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Title: Finite-size effects in lead scandium tantalate relaxor thin films

Authors:
; ORCiD logo; ; ; ORCiD logo
Publication Date:
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
OSTI Identifier:
1603202
Grant/Contract Number:  
[AC02-05-CH11231; SC-0012375]
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
[Journal Name: Physical Review B Journal Volume: 101 Journal Issue: 9]; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society
Country of Publication:
United States
Language:
English

Citation Formats

Fernandez, Abel, Kim, Jieun, Meyers, Derek, Saremi, Sahar, and Martin, Lane W. Finite-size effects in lead scandium tantalate relaxor thin films. United States: N. p., 2020. Web. doi:10.1103/PhysRevB.101.094102.
Fernandez, Abel, Kim, Jieun, Meyers, Derek, Saremi, Sahar, & Martin, Lane W. Finite-size effects in lead scandium tantalate relaxor thin films. United States. doi:10.1103/PhysRevB.101.094102.
Fernandez, Abel, Kim, Jieun, Meyers, Derek, Saremi, Sahar, and Martin, Lane W. Wed . "Finite-size effects in lead scandium tantalate relaxor thin films". United States. doi:10.1103/PhysRevB.101.094102.
@article{osti_1603202,
title = {Finite-size effects in lead scandium tantalate relaxor thin films},
author = {Fernandez, Abel and Kim, Jieun and Meyers, Derek and Saremi, Sahar and Martin, Lane W.},
abstractNote = {},
doi = {10.1103/PhysRevB.101.094102},
journal = {Physical Review B},
number = [9],
volume = [101],
place = {United States},
year = {2020},
month = {3}
}

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Works referenced in this record:

Ferroelectricity in Ultrathin Perovskite Films
journal, June 2004

  • Fong, Dillon D.; Stephenson, G. Brian; Streiffer, Stephen K.
  • Science, Vol. 304, Issue 5677, p. 1650-1653
  • DOI: 10.1126/science.1098252

Diffuse Scattering from Defect Clusters near Bragg Reflections
journal, August 1971


Order and disorder in the relaxor ferroelectric perovskite (PSN): comparison with simple perovskites and
journal, September 1997


In-plane versus out-of-plane dielectric response in the thin-film relaxor Pb ( Sc 1 2 Ta 1 2 ) O 3
journal, June 2006


Polarization rotation mechanism for ultrahigh electromechanical response in single-crystal piezoelectrics
journal, January 2000

  • Fu, Huaxiang; Cohen, Ronald E.
  • Nature, Vol. 403, Issue 6767
  • DOI: 10.1038/35002022

Crystalline Ferroelectrics with a Glassy Polarization Phase
journal, January 1985

  • Burns, Gerald; Dacol, F. H.
  • Japanese Journal of Applied Physics, Vol. 24, Issue S2
  • DOI: 10.7567/JJAPS.24S2.85

Intermediate temperature scale T in lead-based relaxor systems
journal, August 2009


Vogel-Fulcher freezing in relaxor ferroelectrics
journal, July 2007


Ferroelectricity in Pb 1+δ ZrO 3 Thin Films
journal, July 2017


Emergence of room-temperature ferroelectricity at reduced dimensions
journal, September 2015


Pyroelectric energy conversion with large energy and power density in relaxor ferroelectric thin films
journal, April 2018


The theory of diffuse X-ray scattering and its application to the study of point defects and their clusters
journal, February 1973


Particle and grain size effects on the dielectric behavior of the relaxor ferroelectric Pb(Mg 1/3 Nb 2/3 )O 3
journal, December 1990

  • Papet, Philippe; Dougherty, Joseph P.; Shrout, Thomas R.
  • Journal of Materials Research, Vol. 5, Issue 12
  • DOI: 10.1557/JMR.1990.2902

Freezing of the polarization fluctuations in lead magnesium niobate relaxors
journal, September 1990

  • Viehland, Dwight; Jang, S. J.; Cross, L. Eric
  • Journal of Applied Physics, Vol. 68, Issue 6
  • DOI: 10.1063/1.346425

Strain screening by mobile oxygen vacancies in SrTiO3
journal, June 2010

  • Kim, Yongsam; Disa, Ankit S.; Babakol, Timur E.
  • Applied Physics Letters, Vol. 96, Issue 25
  • DOI: 10.1063/1.3455157

Scaling of structure and electrical properties in ultrathin epitaxial ferroelectric heterostructures
journal, September 2006

  • Nagarajan, V.; Junquera, J.; He, J. Q.
  • Journal of Applied Physics, Vol. 100, Issue 5
  • DOI: 10.1063/1.2337363

Electric-field-induced redistribution of polar nano-regions in a relaxor ferroelectric
journal, January 2006

  • Xu, Guangyong; Zhong, Z.; Bing, Y.
  • Nature Materials, Vol. 5, Issue 2
  • DOI: 10.1038/nmat1560

The origin of ultrahigh piezoelectricity in relaxor-ferroelectric solid solution crystals
journal, December 2016

  • Li, Fei; Zhang, Shujun; Yang, Tiannan
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms13807

Dynamics of interacting clusters and dielectric response in relaxor ferroelectrics
journal, April 1998


Diffuse neutron scattering study of a disordered complex perovskite P b ( Z n 1 / 3 Nb 2 / 3 ) O 3 crystal
journal, November 2001


