {United States},
year = {2019},
month = {9}
}
Web of Science
Works referenced in this record:
Generalized Gradient Approximation Made Simple
journal, October 1996
- Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
- Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868
Weyl and Dirac loop superconductors
journal, January 2016
- Nandkishore, Rahul
- Physical Review B, Vol. 93, Issue 2
Magnetic and chemical order in Heusler alloys containing cobalt and manganese
journal, January 1971
- Webster, P. J.
- Journal of Physics and Chemistry of Solids, Vol. 32, Issue 6
Giant anomalous Hall effect in a ferromagnetic kagome-lattice semimetal
journal, July 2018
- Liu, Enke; Sun, Yan; Kumar, Nitesh
- Nature Physics, Vol. 14, Issue 11
Multivariable Scaling for the Anomalous Hall Effect
journal, May 2015
- Hou, Dazhi; Su, Gang; Tian, Yuan
- Physical Review Letters, Vol. 114, Issue 21
Colloquium : Topological band theory
journal, June 2016
- Bansil, A.; Lin, Hsin; Das, Tanmoy
- Reviews of Modern Physics, Vol. 88, Issue 2
Giant anomalous Nernst effect and quantum-critical scaling in a ferromagnetic semimetal
journal, July 2018
- Sakai, Akito; Mizuta, Yo Pierre; Nugroho, Agustinus Agung
- Nature Physics, Vol. 14, Issue 11
From ultrasoft pseudopotentials to the projector augmented-wave method
journal, January 1999
- Kresse, G.; Joubert, D.
- Physical Review B, Vol. 59, Issue 3, p. 1758-1775
Exploring Co 2 MnAl Heusler compound for anomalous Hall effect sensors
journal, September 2011
- Vilanova Vidal, E.; Stryganyuk, G.; Schneider, H.
- Applied Physics Letters, Vol. 99, Issue 13
Proper Scaling of the Anomalous Hall Effect
journal, August 2009
- Tian, Yuan; Ye, Li; Jin, Xiaofeng
- Physical Review Letters, Vol. 103, Issue 8
and other topological semimetals with line nodes and drumhead surface states
journal, May 2016
- Chan, Y. -H.; Chiu, Ching-Kai; Chou, M. Y.
- Physical Review B, Vol. 93, Issue 20
Topological nodal semimetals
journal, December 2011
- Burkov, A. A.; Hook, M. D.; Balents, Leon
- Physical Review B, Vol. 84, Issue 23
Source data for "Discovery of topological Weyl fermion lines and drumhead surface states in a room temperature magnet"
dataset, January 2019
- Belopolski, Ilya; Manna, Kaustuv; Sanchez, Daniel S.
- Zenodo
Classification of topological quantum matter with symmetries
journal, August 2016
- Chiu, Ching-Kai; Teo, Jeffrey C. Y.; Schnyder, Andreas P.
- Reviews of Modern Physics, Vol. 88, Issue 3
Topological Hopf and Chain Link Semimetal States and Their Application to
journal, October 2017
- Chang, Guoqing; Xu, Su-Yang; Zhou, Xiaoting
- Physical Review Letters, Vol. 119, Issue 15
Electronic structure and magnetic exchange coupling in ferromagnetic full Heusler alloys
journal, January 2005
- Kurtulus, Yasemin; Dronskowski, Richard; Samolyuk, German D.
- Physical Review B, Vol. 71, Issue 1
Dirac Line Nodes in Inversion-Symmetric Crystals
journal, July 2015
- Kim, Youngkuk; Wieder, Benjamin J.; Kane, C. L.
- Physical Review Letters, Vol. 115, Issue 3
The strange topology that is reshaping physics
journal, July 2017
- Castelvecchi, Davide
- Nature, Vol. 547, Issue 7663
Discovery of Weyl Fermion Semimetals and Topological Fermi Arc States
journal, March 2017
- Hasan, M. Zahid; Xu, Su-Yang; Belopolski, Ilya
- Annual Review of Condensed Matter Physics, Vol. 8, Issue 1
Topological insulators, topological superconductors and Weyl fermion semimetals: discoveries, perspectives and outlooks
journal, September 2015
- Hasan, M. Zahid; Xu, Su-Yang; Bian, Guang
- Physica Scripta, Vol. T164
Emergent functions of quantum materials
journal, September 2017
- Tokura, Yoshinori; Kawasaki, Masashi; Nagaosa, Naoto
- Nature Physics, Vol. 13, Issue 11
Source data for "Discovery of topological Weyl fermion lines and drumhead surface states in a room temperature magnet"
dataset, January 2019
- Belopolski, Ilya; Manna, Kaustuv; Sanchez, Daniel S.
