Magnetic frustration in a metallic fcc lattice

Stockert, Oliver; Hoffmann, Jens-Uwe; Mühlbauer, Martin; Senyshyn, Anatoliy; Koza, Michael M.; Tsirlin, Alexander A.; Wolf, F. Maximilian; Bachus, Sebastian; Gegenwart, Philipp; Movshovich, Roman; Bobev, Svilen; Fritsch, Veronika

doi:10.1103/PhysRevResearch.2.013183

Title: Magnetic frustration in a metallic fcc lattice

Abstract

Magnetic frustration in metals is scarce and hard to pinpoint, but exciting due to the possibility of the emergence of fascinating novel phases. The cubic intermetallic compound HoInCu₄ with all holmium atoms on an fcc lattice exhibits partial magnetic frustration, yielding a ground state where half of the Ho moments remain without long-range order, as evidenced by our neutron scattering experiments. The substitution of In with Cd results in HoCdCu₄ in a full breakdown of magnetic frustration. Consequently we found a fully ordered magnetic structure in our neutron diffraction experiments. These findings are in agreement with the local energy scales and crystal electric field excitations, which we determined from specific heat and inelastic neutron scattering data. The electronic density of states for the itinerant bands acts as a tuning parameter for the ratio between nearest-neighbor and next-nearest-neighbor interactions and thus for magnetic frustration.

Authors:

Stockert, Oliver; Hoffmann, Jens-Uwe; Mühlbauer, Martin; Senyshyn, Anatoliy; Koza, Michael M.; Tsirlin, Alexander A.; Wolf, F. Maximilian; Bachus, Sebastian; Gegenwart, Philipp; Movshovich, Roman; Bobev, Svilen;

Publication Date:: 2020-02-21

Research Org.:: Univ. of Delaware, Newark, DE (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1601077

Alternate Identifier(s):: OSTI ID: 1697978

Grant/Contract Number:: SC0008885

Resource Type:: Published Article

Journal Name:: Physical Review Research

Additional Journal Information:: Journal Name: Physical Review Research Journal Volume: 2 Journal Issue: 1; Journal ID: ISSN 2643-1564

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Frustrated magnetism; Magnetic phase transitions; Spin-orbit coupling

Citation Formats


                    Stockert, Oliver, Hoffmann, Jens-Uwe, Mühlbauer, Martin, Senyshyn, Anatoliy, Koza, Michael M., Tsirlin, Alexander A., Wolf, F. Maximilian, Bachus, Sebastian, Gegenwart, Philipp, Movshovich, Roman, Bobev, Svilen, and Fritsch, Veronika. Magnetic frustration in a metallic fcc lattice.  United States: N. p., 2020. 
        Web.  doi:10.1103/PhysRevResearch.2.013183.

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                    Stockert, Oliver, Hoffmann, Jens-Uwe, Mühlbauer, Martin, Senyshyn, Anatoliy, Koza, Michael M., Tsirlin, Alexander A., Wolf, F. Maximilian, Bachus, Sebastian, Gegenwart, Philipp, Movshovich, Roman, Bobev, Svilen, & Fritsch, Veronika. Magnetic frustration in a metallic fcc lattice.  United States.  doi:https://doi.org/10.1103/PhysRevResearch.2.013183

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                    Stockert, Oliver, Hoffmann, Jens-Uwe, Mühlbauer, Martin, Senyshyn, Anatoliy, Koza, Michael M., Tsirlin, Alexander A., Wolf, F. Maximilian, Bachus, Sebastian, Gegenwart, Philipp, Movshovich, Roman, Bobev, Svilen, and Fritsch, Veronika. Fri .  
        "Magnetic frustration in a metallic fcc lattice".  United States.  doi:https://doi.org/10.1103/PhysRevResearch.2.013183.

