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Title: Attosecond pulse shaping using a seeded free-electron laser

Abstract

Attosecond pulses are central to the investigation of valence- and core-electron dynamics on their natural timescales. The reproducible generation and characterization of attosecond waveforms has been demonstrated so far only through the process of high-order harmonic generation. Several methods for shaping attosecond waveforms have been proposed, including the use of metallic filters, multilayer mirrors and manipulation of the driving field. However, none of these approaches allows the flexible manipulation of the temporal characteristics of the attosecond waveforms, and they suffer from the low conversion efficiency of the high-order harmonic generation process. Free-electron lasers, by contrast, deliver femtosecond, extreme-ultraviolet and X-ray pulses with energies ranging from tens of microjoules to a few millijoules. Recent experiments have shown that they can generate subfemtosecond spikes, but with temporal characteristics that change shot-to-shot. In this paper we report reproducible generation of high-energy (microjoule level) attosecond waveforms using a seeded free-electron laser. We demonstrate amplitude and phase manipulation of the harmonic components of an attosecond pulse train in combination with an approach for its temporal reconstruction. The results presented here open the way to performing attosecond time-resolved experiments with free-electron lasers.

Authors:
 [1];  [2];  [3];  [1];  [1];  [1];  [3];  [3];  [3];  [4];  [5];  [3];  [3];  [3];  [3];  [3];  [3];  [3];  [3];  [3] more »;  [6];  [7];  [7];  [8];  [9];  [10];  [10];  [11];  [11];  [11];  [11];  [12];  [12];  [12];  [12];  [13];  [13];  [14];  [14];  [14];  [15];  [15];  [3];  [3];  [1] « less
  1. Albert-Ludwigs-Univ., Freiburg (Germany)
  2. The National Research Council (CNR), Trieste (Italy). Inst. of Structure of Matter (ISM)
  3. Elettra-Sincrotrone Trieste (Italy)
  4. Elettra-Sincrotrone Trieste (Italy); Lab. Nazionali di Frascati, Rome (Italy). Istituto Nazionale di Fisica Nucleare
  5. Elettra-Sincrotrone Trieste (Italy); Univ. of Nova Gorica (Slovenia)
  6. SLAC National Accelerator Lab., Menlo Park, CA (United States)
  7. Univ. of Gothenburg (Sweden)
  8. Technische Univ. Wien, Vienna (Austria)
  9. Politecnico di Milano (Italy)
  10. European XFEL GmbH, Schenefeld (Germany)
  11. Lund Univ. (Sweden)
  12. ELI-ALPS, Szeged (Hungary)
  13. Tohoku Univ., Sendai (Japan)
  14. Louisiana State Univ., Baton Rouge, LA (United States)
  15. Lomonosov Moscow State Univ., Moscow (Russia)
Publication Date:
Research Org.:
SLAC National Accelerator Lab., Menlo Park, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC); European Union’s Horizon 2020; Italian Ministry of Research; Ministry of Education, Culture, Sports, Science and Technology of Japan (MEXT); Cooperative Research Program; The National Research Council (CNR); Japan Society for the Promotion of Science (JSPS); IMRAM Project; Swedish Research Council (VR); Knut and Alice Wallenberg Foundation; Foundation for the Advancement of Theoretical Physics and Mathematics; German Research Foundation (DFG)
OSTI Identifier:
1604577
Grant/Contract Number:  
AC02-76SF00515; 641789 MEDEA; SFB925/1; SC0010431
Resource Type:
Accepted Manuscript
Journal Name:
Nature (London)
Additional Journal Information:
Journal Name: Nature (London); Journal Volume: 578; Journal Issue: 7795; Journal ID: ISSN 0028-0836
Publisher:
Nature Publishing Group
Country of Publication:
United States
Language:
English
Subject:
47 OTHER INSTRUMENTATION; Free-electron lasers; High-harmonic generation; Ultrafast lasers

