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Title: Site‐Controlled Uniform Ge/Si Hut Wires with Electrically Tunable Spin–Orbit Coupling

Abstract

Abstract Semiconductor nanowires have been playing a crucial role in the development of nanoscale devices for the realization of spin qubits, Majorana fermions, single photon emitters, nanoprocessors, etc. The monolithic growth of site‐controlled nanowires is a prerequisite toward the next generation of devices that will require addressability and scalability. Here, combining top‐down nanofabrication and bottom‐up self‐assembly, the growth of Ge wires on prepatterned Si (001) substrates with controllable position, distance, length, and structure is reported. This is achieved by a novel growth process that uses a SiGe strain‐relaxation template and can be potentially generalized to other material combinations. Transport measurements show an electrically tunable spin–orbit coupling, with a spin–orbit length similar to that of III–V materials. Also, charge sensing between quantum dots in closely spaced wires is observed, which underlines their potential for the realization of advanced quantum devices. The reported results open a path toward scalable qubit devices using nanowires on silicon.

Authors:
 [1];  [1];  [2];  [3];  [4];  [1];  [5];  [6];  [7];  [2];  [2];  [4];  [4];  [8];  [2]; ORCiD logo [5]
  1. National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences Beijing 100190 China, CAS Center for Excellence in Topological Quantum Computation and School of Physics University of Chinese Academy of Sciences Beijing 100049 China
  2. Institute of Science and Technology Austria Am Campus 1 Klosterneuburg 3400 Austria
  3. Frontier Institute of Science and Technology Xi'an Jiaotong University Xi'an 710054 China
  4. Department of Physics University of Basel Klingelbergstrasse 82 Basel CH‐4056 Switzerland
  5. National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences Beijing 100190 China, CAS Center for Excellence in Topological Quantum Computation and School of Physics University of Chinese Academy of Sciences Beijing 100049 China, Songshan Lake Materials Laboratory Dongguan Guangdong 523808 China
  6. National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences Beijing 100190 China
  7. Institute of Microelectronics Chinese Academy of Sciences Beijing 100029 China
  8. Department of Materials Science and Engineering University of Utah Salt Lake City UT 84112 USA
Publication Date:
Sponsoring Org.:
USDOE
OSTI Identifier:
1602072
Alternate Identifier(s):
OSTI ID: 1602074
Grant/Contract Number:  
DE‐FG02‐04ER46148
Resource Type:
Published Article
Journal Name:
Advanced Materials
Additional Journal Information:
Journal Name: Advanced Materials Journal Volume: 32 Journal Issue: 16; Journal ID: ISSN 0935-9648
Publisher:
Wiley Blackwell (John Wiley & Sons)
Country of Publication:
Germany
Language:
English

Citation Formats

Gao, Fei, Wang, Jian‐Huan, Watzinger, Hannes, Hu, Hao, Rančić, Marko J., Zhang, Jie‐Yin, Wang, Ting, Yao, Yuan, Wang, Gui‐Lei, Kukučka, Josip, Vukušić, Lada, Kloeffel, Christoph, Loss, Daniel, Liu, Feng, Katsaros, Georgios, and Zhang, Jian‐Jun. Site‐Controlled Uniform Ge/Si Hut Wires with Electrically Tunable Spin–Orbit Coupling. Germany: N. p., 2020. Web. doi:10.1002/adma.201906523.
Gao, Fei, Wang, Jian‐Huan, Watzinger, Hannes, Hu, Hao, Rančić, Marko J., Zhang, Jie‐Yin, Wang, Ting, Yao, Yuan, Wang, Gui‐Lei, Kukučka, Josip, Vukušić, Lada, Kloeffel, Christoph, Loss, Daniel, Liu, Feng, Katsaros, Georgios, & Zhang, Jian‐Jun. Site‐Controlled Uniform Ge/Si Hut Wires with Electrically Tunable Spin–Orbit Coupling. Germany. https://doi.org/10.1002/adma.201906523
Gao, Fei, Wang, Jian‐Huan, Watzinger, Hannes, Hu, Hao, Rančić, Marko J., Zhang, Jie‐Yin, Wang, Ting, Yao, Yuan, Wang, Gui‐Lei, Kukučka, Josip, Vukušić, Lada, Kloeffel, Christoph, Loss, Daniel, Liu, Feng, Katsaros, Georgios, and Zhang, Jian‐Jun. Thu . "Site‐Controlled Uniform Ge/Si Hut Wires with Electrically Tunable Spin–Orbit Coupling". Germany. https://doi.org/10.1002/adma.201906523.
@article{osti_1602072,
title = {Site‐Controlled Uniform Ge/Si Hut Wires with Electrically Tunable Spin–Orbit Coupling},
author = {Gao, Fei and Wang, Jian‐Huan and Watzinger, Hannes and Hu, Hao and Rančić, Marko J. and Zhang, Jie‐Yin and Wang, Ting and Yao, Yuan and Wang, Gui‐Lei and Kukučka, Josip and Vukušić, Lada and Kloeffel, Christoph and Loss, Daniel and Liu, Feng and Katsaros, Georgios and Zhang, Jian‐Jun},
abstractNote = {Abstract Semiconductor nanowires have been playing a crucial role in the development of nanoscale devices for the realization of spin qubits, Majorana fermions, single photon emitters, nanoprocessors, etc. The monolithic growth of site‐controlled nanowires is a prerequisite toward the next generation of devices that will require addressability and scalability. Here, combining top‐down nanofabrication and bottom‐up self‐assembly, the growth of Ge wires on prepatterned Si (001) substrates with controllable position, distance, length, and structure is reported. This is achieved by a novel growth process that uses a SiGe strain‐relaxation template and can be potentially generalized to other material combinations. Transport measurements show an electrically tunable spin–orbit coupling, with a spin–orbit length similar to that of III–V materials. Also, charge sensing between quantum dots in closely spaced wires is observed, which underlines their potential for the realization of advanced quantum devices. The reported results open a path toward scalable qubit devices using nanowires on silicon.},
doi = {10.1002/adma.201906523},
journal = {Advanced Materials},
number = 16,
volume = 32,
place = {Germany},
year = {Thu Feb 27 00:00:00 EST 2020},
month = {Thu Feb 27 00:00:00 EST 2020}
}

