Emerging investigator series: influence of marine emissions and atmospheric processing on individual particle composition of summertime Arctic aerosol over the Bering Strait and Chukchi Sea
Abstract
The Arctic is rapidly transforming due to sea ice loss, increasing shipping activity, and oil and gas development. Associated marine and combustion emissions influence atmospheric aerosol composition, impacting complex aerosol–cloud–climate feedbacks. To improve understanding of the sources and processes determining Arctic aerosol composition, atmospheric particles were collected aboard the Korean icebreaker R/V Araon cruising within the Bering Strait and Chukchi Sea during August 2016. Offline analyses of individual particles by microspectroscopic techniques, including scanning electron microscopy with energy dispersive X-ray spectroscopy and atomic force microscopy with infrared spectroscopy, provided information on particle size, morphology, and chemical composition. The most commonly observed particle types were sea spray aerosol (SSA), comprising ~60–90%, by number, of supermicron particles, and organic aerosol (OA), comprising ~50–90%, by number, of submicron particles. Sulfate and nitrate were internally mixed within both SSA and OA particles, consistent with particle multiphase reactions during atmospheric transport. Within the Bering Strait, SSA and OA particles were more aged, with greater number fractions of particles containing sulfate and/or nitrate, compared to particles collected over the Chukchi Sea. This is indicative of greater pollution influence within the Bering Strait from coastal and inland sources, while the Chukchi Sea is primarily influenced by marinemore »
- Authors:
-
- Univ. of Michigan, Ann Arbor, MI (United States). Dept. of Chemistry
- Univ. of California, Irvine, CA (United States). Dept. of Earth System Science
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States). Environmental Molecular Sciences Lab. (EMSL)
- Korea Polar Research Inst., Incheon (South Korea)
- Univ. of Michigan, Ann Arbor, MI (United States). Dept. of Chemistry and Dept. of Environmental Health Sciences
- Univ. of Michigan, Ann Arbor, MI (United States). Dept. of Chemistry and Dept. of Earth & Environmental Sciences
- Publication Date:
- Research Org.:
- Pacific Northwest National Laboratory (PNNL), Richland, WA (United States). Environmental Molecular Sciences Laboratory (EMSL)
- Sponsoring Org.:
- USDOE Office of Science (SC), Biological and Environmental Research (BER); Ministry of Oceans and Fisheries (MOF) South Korea
- OSTI Identifier:
- 1650015
- Alternate Identifier(s):
- OSTI ID: 1601031
- Report Number(s):
- PNNL-SA-148936
Journal ID: ISSN 2050-7887
- Grant/Contract Number:
- AC05-76RL01830; 20160245
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Environmental Science: Processes & Impacts
- Additional Journal Information:
- Journal Volume: 22; Journal Issue: 5; Journal ID: ISSN 2050-7887
- Publisher:
- Royal Society of Chemistry
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 54 ENVIRONMENTAL SCIENCES; marine aerosol; atmospheric chemistry; Arctic; sulfate; summer
Citation Formats
Kirpes, Rachel M., Rodriguez, Blanca, Kim, Saewung, China, Swarup, Laskin, Alexander, Park, Keyhong, Jung, Jinyoung, Ault, Andrew P., and Pratt, Kerri A. Emerging investigator series: influence of marine emissions and atmospheric processing on individual particle composition of summertime Arctic aerosol over the Bering Strait and Chukchi Sea. United States: N. p., 2020.
Web. doi:10.1039/c9em00495e.
Kirpes, Rachel M., Rodriguez, Blanca, Kim, Saewung, China, Swarup, Laskin, Alexander, Park, Keyhong, Jung, Jinyoung, Ault, Andrew P., & Pratt, Kerri A. Emerging investigator series: influence of marine emissions and atmospheric processing on individual particle composition of summertime Arctic aerosol over the Bering Strait and Chukchi Sea. United States. https://doi.org/10.1039/c9em00495e
Kirpes, Rachel M., Rodriguez, Blanca, Kim, Saewung, China, Swarup, Laskin, Alexander, Park, Keyhong, Jung, Jinyoung, Ault, Andrew P., and Pratt, Kerri A. Tue .
"Emerging investigator series: influence of marine emissions and atmospheric processing on individual particle composition of summertime Arctic aerosol over the Bering Strait and Chukchi Sea". United States. https://doi.org/10.1039/c9em00495e. https://www.osti.gov/servlets/purl/1650015.
@article{osti_1650015,
title = {Emerging investigator series: influence of marine emissions and atmospheric processing on individual particle composition of summertime Arctic aerosol over the Bering Strait and Chukchi Sea},
author = {Kirpes, Rachel M. and Rodriguez, Blanca and Kim, Saewung and China, Swarup and Laskin, Alexander and Park, Keyhong and Jung, Jinyoung and Ault, Andrew P. and Pratt, Kerri A.},
abstractNote = {The Arctic is rapidly transforming due to sea ice loss, increasing shipping activity, and oil and gas development. Associated marine and combustion emissions influence atmospheric aerosol composition, impacting complex aerosol–cloud–climate feedbacks. To improve understanding of the sources and processes determining Arctic aerosol composition, atmospheric particles were collected aboard the Korean icebreaker R/V Araon cruising within the Bering Strait and Chukchi Sea during August 2016. Offline analyses of individual particles by microspectroscopic techniques, including scanning electron microscopy with energy dispersive X-ray spectroscopy and atomic force microscopy with infrared spectroscopy, provided information on particle size, morphology, and chemical composition. The most commonly observed particle types were sea spray aerosol (SSA), comprising ~60–90%, by number, of supermicron particles, and organic aerosol (OA), comprising ~50–90%, by number, of submicron particles. Sulfate and nitrate were internally mixed within both SSA and OA particles, consistent with particle multiphase reactions during atmospheric transport. Within the Bering Strait, SSA and OA particles were more aged, with greater number fractions of particles containing sulfate and/or nitrate, compared to particles collected over the Chukchi Sea. This is indicative of greater pollution influence within the Bering Strait from coastal and inland sources, while the Chukchi Sea is primarily influenced by marine sources.},
doi = {10.1039/c9em00495e},
journal = {Environmental Science: Processes & Impacts},
number = 5,
volume = 22,
place = {United States},
year = {Tue Feb 11 00:00:00 EST 2020},
month = {Tue Feb 11 00:00:00 EST 2020}
}
Web of Science
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