Citation Formats

Maroju, Praveen Kumar, Grazioli, Cesare, Di Fraia, Michele, Moioli, Matteo, Ertel, Dominik, Ahmadi, Hamed, Plekan, Oksana, Finetti, Paola, Allaria, Enrico, Giannessi, Luca, De Ninno, Giovanni, Spezzani, Carlo, Penco, Giuseppe, Spampinati, Simone, Demidovich, Alexander, Danailov, Miltcho B., Borghes, Roberto, Kourousias, George, Sanches Dos Reis, Carlos Eduardo, Billé, Fulvio, Lutman, Alberto A., Squibb, Richard J., Feifel, Raimund, Carpeggiani, Paolo, Reduzzi, Maurizio, Mazza, Tommaso, Meyer, Michael, Bengtsson, Samuel, Ibrakovic, Neven, Simpson, Emma Rose, Mauritsson, Johan, Csizmadia, Tamás, Dumergue, Mathieu, Kühn, Sergei, Nandiga Gopalakrishna, Harshitha, You, Daehyun, Ueda, Kiyoshi, Labeye, Marie, Bækhøj, Jens Egebjerg, Schafer, Kenneth J., Gryzlova, Elena V., Grum-Grzhimailo, Alexei N., Prince, Kevin C., Callegari, Carlo, and Sansone, Giuseppe. Attosecond pulse shaping using a seeded free-electron laser. United States: N. p., 2020. Web. https://doi.org/10.1038/s41586-020-2005-6.
Maroju, Praveen Kumar, Grazioli, Cesare, Di Fraia, Michele, Moioli, Matteo, Ertel, Dominik, Ahmadi, Hamed, Plekan, Oksana, Finetti, Paola, Allaria, Enrico, Giannessi, Luca, De Ninno, Giovanni, Spezzani, Carlo, Penco, Giuseppe, Spampinati, Simone, Demidovich, Alexander, Danailov, Miltcho B., Borghes, Roberto, Kourousias, George, Sanches Dos Reis, Carlos Eduardo, Billé, Fulvio, Lutman, Alberto A., Squibb, Richard J., Feifel, Raimund, Carpeggiani, Paolo, Reduzzi, Maurizio, Mazza, Tommaso, Meyer, Michael, Bengtsson, Samuel, Ibrakovic, Neven, Simpson, Emma Rose, Mauritsson, Johan, Csizmadia, Tamás, Dumergue, Mathieu, Kühn, Sergei, Nandiga Gopalakrishna, Harshitha, You, Daehyun, Ueda, Kiyoshi, Labeye, Marie, Bækhøj, Jens Egebjerg, Schafer, Kenneth J., Gryzlova, Elena V., Grum-Grzhimailo, Alexei N., Prince, Kevin C., Callegari, Carlo, & Sansone, Giuseppe. Attosecond pulse shaping using a seeded free-electron laser. United States. https://doi.org/10.1038/s41586-020-2005-6
Maroju, Praveen Kumar, Grazioli, Cesare, Di Fraia, Michele, Moioli, Matteo, Ertel, Dominik, Ahmadi, Hamed, Plekan, Oksana, Finetti, Paola, Allaria, Enrico, Giannessi, Luca, De Ninno, Giovanni, Spezzani, Carlo, Penco, Giuseppe, Spampinati, Simone, Demidovich, Alexander, Danailov, Miltcho B., Borghes, Roberto, Kourousias, George, Sanches Dos Reis, Carlos Eduardo, Billé, Fulvio, Lutman, Alberto A., Squibb, Richard J., Feifel, Raimund, Carpeggiani, Paolo, Reduzzi, Maurizio, Mazza, Tommaso, Meyer, Michael, Bengtsson, Samuel, Ibrakovic, Neven, Simpson, Emma Rose, Mauritsson, Johan, Csizmadia, Tamás, Dumergue, Mathieu, Kühn, Sergei, Nandiga Gopalakrishna, Harshitha, You, Daehyun, Ueda, Kiyoshi, Labeye, Marie, Bækhøj, Jens Egebjerg, Schafer, Kenneth J., Gryzlova, Elena V., Grum-Grzhimailo, Alexei N., Prince, Kevin C., Callegari, Carlo, and Sansone, Giuseppe. Mon . "Attosecond pulse shaping using a seeded free-electron laser". United States. https://doi.org/10.1038/s41586-020-2005-6. https://www.osti.gov/servlets/purl/1604577.