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@article{osti_1601077,

  title        = {Magnetic frustration in a metallic fcc lattice},

  author       = {Stockert, Oliver and Hoffmann, Jens-Uwe and Mühlbauer, Martin and Senyshyn, Anatoliy and Koza, Michael M. and Tsirlin, Alexander A. and Wolf, F. Maximilian and Bachus, Sebastian and Gegenwart, Philipp and Movshovich, Roman and Bobev, Svilen and Fritsch, Veronika},

  abstractNote = {Magnetic frustration in metals is scarce and hard to pinpoint, but exciting due to the possibility of the emergence of fascinating novel phases. The cubic intermetallic compound HoInCu4 with all holmium atoms on an fcc lattice exhibits partial magnetic frustration, yielding a ground state where half of the Ho moments remain without long-range order, as evidenced by our neutron scattering experiments. The substitution of In with Cd results in HoCdCu4 in a full breakdown of magnetic frustration. Consequently we found a fully ordered magnetic structure in our neutron diffraction experiments. These findings are in agreement with the local energy scales and crystal electric field excitations, which we determined from specific heat and inelastic neutron scattering data. The electronic density of states for the itinerant bands acts as a tuning parameter for the ratio between nearest-neighbor and next-nearest-neighbor interactions and thus for magnetic frustration.},

  doi          = {10.1103/PhysRevResearch.2.013183},

  journal      = {Physical Review Research},

  number       = 1,

  volume       = 2,

  place        = {United States},

  year         = {2020},

  month        = {2}

}

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Title: Magnetic frustration in a metallic fcc lattice

Abstract

Citation Formats

Green Functions in the Theory of Antiferromagnetism journal, August 1964

Phase diagram and magnetic structure investigation of the fcc antiferromagnet Ho B 12 journal, December 2004

Spin liquids in frustrated magnets journal, March 2010

The partially disordered state of the frustrated face-centred cubic antiferromagnet journal, January 1999

Cubic symmetry and magnetic frustration on the fcc spin lattice in K 2 IrCl 6 journal, April 2019

The raising of angular momentum degeneracy of f-Electron terms by cubic crystal fields journal, October 1962

Transport properties of RInCu4 with C15b-type structure journal, February 1995

Multi-functional properties of non-centrosymmetric ternary half-Heuslers, RPdSb (R = Er and Ho) journal, June 2018

Anomalous magnetism of the frustrated compound GdInCu4 journal, May 1993

Direct Observation of a Nuclear Spin Excitation in Ho 2 Ti 2 O 7 journal, January 2009

Magnetic Properties of the Frustrated fcc – Antiferromagnet HoB12 Above and Below T N journal, January 2007

Magnetic structures of (Gd 1-x Y x )Mn 2 Ge 2 and (Tb 1-x Y x )Mn 2 Ge 2 studied by neutron powder diffraction journal, January 2018

Correlation between magnetic frustration and electrical conductivity in R In Cu 4 compounds ( R = Gd − Tm ) journal, March 2006

Effect of vertical divergence on the displacement and breadth of X-ray powder diffraction lines journal, November 1952

Direct observation of low energy nuclear spin excitations in HoCrO 3 by high resolution neutron spectroscopy journal, June 2013

Kitaev-Heisenberg models for iridates on the triangular, hyperkagome, kagome, fcc, and pyrochlore lattices journal, January 2014

Accurate and simple analytic representation of the electron-gas correlation energy journal, June 1992

Highly anisotropic exchange interactions of j eff = 1 2 iridium moments on the fcc lattice in La 2 B IrO 6 ( B = Mg , Zn ) journal, June 2016

Spin and orbital frustration in R In Cu 4 ( R = Gd , Dy, Ho, and Er) journal, April 2005

Specific Heat of Holmium Metal between 0.38 and 4.2°K journal, November 1962

Low energy nuclear spin excitations in Ho metal investigated by high resolution neutron spectroscopy journal, March 2013

La structure des substances magnetiques journal, October 1959

The magnetic order of GdMn 2 Ge 2 studied by neutron diffraction and x-ray resonant magnetic scattering journal, May 2010

Hyperfine and crystal field interactions in multiferroic HoCrO 3 journal, September 2016

Generalizations of the Weiss Molecular Field Theory of Antiferromagnetism journal, August 1950

Anisotropic magnetic phase diagrams of HoB4 single crystal journal, April 2009

A correction for powder diffraction peak asymmetry due to axial divergence journal, December 1994

Influence of 3 d − 4 f interactions in the magnetic phases of R Fe x Mn 12 − x ( R = Gd , Tb, and Dy) compounds: Coexistence of ferromagnetism and antiferromagnetism at different crystallographic sites journal, June 2007

Spin Ice State in Frustrated Magnetic Pyrochlore Materials journal, November 2001

