Observation of persistent species temperature separation in inertial confinement fusion mixtures
Abstract
The injection and mixing of contaminant mass into the fuel in inertial confinement fusion (ICF) implosions is a primary factor preventing ignition. ICF experiments have recently achieved an alpha-heating regime, in which fusion self-heating is the dominant source of yield, by reducing the susceptibility of implosions to instabilities that inject this mass. We report the results of unique separated reactants implosion experiments studying pre-mixed contaminant as well as detailed high-resolution three-dimensional simulations that are in good agreement with experiments. At conditions relevant to mixing regions in high-yield implosions, we observe persistent chunks of contaminant that do not achieve thermal equilibrium with the fuel throughout the burn phase. The assumption of thermal equilibrium is made in nearly all computational ICF modeling and methods used to infer levels of contaminant from experiments. We estimate that these methods may underestimate the amount of contaminant by a factor of two or more.
- Authors:
-
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Univ. of Rochester, NY (United States). Lab. for Laser Energetics
- Publication Date:
- Research Org.:
- Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
- Sponsoring Org.:
- USDOE National Nuclear Security Administration (NNSA)
- OSTI Identifier:
- 1604025
- Report Number(s):
- LA-UR-19-20184
Journal ID: ISSN 2041-1723; TRN: US2104180
- Grant/Contract Number:
- 89233218CNA000001
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 11; Journal Issue: 1; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 70 PLASMA PHYSICS AND FUSION TECHNOLOGY
Citation Formats
Haines, Brian Michael, Shah, Rahul C, Smidt, Joseph Michael, Albright, Brian James, Cardenas, Tana, Douglas, Melissa Rae, Forrest, Chad, Glebov, Vladimir Yu, Gunderson, Mark A., Hamilton, Christopher Eric, Henderson, Kevin C., Kim, Yong Ho, Lee, Matthew Nicholson, Murphy, Thomas Joseph, Oertel, John A., Olson, Richard Edward, Patterson, Brian M., Randolph, Randall Blaine, and Schmidt, Derek William. Observation of persistent species temperature separation in inertial confinement fusion mixtures. United States: N. p., 2020.
Web. doi:10.1038/s41467-020-14412-y.
Haines, Brian Michael, Shah, Rahul C, Smidt, Joseph Michael, Albright, Brian James, Cardenas, Tana, Douglas, Melissa Rae, Forrest, Chad, Glebov, Vladimir Yu, Gunderson, Mark A., Hamilton, Christopher Eric, Henderson, Kevin C., Kim, Yong Ho, Lee, Matthew Nicholson, Murphy, Thomas Joseph, Oertel, John A., Olson, Richard Edward, Patterson, Brian M., Randolph, Randall Blaine, & Schmidt, Derek William. Observation of persistent species temperature separation in inertial confinement fusion mixtures. United States. https://doi.org/10.1038/s41467-020-14412-y
Haines, Brian Michael, Shah, Rahul C, Smidt, Joseph Michael, Albright, Brian James, Cardenas, Tana, Douglas, Melissa Rae, Forrest, Chad, Glebov, Vladimir Yu, Gunderson, Mark A., Hamilton, Christopher Eric, Henderson, Kevin C., Kim, Yong Ho, Lee, Matthew Nicholson, Murphy, Thomas Joseph, Oertel, John A., Olson, Richard Edward, Patterson, Brian M., Randolph, Randall Blaine, and Schmidt, Derek William. Tue .
"Observation of persistent species temperature separation in inertial confinement fusion mixtures". United States. https://doi.org/10.1038/s41467-020-14412-y. https://www.osti.gov/servlets/purl/1604025.
