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Title: Extreme Fermi Surface Smearing in a Maximally Disordered Concentrated Solid Solution

Abstract

We show that the Fermi surface can survive the presence of extreme compositional disorder in the equiatomic alloy Ni0.25Fe0.25Co0.25Cr0.25. Our high-resolution Compton scattering experiments reveal a Fermi surface which is smeared across a significant fraction of the Brillouin zone (up to 40% of $$\frac{2π}{a}$$). The extent of this smearing and its variation on and between different sheets of the Fermi surface have been determined, and estimates of the electron mean free path and residual resistivity have been made by connecting this smearing with the coherence length of the quasiparticle states.

Authors:
 [1];  [1];  [1]; ORCiD logo [1];  [2];  [3];  [3];  [2];  [4]; ORCiD logo [5]; ORCiD logo [5]; ORCiD logo [6]; ORCiD logo [6]; ORCiD logo [6]; ORCiD logo [6]; ORCiD logo [1]
+ Show Author Affiliations
  1. Univ. of Bristol (United Kingdom)
  2. Cardiff Univ. (United Kingdom)
  3. Univ. of Warwick (United Kingdom)
  4. Data Management and Software Center of the European Spallation Source, Copenhagen (Denmark)
  5. Polish Academy of Sciences (PAS), Krakow (Poland). Inst. of Low Temperature and Structure Research
  6. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Publication Date:
Research Org.:
Energy Frontier Research Centers (EFRC) (United States). Energy Dissipation to Defect Evolution (EDDE); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
OSTI Identifier:
1606651
Grant/Contract Number:  
AC05-00OR22725
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review Letters
Additional Journal Information:
Journal Volume: 124; Journal Issue: 4; Journal ID: ISSN 0031-9007
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; Electronic structure; Fermi surface; Disordered alloys; Transition-metal alloys; Compton scattering; Density functional theory

Citation Formats

Robarts, Hannah C., Millichamp, Thomas E., Lagos, Daniel A., Laverock, Jude, Billington, David, Duffy, Jonathan A., O’Neill, Daniel, Giblin, Sean R., Taylor, Jonathan W., Kontrym-Sznajd, Grazyna, Samsel-Czekala, Malgorzata, Bei, Hongbin, Mu, Sai, Samolyuk, German D., Stocks, George, and Dugdale, Stephen B. Extreme Fermi Surface Smearing in a Maximally Disordered Concentrated Solid Solution. United States: N. p., 2020. Web. doi:10.1103/PhysRevLett.124.046402.
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Robarts, Hannah C., Millichamp, Thomas E., Lagos, Daniel A., Laverock, Jude, Billington, David, Duffy, Jonathan A., O’Neill, Daniel, Giblin, Sean R., Taylor, Jonathan W., Kontrym-Sznajd, Grazyna, Samsel-Czekala, Malgorzata, Bei, Hongbin, Mu, Sai, Samolyuk, German D., Stocks, George, & Dugdale, Stephen B. Extreme Fermi Surface Smearing in a Maximally Disordered Concentrated Solid Solution. United States. https://doi.org/10.1103/PhysRevLett.124.046402
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Robarts, Hannah C., Millichamp, Thomas E., Lagos, Daniel A., Laverock, Jude, Billington, David, Duffy, Jonathan A., O’Neill, Daniel, Giblin, Sean R., Taylor, Jonathan W., Kontrym-Sznajd, Grazyna, Samsel-Czekala, Malgorzata, Bei, Hongbin, Mu, Sai, Samolyuk, German D., Stocks, George, and Dugdale, Stephen B. Thu . "Extreme Fermi Surface Smearing in a Maximally Disordered Concentrated Solid Solution". United States. https://doi.org/10.1103/PhysRevLett.124.046402. https://www.osti.gov/servlets/purl/1606651.
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@article{osti_1606651,
title = {Extreme Fermi Surface Smearing in a Maximally Disordered Concentrated Solid Solution},
author = {Robarts, Hannah C. and Millichamp, Thomas E. and Lagos, Daniel A. and Laverock, Jude and Billington, David and Duffy, Jonathan A. and O’Neill, Daniel and Giblin, Sean R. and Taylor, Jonathan W. and Kontrym-Sznajd, Grazyna and Samsel-Czekala, Malgorzata and Bei, Hongbin and Mu, Sai and Samolyuk, German D. and Stocks, George and Dugdale, Stephen B.},
abstractNote = {We show that the Fermi surface can survive the presence of extreme compositional disorder in the equiatomic alloy Ni0.25Fe0.25Co0.25Cr0.25. Our high-resolution Compton scattering experiments reveal a Fermi surface which is smeared across a significant fraction of the Brillouin zone (up to 40% of $\frac{2π}{a}$). The extent of this smearing and its variation on and between different sheets of the Fermi surface have been determined, and estimates of the electron mean free path and residual resistivity have been made by connecting this smearing with the coherence length of the quasiparticle states.},
doi = {10.1103/PhysRevLett.124.046402},
journal = {Physical Review Letters},
number = 4,
volume = 124,
place = {United States},
year = {2020},
month = {1}
}
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https://doi.org/10.1103/PhysRevLett.124.046402
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Works referenced in this record:

Universality of the Mott–Ioffe–Regel limit in metals
journal, September 2004

Electronic properties of random alloys: Special quasirandom structures
journal, November 1990

Microstructural development in equiatomic multicomponent alloys
journal, July 2004

Solution of the Schrödinger Equation in Periodic Lattices with an Application to Metallic Lithium
journal, June 1954

A product representation for cubic harmonics and special directions for the determination of the Fermi surface and related properties
journal, November 1976

  • Fehlner, W. R.; Vosko, S. H.
  • Canadian Journal of Physics, Vol. 54, Issue 21
  • DOI: 10.1139/p76-256

Ferrimagnetism in Fe-rich NbFe 2
journal, March 2012

Accurate spin-dependent electron liquid correlation energies for local spin density calculations: a critical analysis
journal, August 1980

  • Vosko, S. H.; Wilk, L.; Nusair, M.
  • Canadian Journal of Physics, Vol. 58, Issue 8
  • DOI: 10.1139/p80-159

X-Ray Scattering from an Electron Gas
journal, July 1965

Thermophysical properties of Ni-containing single-phase concentrated solid solution alloys
journal, March 2017

Phonon broadening in high entropy alloys
journal, September 2017

  • Körmann, Fritz; Ikeda, Yuji; Grabowski, Blazej
  • npj Computational Materials, Vol. 3, Issue 1
  • DOI: 10.1038/s41524-017-0037-8

Calculating the Berry curvature of Bloch electrons using the KKR method
journal, August 2011

Calculating electron momentum densities and Compton profiles using the linear tetrahedron method
journal, November 2014

Compton Scattering of X Rays from Bound Electrons
journal, August 1970

Electrical, magnetic, and Hall properties of AlxCoCrFeNi high-entropy alloys
journal, February 2011

Positron annihilation and Fermi surface studies: a new approach
journal, March 1973

  • Lock, D. G.; Crisp, V. H. C.; West, R. N.
  • Journal of Physics F: Metal Physics, Vol. 3, Issue 3
  • DOI: 10.1088/0305-4608/3/3/014

Hartree-Fock Compton profiles for the elements
journal, September 1975

Uncovering electron scattering mechanisms in NiFeCoCrMn derived concentrated solid solution and high entropy alloys
journal, January 2019

  • Mu, Sai; Samolyuk, German D.; Wimmer, Sebastian
  • npj Computational Materials, Vol. 5, Issue 1
  • DOI: 10.1038/s41524-018-0138-z

A first-principles theory of ferromagnetic phase transitions in metals
journal, June 1985

  • Gyorffy, B. L.; Pindor, A. J.; Staunton, J.
  • Journal of Physics F: Metal Physics, Vol. 15, Issue 6
  • DOI: 10.1088/0305-4608/15/6/018

Concentration Waves and Fermi Surfaces in Random Metallic Alloys
journal, January 1983

On the calculation of the energy of a Bloch wave in a metal
journal, August 1947

NiFeCoCr
dataset, January 2019

Efficient stochastic generation of special quasirandom structures
journal, September 2013

Momentum Distribution and Renormalization Factor in Sodium and the Electron Gas
journal, August 2010

