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Title: Strengthened relaxor behavior in (1− x )Pb(Fe 0.5 Nb 0.5 )O 3x BiFeO 3

Abstract

A systematic study of (1− x )Pb(Fe 0.5 Nb 0.5 )O 3 – x BiFeO 3 ( x = 0–0.5) was performed in order to investigate the strengthening of the relaxor properties when adding BiFeO 3 into Pb(Fe 0.5 Nb 0.5 )O 3 and forming a solid solution.

Authors:
 [1];  [2];  [1];  [1];  [3];  [4];  [3];  [5]; ORCiD logo [5]; ORCiD logo [1]
  1. Jožef Stefan Institute, 1000 Ljubljana, Slovenia, Jožef Stefan International Postgraduate School, 1000 Ljubljana
  2. Jožef Stefan Institute, 1000 Ljubljana, Slovenia
  3. Department of Materials Science and Engineering, North Carolina State University, Raleigh, USA
  4. Analytical Instrumentation Facility, North Carolina State University, Raleigh, USA
  5. Colorado School of Mines, Golden, USA
Publication Date:
Sponsoring Org.:
USDOE
OSTI Identifier:
1598715
Grant/Contract Number:  
AC02-06CH11357
Resource Type:
Published Article
Journal Name:
Journal of Materials Chemistry C
Additional Journal Information:
Journal Name: Journal of Materials Chemistry C; Journal ID: ISSN 2050-7526
Publisher:
Royal Society of Chemistry (RSC)
Country of Publication:
United Kingdom
Language:
English

Citation Formats

Prah, Uroš, Dragomir, Mirela, Rojac, Tadej, Benčan, Andreja, Broughton, Rachel, Chung, Ching-Chang, Jones, Jacob L., Sherbondy, Rachel, Brennecka, Geoff, and Uršič, Hana. Strengthened relaxor behavior in (1− x )Pb(Fe 0.5 Nb 0.5 )O 3 – x BiFeO 3. United Kingdom: N. p., 2020. Web. doi:10.1039/C9TC05883D.
Prah, Uroš, Dragomir, Mirela, Rojac, Tadej, Benčan, Andreja, Broughton, Rachel, Chung, Ching-Chang, Jones, Jacob L., Sherbondy, Rachel, Brennecka, Geoff, & Uršič, Hana. Strengthened relaxor behavior in (1− x )Pb(Fe 0.5 Nb 0.5 )O 3 – x BiFeO 3. United Kingdom. doi:10.1039/C9TC05883D.
Prah, Uroš, Dragomir, Mirela, Rojac, Tadej, Benčan, Andreja, Broughton, Rachel, Chung, Ching-Chang, Jones, Jacob L., Sherbondy, Rachel, Brennecka, Geoff, and Uršič, Hana. Wed . "Strengthened relaxor behavior in (1− x )Pb(Fe 0.5 Nb 0.5 )O 3 – x BiFeO 3". United Kingdom. doi:10.1039/C9TC05883D.
@article{osti_1598715,
title = {Strengthened relaxor behavior in (1− x )Pb(Fe 0.5 Nb 0.5 )O 3 – x BiFeO 3},
author = {Prah, Uroš and Dragomir, Mirela and Rojac, Tadej and Benčan, Andreja and Broughton, Rachel and Chung, Ching-Chang and Jones, Jacob L. and Sherbondy, Rachel and Brennecka, Geoff and Uršič, Hana},
abstractNote = {A systematic study of (1− x )Pb(Fe 0.5 Nb 0.5 )O 3 – x BiFeO 3 ( x = 0–0.5) was performed in order to investigate the strengthening of the relaxor properties when adding BiFeO 3 into Pb(Fe 0.5 Nb 0.5 )O 3 and forming a solid solution.},
doi = {10.1039/C9TC05883D},
journal = {Journal of Materials Chemistry C},
number = ,
volume = ,
place = {United Kingdom},
year = {2020},
month = {1}
}

Journal Article:
Free Publicly Available Full Text
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DOI: 10.1039/C9TC05883D

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Works referenced in this record:

Structural properties of multiferroic 0.5BiFeO3–0.5Pb(Fe0.5Nb0.5)O3 solid solution
journal, April 2017


Ferroelectromagnetic Smart Structures (1-x)Pb(Fe 0.5 Nb 0.5 )O 3 -(x)BiFeO 3
journal, September 2009


Magnetoelectric and electric measurements of the (1− x )BiFeO 3 –( x )Pb(Fe 1/2 Nb 1/2 )O 3 solid solutions
journal, July 2017


