Extreme tensile strain states in La 0.7 Ca 0.3 MnO 3 membranes

Hong, Seung Sae; Gu, Mingqiang; Verma, Manish; Harbola, Varun; Wang, Bai Yang; Lu, Di; Vailionis, Arturas; Hikita, Yasuyuki; Pentcheva, Rossitza; Rondinelli, James M.; Hwang, Harold Y.

doi:10.1126/science.aax9753

Title: Extreme tensile strain states in La _0.7 Ca _0.3 MnO ₃ membranes

Abstract

A defining feature of emergent phenomena in complex oxides is the competition and cooperation between ground states. In manganites, the balance between metallic and insulating phases can be tuned by the lattice; extending the range of lattice control would enhance the ability to access other phases. We stabilized uniform extreme tensile strain in nanoscale La _0.7 Ca _0.3 MnO ₃ membranes, exceeding 8% uniaxially and 5% biaxially. Uniaxial and biaxial strain suppresses the ferromagnetic metal at distinctly different strain values, inducing an insulator that can be extinguished by a magnetic field. Electronic structure calculations indicate that the insulator consists of charge-ordered Mn ⁴⁺ and Mn ³⁺ with staggered strain-enhanced Jahn-Teller distortions within the plane. This highly tunable strained membrane approach provides a broad opportunity to design and manipulate correlated electron states.

Authors:

^[1];

^[2]; Verma, Manish ^[3];

^[4];

^[4]; Lu, Di ^[5];

^[6];

^[7];

^[3];

^[8];

^[9]

Department of Applied Physics, Stanford University, Stanford, CA 94305, USA., Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA., Department of Materials Science and Engineering, University of California, Davis, CA 95616, USA.
Department of Materials Science and Engineering, Northwestern University, Evanston, IL 60208, USA., Department of Physics, Southern University of Science and Technology, Shenzhen 518055, China.
Department of Physics and Center for Nanointegration (CENIDE), University of Duisburg-Essen, 47053 Duisburg, Germany.
Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA., Department of Physics, Stanford University, Stanford, CA 94305, USA.
Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA., Department of Materials Science and Engineering, Northwestern University, Evanston, IL 60208, USA., Department of Physics, Stanford University, Stanford, CA 94305, USA.
Stanford Nano Shared Facilities, Stanford University, Stanford, CA 94305, USA., Department of Physics, Kaunas University of Technology, LT-51368 Kaunas, Lithuania.
Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA.
Department of Materials Science and Engineering, Northwestern University, Evanston, IL 60208, USA.
Department of Applied Physics, Stanford University, Stanford, CA 94305, USA., Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, Menlo Park, CA 94025, USA.

Publication Date:: Thu Apr 02 00:00:00 EDT 2020

Research Org.:: SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., CA (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; Gordon and Betty Moore Foundation; US Air Force Office of Scientific Research (AFOSR); Army Research Office (ARO); German Science Foundation (DFG); National Science Foundation (NSF)

OSTI Identifier:: 1608079

Alternate Identifier(s):: OSTI ID: 1614877

Grant/Contract Number:: AC02-76SF00515; SC0012375; AC02-06CH11357; GBMF4415; FA9550-18-1-0480; W911NF-15-1-0017; ACI-1548562; INST20876/209-1 FUGG; INST20876/243-1 FUGG; ECCS-1542152

Resource Type:: Published Article

Journal Name:: Science

Additional Journal Information:: Journal Name: Science Journal Volume: 368 Journal Issue: 6486; Journal ID: ISSN 0036-8075

Publisher:: AAAS

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE

Citation Formats


                    Hong, Seung Sae, Gu, Mingqiang, Verma, Manish, Harbola, Varun, Wang, Bai Yang, Lu, Di, Vailionis, Arturas, Hikita, Yasuyuki, Pentcheva, Rossitza, Rondinelli, James M., and Hwang, Harold Y. Extreme tensile strain states in La 0.7 Ca 0.3 MnO 3 membranes.  United States: N. p., 2020. 
Web.  doi:10.1126/science.aax9753.

