Co-feeding copper catalysts couple carbon
Abstract
Here, the mechanistic electrochemical mass spectrometry study of ethylene production on Cu-based nanocatalysts under CO2/CO co-feeds indicates the existence of separate, reactant-specific surface adsorption sites for CO2 and CO, which guided the design of a multi-component CO2RR electrocatalyst.
- Authors:
-
- Univ. of California, Berkeley, CA (United States). Kavli Energy NanoScience Inst.; Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC)
- OSTI Identifier:
- 1605258
- Grant/Contract Number:
- AC02-05CH11231
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Nanotechnology
- Additional Journal Information:
- Journal Volume: 14; Journal Issue: 11; Journal ID: ISSN 1748-3387
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
Citation Formats
Li, Yifan, and Yang, Peidong. Co-feeding copper catalysts couple carbon. United States: N. p., 2019.
Web. doi:10.1038/s41565-019-0575-y.
Li, Yifan, & Yang, Peidong. Co-feeding copper catalysts couple carbon. United States. https://doi.org/10.1038/s41565-019-0575-y
Li, Yifan, and Yang, Peidong. Tue .
"Co-feeding copper catalysts couple carbon". United States. https://doi.org/10.1038/s41565-019-0575-y. https://www.osti.gov/servlets/purl/1605258.
@article{osti_1605258,
title = {Co-feeding copper catalysts couple carbon},
author = {Li, Yifan and Yang, Peidong},
abstractNote = {Here, the mechanistic electrochemical mass spectrometry study of ethylene production on Cu-based nanocatalysts under CO2/CO co-feeds indicates the existence of separate, reactant-specific surface adsorption sites for CO2 and CO, which guided the design of a multi-component CO2RR electrocatalyst.},
doi = {10.1038/s41565-019-0575-y},
journal = {Nature Nanotechnology},
number = 11,
volume = 14,
place = {United States},
year = {Tue Oct 22 00:00:00 EDT 2019},
month = {Tue Oct 22 00:00:00 EDT 2019}
}
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Cited by: 3 works
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Figures / Tables:
Figure 1: Cross-coupling of CO and CO2-derived species to result in increased C2H4 yields in co-feed conditions on copper oxide derived nanoparticle catalysts. (a) Isotopic labeling in combination with operando DEMS in co-feed conditions shows a plurality of cross-coupled C2H4 from 13CO and 12CO2 sources. (b) A sequential bifunctional catalystmore »
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Works referenced in this record:
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Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.