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This content will become publicly available on February 27, 2021

Title: Building Electron/Proton Nanohighways for Full Utilization of Water Splitting Catalysts

Authors:
 [1];  [1];  [2];  [1];  [3];  [3];  [3];  [4]; ORCiD logo [1]
  1. Department of MechanicalAerospace and Biomedical EngineeringUT Space InstituteUniversity of Tennessee, Knoxville Tullahoma TN 37388 USA
  2. Department of MechanicalAerospace and Biomedical EngineeringUT Space InstituteUniversity of Tennessee, Knoxville Tullahoma TN 37388 USA, Chemistry and Nanoscience DepartmentNational Renewable Energy Lab Golden CO 80401 USA
  3. Chemistry and Nanoscience DepartmentNational Renewable Energy Lab Golden CO 80401 USA
  4. Center for Nanophase Materials SciencesOak Ridge National Lab Oak Ridge TN 37831 USA
Publication Date:
Sponsoring Org.:
USDOE Office of Energy Efficiency and Renewable Energy (EERE)
OSTI Identifier:
1602091
Grant/Contract Number:  
[DE‐EE0008426; DE‐AC36‐08GO28308; DE‐FE0011585]
Resource Type:
Publisher's Accepted Manuscript
Journal Name:
Advanced Energy Materials
Additional Journal Information:
[Journal Name: Advanced Energy Materials]; Journal ID: ISSN 1614-6832
Publisher:
Wiley Blackwell (John Wiley & Sons)
Country of Publication:
Germany
Language:
English

Citation Formats

Yang, Gaoqiang, Yu, Shule, Kang, Zhenye, Li, Yifan, Bender, Guido, Pivovar, Bryan S., Green, Jr., Johney B., Cullen, David A., and Zhang, Feng‐Yuan. Building Electron/Proton Nanohighways for Full Utilization of Water Splitting Catalysts. Germany: N. p., 2020. Web. doi:10.1002/aenm.201903871.
Yang, Gaoqiang, Yu, Shule, Kang, Zhenye, Li, Yifan, Bender, Guido, Pivovar, Bryan S., Green, Jr., Johney B., Cullen, David A., & Zhang, Feng‐Yuan. Building Electron/Proton Nanohighways for Full Utilization of Water Splitting Catalysts. Germany. doi:10.1002/aenm.201903871.
Yang, Gaoqiang, Yu, Shule, Kang, Zhenye, Li, Yifan, Bender, Guido, Pivovar, Bryan S., Green, Jr., Johney B., Cullen, David A., and Zhang, Feng‐Yuan. Fri . "Building Electron/Proton Nanohighways for Full Utilization of Water Splitting Catalysts". Germany. doi:10.1002/aenm.201903871.
@article{osti_1602091,
title = {Building Electron/Proton Nanohighways for Full Utilization of Water Splitting Catalysts},
author = {Yang, Gaoqiang and Yu, Shule and Kang, Zhenye and Li, Yifan and Bender, Guido and Pivovar, Bryan S. and Green, Jr., Johney B. and Cullen, David A. and Zhang, Feng‐Yuan},
abstractNote = {},
doi = {10.1002/aenm.201903871},
journal = {Advanced Energy Materials},
number = ,
volume = ,
place = {Germany},
year = {2020},
month = {2}
}

Journal Article:
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Works referenced in this record:

Efficient oxygen evolution electrocatalysis in acid by a perovskite with face-sharing IrO6 octahedral dimers
journal, December 2018


U.S. DOE Progress Towards Developing Low-Cost, High Performance, Durable Polymer Electrolyte Membranes for Fuel Cell Applications
journal, December 2012


Uncovering the Stabilization Mechanism in Bimetallic Ruthenium–Iridium Anodes for Proton Exchange Membrane Electrolyzers
journal, August 2016

  • Saveleva, Viktoriia A.; Wang, Li; Luo, Wen
  • The Journal of Physical Chemistry Letters, Vol. 7, Issue 16
  • DOI: 10.1021/acs.jpclett.6b01500

