Designing and transforming yield-stress fluids

Nelson, Arif Z.; Schweizer, Kenneth S.; Rauzan, Brittany M.; Nuzzo, Ralph G.; Vermant, Jan; Ewoldt, Randy H.

doi:10.1016/j.cossms.2019.06.002

Title: Designing and transforming yield-stress fluids

Journal Article · 29 July 2019 · Current Opinion in Solid State and Materials Science

DOI: https://doi.org/10.1016/j.cossms.2019.06.002 · OSTI ID:1607400

Nelson, Arif Z. ^[1]; Schweizer, Kenneth S. ^[2]; Rauzan, Brittany M. ^[2]; Nuzzo, Ralph G. ^[3]; Vermant, Jan ^[4]; Ewoldt, Randy H. ^[2]

Univ. of Illinois at Urbana-Champaign, IL (United States); Singapore-MIT Alliance for Research and Technology (Singapore)
Univ. of Illinois at Urbana-Champaign, IL (United States)
Univ. of Illinois at Urbana-Champaign, IL (United States); KTH Royal Inst. of Technology, Stockholm (Sweden)
ETH Zurich (Switzerland)

We review progress in designing and transforming multi-functional yield-stress fluids and give a perspective on the current state of knowledge that supports each step in the design process. We focus mainly on the rheological properties that make yield-stress fluids so useful and the trade-offs which need to be considered when working with these materials. Thinking in terms of "design with" and "design of' yield-stress fluids motivates how we can organize our scientific understanding of this field. "Design with" involves identification of rheological property requirements independent of the chemical formulation, e.g. for 3D direct-write printing which needs to accommodate a wide range of chemistry and material structures. "Design of includes microstructural considerations: conceptual models relating formulation to properties, quantitative models of formulation-structureproperty relations, and chemical transformation strategies for converting effective yield-stress fluids to be more useful solid engineering materials. Finally, future research directions are suggested at the intersection of chemistry, soft-matter physics, and material science in the context of our desire to design useful Theologically-complex functional materials.

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Research Organization:: Univ. of Illinois at Urbana-Champaign, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: FG02-07ER46471

OSTI ID:: 1607400

Alternate ID(s):: OSTI ID: 1606468

Journal Information:: Current Opinion in Solid State and Materials Science, Vol. 23, Issue 5; ISSN 1359-0286

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Viscoplastic drop impact on thin films Sen, Samya; Morales, Anthony G.; Ewoldt, Randy H. Journal of Fluid Mechanics, Vol. 891 https://doi.org/10.1017/jfm.2020.147	journal	March 2020

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Related Subjects

36 MATERIALS SCIENCE
soft matter
yield-stress fluid
design
engineering
extension
thixotropy
elasticity
colloids
emulsions
polymers
3D printing
chemistry
physics
rheology
complex fluids