Gap-like feature observed in the non-magnetic topological insulators
Abstract
Non-magnetic gap at the Dirac point of topological insulators remains an open question in the field. Here, we present angle-resolved photoemission spectroscopy experiments performed on Cr-doped Bi2Se3 and showed that the Dirac point is progressively buried by the bulk bands and a low spectral weight region in the vicinity of the Dirac point appears. These two mechanisms lead to spectral weight suppression region being mistakenly identified as an energy gap in earlier studies. We further calculated the band structure and found that the original Dirac point splits into two nodes due to the impurity resonant states and the energy separation between the nodes is the low density of state region which appears to be like an energy gap in potoemission experiments. Furthermore, we supported our arguments by presenting photoemission experiments carried out with on- and off- resonant photon energies. Our observation resolves the widely debated questions of apparent energy gap opening at the Dirac point without long range ferromagnetic order in topological insulators.
- Authors:
- Publication Date:
- Research Org.:
- Brookhaven National Lab. (BNL), Upton, NY (United States). National Synchrotron Light Source II (NSLS-II)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); University of Connecticut; USDOE Laboratory Directed Research and Development (LDRD) Program
- OSTI Identifier:
- 1604317
- Report Number(s):
- BNL-213701-2020-JAAM
Journal ID: ISSN 0953-8984
- Grant/Contract Number:
- SC0012704; 4626510
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Physics. Condensed Matter
- Additional Journal Information:
- Journal Volume: 32; Journal Issue: 14; Journal ID: ISSN 0953-8984
- Publisher:
- IOP Publishing
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; topological insulators; time reversal symmetry; ARPES
Citation Formats
Yilmaz, T., Pertsova, A., Hines, W., Vescovo, E., Kaznatcheev, K., Balatsky, A. V., and Sinkovic, B. Gap-like feature observed in the non-magnetic topological insulators. United States: N. p., 2020.
Web. doi:10.1088/1361-648X/ab6349.
Yilmaz, T., Pertsova, A., Hines, W., Vescovo, E., Kaznatcheev, K., Balatsky, A. V., & Sinkovic, B. Gap-like feature observed in the non-magnetic topological insulators. United States. https://doi.org/10.1088/1361-648X/ab6349
Yilmaz, T., Pertsova, A., Hines, W., Vescovo, E., Kaznatcheev, K., Balatsky, A. V., and Sinkovic, B. Wed .
"Gap-like feature observed in the non-magnetic topological insulators". United States. https://doi.org/10.1088/1361-648X/ab6349. https://www.osti.gov/servlets/purl/1604317.
@article{osti_1604317,
title = {Gap-like feature observed in the non-magnetic topological insulators},
author = {Yilmaz, T. and Pertsova, A. and Hines, W. and Vescovo, E. and Kaznatcheev, K. and Balatsky, A. V. and Sinkovic, B.},
abstractNote = {Non-magnetic gap at the Dirac point of topological insulators remains an open question in the field. Here, we present angle-resolved photoemission spectroscopy experiments performed on Cr-doped Bi2Se3 and showed that the Dirac point is progressively buried by the bulk bands and a low spectral weight region in the vicinity of the Dirac point appears. These two mechanisms lead to spectral weight suppression region being mistakenly identified as an energy gap in earlier studies. We further calculated the band structure and found that the original Dirac point splits into two nodes due to the impurity resonant states and the energy separation between the nodes is the low density of state region which appears to be like an energy gap in potoemission experiments. Furthermore, we supported our arguments by presenting photoemission experiments carried out with on- and off- resonant photon energies. Our observation resolves the widely debated questions of apparent energy gap opening at the Dirac point without long range ferromagnetic order in topological insulators.},
doi = {10.1088/1361-648X/ab6349},
journal = {Journal of Physics. Condensed Matter},
number = 14,
volume = 32,
place = {United States},
year = {2020},
month = {1}
}
Works referenced in this record:
Topological Insulators in Three Dimensions
journal, March 2007
- Fu, Liang; Kane, C. L.; Mele, E. J.