@article{osti_1604025,
title = {Observation of persistent species temperature separation in inertial confinement fusion mixtures},
author = {Haines, Brian Michael and Shah, Rahul C and Smidt, Joseph Michael and Albright, Brian James and Cardenas, Tana and Douglas, Melissa Rae and Forrest, Chad and Glebov, Vladimir Yu and Gunderson, Mark A. and Hamilton, Christopher Eric and Henderson, Kevin C. and Kim, Yong Ho and Lee, Matthew Nicholson and Murphy, Thomas Joseph and Oertel, John A. and Olson, Richard Edward and Patterson, Brian M. and Randolph, Randall Blaine and Schmidt, Derek William},
abstractNote = {The injection and mixing of contaminant mass into the fuel in inertial confinement fusion (ICF) implosions is a primary factor preventing ignition. ICF experiments have recently achieved an alpha-heating regime, in which fusion self-heating is the dominant source of yield, by reducing the susceptibility of implosions to instabilities that inject this mass. We report the results of unique separated reactants implosion experiments studying pre-mixed contaminant as well as detailed high-resolution three-dimensional simulations that are in good agreement with experiments. At conditions relevant to mixing regions in high-yield implosions, we observe persistent chunks of contaminant that do not achieve thermal equilibrium with the fuel throughout the burn phase. The assumption of thermal equilibrium is made in nearly all computational ICF modeling and methods used to infer levels of contaminant from experiments. We estimate that these methods may underestimate the amount of contaminant by a factor of two or more.},
doi = {10.1038/s41467-020-14412-y},
journal = {Nature Communications},
number = 1,
volume = 11,
place = {United States},
year = {2020},
month = {1}
}
Web of Science
Works referenced in this record:
Thermo-diffusion in inertially confined plasmas
journal, April 2014
- Kagan, Grigory; Tang, Xian-Zhu
- Physics Letters A, Vol. 378, Issue 21
The mixing transition in turbulent flows
journal, April 2000
- Dimotakis, Paul E.
- Journal of Fluid Mechanics, Vol. 409
Measure of morphological and performance properties in polymeric silicone foams by X-ray tomography
journal, October 2012
- Patterson, Brian M.; Henderson, Kevin; Smith, Zachary
- Journal of Materials Science, Vol. 48, Issue 5
Fuel gain exceeding unity in an inertially confined fusion implosion
journal, February 2014
- Hurricane, O. A.; Callahan, D. A.; Casey, D. T.
- Nature, Vol. 506, Issue 7488
Process Development and Micro-Machining of MARBLE Foam-Cored Rexolite Hemi-Shell Ablator Capsules
journal, September 2016
- Randolph, Randall B.; Oertel, John A.; Schmidt, Derek W.
- Fusion Science and Technology, Vol. 70, Issue 2
First Liquid Layer Inertial Confinement Fusion Implosions at the National Ignition Facility
journal, December 2016
- Olson, R. E.; Leeper, R. J.; Kline, J. L.
- Physical Review Letters, Vol. 117, Issue 24
The modeling of delayed-onset Rayleigh-Taylor and transition to mixing in laser-driven HED experiments
journal, May 2019
- Di Stefano, C. A.; Doss, F. W.; Rasmus, A. M.
- Physics of Plasmas, Vol. 26, Issue 5
Variable convergence liquid layer implosions on the National Ignition Facility
journal, May 2018
- Zylstra, A. B.; Yi, S. A.; Haines, B. M.
- Physics of Plasmas, Vol. 25, Issue 5
Onset of Hydrodynamic Mix in High-Velocity, Highly Compressed Inertial Confinement Fusion Implosions
journal, August 2013
- Ma, T.; Patel, P. K.; Izumi, N.
- Physical Review Letters, Vol. 111, Issue 8
Effects of Fuel-Shell Mix upon Direct-Drive, Spherical Implosions on OMEGA
journal, September 2002
- Li, C. K.; Séguin, F. H.; Frenje, J. A.
- Physical Review Letters, Vol. 89, Issue 16
Hot-spot mix in ignition-scale implosions on the NIF
journal, May 2012
- Regan, S. P.; Epstein, R.; Hammel, B. A.
- Physics of Plasmas, Vol. 19, Issue 5
Unification and extension of the similarity scaling criteria and mixing transition for studying astrophysics using high energy density laboratory experiments or numerical simulations
journal, August 2007
- Zhou, Ye
- Physics of Plasmas, Vol. 14, Issue 8
Absolute calibration method for laser megajoule neutron yield measurement by activation diagnostics
journal, July 2011
- Landoas, Olivier; Yu Glebov, Vladimir; Rossé, Bertrand
- Review of Scientific Instruments, Vol. 82, Issue 7
Turbulent stagnation in a -pinch plasma
journal, January 2018
- Kroupp, E.; Stambulchik, E.; Starobinets, A.
- Physical Review E, Vol. 97, Issue 1
Exact statistical results for binary mixing and reaction in variable density turbulence
journal, February 2017
- Ristorcelli, J. R.
- Physics of Fluids, Vol. 29, Issue 2
Simulation ensemble for a laser–driven shear experiment
journal, September 2013
- Haines, Brian M.; Grinstein, Fernando F.; Welser–Sherrill, Leslie
- Physics of Plasmas, Vol. 20, Issue 9
Species separation and modification of neutron diagnostics in inertial-confinement fusion
journal, September 2014
- Inglebert, A.; Canaud, B.; Larroche, O.