Balancing activity, stability and conductivity of nanoporous core-shell iridium/iridium oxide oxygen evolution catalysts
journal, November 2017


Terahertz conductivity of thin gold films at the metal-insulator percolation transition
journal, September 2007


Electrocatalysis for the oxygen evolution reaction: recent development and future perspectives
journal, January 2017

  • Suen, Nian-Tzu; Hung, Sung-Fu; Quan, Quan
  • Chemical Society Reviews, Vol. 46, Issue 2
  • DOI: 10.1039/C6CS00328A

Field-Assisted Splitting of Pure Water Based on Deep-Sub-Debye-Length Nanogap Electrochemical Cells
journal, July 2017


Engineering the Electronic State of a Perovskite Electrocatalyst for Synergistically Enhanced Oxygen Evolution Reaction
journal, August 2015


Discovery of true electrochemical reactions for ultrahigh catalyst mass activity in water splitting
journal, November 2016


Investigation of Charge-Transfer and Mass-Transport Resistances in PEMFCs with Microporous Layer Using Electrochemical Impedance Spectroscopy
journal, January 2009

  • Malevich, Dzmitry; Halliop, Ela; Peppley, Brant A.
  • Journal of The Electrochemical Society, Vol. 156, Issue 2
  • DOI: 10.1149/1.3033408

Investigation of thin/well-tunable liquid/gas diffusion layers exhibiting superior multifunctional performance in low-temperature electrolytic water splitting
journal, January 2017

  • Kang, Zhenye; Mo, Jingke; Yang, Gaoqiang
  • Energy & Environmental Science, Vol. 10, Issue 1
  • DOI: 10.1039/C6EE02368A

A highly active and stable hydrogen evolution catalyst based on pyrite-structured cobalt phosphosulfide
journal, February 2016

  • Liu, Wen; Hu, Enyuan; Jiang, Hong
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms10771

Nanoporous gold supported chromium-doped NiFe oxyhydroxides as high-performance catalysts for the oxygen evolution reaction
journal, January 2019

  • Sun, Jie-Song; Zhou, Yi-Tong; Yao, Rui-Qi
  • Journal of Materials Chemistry A, Vol. 7, Issue 16
  • DOI: 10.1039/C9TA01027K

A Thin NiFe Hydroxide Film Formed by Stepwise Electrodeposition Strategy with Significantly Improved Catalytic Water Oxidation Efficiency
journal, January 2017


Trapping an Iron(VI) Water-Splitting Intermediate in Nonaqueous Media
journal, April 2018


Analysis of Voltage Losses in PEM Water Electrolyzers with Low Platinum Group Metal Loadings
journal, January 2018

  • Bernt, Maximilian; Siebel, Armin; Gasteiger, Hubert A.
  • Journal of The Electrochemical Society, Vol. 165, Issue 5
  • DOI: 10.1149/2.0641805jes

Comprehensive investigation of novel pore-graded gas diffusion layers for high-performance and cost-effective proton exchange membrane electrolyzers
journal, January 2017

  • Lettenmeier, P.; Kolb, S.; Sata, N.
  • Energy & Environmental Science, Vol. 10, Issue 12
  • DOI: 10.1039/C7EE01240C

Metal overlayer on metal carbide substrate: unique bimetallic properties for catalysis and electrocatalysis
journal, January 2012

  • Kelly, Thomas G.; Chen, Jingguang G.
  • Chemical Society Reviews, Vol. 41, Issue 24
  • DOI: 10.1039/c2cs35165j

Substantial Impact of Charge on Electrochemical Reactions of Two-Dimensional Materials
journal, June 2018

  • Kim, Donghoon; Shi, Jianjian; Liu, Yuanyue
  • Journal of the American Chemical Society, Vol. 140, Issue 29
  • DOI: 10.1021/jacs.8b03002

