Two-Dimensional Hybrid Halide Perovskites: Principles and Promises

Mao, Lingling; Stoumpos, Constantinos C.; Kanatzidis, Mercouri G.

doi:10.1021/jacs.8b10851

Title: Two-Dimensional Hybrid Halide Perovskites: Principles and Promises

Journal Article · 06 November 2018 · Journal of the American Chemical Society

DOI: https://doi.org/10.1021/jacs.8b10851 · OSTI ID:1599730

^[1]; Stoumpos, Constantinos C. ^[1];

^[1]

Northwestern Univ., Evanston, IL (United States)

Hybrid halide perovskites have become the “next big thing” in emerging semiconductor materials as the past decade witnessed their successful application in high-performance photovoltaics. This resurgence has seen enormous and widespread development of the three-dimensional (3D) perovskites, spearheaded by CH₃NH₃PbI₃. The next generation of halide perovskites, however, is characterized by reduced dimensionality perovskites, emphasizing on the two-dimensional (2D) perovskite derivatives which expand as a more diverse subgroup of semiconducting hybrids that possesses even higher tunability and excellent photophysical properties. In this perspective, we start with a histori-cal flashback that traces back to early reports before the “perovskite fever” and we follow this original work to its fruition in the present day, where 2D halide perov-skites are on the spotlight of current research, thriving on several aspects of high-performance optoelectronics. We approach the evolution of 2D halide perovskites from a structural perspective, providing a classification for the diverse structure-types of the materials, which largely dictate the unusual physical properties ob-served. We sort out the 2D hybrid halide perovskite based on two key components: the inorganic layers and their modification and the organic cation diversity. As these two heterogeneous components blend, either by synthetic manipulation (shuffling the organic cations or inorganic elements) or by external stimuli (temperature and pressure), the modular perovskite structure evolves to construct crystallographically defined quantum wells (QW). The complex electronic structure that arises is sensitive to the structural features that could be in turn used as a knob to control the dielectric and optical properties the QWs. We end this perspective with the most notable optoelectronic device achievements that have been demonstrated to date with an eye to-wards future material discovery and potential techno-logical developments.

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Research Organization:: Univ. of California, Santa Barbara, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0012541

OSTI ID:: 1599730

Journal Information:: Journal of the American Chemical Society, Vol. 141, Issue 3; ISSN 0002-7863