- EPL (Europhysics Letters), Vol. 107, Issue 6
Wavelength-detuning cross-beam energy transfer mitigation scheme for direct drive: Modeling and evidence from National Ignition Facility implosions
journal, May 2018
- Marozas, J. A.; Hohenberger, M.; Rosenberg, M. J.
- Physics of Plasmas, Vol. 25, Issue 5
Three-dimensional hydrodynamics of the deceleration stage in inertial confinement fusion
journal, March 2015
- Weber, C. R.; Clark, D. S.; Cook, A. W.
- Physics of Plasmas, Vol. 22, Issue 3
Indications of flow near maximum compression in layered deuterium-tritium implosions at the National Ignition Facility
journal, August 2016
- Gatu Johnson, M.; Knauer, J. P.; Cerjan, C. J.
- Physical Review E, Vol. 94, Issue 2
Robustness to hydrodynamic instabilities in indirectly driven layered capsule implosions
journal, January 2019
- Haines, Brian M.; Olson, R. E.; Sweet, W.
- Physics of Plasmas, Vol. 26, Issue 1
Fusion neutrons from the gas–pusher interface in deuterated-shell inertial confinement fusion implosions
journal, March 1998
- Chrien, R. E.; Hoffman, N. M.; Colvin, J. D.
- Physics of Plasmas, Vol. 5, Issue 3
Morphological and Performance Measures of Polyurethane Foams Using X-Ray CT and Mechanical Testing
journal, May 2014
- Patterson, Brian M.; Henderson, Kevin; Gilbertson, Robert D.
- Microscopy and Microanalysis, Vol. 20, Issue 4
Three-dimensional simulations of low foot and high foot implosion experiments on the National Ignition Facility
journal, March 2016
- Clark, D. S.; Weber, C. R.; Milovich, J. L.
- Physics of Plasmas, Vol. 23, Issue 5
The RAGE radiation-hydrodynamic code
journal, October 2008
- Gittings, Michael; Weaver, Robert; Clover, Michael
- Computational Science & Discovery, Vol. 1, Issue 1
Core performance and mix in direct-drive spherical implosions with high uniformity
journal, May 2001
- Meyerhofer, D. D.; Delettrez, J. A.; Epstein, R.
- Physics of Plasmas, Vol. 8, Issue 5
Experimental study of initial condition dependence on Richtmyer-Meshkov instability in the presence of reshock
journal, March 2012
- Balasubramanian, S.; Orlicz, G. C.; Prestridge, K. P.
- Physics of Fluids, Vol. 24, Issue 3
The role of hot spot mix in the low-foot and high-foot implosions on the NIF
journal, May 2017
- Ma, T.; Patel, P. K.; Izumi, N.
- Physics of Plasmas, Vol. 24, Issue 5
A subgrid model for equilibrium chemistry in turbulent flows
journal, August 1994
- Cook, Andrew W.; Riley, James J.
- Physics of Fluids, Vol. 6, Issue 8
Inhibition of turbulence in inertial-confinement-fusion hot spots by viscous dissipation
journal, May 2014
- Weber, C. R.; Clark, D. S.; Cook, A. W.
- Physical Review E, Vol. 89, Issue 5
The effects of convergence ratio on the implosion behavior of DT layered inertial confinement fusion capsules
journal, July 2017
- Haines, Brian M.; Yi, S. A.; Olson, R. E.
- Physics of Plasmas, Vol. 24, Issue 7
Multifrequency-Gray Method for Radiation Diffusion with Compton Scattering
journal, March 1995
- Winslow, Alan M.
- Journal of Computational Physics, Vol. 117, Issue 2
On Upstream Differencing and Godunov-Type Schemes for Hyperbolic Conservation Laws
journal, January 1983
- Harten, Amiram; Lax, Peter D.; Leer, Bram van
- SIAM Review, Vol. 25, Issue 1
Hot-Spot Mix in Ignition-Scale Inertial Confinement Fusion Targets
journal, July 2013
- Regan, S. P.; Epstein, R.; Hammel, B. A.
- Physical Review Letters, Vol. 111, Issue 4
Relativistically correct DD and DT neutron spectra
journal, June 2014
- Appelbe, B.; Chittenden, J.
- High Energy Density Physics, Vol. 11
An electron conductivity model for dense plasmas
journal, January 1984
- Lee, Y. T.; More, R. M.