- Zenodo
Giant and anisotropic many-body spin–orbit tunability in a strongly correlated kagome magnet
journal, September 2018
- Yin, Jia-Xin; Zhang, Songtian S.; Li, Hang
- Nature, Vol. 562, Issue 7725
Anomalous Hall effect
journal, May 2010
- Nagaosa, Naoto; Sinova, Jairo; Onoda, Shigeki
- Reviews of Modern Physics, Vol. 82, Issue 2
Anomalous Hall effect in localization regime
journal, June 2016
- Wu, Lin; Zhu, Kai; Yue, Di
- Physical Review B, Vol. 93, Issue 21
Twisting the thermoelectric potential
journal, January 2021
- May, Andrew F.; Sales, Brian C.
- Nature Materials, Vol. 20, Issue 4
Weyl and Dirac semimetals in three-dimensional solids
journal, January 2018
- Armitage, N. P.; Mele, E. J.; Vishwanath, Ashvin
- Reviews of Modern Physics, Vol. 90, Issue 1
Towards properties on demand in quantum materials
journal, October 2017
- Basov, D. N.; Averitt, R. D.; Hsieh, D.
- Nature Materials, Vol. 16, Issue 11
Nodal-chain metals
journal, August 2016
- Bzdušek, Tomáš; Wu, QuanSheng; Rüegg, Andreas
- Nature, Vol. 538, Issue 7623
Topological nodal-line fermions in spin-orbit metal PbTaSe2
journal, February 2016
- Bian, Guang; Chang, Tay-Rong; Sankar, Raman
- Nature Communications, Vol. 7, Issue 1
Topological Phonons and Weyl Lines in Three Dimensions
journal, August 2016
- Stenull, Olaf; Kane, C. L.; Lubensky, T. C.
- Physical Review Letters, Vol. 117, Issue 6
The physics of quantum materials
journal, October 2017
- Keimer, B.; Moore, J. E.
- Nature Physics, Vol. 13, Issue 11
Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set
journal, October 1996
- Kresse, G.; Furthmüller, J.
- Physical Review B, Vol. 54, Issue 16, p. 11169-11186
Classification of reflection-symmetry-protected topological semimetals and nodal superconductors
journal, November 2014
- Chiu, Ching-Kai; Schnyder, Andreas P.
- Physical Review B, Vol. 90, Issue 20
Large anomalous Hall current induced by topological nodal lines in a ferromagnetic van der Waals semimetal
journal, July 2018
- Kim, Kyoo; Seo, Junho; Lee, Eunwoo
- Nature Materials, Vol. 17, Issue 9
Topological surface superconductivity in doped Weyl loop materials
journal, February 2017
- Wang, Yuxuan; Nandkishore, Rahul M.
- Physical Review B, Vol. 95, Issue 6
Classification of topological insulators and superconductors in three spatial dimensions
journal, November 2008
- Schnyder, Andreas P.; Ryu, Shinsei; Furusaki, Akira
- Physical Review B, Vol. 78, Issue 19
From Colossal to Zero: Controlling the Anomalous Hall Effect in Magnetic Heusler Compounds via Berry Curvature Design
journal, December 2018
- Manna, Kaustuv; Muechler, Lukas; Kao, Ting-Hui
- Physical Review X, Vol. 8, Issue 4
Reducing Dzyaloshinskii-Moriya interaction and field-free spin-orbit torque switching in synthetic antiferromagnets
journal, May 2021
- Chen, Ruyi; Cui, Qirui; Liao, Liyang
- Nature Communications, Vol. 12, Issue 1
Temperature dependence of the intrinsic anomalous Hall effect in nickel
journal, June 2012
- Ye, Li; Tian, Yuan; Jin, Xiaofeng
- Physical Review B, Vol. 85, Issue 22
Surface states of ternary semiconductor alloys: Effect of alloy fluctuations in one-dimensional models with realistic atoms
journal, April 1985
- Bryant, Garnett W.
- Physical Review B, Vol. 31, Issue 8
MAGNETIC PROPERTIES OF Co-HEUSLER AND RELATED MIXED ALLOYS
journal, December 1988
- Ido, H.; Yasuda, S.
- Le Journal de Physique Colloques, Vol. 49, Issue C8
Source data for "Discovery of topological Weyl fermion lines and drumhead surface states in a room temperature magnet"
dataset, January 2019
- Belopolski, Ilya; Manna, Kaustuv; Sanchez, Daniel S.
- Zenodo
Classification of topological insulators and superconductors in three spatial dimensions
text, January 2008
- Schnyder, Andreas P.; Ryu, Shinsei; Furusaki, Akira
- arXiv
Temperature Dependence of the Intrinsic Anomalous Hall Effect in Nickel
text, January 2011
- Ye, Li; Tian, Yuan; Xiao, Di
- arXiv
Classification of reflection symmetry protected topological semimetals and nodal superconductors
text, January 2014
- Chiu, Ching-Kai; Schnyder, Andreas P.
