Metal- and covalent-organic frameworks as solid-state electrolytes for metal-ion batteries

Miner, Elise M.; Dincă, Mircea

doi:10.1098/rsta.2018.0225

Title: Metal- and covalent-organic frameworks as solid-state electrolytes for metal-ion batteries

Journal Article · 27 May 2019 · Philosophical Transactions of the Royal Society. A, Mathematical, Physical and Engineering Sciences

DOI: https://doi.org/10.1098/rsta.2018.0225 · OSTI ID:1601987

Miner, Elise M. ^[1];

^[1]

Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)

Society’s long-standing energy demands have fuelled for centuries the quest for power-dense, portable and economically viable energy carriers. Since the birth of the first rechargeable battery in 1860, emerging battery technologies have provided both answers to these demands as well as additional obstacles. One ubiquitous energy storage device, the metal or metalion battery, offers quintessential examples of both. The strongly reducing nature of Group 1 and 2 metal ions qualifies these elements as viable energy-dense anode materials: standard reduction potentials several volts below that of the standard hydrogen electrode (SHE) allow a thermodynamically favourable oxidation of these metals to readily release electrons that shuttle through an external circuit, generating the electric current that serves as the power supply during battery discharge. Integration of energy-dense materials into devices allows power sources to be compact and portable, by maximizing energy output per unit mass of material. Further, the reversibility of these oxidation events makes possible extensive battery cycling, thus providing a rechargeable power source. Indeed, current Li-ion batteries boast an energy density of 265 Wh kg^-1, with the potential of a 20% improvement, and are operable for over 1000 charge–discharge cycles.

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Research Organization:: Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0018235

OSTI ID:: 1601987

Journal Information:: Philosophical Transactions of the Royal Society. A, Mathematical, Physical and Engineering Sciences, Vol. 377, Issue 2149; ISSN 1364-503X

Publisher:: The Royal Society PublishingCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 46 works

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Boosting interfacial Li+ transport with a MOF-based ionic conductor for solid-state batteries Wang, Ziqi; Wang, Zijian; Yang, Luyi Nano Energy, Vol. 49 https://doi.org/10.1016/j.nanoen.2018.04.076	journal	July 2018
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Superionic Conductivity in Lithium-Rich Anti-Perovskites Zhao, Yusheng; Daemen, Luke L. Journal of the American Chemical Society, Vol. 134, Issue 36 https://doi.org/10.1021/ja305709z	journal	August 2012
Mechanically Shaped Two-Dimensional Covalent Organic Frameworks Reveal Crystallographic Alignment and Fast Li-Ion Conductivity Vazquez-Molina, Demetrius A.; Mohammad-Pour, Gavin S.; Lee, Chain Journal of the American Chemical Society, Vol. 138, Issue 31 https://doi.org/10.1021/jacs.6b05568	journal	July 2016
Achieving Superprotonic Conduction in Metal–Organic Frameworks through Iterative Design Advances Kim, SiRim; Joarder, Biplab; Hurd, Jeff A. Journal of the American Chemical Society, Vol. 140, Issue 3 https://doi.org/10.1021/jacs.7b11364	journal	January 2018
Stabilization of Hexaaminobenzene in a 2D Conductive Metal–Organic Framework for High Power Sodium Storage Park, Jihye; Lee, Minah; Feng, Dawei Journal of the American Chemical Society, Vol. 140, Issue 32 https://doi.org/10.1021/jacs.8b06020	journal	July 2018
Reactions of the Lithium Salts of the Tribenzylidenemethane Dianion, Diphenylacetone Dianion, and Related Compounds Witt, Ortrun; Mauser, Harald; Friedl, Thomas The Journal of Organic Chemistry, Vol. 63, Issue 4 https://doi.org/10.1021/jo971113c	journal	February 1998
Composite Polymer Electrolytes Encompassing Metal Organic Frame Works: A New Strategy for All-Solid-State Lithium Batteries Angulakshmi, N.; Kumar, R. Senthil; Kulandainathan, M. Anbu The Journal of Physical Chemistry C, Vol. 118, Issue 42 https://doi.org/10.1021/jp506464v	journal	October 2014
Chloride ion conductivity in a plasticized quaternary ammonium polymer Hardy, L. C.; Shriver, D. F. Macromolecules, Vol. 17, Issue 4 https://doi.org/10.1021/ma00134a077	journal	July 1984
Electrolytes for solid-state lithium rechargeable batteries: recent advances and perspectives Quartarone, Eliana; Mustarelli, Piercarlo Chemical Society Reviews, Vol. 40, Issue 5 https://doi.org/10.1039/c0cs00081g	journal	January 2011
Plastic crystalline lithium salt with solid-state ionic conductivity and high lithium transport number Moriya, Makoto; Kato, Daiki; Sakamoto, Wataru Chemical Communications, Vol. 47, Issue 22 https://doi.org/10.1039/c1cc00070e	journal	January 2011
Designer coordination polymers: dimensional crossover architectures and proton conduction Yamada, Teppei; Otsubo, Kazuya; Makiura, Rie Chemical Society Reviews, Vol. 42, Issue 16 https://doi.org/10.1039/c3cs60028a	journal	January 2013
Metal-organic frameworks and their derived materials for electrochemical energy storage and conversion: Promises and challenges Wu, Hao Bin; Lou, Xiong Wen (David) Science Advances, Vol. 3, Issue 12 https://doi.org/10.1126/sciadv.aap9252	journal	December 2017
Modified Metal Organic Frameworks (MOFs)/Ionic Liquid Matrices for Efficient Charge Storage Singh, Ankit; Vedarajan, Raman; Matsumi, Noriyoshi Journal of The Electrochemical Society, Vol. 164, Issue 8 https://doi.org/10.1149/2.0191708jes	journal	January 2017
Proton-Conductive Metal–Organic Frameworks Yamada, Teppei; Sadakiyo, Masaaki; Shigematsu, Akihito Bulletin of the Chemical Society of Japan, Vol. 89, Issue 1 https://doi.org/10.1246/bcsj.20150308	journal	January 2016

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A pre-synthetic strategy to construct single ion conductive covalent organic frameworks Li, Juan; Zhang, Fu-Qiang; Li, Falian Chemical Communications, Vol. 56, Issue 18 https://doi.org/10.1039/d0cc00454e	journal	January 2020
Introduction: minerals to metal-organic frameworks Phillips, Anthony E. Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Vol. 377, Issue 2149 https://doi.org/10.1098/rsta.2019.0153	journal	May 2019

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