The Three Characteristic Temperatures of Relaxor Dynamics and Their Meaning
journal, October 2008


Origin of ferroelectricity in perovskite oxides
journal, July 1992


Evidence for domain-type dynamics in the ergodic phase of the PbMg 1 / 3 Nb 2 / 3 O 3 relaxor ferroelectric
journal, May 1996


The contribution of structural disorder to diffuse phase transitions in ferroelectrics
journal, October 1980

  • Setter, N.; Cross, L. E.
  • Journal of Materials Science, Vol. 15, Issue 10
  • DOI: 10.1007/BF00550750

Relationship between Local Structure and Relaxor Behavior in Perovskite Oxides
journal, December 2007


Relaxorferroelectrics: An overview
journal, January 1994


Dipole glass and ferroelectricity in random-site electric dipole systems
journal, October 1990


Cold neutron study on the diffuse scattering and phonon excitations in the relaxor Pb ( Mg 1 3 Nb 2 3 ) O 3
journal, November 2004


Nonstoichiometry, Structure, and Properties of BiFeO 3 Films
journal, August 2016


Grain size dependence of relaxor characteristics in La-modified lead zirconate titanate
journal, March 1997


Local and long range polar order in the relaxor-ferroelectric compounds PbMg 1 / 3 Nb 2 / 3 O 3 and PbMg 0.3 Nb 0.6 Ti 0.1 O 3
journal, December 2001


The spontaneous relaxor‐ferroelectric transition of Pb(Sc 0.5 Ta 0.5 )O 3
journal, October 1993

  • Chu, F.; Setter, N.; Tagantsev, A. K.
  • Journal of Applied Physics, Vol. 74, Issue 8
  • DOI: 10.1063/1.354300

Processing and properties of ferroelectric relaxor lead scandium tantalate Pb(Sc 1/2 Ta 1/2 )O 3 thin films
journal, January 2007

  • Brinkman, K.; Wang, Y.; Cantoni, M.
  • Journal of Materials Research, Vol. 22, Issue 1
  • DOI: 10.1557/jmr.2007.0023

Size-driven relaxation and polar states in PbMg 1 3 Nb 2 3 O 3 -based system
journal, November 2005


Extrinsic contributions to the grain size dependence of relaxor ferroelectric Pb(Mg 1/3 Nb 2/3 )O 3 : PbTiO 3 ceramics
journal, April 1993

  • Randall, C. A.; Hilton, A. D.; Barber, D. J.
  • Journal of Materials Research, Vol. 8, Issue 4
  • DOI: 10.1557/JMR.1993.0880

Vogel-Fulcher relationship for the dielectric permittivity of relaxor ferroelectrics
journal, February 1994


Mechanism of polarization response in the ergodic phase of a relaxor ferroelectric
journal, January 1998


Phase instability induced by polar nanoregions in a relaxor ferroelectric system
journal, May 2008

  • Xu, Guangyong; Wen, Jinsheng; Stock, C.
  • Nature Materials, Vol. 7, Issue 7
  • DOI: 10.1038/nmat2196

Particle-size effect on the ferroelectric phase transition in PbSc1/2Ta1/2O3 ceramics
journal, June 1998

  • Park, Yung; Knowles, Kevin M.; Cho, Kurn
  • Journal of Applied Physics, Vol. 83, Issue 11
  • DOI: 10.1063/1.367424

Contributions to the nonlinear dielectric and piezoelectric response of ferroelectric thin films and ceramics
journal, January 1999


The role of B‐site cation disorder in diffuse phase transition behavior of perovskite ferroelectrics
journal, August 1980

  • Setter, N.; Cross, L. E.
  • Journal of Applied Physics, Vol. 51, Issue 8
  • DOI: 10.1063/1.328296

The dielectric relaxation of lead magnesium niobate relaxor ferroelectrics
journal, September 1991


Neutron elastic diffuse scattering study of Pb ( Mg 1 / 3 Nb 2 / 3 ) O 3
journal, February 2004


Identification of two lead perovskites, Pb 2 ScTaO 6 and Pb(Sc 0.5 Nb 0.5 )O 3 , by X-ray powder diffraction patterns
journal, September 1993


Nonlinear dynamics of polar regions in paraelectric phase of (Ba 1-x ,Sr x )TiO 3 ceramics
journal, May 2017

  • Hashemizadeh, Sina; Damjanovic, Dragan
  • Applied Physics Letters, Vol. 110, Issue 19
  • DOI: 10.1063/1.4983366

Epitaxial Strain Control of Relaxor Ferroelectric Phase Evolution
journal, April 2019


Ultrahigh–energy density lead-free dielectric films via polymorphic nanodomain design
journal, August 2019


Critical thickness for ferroelectricity in perovskite ultrathin films
journal, April 2003

  • Junquera, Javier; Ghosez, Philippe
  • Nature, Vol. 422, Issue 6931, p. 506-509
  • DOI: 10.1038/nature01501

Slush-like polar structures in single-crystal relaxors
journal, June 2017

  • Takenaka, Hiroyuki; Grinberg, Ilya; Liu, Shi
  • Nature, Vol. 546, Issue 7658
  • DOI: 10.1038/nature22068

The Rayleigh law in piezoelectric ceramics
journal, July 1996