Electrical and Electromechanical Properties of Hot-Pressed Pb(Fe 1/2 Nb 1/2 )O 3 Ferroelectric Ceramics
journal, March 1993

  • Yokosuka, Masaru
  • Japanese Journal of Applied Physics, Vol. 32, Issue Part 1, No. 3A
  • DOI: 10.1143/JJAP.32.1142

Role of charged defects on the electrical and electromechanical properties of rhombohedral Pb ( Zr , Ti ) O 3 with oxygen octahedra tilts
journal, January 2016


Hardening-softening transition in Fe-doped Pb(Zr,Ti)O3 ceramics and evolution of the third harmonic of the polarization response
journal, August 2008

  • Morozov, Maxim I.; Damjanovic, Dragan
  • Journal of Applied Physics, Vol. 104, Issue 3
  • DOI: 10.1063/1.2963704

Large electrocaloric effect in grain-size-engineered 0.9Pb(Mg 1/3 Nb 2/3 )O 3 –0.1PbTiO 3
journal, January 2016


Recent progress in relaxor ferroelectrics with perovskite structure
journal, January 2006


Improvement of the dielectric and ferroelectric properties of multiferroic Pb(Fe1/2Nb1/2)O3 ceramics processed in oxygen atmosphere
journal, April 2016

  • Font, Reynaldo; Raymond-Herrera, Oscar; Mestres, Lourdes
  • Journal of Materials Science, Vol. 51, Issue 13
  • DOI: 10.1007/s10853-016-9928-1

Ferroelectric hysteresis and aging effect analysis in multiferroic Pb(Fe0.5Nb0.5)O3 ceramics
journal, June 2009

  • Font, R.; Raymond, O.; Martinez, E.
  • Journal of Applied Physics, Vol. 105, Issue 11
  • DOI: 10.1063/1.3142420

Magnetoelectric investigation of the system BiFeO3Pb(Fe0.5Nb0.5)O3
journal, January 1980

  • Ismailzade, I. H.; Ismailov, R. M.; Alekperov, A. I.
  • Physica Status Solidi (a), Vol. 57, Issue 1
  • DOI: 10.1002/pssa.2210570108

The spontaneous relaxor‐ferroelectric transition of Pb(Sc 0.5 Ta 0.5 )O 3
journal, October 1993

  • Chu, F.; Setter, N.; Tagantsev, A. K.
  • Journal of Applied Physics, Vol. 74, Issue 8
  • DOI: 10.1063/1.354300

Positive temperature coefficient of resistivity in Pb(Fe 1/2 Nb 1/2 )O 3 ceramics
journal, July 2004


Analysis of Recent Measurements of the Viscosity of Glasses
journal, June 1925


Vogel-Fulcher freezing in relaxor ferroelectrics
journal, July 2007


A fundamental parameters approach to X-ray line-profile fitting
journal, April 1992


Polar nanodomains and local ferroelectric phenomena in relaxor lead lanthanum zirconate titanate ceramics
journal, May 2005

  • Shvartsman, V. V.; Kholkin, A. L.; Orlova, A.
  • Applied Physics Letters, Vol. 86, Issue 20
  • DOI: 10.1063/1.1923756

Simple ways of determining perovskite structures
journal, November 1975


Local Structural Heterogeneity and Electromechanical Responses of Ferroelectrics: Learning from Relaxor Ferroelectrics
journal, July 2018

  • Li, Fei; Zhang, Shujun; Damjanovic, Dragan
  • Advanced Functional Materials, Vol. 28, Issue 37
  • DOI: 10.1002/adfm.201801504

Origin of the large electrostrain in BiFeO 3 -BaTiO 3 based lead-free ceramics
journal, January 2019

  • Wang, Ge; Fan, Zhongming; Murakami, Shunsuke
  • Journal of Materials Chemistry A, Vol. 7, Issue 37
  • DOI: 10.1039/C9TA07904A

Improving the multicaloric properties of Pb(Fe0.5Nb0.5)O3 by controlling the sintering conditions and doping with manganese
journal, November 2019


Some Properties of Bismuth Perovskites
journal, February 1962

  • Buhrer, Carl F.
  • The Journal of Chemical Physics, Vol. 36, Issue 3
  • DOI: 10.1063/1.1732613

Feret‘s Statistical Diameter as a Measure of Particle Size
journal, August 1948


Short- and medium-range structure of multiferroic Pb(Fe 1 / 2 Nb 1 / 2 )O 3 studied using neutron total scattering analysis
journal, February 2011