Journal Article:
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1002/adma.201906523

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Works referenced in this record:

Programmable nanowire circuits for nanoprocessors
journal, February 2011

  • Yan, Hao; Choe, Hwan Sung; Nam, SungWoo
  • Nature, Vol. 470, Issue 7333
  • DOI: 10.1038/nature09749

Monolithic Growth of Ultrathin Ge Nanowires on Si(001)
journal, August 2012


Spin relaxation at the singlet-triplet crossing in a quantum dot
journal, January 2008


Direct Measurement of the Spin-Orbit Interaction in a Two-Electron InAs Nanowire Quantum Dot
journal, June 2007


Shallow and Undoped Germanium Quantum Wells: A Playground for Spin and Hybrid Quantum Technology
journal, January 2019

  • Sammak, Amir; Sabbagh, Diego; Hendrickx, Nico W.
  • Advanced Functional Materials, Vol. 29, Issue 14
  • DOI: 10.1002/adfm.201807613

Template-Assisted Scalable Nanowire Networks
journal, March 2018


Metallization of a Rashba wire by a superconducting layer in the strong-proximity regime
journal, April 2018


Towards Realistic Implementations of a Majorana Surface Code
journal, February 2016


Andreev bound states in supercurrent-carrying carbon nanotubes revealed
journal, November 2010

  • Pillet, J-D.; Quay, C. H. L.; Morfin, P.
  • Nature Physics, Vol. 6, Issue 12
  • DOI: 10.1038/nphys1811

Heavy-Hole States in Germanium Hut Wires
journal, October 2016


Hybrid superconductor–semiconductor devices made from self-assembled SiGe nanocrystals on silicon
journal, May 2010

  • Katsaros, G.; Spathis, P.; Stoffel, M.
  • Nature Nanotechnology, Vol. 5, Issue 6
  • DOI: 10.1038/nnano.2010.84

One-dimensional hole gas in germanium/silicon nanowire heterostructures
journal, July 2005

  • Lu, W.; Xiang, J.; Timko, B. P.
  • Proceedings of the National Academy of Sciences, Vol. 102, Issue 29, p. 10046-10051
  • DOI: 10.1073/pnas.0504581102

Ge/Si nanowire mesoscopic Josephson junctions
journal, December 2006


Effective mass measurement: the influence of hole band nonparabolicity in SiGe/Ge quantum wells
journal, December 2006

  • Rössner, Benjamin; Känel, Hans von; Chrastina, Daniel
  • Semiconductor Science and Technology, Vol. 22, Issue 1
  • DOI: 10.1088/0268-1242/22/1/S45

Self-assembled in-plane Ge nanowires on rib-patterned Si (1 1 10) templates
journal, August 2014


Gate-controlled quantum dots and superconductivity in planar germanium
journal, July 2018


Barrierless Formation and Faceting of SiGe Islands on Si(001)
journal, October 2002


Fast two-qubit logic with holes in germanium
journal, January 2020


Monoisotopic varieties of silicon and germanium with a high chemical and isotopic purity
journal, February 2013


Strain effect on adatom binding and diffusion in homo- and heteroepitaxies of Si and Ge on ( 001 ) Surfaces
journal, October 2004


Circuit QED with hole-spin qubits in Ge/Si nanowire quantum dots
journal, December 2013