The Boltzmann Equation in the Theory of Electrical Conduction in Metals
journal, April 1958

Electron and electron-positron momentum distributions in concentrated random alloys
journal, November 1984

Discovery of a Superconducting High-Entropy Alloy
journal, September 2014

A key concept from the electron theory of metals: history of the fermi surface 1933–60
journal, January 1983

Fermi Surface Nesting in Disordered Cu 1 − x Pd x Alloys
journal, October 2001

Electronic structure of metallic ferromagnets above the Curie temperature
journal, June 1985

  • Staunton, J.; Gyorffy, B. L.; Pindor, A. J.
  • Journal of Physics F: Metal Physics, Vol. 15, Issue 6
  • DOI: 10.1088/0305-4608/15/6/019

Simulation of Compton Double Scatterings of Circularly Polarized γ-Rays by Magnetic Electrons
journal, July 1987

  • Sakai, Nobuhiko
  • Journal of the Physical Society of Japan, Vol. 56, Issue 7
  • DOI: 10.1143/JPSJ.56.2477

Special directions in momentum space. I. Cubic symmetries
journal, October 2011

  • Kontrym-Sznajd, G.; Samsel-Czekała, M.
  • Journal of Applied Crystallography, Vol. 44, Issue 6
  • DOI: 10.1107/S0021889811037411

Probing the Fermi surface by positron annihilation and Compton scattering
journal, April 2014

Mean Free Path of Electrons and Magnetomorphic Effects in Small Single Crystals of Gallium
journal, February 1965

Electronic correlations in vanadium revealed by electron-positron annihilation measurements
journal, February 2017

Fermi Surface and Some Simple Equilibrium Properties of a System of Interacting Fermions
journal, August 1960

A critical review of high entropy alloys and related concepts
journal, January 2017

Theory of electronic transport in random alloys with short-range order: Korringa-Kohn-Rostoker nonlocal coherent potential approximation
journal, April 2008

Optical conductivity of metal alloys with residual resistivities near or above the Mott-Ioffe-Regel limit
journal, August 2019

The alloy theoretic automated toolkit: A user guide
journal, December 2002

A new X-ray spectrometer for high-resolution Compton profile measurements at SPring-8
journal, January 2001

Accurate and simple analytic representation of the electron-gas correlation energy
journal, June 1992

Calculating properties with the coherent-potential approximation
journal, April 1980

Tailoring the physical properties of Ni-based single-phase equiatomic alloys by modifying the chemical complexity
journal, February 2016

  • Jin, K.; Sales, B. C.; Stocks, G. M.
  • Scientific Reports, Vol. 6, Issue 1
  • DOI: 10.1038/srep20159

Special quasirandom structures
journal, July 1990

Simulation of Compton Double Scatterings of Circularly Polarized γ-Rays by Magnetic Electrons
journal, July 1991

  • Sakai, Nobuhiko
  • Journal of the Physical Society of Japan, Vol. 60, Issue 7
  • DOI: 10.1143/jpsj.60.2483

How to estimate isotropic distributions and mean values in crystalline solids
journal, October 2015

Alloying effect of tungsten on the structural and magnetic properties of CoCrFeNiW high entropy alloys
journal, September 2018

New reconstruction method of electron momentum densities from Compton profiles
journal, January 2000

  • Kontrym-Sznajd, G.; Samsel-Czekała, M.
  • Applied Physics A: Materials Science & Processing, Vol. 70, Issue 1
  • DOI: 10.1007/s003390050017

Coherent-Potential Model of Substitutional Disordered Alloys
journal, April 1967

Microstructures and mechanical properties of a directionally solidified NiAl–Mo eutectic alloy
journal, January 2005

Local lattice distortion in high-entropy alloys
journal, July 2017

Electron mean free path in elemental metals
journal, February 2016

Momentum Distribution and Renormalization Factor in Sodium and the Electron Gas
text, January 2010

On calculating the Berry curvature of Bloch electrons using the KKR method
text, January 2011

Calculating electron momentum densities and Compton profiles using the linear tetrahedron method
text, January 2014

Electronic Correlations in Vanadium Revealed by Electron-Positron Annihilation Measurements
text, January 2016

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