Reducing Iridium Loading in Oxygen Evolution Reaction Electrocatalysts Using Core–Shell Particles with Nitride Cores
journal, January 2018


Considerations for the scaling-up of water splitting catalysts
journal, May 2019


Engineering the Electrical Conductivity of Lamellar Silver-Doped Cobalt(II) Selenide Nanobelts for Enhanced Oxygen Evolution
journal, November 2016

  • Zhao, Xu; Zhang, Hantao; Yan, Yu
  • Angewandte Chemie International Edition, Vol. 56, Issue 1
  • DOI: 10.1002/anie.201609080

In situ click chemistry generation of cyclooxygenase-2 inhibitors
journal, February 2017


Opportunities and Challenges in Utilizing Metal-Modified Transition Metal Carbides as Low-Cost Electrocatalysts
journal, October 2017


Design of Highly Active Perovskite Oxides for Oxygen Evolution Reaction by Combining Experimental and ab Initio Studies
journal, June 2015


Hydrogen at Scale (H 2 @Scale): Key to a Clean, Economic, and Sustainable Energy System
journal, January 2018

  • Pivovar, Bryan; Rustagi, Neha; Satyapal, Sunita
  • The Electrochemical Society Interface, Vol. 27, Issue 1
  • DOI: 10.1149/2.F04181if

A review of graphene and graphene oxide sponge: material synthesis and applications to energy and the environment
journal, January 2014

  • Chabot, Victor; Higgins, Drew; Yu, Aiping
  • Energy & Environmental Science, Vol. 7, Issue 5
  • DOI: 10.1039/c3ee43385d

Oxygen Reduction at Very Low Overpotential on Nanoporous Ag Catalysts
journal, May 2015

  • Zhou, Yang; Lu, Qi; Zhuang, Zhongbin
  • Advanced Energy Materials, Vol. 5, Issue 13
  • DOI: 10.1002/aenm.201500149

Behaviors of a proton exchange membrane electrolyzer under water starvation
journal, January 2015

  • Sun, Shucheng; Xiao, Yu; Liang, Dong
  • RSC Advances, Vol. 5, Issue 19
  • DOI: 10.1039/C4RA14104K

Tailoring FeN 4 Sites with Edge Enrichment for Boosted Oxygen Reduction Performance in Proton Exchange Membrane Fuel Cell
journal, January 2019


Properties of gold nanostructures sputtered on glass
journal, January 2011

  • Siegel, Jakub; Lyutakov, Olexiy; Rybka, Vladimír
  • Nanoscale Research Letters, Vol. 6, Issue 1
  • DOI: 10.1186/1556-276X-6-96

Highly Active and Stable Water Splitting in Acidic Media Using a Bifunctional Iridium/Cucurbit[6]uril Catalyst
journal, April 2019


Reaction mechanism for oxygen evolution on RuO2, IrO2, and RuO2@IrO2 core-shell nanocatalysts
journal, June 2018


Electrocatalytic Oxygen Evolution at Surface-Oxidized Multiwall Carbon Nanotubes
journal, February 2015

  • Lu, Xunyu; Yim, Wai-Leung; Suryanto, Bryan H. R.
  • Journal of the American Chemical Society, Vol. 137, Issue 8
  • DOI: 10.1021/ja509879r

Calculating the Electrochemically Active Surface Area of Iridium Oxide in Operating Proton Exchange Membrane Electrolyzers
journal, January 2015

  • Zhao, Shuai; Yu, Haoran; Maric, Radenka
  • Journal of The Electrochemical Society, Vol. 162, Issue 12
  • DOI: 10.1149/2.0211512jes

Modeling, Simulation, and Implementation of Solar-Driven Water-Splitting Devices
journal, October 2016

  • Xiang, Chengxiang; Weber, Adam Z.; Ardo, Shane
  • Angewandte Chemie International Edition, Vol. 55, Issue 42
  • DOI: 10.1002/anie.201510463