Anelastic relaxor behavior of Pb(Mg 1/3 Nb 2/3 )O 3
journal, August 2013

  • Uršič, Hana; Damjanovic, Dragan
  • Applied Physics Letters, Vol. 103, Issue 7
  • DOI: 10.1063/1.4818665

Microstructure and properties of lead ferroniobate ceramics (Pb(Fe0.5Nb0.5)O3)
journal, September 1993


Physics and Applications of Bismuth Ferrite
journal, June 2009


Unusual structural-disorder stability of mechanochemically derived-Pb(Sc 0.5 Nb 0.5 )O 3
journal, January 2015

  • Uršič, Hana; Benčan, Andreja; Dražič, Goran
  • Journal of Materials Chemistry C, Vol. 3, Issue 39
  • DOI: 10.1039/C5TC02205C

Electrical after-effects in Pb(Ti, Zr)O3 ceramics
journal, January 1977


Magnetoelectric properties of 0.5BiFeO3–0.5Pb(Fe0.5Nb0.5)O3 solid solution
journal, August 2018


Lattice dynamics and broad-band dielectric properties of multiferroic Pb(Fe 1/2 Nb 1/2 )O 3 ceramics
journal, February 2015

  • Mackeviciute, R.; Goian, V.; Greicius, S.
  • Journal of Applied Physics, Vol. 117, Issue 8
  • DOI: 10.1063/1.4913286

Crystal-structure and magnetic phase transformations in solid solutions of BiFeO3-AFe0.5Nb0.5O3 (A = Ca, Sr, Ba, Pb)
journal, August 2008

  • Troyanchuk, I. O.; Bushinsky, M. V.; Chobot, A. N.
  • Journal of Experimental and Theoretical Physics, Vol. 107, Issue 2
  • DOI: 10.1134/S1063776108080086

Spontaneous (zero‐field) relaxor–to–ferroelectric‐phase transition in disordered Pb(Sc 1/2 Nb 1/2 )O 3
journal, February 1995

  • Chu, F.; Reaney, I. M.; Setter, N.
  • Journal of Applied Physics, Vol. 77, Issue 4
  • DOI: 10.1063/1.358856

Nature of ferroelectric to paraelectric phase transition in multiferroic 0.8BiFeO3–0.2Pb(Fe1/2Nb1/2)O3 ceramics
journal, May 2010

  • Patel, Jay Prakash; Singh, Anar; Pandey, Dhananjai
  • Journal of Applied Physics, Vol. 107, Issue 10
  • DOI: 10.1063/1.3428410

Phase diagram of the system of (1–х)BiFeO3–x PbFe0.5Nb0.5O3 solid solutions at room temperature
journal, March 2016

  • Shilkina, L. A.; Pavlenko, A. V.; Reznitchenko, L. A.
  • Crystallography Reports, Vol. 61, Issue 2
  • DOI: 10.1134/S1063774516020231

Electrostrictive and Piezoelectric Materials for Actuator Applications
journal, April 1992

  • Damjanovic, D.; Newnham, R. E.
  • Journal of Intelligent Material Systems and Structures, Vol. 3, Issue 2
  • DOI: 10.1177/1045389X9200300201

Fabrication of PMN and PFN ceramics by a two-stage sintering technique
journal, December 1999


Anti-ferrodistortive Nanodomains in PMN Relaxor
conference, January 2003

  • Tkachuk, A.
  • Fundamental Physics of Ferroelectrics 2003, AIP Conference Proceedings
  • DOI: 10.1063/1.1609938

Relationship between Local Structure and Relaxor Behavior in Perovskite Oxides
journal, December 2007


BiFeO 3 Ceramics: Processing, Electrical, and Electromechanical Properties
journal, May 2014

  • Rojac, Tadej; Bencan, Andreja; Malic, Barbara
  • Journal of the American Ceramic Society, Vol. 97, Issue 7
  • DOI: 10.1111/jace.12982

Coupled short-range ferroelectric and magnetic order in PbFe 1 / 2 Nb 1 / 2 O 3
journal, September 2013


Piezoelectric response of BiFeO 3 ceramics at elevated temperatures
journal, July 2016

  • Rojac, Tadej; Makarovic, Maja; Walker, Julian
  • Applied Physics Letters, Vol. 109, Issue 4
  • DOI: 10.1063/1.4960103

About the deformation of ferroelectric hystereses
journal, December 2014

  • Schenk, T.; Yurchuk, E.; Mueller, S.
  • Applied Physics Reviews, Vol. 1, Issue 4
  • DOI: 10.1063/1.4902396

Room Temperature Multiferroic Behavior in Pb(Fe 1/2 Nb 1/2 )O 3 Ceramics
journal, October 2014