- Physical Review Letters, Vol. 98, Issue 10, Article No. 106803
Colloquium: Topological insulators
journal, November 2010
- Hasan, M. Z.; Kane, C. L.
- Reviews of Modern Physics, Vol. 82, Issue 4, p. 3045-3067
Quantum Spin Hall Insulator State in HgTe Quantum Wells
journal, November 2007
- Konig, M.; Wiedmann, S.; Brune, C.
- Science, Vol. 318, Issue 5851, p. 766-770
Quantum Anomalous Hall Effect in Quantum Wells
journal, October 2008
- Liu, Chao-Xing; Qi, Xiao-Liang; Dai, Xi
- Physical Review Letters, Vol. 101, Issue 14
Massive Dirac Fermion on the Surface of a Magnetically Doped Topological Insulator
journal, August 2010
- Chen, Y. L.; Chu, J. - H.; Analytis, J. G.
- Science, Vol. 329, Issue 5992
Topological insulators and superconductors
journal, October 2011
- Qi, Xiao-Liang; Zhang, Shou-Cheng
- Reviews of Modern Physics, Vol. 83, Issue 4
Experimental Observation of the Quantum Anomalous Hall Effect in a Magnetic Topological Insulator
journal, March 2013
- Chang, C. -Z.; Zhang, J.; Feng, X.
- Science, Vol. 340, Issue 6129
Ferromagnetism in vanadium-doped Bi 2 Se 3 topological insulator films
journal, July 2017
- Zhang, Liguo; Zhao, Dapeng; Zang, Yunyi
- APL Materials, Vol. 5, Issue 7
Topology-Driven Magnetic Quantum Phase Transition in Topological Insulators
journal, March 2013
- Zhang, J.; Chang, C. -Z.; Tang, P.
- Science, Vol. 339, Issue 6127
Nonmagnetic band gap at the Dirac point of the magnetic topological insulator (Bi1−xMnx)2Se3
journal, February 2016
- Sánchez-Barriga, J.; Varykhalov, A.; Springholz, G.
- Nature Communications, Vol. 7, Issue 1
Systematics of electronic and magnetic properties in the transition metal doped quantum anomalous Hall platform
journal, April 2018
- Islam, M. F.; Canali, C. M.; Pertsova, A.
- Physical Review B, Vol. 97, Issue 15
Dual nature of magnetic dopants and competing trends in topological insulators
journal, June 2016
- Sessi, Paolo; Biswas, Rudro R.; Bathon, Thomas
- Nature Communications, Vol. 7, Issue 1
Disorder enabled band structure engineering of a topological insulator surface
journal, February 2017
- Xu, Yishuai; Chiu, Janet; Miao, Lin
- Nature Communications, Vol. 8, Issue 1
Strong potential impurities on the surface of a topological insulator
journal, March 2012
- Black-Schaffer, Annica M.; Balatsky, Alexander V.
- Physical Review B, Vol. 85, Issue 12
Determining the strength of magnetic and potential scattering of magnetic impurities on the surface of a topological insulator via quantum corrals
journal, December 2017
- Zheng, C.; Li, Q. L.; Miao, B. F.
- Physical Review B, Vol. 96, Issue 23
Subsurface impurities and vacancies in a three-dimensional topological insulator
journal, September 2012
- Black-Schaffer, Annica M.; Balatsky, Alexander V.
- Physical Review B, Vol. 86, Issue 11
Observation of Fermi-energy dependent unitary impurity resonances in a strong topological insulator Bi2Se3 with scanning tunneling spectroscopy
journal, May 2012
- Teague, M. L.; Chu, H.; Xiu, F. -X.
- Solid State Communications, Vol. 152, Issue 9
Impurity-induced states on the surface of three-dimensional topological insulators
journal, June 2010
- Biswas, Rudro R.; Balatsky, A. V.
- Physical Review B, Vol. 81, Issue 23
Filling of magnetic-impurity-induced gap in topological insulators by potential scattering
journal, May 2015
- Black-Schaffer, A. M.; Balatsky, A. V.; Fransson, J.