Magnetic and transport properties of the rare-earth-based Heusler phases R Pd Z and R Pd 2 Z ( Z = Sb , Bi ) journal, September 2005

Magnetic phase transition in studied by neutron diffraction journal, March 2007

Strongly Geometrically Frustrated Magnets journal, August 1994

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The J 1 - J 2 model on the face-centered-cubic lattices journal, May 2018

Low temperature magnetocaloric properties of HoNi2 journal, May 2003

Magnetic Properties and Nuclear Magnetic Resonance of Cubic RCu 5 Intermetallic Compounds journal, October 1970

Green Functions in the Theory of Antiferromagnetism
journal, August 1964

Phase diagram and magnetic structure investigation of the fcc antiferromagnet $Ho B_{12}$
journal, December 2004

Spin liquids in frustrated magnets
journal, March 2010

The partially disordered state of the frustrated face-centred cubic antiferromagnet
journal, January 1999

Cubic symmetry and magnetic frustration on the fcc spin lattice in $K_{2} {IrCl}_{6}$
journal, April 2019

The raising of angular momentum degeneracy of f-Electron terms by cubic crystal fields
journal, October 1962

Transport properties of RInCu4 with C15b-type structure
journal, February 1995

Multi-functional properties of non-centrosymmetric ternary half-Heuslers, RPdSb (R = Er and Ho)
journal, June 2018

Anomalous magnetism of the frustrated compound GdInCu4
journal, May 1993

Direct Observation of a Nuclear Spin Excitation in ${Ho}_{2} {Ti}_{2} O_{7}$
journal, January 2009

Magnetic Properties of the Frustrated fcc – Antiferromagnet HoB12 Above and Below T N
journal, January 2007

Magnetic structures of (Gd _1-x Y _x )Mn ₂ Ge ₂ and (Tb _1-x Y _x )Mn ₂ Ge ₂ studied by neutron powder diffraction
journal, January 2018

Correlation between magnetic frustration and electrical conductivity in $R In {Cu}_{4}$ compounds $(R = Gd − Tm)$
journal, March 2006

Effect of vertical divergence on the displacement and breadth of X-ray powder diffraction lines
journal, November 1952

Direct observation of low energy nuclear spin excitations in HoCrO ₃ by high resolution neutron spectroscopy
journal, June 2013

Kitaev-Heisenberg models for iridates on the triangular, hyperkagome, kagome, fcc, and pyrochlore lattices
journal, January 2014

Accurate and simple analytic representation of the electron-gas correlation energy
journal, June 1992

Highly anisotropic exchange interactions of $j_{eff} = \frac{1}{2}$ iridium moments on the fcc lattice in ${La}_{2} B {IrO}_{6} (B = Mg, Zn)$
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Spin and orbital frustration in $R In {Cu}_{4}$ ( $R = Gd$ , Dy, Ho, and Er)
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Specific Heat of Holmium Metal between 0.38 and 4.2°K
journal, November 1962

Low energy nuclear spin excitations in Ho metal investigated by high resolution neutron spectroscopy
journal, March 2013

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The magnetic order of GdMn ₂ Ge ₂ studied by neutron diffraction and x-ray resonant magnetic scattering
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Hyperfine and crystal field interactions in multiferroic HoCrO ₃
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Generalizations of the Weiss Molecular Field Theory of Antiferromagnetism
journal, August 1950

Anisotropic magnetic phase diagrams of HoB4 single crystal
journal, April 2009

A correction for powder diffraction peak asymmetry due to axial divergence
journal, December 1994

Influence of $3 d − 4 f$ interactions in the magnetic phases of $R {Fe}_{x} {Mn}_{12 - x}$ ( $R = Gd$ , Tb, and Dy) compounds: Coexistence of ferromagnetism and antiferromagnetism at different crystallographic sites
journal, June 2007

Spin Ice State in Frustrated Magnetic Pyrochlore Materials
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Magnetic and transport properties of the rare-earth-based Heusler phases $R Pd Z$ and $R {Pd}_{2} Z$ $(Z = Sb, Bi)$
journal, September 2005

Magnetic phase transition in studied by neutron diffraction
journal, March 2007

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journal, August 1994

Full-potential nonorthogonal local-orbital minimum-basis band-structure scheme
journal, January 1999

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journal, May 2018

Low temperature magnetocaloric properties of HoNi2
journal, May 2003

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journal, October 1970