@article{osti_1604577,
title = {Attosecond pulse shaping using a seeded free-electron laser},
author = {Maroju, Praveen Kumar and Grazioli, Cesare and Di Fraia, Michele and Moioli, Matteo and Ertel, Dominik and Ahmadi, Hamed and Plekan, Oksana and Finetti, Paola and Allaria, Enrico and Giannessi, Luca and De Ninno, Giovanni and Spezzani, Carlo and Penco, Giuseppe and Spampinati, Simone and Demidovich, Alexander and Danailov, Miltcho B. and Borghes, Roberto and Kourousias, George and Sanches Dos Reis, Carlos Eduardo and Billé, Fulvio and Lutman, Alberto A. and Squibb, Richard J. and Feifel, Raimund and Carpeggiani, Paolo and Reduzzi, Maurizio and Mazza, Tommaso and Meyer, Michael and Bengtsson, Samuel and Ibrakovic, Neven and Simpson, Emma Rose and Mauritsson, Johan and Csizmadia, Tamás and Dumergue, Mathieu and Kühn, Sergei and Nandiga Gopalakrishna, Harshitha and You, Daehyun and Ueda, Kiyoshi and Labeye, Marie and Bækhøj, Jens Egebjerg and Schafer, Kenneth J. and Gryzlova, Elena V. and Grum-Grzhimailo, Alexei N. and Prince, Kevin C. and Callegari, Carlo and Sansone, Giuseppe},
abstractNote = {Attosecond pulses are central to the investigation of valence- and core-electron dynamics on their natural timescales. The reproducible generation and characterization of attosecond waveforms has been demonstrated so far only through the process of high-order harmonic generation. Several methods for shaping attosecond waveforms have been proposed, including the use of metallic filters, multilayer mirrors and manipulation of the driving field. However, none of these approaches allows the flexible manipulation of the temporal characteristics of the attosecond waveforms, and they suffer from the low conversion efficiency of the high-order harmonic generation process. Free-electron lasers, by contrast, deliver femtosecond, extreme-ultraviolet and X-ray pulses with energies ranging from tens of microjoules to a few millijoules. Recent experiments have shown that they can generate subfemtosecond spikes, but with temporal characteristics that change shot-to-shot. In this paper we report reproducible generation of high-energy (microjoule level) attosecond waveforms using a seeded free-electron laser. We demonstrate amplitude and phase manipulation of the harmonic components of an attosecond pulse train in combination with an approach for its temporal reconstruction. The results presented here open the way to performing attosecond time-resolved experiments with free-electron lasers.},
doi = {10.1038/s41586-020-2005-6},
journal = {Nature (London)},
number = 7795,
volume = 578,
place = {United States},
year = {2020},
month = {2}
}