Spin–orbit qubit in a semiconductor nanowire
journal, December 2010

  • Nadj-Perge, S.; Frolov, S. M.; Bakkers, E. P. A. M.
  • Nature, Vol. 468, Issue 7327
  • DOI: 10.1038/nature09682

Majorana fermions in Ge/Si hole nanowires
journal, November 2014


Majorana Kramers pairs in Rashba double nanowires with interactions and disorder
journal, January 2018


Spectroscopy of Spin-Orbit Quantum Bits in Indium Antimonide Nanowires
journal, April 2012


Theory of Directed Nucleation of Strained Islands on Patterned Substrates
journal, November 2008


Light effective hole mass in undoped Ge/SiGe quantum wells
journal, July 2019


How pit facet inclination drives heteroepitaxial island positioning on patterned substrates
journal, October 2011


Academic and industry research progress in germanium nanodevices
journal, November 2011


Field effect enhancement in buffered quantum nanowire networks
journal, September 2018


Strong spin-orbit interaction and helical hole states in Ge/Si nanowires
journal, November 2011


Ultra-high hole mobility exceeding one million in a strained germanium quantum well
journal, October 2012

  • Dobbie, A.; Myronov, M.; Morris, R. J. H.
  • Applied Physics Letters, Vol. 101, Issue 17
  • DOI: 10.1063/1.4763476

Strong and Tunable Spin−Orbit Coupling of One-Dimensional Holes in Ge/Si Core/Shell Nanowires
journal, August 2010

  • Hao, Xiao-Jie; Tu, Tao; Cao, Gang
  • Nano Letters, Vol. 10, Issue 8
  • DOI: 10.1021/nl101181e

Simple generic method for predicting the effect of strain on surface diffusion
journal, November 2001


Spin-resolved Andreev levels and parity crossings in hybrid superconductor–semiconductor nanostructures
journal, December 2013

  • Lee, Eduardo J. H.; Jiang, Xiaocheng; Houzet, Manuel
  • Nature Nanotechnology, Vol. 9, Issue 1
  • DOI: 10.1038/nnano.2013.267

Mechanics of coherent and dislocated island morphologies in strained epitaxial material systems
journal, May 1997

  • Johnson, H. T.; Freund, L. B.
  • Journal of Applied Physics, Vol. 81, Issue 9
  • DOI: 10.1063/1.364357

Quantitative Model of Heterogeneous Nucleation and Growth of SiGe Quantum Dot Molecules
journal, September 2012


Shape transition in growth of strained islands: Spontaneous formation of quantum wires
journal, May 1993


Solution-processed core–shell nanowires for efficient photovoltaic cells
journal, August 2011

  • Tang, Jinyao; Huo, Ziyang; Brittman, Sarah
  • Nature Nanotechnology, Vol. 6, Issue 9
  • DOI: 10.1038/nnano.2011.139

Epitaxy of advanced nanowire quantum devices
journal, August 2017

  • Gazibegovic, Sasa; Car, Diana; Zhang, Hao
  • Nature, Vol. 548, Issue 7668
  • DOI: 10.1038/nature23468

Signatures of Majorana Fermions in Hybrid Superconductor-Semiconductor Nanowire Devices
journal, April 2012


A germanium hole spin qubit
journal, September 2018


SiGe growth on patterned Si(001) substrates: Surface evolution and evidence of modified island coarsening
journal, October 2007

  • Zhang, J. J.; Stoffel, M.; Rastelli, A.
  • Applied Physics Letters, Vol. 91, Issue 17
  • DOI: 10.1063/1.2802555

Spins in few-electron quantum dots
journal, October 2007


Antilocalization of Coulomb Blockade in a Ge/Si Nanowire
journal, May 2014


Exponential protection of zero modes in Majorana islands
journal, March 2016

  • Albrecht, S. M.; Higginbotham, A. P.; Madsen, M.
  • Nature, Vol. 531, Issue 7593
  • DOI: 10.1038/nature17162

Selective area heteroepitaxy of GaSb on GaAs (001) for in-plane InAs nanowire achievement
journal, November 2016


Direct Rashba spin-orbit interaction in Si and Ge nanowires with different growth directions
journal, June 2018


Spin–Orbit Interaction and Induced Superconductivity in a One-Dimensional Hole Gas
journal, September 2018


Room-Temperature Ultraviolet Nanowire Nanolasers
journal, June 2001

  • Huang, Michael H.; Mao, Samuel; Feick, Henning
  • Science, Vol. 292, Issue 5523, p. 1897-1899
  • DOI: 10.1126/science.1060367

Fermi-level pinning and charge neutrality level in germanium
journal, December 2006

  • Dimoulas, A.; Tsipas, P.; Sotiropoulos, A.
  • Applied Physics Letters, Vol. 89, Issue 25
  • DOI: 10.1063/1.2410241