- Physics of Fluids, Vol. 27, Issue 5
Three-dimensional simulation strategy to determine the effects of turbulent mixing on inertial-confinement-fusion capsule performance
journal, May 2014
- Haines, Brian M.; Grinstein, Fernando F.; Fincke, James R.
- Physical Review E, Vol. 89, Issue 5
Atomic mix in directly driven inertial confinement implosions
journal, November 2011
- Wilson, D. C.; Ebey, P. S.; Sangster, T. C.
- Physics of Plasmas, Vol. 18, Issue 11
Development of Hierarchical, Tunable Pore Size Polymer Foams for ICF Targets
journal, September 2016
- Hamilton, Christopher E.; Lee, Matthew N.; Parra-Vasquez, A. Nicholas G.
- Fusion Science and Technology, Vol. 70, Issue 2
Transport properties of an asymmetric mixture in the dense plasma regime
journal, June 2016
- Ticknor, Christopher; Kress, Joel D.; Collins, Lee A.
- Physical Review E, Vol. 93, Issue 6
Modeling of direct-drive cylindrical implosion experiments with an Eulerian radiation-hydrodynamics code
journal, April 2019
- Sauppe, J. P.; Haines, B. M.; Palaniyappan, S.
- Physics of Plasmas, Vol. 26, Issue 4
High-dynamic-range neutron time-of-flight detector used to infer the D(t,n)4He and D(d,n)3He reaction yield and ion temperature on OMEGA
journal, August 2016
- Forrest, C. J.; Glebov, V. Yu.; Goncharov, V. N.
- Review of Scientific Instruments, Vol. 87, Issue 11
Fusion Energy Output Greater than the Kinetic Energy of an Imploding Shell at the National Ignition Facility
journal, June 2018
- Le Pape, S.; Berzak Hopkins, L. F.; Divol, L.
- Physical Review Letters, Vol. 120, Issue 24
Large-eddy simulation and Reynolds-averaged Navier-Stokes modeling of a reacting Rayleigh-Taylor mixing layer in a spherical geometry
journal, September 2018
- Morgan, Brandon E.; Olson, Britton J.; Black, Wolfgang J.
- Physical Review E, Vol. 98, Issue 3
A platform for studying the Rayleigh–Taylor and Richtmyer–Meshkov instabilities in a planar geometry at high energy density at the National Ignition Facility
journal, July 2017
- Nagel, S. R.; Raman, K. S.; Huntington, C. M.
- Physics of Plasmas, Vol. 24, Issue 7
Simulations of material mixing in laser-driven reshock experiments
journal, February 2013
- Haines, Brian M.; Grinstein, Fernando F.; Welser-Sherrill, Leslie
- Physics of Plasmas, Vol. 20, Issue 2
Kinetic simulations of fusion ignition with hot-spot ablator mix
journal, September 2019
- Sadler, James D.; Lu, Yingchao; Spiers, Benjamin
- Physical Review E, Vol. 100, Issue 3
A monochromatic x-ray imaging system for characterizing low-density foams
journal, October 2012
- Lanier, N. E.; Hamilton, C.; Taccetti, J. M.
- Review of Scientific Instruments, Vol. 83, Issue 10
Time-Dependent Nuclear Measurements of Mix in Inertial Confinement Fusion
journal, May 2007
- Rygg, J. R.; Frenje, J. A.; Li, C. K.
- Physical Review Letters, Vol. 98, Issue 21
Laser Compression of Matter to Super-High Densities: Thermonuclear (CTR) Applications
journal, September 1972
- Nuckolls, John; Wood, Lowell; Thiessen, Albert
- Nature, Vol. 239, Issue 5368, p. 139-142
Diagnosing and controlling mix in National Ignition Facility implosion experiments
journal, May 2011
- Hammel, B. A.; Scott, H. A.; Regan, S. P.
- Physics of Plasmas, Vol. 18, Issue 5
25 ps neutron detector for measuring ICF‐target burn history
journal, January 1995
- Lerche, R. A.; Phillion, D. W.; Tietbohl, G. L.
- Review of Scientific Instruments, Vol. 66, Issue 1
Plasma kinetic effects on interfacial mix and burn rates in multispatial dimensions
journal, June 2019
- Yin, L.; Albright, B. J.; Vold, E. L.
- Physics of Plasmas, Vol. 26, Issue 6
Three‐dimensional numerical simulation of turbulent mixing by Rayleigh–Taylor instability
journal, May 1991
- Youngs, David L.