- arXiv
Dirac Line Nodes in Inversion Symmetric Crystals
text, January 2015
- Kim, Youngkuk; Wieder, Benjamin J.; Kane, C. L.
- arXiv
Classification of topological quantum matter with symmetries
text, January 2015
- Chiu, Ching-Kai; Teo, Jeffrey C. Y.; Schnyder, Andreas P.
- arXiv
Discovery of Weyl fermion semimetals and topological Fermi arc states
text, January 2017
- Hasan, M. Zahid; Xu, Su-Yang; Belopolski, Ilya
- arXiv
Weyl and Dirac Semimetals in Three Dimensional Solids
text, January 2017
- Armitage, N. P.; Mele, E. J.; Vishwanath, Ashvin
- arXiv
Giant anomalous Hall effect in a ferromagnetic Kagome-lattice semimetal
text, January 2017
- Liu, Enke; Sun, Yan; Kumar, Nitesh
- arXiv
From colossal to zero: Controlling the Anomalous Hall Effect in Magnetic Heusler Compounds via Berry Curvature Design
text, January 2017
- Manna, Kaustuv; Muechler, Lukas; Kao, Ting-Hui
- arXiv
Giant anomalous Nernst effect and quantum-critical scaling in a ferromagnetic semimetal
text, January 2018
- Sakai, Akito; Mizuta, Yo Pierre; Nugroho, Agustinus Agung
- arXiv
Giant and anisotropic many-body spin-orbit tunability in a strongly correlated kagome magnet
text, January 2018
- Yin, Jia-Xin; Zhang, Songtian S.; Li, Hang
- arXiv
Works referencing / citing this record:
Finite bulk Josephson currents and chirality blockade removal from interorbital pairing in magnetic Weyl semimetals
journal, February 2020
- Dutta, Paramita; Parhizgar, Fariborz; Black-Schaffer, Annica M.
- Physical Review B, Vol. 101, Issue 6
“Weyl”ing away time-reversal symmetry
journal, September 2019
- da Silva Neto, Eduardo H.
- Science, Vol. 365, Issue 6459
Weyl nodes and magnetostructural instability in antiperovskite Mn 3 ZnC
journal, December 2019
- Teicher, S. M. L.; Svenningsson, I. K.; Schoop, L. M.
- APL Materials, Vol. 7, Issue 12
Magnetism and anomalous transport in the Weyl semimetal PrAlGe: possible route to axial gauge fields
journal, January 2020
- Destraz, Daniel; Das, Lakshmi; Tsirkin, Stepan S.
- npj Quantum Materials, Vol. 5, Issue 1
Modular Arithmetic with Nodal Lines: Drumhead Surface States in ZrSiTe
journal, February 2020
- Muechler, Lukas; Topp, Andreas; Queiroz, Raquel
- Physical Review X, Vol. 10, Issue 1
Inverse-perovskites A 3 B O ( A = Sr, Ca, Eu/ B = Pb, Sn): A platform for control of Dirac and Weyl Fermions
journal, December 2019
- Rost, A. W.; Kim, J.; Suetsugu, S.
- APL Materials, Vol. 7, Issue 12
Spin-to-Charge Conversion in Magnetic Weyl Semimetals
journal, October 2019
- Zhang, Steven S. -L.; Burkov, Anton A.; Martin, Ivar
- Physical Review Letters, Vol. 123, Issue 18
Transition from intrinsic to extrinsic anomalous Hall effect in the ferromagnetic Weyl semimetal PrAlGe 1− x Si x
journal, January 2020
- Yang, Hung-Yu; Singh, Bahadur; Lu, Baozhu
- APL Materials, Vol. 8, Issue 1
Magnetism and anomalous transport in the Weyl semimetal PrAlGe: possible route to axial gauge fields
text, January 2020
- Destraz, Daniel; Das, Lakshmi; Tsirkin, Stepan S.
- Nature Publishing Group
Spin-to-charge conversion in magnetic Weyl semimetals
text, January 2019
- Zhang, Steven S. -L.; Burkov, Anton A.; Martin, Ivar
- arXiv
Modular Arithmetic with Nodal Lines: Drumhead Surface States in ZrSiTe
text, January 2019
- Muechler, Lukas; Topp, Andreas; Queiroz, Raquel
- arXiv
Transition from Intrinsic to Extrinsic Anomalous Hall Effect in the Ferromagnetic Weyl Semimetal PrAlGe$_{1-x}$Si$_x$
text, January 2019
- Yang, Hung-Yu; Singh, Bahadur; Lu, Baozhu
- arXiv