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 892 works

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Compositional and Dimensional Control of 2D and Quasi‐2D Lead Halide Perovskites in Water Jana, Atanu; Ba, Qiankai; Kim, Kwang S. Advanced Functional Materials, Vol. 29, Issue 28 https://doi.org/10.1002/adfm.201900966	journal	May 2019
Tin Halide Perovskites: Progress and Challenges Yang, Wen‐Fan; Igbari, Femi; Lou, Yan‐Hui Advanced Energy Materials, Vol. 10, Issue 13 https://doi.org/10.1002/aenm.201902584	journal	April 2020
Synthesis of triphenylpyridines via an oxidative cyclization reaction using Sr-doped LaCoO ₃ perovskite as a recyclable heterogeneous catalyst Le, Thu N. M.; Doan, Son H.; Pham, Phuc H. RSC Advances, Vol. 9, Issue 41 https://doi.org/10.1039/c9ra04096j	journal	January 2019
Switching hydrogen bonds to readily interconvert two room-temperature long-term stable crystalline polymorphs in chiral molecular perovskites Hu, Wang-Hua; Xu, Wei-Jian; Meng, Qian-Ru Chemical Communications, Vol. 55, Issue 77 https://doi.org/10.1039/c9cc05967a	journal	January 2019
Intrinsic Self‐Trapped Emission in 0D Lead‐Free (C ₄ H ₁₄ N ₂ ) ₂ In ₂ Br ₁₀ Single Crystal Zhou, Lei; Liao, Jin‐Feng; Huang, Zeng‐Guang Angewandte Chemie International Edition, Vol. 58, Issue 43 https://doi.org/10.1002/anie.201907503	journal	October 2019
Benzodithiophene Hole‐Transporting Materials for Efficient Tin‐Based Perovskite Solar Cells Vegiraju, Sureshraju; Ke, Weijun; Priyanka, Pragya Advanced Functional Materials, Vol. 29, Issue 45 https://doi.org/10.1002/adfm.201905393	journal	September 2019
Resurfacing halide perovskite nanocrystals Almeida, Guilherme; Infante, Ivan; Manna, Liberato Science, Vol. 364, Issue 6443 https://doi.org/10.1126/science.aax5825	journal	May 2019
Synthesis of a two-dimensional organic–inorganic bismuth iodide metalate through in situ formation of iminium cations Dehnhardt, Natalie; Luy, Jan-Niclas; Szabo, Marvin Chemical Communications, Vol. 55, Issue 98 https://doi.org/10.1039/c9cc06625j	journal	January 2019
Direct oxidative C(sp ³ )─H/C(sp ² )─H coupling reaction using recyclable Sr‐doped LaCoO ₃ perovskite catalyst Trinh, Khang H.; Tran, Phuong H.; Nguyen, Thanh T. Applied Organometallic Chemistry, Vol. 34, Issue 4 https://doi.org/10.1002/aoc.5515	journal	January 2020
Constructing moisture-stable hybrid lead iodine semiconductors based on hydrogen-bond-free and dual-iodine strategies Liu, Guang-Ning; Zhao, Ruo-Yu; Xu, Rang-Dong Journal of Materials Chemistry C, Vol. 7, Issue 25 https://doi.org/10.1039/c9tc01967g	journal	January 2019
(TMT–TTF)[Pb _2.6/3 □ _0.4/3 I ₂ ] ₃ : a TTF-intercalated two-dimensional hybrid lead iodide: crystal structure and properties Yin, Wen-Yu; Weng, Yi-Gang; Jiang, Miao New Journal of Chemistry, Vol. 44, Issue 4 https://doi.org/10.1039/c9nj04316k	journal	January 2020
Organic intercalation engineering of quasi-2D Dion–Jacobson α-CsPbI ₃ perovskites Fang, Zhi; Shang, Minghui; Zheng, Yapeng Materials Horizons, Vol. 7, Issue 4 https://doi.org/10.1039/c9mh01788g	journal	January 2020
Engineering Multiphase Metal Halide Perovskites Thin Films for Stable and Efficient Solar Cells Kim, Min; Figueroa-Tapia, Jetsabel M.; Prato, Mirko Zenodo https://doi.org/10.5281/zenodo.3738931	text	January 2020
Polarized near-infrared intersubband absorptions in CdSe colloidal quantum wells Diroll, Benjamin T.; Chen, Menglu; Coropceanu, Igor Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-12503-z	journal	October 2019
Exploring the role of halide mixing in lead-free BZA ₂ SnX ₄ two dimensional hybrid perovskites Pisanu, Ambra; Coduri, Mauro; Morana, Marta Journal of Materials Chemistry A, Vol. 8, Issue 4 https://doi.org/10.1039/c9ta11923j	journal	January 2020
Research Direction toward Scalable, Stable, and High Efficiency Perovskite Solar Cells Park, Nam‐Gyu Advanced Energy Materials, Vol. 10, Issue 13 https://doi.org/10.1002/aenm.201903106	journal	April 2020
(CH ₃ NH ₃ )AuX ₄ ⋅H ₂ O (X=Cl, Br) and (CH ₃ NH ₃ )AuCl ₄ : Low‐Band Gap Lead‐Free Layered Gold Halide Perovskite Materials Worley, Chris; Yangui, Aymen; Roccanova, Rachel Chemistry – A European Journal, Vol. 25, Issue 42 https://doi.org/10.1002/chem.201901112	journal	July 2019
Structure-directing effects in (110)-layered hybrid perovskites containing two distinct organic moieties Guo, Yuan-Yuan; McNulty, Jason A.; Mica, Natalie A. Chemical Communications, Vol. 55, Issue 67 https://doi.org/10.1039/c9cc04964a	journal	January 2019
An Effective Strategy for Photoelectric Performance Enhancement of 2D Perovskite via Halogenating Organic Cation: A Theoretical Prediction Tang, Yong; Zhou, Yingtang; Zhong, Xiangli physica status solidi (b), Vol. 257, Issue 5 https://doi.org/10.1002/pssb.201900599	journal	January 2020
Guanine‐Stabilized Formamidinium Lead Iodide Perovskites Hong, Li; Milić, Jovana V.; Ahlawat, Paramvir Angewandte Chemie, Vol. 132, Issue 12 https://doi.org/10.1002/ange.201912051	journal	February 2020
Ruddlesden–Popper Perovskites: Synthesis and Optical Properties for Optoelectronic Applications Gao, Xupeng; Zhang, Xiangtong; Yin, Wenxu Advanced Science, Vol. 6, Issue 22 https://doi.org/10.1002/advs.201900941	journal	October 2019
Intrinsic Self‐Trapped Emission in 0D Lead‐Free (C ₄ H ₁₄ N ₂ ) ₂ In ₂ Br ₁₀ Single Crystal Zhou, Lei; Liao, Jin‐Feng; Huang, Zeng‐Guang Angewandte Chemie, Vol. 131, Issue 43 https://doi.org/10.1002/ange.201907503	journal	September 2019
Exciton-band tuning induced by the width of the cation in 2D lead iodide perovskite hybrids Tremblay, Marie-Hélène; Bacsa, John; Barlow, Stephen Materials Chemistry Frontiers https://doi.org/10.1039/d0qm00118j	journal	January 2020
Engineering Multiphase Metal Halide Perovskites Thin Films for Stable and Efficient Solar Cells Kim, Min; Figueroa‐Tapia, Jetsabel M.; Prato, Mirko Advanced Energy Materials, Vol. 10, Issue 8 https://doi.org/10.1002/aenm.201903221	journal	January 2020
Hybrid Halide Perovskites: Discussions on Terminology and Materials Mercier, Nicolas Angewandte Chemie, Vol. 131, Issue 50 https://doi.org/10.1002/ange.201909601	journal	October 2019
Inducing Charge Separation in Solid-State Two-Dimensional Hybrid Perovskites through the Incorporation of Organic Charge-Transfer Complexes Gélvez-Rueda, María C.; Van Gompel, Wouter T. M.; Herckens, Roald The Journal of Physical Chemistry Letters, Vol. 11, Issue 3 https://doi.org/10.1021/acs.jpclett.9b03746	journal	January 2020
Incorporating Large A Cations into Lead Iodide Perovskite Cages: Relaxed Goldschmidt Tolerance Factor and Impact on Exciton–Phonon Interaction Fu, Yongping; Hautzinger, Matthew P.; Luo, Ziyu ACS Central Science, Vol. 5, Issue 8 https://doi.org/10.1021/acscentsci.9b00367	journal	July 2019
Prospects for low-toxicity lead-free perovskite solar cells Ke, Weijun; Kanatzidis, Mercouri G. Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-08918-3	journal	February 2019
Polarized near-infrared intersubband absorptions in CdSe colloidal quantum wells Diroll, Benjamin T.; Chen, Menglu; Coropceanu, Igor Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-12503-z	journal	October 2019

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