- Physics of Fluids A: Fluid Dynamics, Vol. 3, Issue 5
Detailed high-resolution three-dimensional simulations of OMEGA separated reactants inertial confinement fusion experiments
journal, July 2016
- Haines, Brian M.; Grim, Gary P.; Fincke, James R.
- Physics of Plasmas, Vol. 23, Issue 7
Inference of mix in direct-drive implosions on OMEGA
journal, May 2002
- Radha, P. B.; Delettrez, J.; Epstein, R.
- Physics of Plasmas, Vol. 9, Issue 5
Ion Thermal Decoupling and Species Separation in Shock-Driven Implosions
journal, January 2015
- Rinderknecht, Hans G.; Rosenberg, M. J.; Li, C. K.
- Physical Review Letters, Vol. 114, Issue 2
Instability of the interface of two gases accelerated by a shock wave
journal, January 1972
- Meshkov, E. E.
- Fluid Dynamics, Vol. 4, Issue 5
Transport Phenomena in a Completely Ionized Gas
journal, March 1953
- Spitzer, Lyman; Härm, Richard
- Physical Review, Vol. 89, Issue 5
High-resolution modeling of indirectly driven high-convergence layered inertial confinement fusion capsule implosions
journal, May 2017
- Haines, Brian M.; Aldrich, C. H.; Campbell, J. M.
- Physics of Plasmas, Vol. 24, Issue 5
A new Generation of los Alamos Opacity Tables
journal, January 2016
- Colgan, J.; Kilcrease, D. P.; Magee, N. H.
- The Astrophysical Journal, Vol. 817, Issue 2
Measurements of an Ablator-Gas Atomic Mix in Indirectly Driven Implosions at the National Ignition Facility
journal, January 2014
- Smalyuk, V. A.; Tipton, R. E.; Pino, J. E.
- Physical Review Letters, Vol. 112, Issue 2
Taylor instability in shock acceleration of compressible fluids
journal, May 1960
- Richtmyer, Robert D.
- Communications on Pure and Applied Mathematics, Vol. 13, Issue 2
Short-wavelength and three-dimensional instability evolution in National Ignition Facility ignition capsule designs
journal, August 2011
- Clark, D. S.; Haan, S. W.; Cook, A. W.
- Physics of Plasmas, Vol. 18, Issue 8
Dry-Machining of Aerogel Foams, CH Foams, and Specially Engineered Foams Using Turn-Milling Techniques
journal, November 2017
- Randolph, Randall B.; Oertel, John A.; Cardenas, Tana
- Fusion Science and Technology, Vol. 73, Issue 2
Species separation and modification of neutron diagnostics in inertial-confinement fusion
text, January 2014
- Inglebert, Aurelie; Canaud, Benoit; Larroche, Olivier
- arXiv
A New Generation of Los Alamos Opacity Tables
text, January 2016
- Colgan, J.; Kilcrease, D. P.; Magee, N. H.
- arXiv
Works referencing / citing this record:
Mitigation of cross-beam energy transfer in ignition-scale polar-direct-drive target designs for the National Ignition Facility
journal, July 2018
- Collins, T. J. B.; Marozas, J. A.
- Physics of Plasmas, Vol. 25, Issue 7
Using cylindrical implosions to investigate hydrodynamic instabilities in convergent geometry
journal, November 2019
- Sauppe, J. P.; Palaniyappan, S.; Loomis, E. N.
- Matter and Radiation at Extremes, Vol. 4, Issue 6
Mitigating laser-imprint effects in direct-drive inertial confinement fusion implosions with an above-critical-density foam layer
journal, August 2018
- Hu, S. X.; Theobald, W.; Radha, P. B.
- Physics of Plasmas, Vol. 25, Issue 8
Modeling of direct-drive cylindrical implosion experiments with an Eulerian radiation-hydrodynamics code
journal, April 2019
- Sauppe, J. P.; Haines, B. M.; Palaniyappan, S.
- Physics of Plasmas, Vol. 26, Issue 4
Direct-drive double-shell implosion: A platform for burning-plasma physics studies
journal, December 2019
- Hu, S. X.; Epstein, R.; Theobald, W.
- Physical Review E, Vol. 100, Issue 6
Real and complex valued geometrical optics inverse ray-tracing for inline field calculations
journal, March 2019
- Colaïtis, A.; Palastro, J. P.; Follett, R. K.
- Physics of Plasmas, Vol. 26, Issue 3