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Works referenced in this record:

Atomic transient recorder
journal, February 2004

  • Kienberger, R.; Goulielmakis, E.; Uiberacker, M.
  • Nature, Vol. 427, Issue 6977
  • DOI: 10.1038/nature02277

Operation of a free-electron laser from the extreme ultraviolet to the water window
journal, June 2007


Shaped-pulse optimization of coherent emission of high-harmonic soft X-rays
journal, July 2000

  • Bartels, R.; Backus, S.; Zeek, E.
  • Nature, Vol. 406, Issue 6792, p. 164-166
  • DOI: 10.1038/35018029

First lasing and operation of an ångstrom-wavelength free-electron laser
journal, August 2010


Broadband attosecond pulse shaping
journal, January 2007

  • Gustafsson, E.; Ruchon, T.; Swoboda, M.
  • Optics Letters, Vol. 32, Issue 11
  • DOI: 10.1364/OL.32.001353

Attosecond science
journal, June 2007

  • Corkum, P. B.; Krausz, Ferenc
  • Nature Physics, Vol. 3, Issue 6
  • DOI: 10.1038/nphys620

Experimental demonstration of a single-spike hard-X-ray free-electron laser starting from noise
journal, October 2017

  • Marinelli, A.; MacArthur, J.; Emma, P.
  • Applied Physics Letters, Vol. 111, Issue 15
  • DOI: 10.1063/1.4990716

Amplitude and Phase Control of Attosecond Light Pulses
journal, January 2005


Observation and Control of Laser-Enabled Auger Decay
journal, August 2017


Interferometric Autocorrelation of an Attosecond Pulse Train in the Single-Cycle Regime
journal, October 2006


Multiple ionization of argon via multi-XUV-photon absorption induced by 20-GW high-order harmonic laser pulses
journal, August 2018


Attosecond nonlinear optics using gigawatt-scale isolated attosecond pulses
journal, October 2013

  • Takahashi, Eiji J.; Lan, Pengfei; Mücke, Oliver D.
  • Nature Communications, Vol. 4, Issue 1
  • DOI: 10.1038/ncomms3691

Coherent soft X-ray pulses from an echo-enabled harmonic generation free-electron laser
journal, May 2019

  • Rebernik Ribič, Primož; Abrami, Alessandro; Badano, Laura
  • Nature Photonics, Vol. 13, Issue 8
  • DOI: 10.1038/s41566-019-0427-1

Attosecond physics
journal, February 2009


Observation of a Train of Attosecond Pulses from High Harmonic Generation
journal, June 2001


Mode Locking in a Free-Electron Laser Amplifier
journal, May 2008


Coherent control with a short-wavelength free-electron laser
journal, February 2016


Highly coherent and stable pulses from the FERMI seeded free-electron laser in the extreme ultraviolet
journal, September 2012


Harnessing Attosecond Science in the Quest for Coherent X-rays
journal, August 2007


Femtosecond all-optical synchronization of an X-ray free-electron laser
journal, January 2015

  • Schulz, S.; Grguraš, I.; Behrens, C.
  • Nature Communications, Vol. 6, Issue 1
  • DOI: 10.1038/ncomms6938

Recent results of PADReS, the Photon Analysis Delivery and REduction System, from the FERMI FEL commissioning and user operations
journal, April 2015

  • Zangrando, Marco; Cocco, Daniele; Fava, Claudio
  • Journal of Synchrotron Radiation, Vol. 22, Issue 3
  • DOI: 10.1107/S1600577515004580

Attosecond time–energy structure of X-ray free-electron laser pulses
journal, March 2018


Generating Single-Spike Hard X-Ray Pulses with Nonlinear Bunch Compression in Free-Electron Lasers
journal, October 2017


Attosecond Synchronization of High-Harmonic Soft X-rays
journal, November 2003


Direct observation of attosecond light bunching
journal, November 2003

  • Tzallas, P.; Charalambidis, D.; Papadogiannis, N. A.
  • Nature, Vol. 426, Issue 6964
  • DOI: 10.1038/nature02091

Attosecond dispersion control by extreme ultraviolet multilayer mirrors
journal, January 2011

  • Hofstetter, Michael; Schultze, Martin; Fieß, Markus
  • Optics Express, Vol. 19, Issue 3
  • DOI: 10.1364/OE.19.001767

Towards jitter-free pump-probe measurements at seeded free electron laser facilities
journal, January 2014

  • Danailov, Miltcho B.; Bencivenga, Filippo; Capotondi, Flavio
  • Optics Express, Vol. 22, Issue 11
  • DOI: 10.1364/OE.22.012869

Method of an enhanced self-amplified spontaneous emission for x-ray free electron lasers
journal, April 2005


    Works referencing / citing this record:

    Attosecond resolution from free running interferometric measurements
    journal, January 2020

    • Krüger, Constantin; Fuchs, Jaco; Cattaneo, Laura
    • Optics Express, Vol. 28, Issue 9
    • DOI: 10.1364/oe.391791