A Precious-Metal-Free Regenerative Fuel Cell for Storing Renewable Electricity
journal, July 2013

  • Desmond Ng, Jia Wei; Gorlin, Yelena; Hatsukade, Toru
  • Advanced Energy Materials, Vol. 3, Issue 12
  • DOI: 10.1002/aenm.201300492

Critical Review—Identifying Critical Gaps for Polymer Electrolyte Water Electrolysis Development
journal, January 2017

  • Babic, Ugljesa; Suermann, Michel; Büchi, Felix N.
  • Journal of The Electrochemical Society, Vol. 164, Issue 4
  • DOI: 10.1149/2.1441704jes

The structure of interfacial water on gold electrodes studied by x-ray absorption spectroscopy
journal, October 2014


Identifying the forefront of electrocatalytic oxygen evolution reaction: Electronic double layer
journal, December 2018


Electrical and structural engineering of cobalt selenide nanosheets by Mn modulation for efficient oxygen evolution
journal, November 2018


Activation of surface oxygen sites on an iridium-based model catalyst for the oxygen evolution reaction
journal, December 2016

  • Grimaud, Alexis; Demortière, Arnaud; Saubanère, Matthieu
  • Nature Energy, Vol. 2, Issue 1
  • DOI: 10.1038/nenergy.2016.189

Early stages of growth of gold layers sputter deposited on glass and silicon substrates
journal, January 2012

  • Malinský, Petr; Slepička, Petr; Hnatowicz, Vladimír
  • Nanoscale Research Letters, Vol. 7, Issue 1
  • DOI: 10.1186/1556-276X-7-241

Ror2 signaling regulates Golgi structure and transport through IFT20 for tumor invasiveness
journal, January 2017


Nanosized IrO x -Ir Catalyst with Relevant Activity for Anodes of Proton Exchange Membrane Electrolysis Produced by a Cost-Effective Procedure
journal, November 2015

  • Lettenmeier, Philipp; Wang, Li; Golla-Schindler, Ute
  • Angewandte Chemie, Vol. 128, Issue 2
  • DOI: 10.1002/ange.201507626

A Perovskite Nanorod as Bifunctional Electrocatalyst for Overall Water Splitting
journal, December 2016

  • Zhu, Yinlong; Zhou, Wei; Zhong, Yijun
  • Advanced Energy Materials, Vol. 7, Issue 8
  • DOI: 10.1002/aenm.201602122

Electrocatalytic Oxygen Evolution Reaction in Acidic Environments - Reaction Mechanisms and Catalysts
journal, October 2016

  • Reier, Tobias; Nong, Hong Nhan; Teschner, Detre
  • Advanced Energy Materials, Vol. 7, Issue 1
  • DOI: 10.1002/aenm.201601275

Iridium-based double perovskites for efficient water oxidation in acid media
journal, August 2016

  • Diaz-Morales, Oscar; Raaijman, Stefan; Kortlever, Ruud
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms12363

Bivalence Mn5O8 with hydroxylated interphase for high-voltage aqueous sodium-ion storage
journal, November 2016

  • Shan, Xiaoqiang; Charles, Daniel S.; Lei, Yinkai
  • Nature Communications, Vol. 7, Issue 1
  • DOI: 10.1038/ncomms13370

Combining theory and experiment in electrocatalysis: Insights into materials design
journal, January 2017


Electrochemical water splitting by layered and 3D cross-linked manganese oxides: correlating structural motifs and catalytic activity
journal, January 2013

  • Bergmann, Arno; Zaharieva, Ivelina; Dau, Holger
  • Energy & Environmental Science, Vol. 6, Issue 9
  • DOI: 10.1039/c3ee41194j

Nanoporous Gold: Understanding the Origin of the Reactivity of a 21st Century Catalyst Made by Pre-Columbian Technology
journal, September 2015


Anode-Design Strategies for Improved Performance of Polymer-Electrolyte Fuel Cells with Ultra-Thin Electrodes
journal, July 2018