- Physical Review B, Vol. 91, Issue 20
Observation of a topological insulator Dirac cone reshaped by non-magnetic impurity resonance
journal, June 2018
- Miao, Lin; Xu, Yishuai; Zhang, Wenhan
- npj Quantum Materials, Vol. 3, Issue 1
Hedgehog spin texture and Berry’s phase tuning in a magnetic topological insulator
journal, June 2012
- Xu, Su-Yang; Neupane, Madhab; Liu, Chang
- Nature Physics, Vol. 8, Issue 8
Tolerance of Topological Surface States towards Magnetic Moments: Fe on
journal, June 2012
- Scholz, M. R.; Sánchez-Barriga, J.; Marchenko, D.
- Physical Review Letters, Vol. 108, Issue 25
Identifying Magnetic Anisotropy of the Topological Surface State of with Spin-Polarized STM
journal, October 2013
- Yang, Fang; Song, Y. R.; Li, H.
- Physical Review Letters, Vol. 111, Issue 17
Direct Observation of Broken Time-Reversal Symmetry on the Surface of a Magnetically Doped Topological Insulator
journal, May 2011
- Okada, Yoshinori; Dhital, Chetan; Zhou, Wenwen
- Physical Review Letters, Vol. 106, Issue 20
Electron transmission through atomic steps of Bi Se and Bi Te surfaces
journal, November 2011
- Kobayashi, Katsuyoshi
- Physical Review B, Vol. 84, Issue 20
Probing the wavefunction of the surface states in Bi 2 Se 3 topological insulator: a realistic tight-binding approach
journal, June 2014
- Pertsova, A.; Canali, C. M.
- New Journal of Physics, Vol. 16, Issue 6
Interplay between Mn-acceptor state and Dirac surface states in Mn-doped topological insulator
journal, November 2014
- Mahani, M. R.; Pertsova, A.; Islam, M. Fhokrul
- Physical Review B, Vol. 90, Issue 19
The electronic structure of clean and adsorbate-covered Bi 2 Se 3 : an angle-resolved photoemission study
journal, November 2012
- Bianchi, Marco; Hatch, Richard C.; Guan, Dandan
- Semiconductor Science and Technology, Vol. 27, Issue 12
Magnetic ordering in Cr-doped Bi 2 Se 3 thin films
journal, September 2014
- Collins-McIntyre, L. J.; Harrison, S. E.; Schönherr, P.
- EPL (Europhysics Letters), Vol. 107, Issue 5
Photoemission studies on (1 1 1) textured Cr doped Eu2O3 thin film
journal, March 2018
- Kumar, Sandeep; Prakash, Ram; Choudhary, R. J.
- Journal of Alloys and Compounds, Vol. 738
Distinct effects of Cr bulk doping and surface deposition on the chemical environment and electronic structure of the topological insulator Bi2Se3
journal, June 2017
- Yilmaz, Turgut; Hines, William; Sun, Fu-Chang
- Applied Surface Science, Vol. 407
Systematics of electronic and magnetic properties in the transition metal doped $Sb_{2}Te_{3}$ quantum anomalous Hall platform
text, January 2018
- Islam, M. F.; Canali, C. M.; Pertsova, A.
- Deutsches Elektronen-Synchrotron, DESY, Hamburg
Probing the wavefunction of the surface states in Bi$_2$Se$_3$ topological insulator: a realistic tight-binding approach
text, January 2013
- Pertsova, A.; Canali, C. M.
- arXiv
Dual nature of magnetic dopants and competing trends in topological insulators
text, January 2016
- Sessi, Paolo; Biswas, Rudro; Bathon, Thomas
- arXiv
Experimental Observation of the Quantum Anomalous Hall Effect in a Magnetic Topological Insulator
text, January 2016
- Chang, Cui-Zu; Zhang, Jinsong; Feng, Xiao
- arXiv
Topological Insulators in Three Dimensions
text, January 2006
- Fu, Liang; Kane, C. L.; Mele, E. J.
- arXiv