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                    Hong, Seung Sae, Gu, Mingqiang, Verma, Manish, Harbola, Varun, Wang, Bai Yang, Lu, Di, Vailionis, Arturas, Hikita, Yasuyuki, Pentcheva, Rossitza, Rondinelli, James M., & Hwang, Harold Y. Extreme tensile strain states in La 0.7 Ca 0.3 MnO 3 membranes.  United States.  https://doi.org/10.1126/science.aax9753

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                    Hong, Seung Sae, Gu, Mingqiang, Verma, Manish, Harbola, Varun, Wang, Bai Yang, Lu, Di, Vailionis, Arturas, Hikita, Yasuyuki, Pentcheva, Rossitza, Rondinelli, James M., and Hwang, Harold Y. Thu .  
"Extreme tensile strain states in La 0.7 Ca 0.3 MnO 3 membranes".  United States.  https://doi.org/10.1126/science.aax9753.

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@article{osti_1608079,

  title        = {Extreme tensile strain states in La 0.7 Ca 0.3 MnO 3 membranes},

  author       = {Hong, Seung Sae and Gu, Mingqiang and Verma, Manish and Harbola, Varun and Wang, Bai Yang and Lu, Di and Vailionis, Arturas and Hikita, Yasuyuki and Pentcheva, Rossitza and Rondinelli, James M. and Hwang, Harold Y.},

  abstractNote = {A defining feature of emergent phenomena in complex oxides is the competition and cooperation between ground states. In manganites, the balance between metallic and insulating phases can be tuned by the lattice; extending the range of lattice control would enhance the ability to access other phases. We stabilized uniform extreme tensile strain in nanoscale La 0.7 Ca 0.3 MnO 3 membranes, exceeding 8% uniaxially and 5% biaxially. Uniaxial and biaxial strain suppresses the ferromagnetic metal at distinctly different strain values, inducing an insulator that can be extinguished by a magnetic field. Electronic structure calculations indicate that the insulator consists of charge-ordered Mn 4+ and Mn 3+ with staggered strain-enhanced Jahn-Teller distortions within the plane. This highly tunable strained membrane approach provides a broad opportunity to design and manipulate correlated electron states.},

  doi          = {10.1126/science.aax9753},

  journal      = {Science},

  number       = 6486,

  volume       = 368,

  place        = {United States},

  year         = {Thu Apr 02 00:00:00 EDT 2020},

  month        = {Thu Apr 02 00:00:00 EDT 2020}

}

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Title: Extreme tensile strain states in La 0.7 Ca 0.3 MnO 3 membranes

Abstract

Citation Formats

Jahn-Teller distortion and magnetic structure in LaMnO 3 : A first-principles theoretical study with full structure optimizations journal, July 2010

Magnetic-field-induced metal-insulator phenomena in Pr 1 − x Ca x Mn O 3 with controlled charge-ordering instability journal, January 1996

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Pressure effects on the magnetoresistance in doped manganese perovskites journal, December 1995

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Title: Extreme tensile strain states in La _0.7 Ca _0.3 MnO ₃ membranes

Jahn-Teller distortion and magnetic structure in ${LaMnO}_{3}$ : A first-principles theoretical study with full structure optimizations
journal, July 2010

Magnetic-field-induced metal-insulator phenomena in $\Pr_{1 - x} {Ca}_{x} Mn O_{3}$ with controlled charge-ordering instability
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Synthesis and Structural Studies of Strontium-Substituted Tricalcium Aluminate Ca3-xSrxAl2O6
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Pairing of charge-ordered stripes in (La,Ca)MnO3
journal, April 1998

Uniaxial pressure control of competing orders in a high-temperature superconductor
journal, November 2018

Doubling the critical temperature of La1.9Sr0.1CuO4 using epitaxial strain
journal, July 1998

Elastic strain engineering of ferroic oxides
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Synthesis of freestanding single-crystal perovskite films and heterostructures by etching of sacrificial water-soluble layers
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Strong Increase of Tc of Sr2RuO4 Under Both Tensile and Compressive Strain
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From quantum matter to high-temperature superconductivity in copper oxides
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Cooperative photoinduced metastable phase control in strained manganite films
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Density-functional theory and strong interactions: Orbital ordering in Mott-Hubbard insulators
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Emergent phenomena at oxide interfaces
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Ultrathin Epitaxial Barrier Layer to Avoid Thermally Induced Phase Transformation in Oxide Heterostructures
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Assessing the Perdew-Burke-Ernzerhof exchange-correlation density functional revised for metallic bulk and surface systems
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