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Title: A portable on-axis laser-heating system for near-90° X-ray spectroscopy: application to ferropericlase and iron silicide

Abstract

A portable IR fiber laser-heating system, optimized for X-ray emission spectroscopy (XES) and nuclear inelastic scattering (NIS) spectroscopy with signal collection through the radial opening of diamond anvil cells near 90°with respect to the incident X-ray beam, is presented. The system offers double-sided on-axis heating by a single laser source and zero attenuation of incoming X-rays other than by the high-pressure environment. A description of the system, which has been tested for pressures above 100 GPa and temperatures up to 3000 K, is given. The XES spectra of laser-heated Mg0.67Fe0.33O demonstrate the potential to map the iron spin state in the pressure–temperature range of the Earth's lower mantle, and the NIS spectra of laser-heated FeSi give access to the sound velocity of this candidate of a phase inside the Earth's core. This portable system represents one of the few bridges across the gap between laser heating and high-resolution X-ray spectroscopies with signal collection near 90°.

Authors:
 [1];  [2];  [3];  [4];  [5];  [5];  [5];  [6];  [7]; ORCiD logo [8];  [9]; ORCiD logo [4];  [9];  [10];  [11];  [4];  [12]; ORCiD logo [13];  [5]; ORCiD logo [5] more »;  [7] « less
  1. Univ. of Potsdam (Germany); Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); GFZ German Research Centre for Geosciences, Potsdam (Germany)
  2. Univ. Munster (Germany)
  3. ETH, Zurich (Switzerland)
  4. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)
  5. Technische Univ. Dortmund (Germany)
  6. Univ. of Potsdam (Germany); European XFEL, Schenefeld (Germany)
  7. Univ. of Potsdam (Germany)
  8. The European Synchrotron (ESRF), Grenoble (France)
  9. European XFEL, Schenefeld (Germany)
  10. Meiji Univ., Kanagawa (Japan)
  11. Univ. Frankfurt (Germany)
  12. Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); SLAC National Accelerator Lab., Menlo Park, CA (United States)
  13. Bayerisches Geoinstitut (BGI), Bayreuth (Germany)
Publication Date:
Research Org.:
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Sponsoring Org.:
USDOE; Federal Ministry of Education and Research (BMBF); German Research Foundation (DFG)
OSTI Identifier:
1608571
Grant/Contract Number:  
AC02-76SF00515; STE 1079/4-1; 05K16RFB; 05K10PEC; 05K13PE2; 05K16PE1
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Synchrotron Radiation (Online)
Additional Journal Information:
Journal Name: Journal of Synchrotron Radiation (Online); Journal Volume: 27; Journal Issue: 2; Journal ID: ISSN 1600-5775
Publisher:
International Union of Crystallography
Country of Publication:
United States
Language:
English
Subject:
46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND TECHNOLOGY; laser heating; extreme conditions; X-ray emission spectroscopy; high pressure; nuclear resonant inelastic scattering

Citation Formats

Spiekermann, Georg, Kupenko, Ilya, Petitgirard, Sylvain, Harder, Manuel, Nyrow, Alexander, Weis, Christopher, Albers, Christian, Biedermann, Nicole, Libon, Lélia, Sahle, Christoph J., Cerantola, Valerio, Glazyrin, Konstantin, Konôpková, Zuzana, Sinmyo, Ryosuke, Morgenroth, Wolfgang, Sergueev, Ilya, Yavaş, Hasan, Dubrovinsky, Leonid, Tolan, Metin, Sternemann, Christian, and Wilke, Max. A portable on-axis laser-heating system for near-90° X-ray spectroscopy: application to ferropericlase and iron silicide. United States: N. p., 2020. Web. https://doi.org/10.1107/s1600577519017041.
Spiekermann, Georg, Kupenko, Ilya, Petitgirard, Sylvain, Harder, Manuel, Nyrow, Alexander, Weis, Christopher, Albers, Christian, Biedermann, Nicole, Libon, Lélia, Sahle, Christoph J., Cerantola, Valerio, Glazyrin, Konstantin, Konôpková, Zuzana, Sinmyo, Ryosuke, Morgenroth, Wolfgang, Sergueev, Ilya, Yavaş, Hasan, Dubrovinsky, Leonid, Tolan, Metin, Sternemann, Christian, & Wilke, Max. A portable on-axis laser-heating system for near-90° X-ray spectroscopy: application to ferropericlase and iron silicide. United States. https://doi.org/10.1107/s1600577519017041
Spiekermann, Georg, Kupenko, Ilya, Petitgirard, Sylvain, Harder, Manuel, Nyrow, Alexander, Weis, Christopher, Albers, Christian, Biedermann, Nicole, Libon, Lélia, Sahle, Christoph J., Cerantola, Valerio, Glazyrin, Konstantin, Konôpková, Zuzana, Sinmyo, Ryosuke, Morgenroth, Wolfgang, Sergueev, Ilya, Yavaş, Hasan, Dubrovinsky, Leonid, Tolan, Metin, Sternemann, Christian, and Wilke, Max. Thu . "A portable on-axis laser-heating system for near-90° X-ray spectroscopy: application to ferropericlase and iron silicide". United States. https://doi.org/10.1107/s1600577519017041. https://www.osti.gov/servlets/purl/1608571.
@article{osti_1608571,
title = {A portable on-axis laser-heating system for near-90° X-ray spectroscopy: application to ferropericlase and iron silicide},
author = {Spiekermann, Georg and Kupenko, Ilya and Petitgirard, Sylvain and Harder, Manuel and Nyrow, Alexander and Weis, Christopher and Albers, Christian and Biedermann, Nicole and Libon, Lélia and Sahle, Christoph J. and Cerantola, Valerio and Glazyrin, Konstantin and Konôpková, Zuzana and Sinmyo, Ryosuke and Morgenroth, Wolfgang and Sergueev, Ilya and Yavaş, Hasan and Dubrovinsky, Leonid and Tolan, Metin and Sternemann, Christian and Wilke, Max},
abstractNote = {A portable IR fiber laser-heating system, optimized for X-ray emission spectroscopy (XES) and nuclear inelastic scattering (NIS) spectroscopy with signal collection through the radial opening of diamond anvil cells near 90°with respect to the incident X-ray beam, is presented. The system offers double-sided on-axis heating by a single laser source and zero attenuation of incoming X-rays other than by the high-pressure environment. A description of the system, which has been tested for pressures above 100 GPa and temperatures up to 3000 K, is given. The XES spectra of laser-heated Mg0.67Fe0.33O demonstrate the potential to map the iron spin state in the pressure–temperature range of the Earth's lower mantle, and the NIS spectra of laser-heated FeSi give access to the sound velocity of this candidate of a phase inside the Earth's core. This portable system represents one of the few bridges across the gap between laser heating and high-resolution X-ray spectroscopies with signal collection near 90°.},
doi = {10.1107/s1600577519017041},
journal = {Journal of Synchrotron Radiation (Online)},
number = 2,
volume = 27,
place = {United States},
year = {2020},
month = {2}
}

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    Works referencing / citing this record:

    A portable on-axis laser-heating system for near-90° X-ray spectroscopy: application to ferropericlase and iron silicide
    text, January 2020

    • Spiekermann, Georg; Kupenko, Ilya; Petitgirard, Sylvain
    • Deutsches Elektronen-Synchrotron, DESY, Hamburg
    • DOI: 10.3204/pubdb-2020-00771