Synthesis of Co‐Doped MoS 2 Monolayers with Enhanced Valley Splitting

Zhou, Jiadong; Lin, Junhao; Sims, Hunter; Jiang, Chongyun; Cong, Chunxiao; Brehm, John A.; Zhang, Zhaowei; Niu, Lin; Chen, Yu; Zhou, Yao; Wang, Yanlong; Liu, Fucai; Zhu, Chao; Yu, Ting; Suenaga, Kazu; Mishra, Rohan; Pantelides, Sokrates T.; Zhu, Zhen‐Gang; Gao, Weibo; Liu, Zheng; Zhou, Wu

doi:10.1002/adma.201906536

Title: Synthesis of Co‐Doped MoS ₂ Monolayers with Enhanced Valley Splitting

Authors:

Zhou, Jiadong ^[1]; Lin, Junhao ^[2]; Sims, Hunter ^[3]; Jiang, Chongyun ^[4]; Cong, Chunxiao ^[5]; Brehm, John A. ^[3]; Zhang, Zhaowei ^[6]; Niu, Lin ^[1]; Chen, Yu ^[6]; Zhou, Yao ^[6]; Wang, Yanlong ^[6]; Liu, Fucai ^[1]; Zhu, Chao ^[1]; Yu, Ting ^[6]; Suenaga, Kazu ^[7]; Mishra, Rohan ^[8]; Pantelides, Sokrates T. ^[3]; Zhu, Zhen‐Gang ^[9]; Gao, Weibo ^[6];

^[10] more »

School of Materials Science and Engineering Nanyang Technological University Singapore 639798 Singapore
National Institute of Advanced Industrial Science and Technology (AIST) Tsukuba 305–8565 Japan, Department of Physics Southern University of Science and Technology Shenzhen 518055 China
Department of Physics and Astronomy Vanderbilt University Nashville TN 37235 USA, Materials Science and Technology Division Oak Ridge National Lab Oak Ridge TN 37831 USA
Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University Singapore 637371 Singapore, College of electronic information and optical engineering Nankai University Tianjin 300350 China
Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University Singapore 637371 Singapore, State Key Laboratory of ASIC &, System School of Information Science and Technology Fudan University Shanghai 200433 P. R. China
Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University Singapore 637371 Singapore
National Institute of Advanced Industrial Science and Technology (AIST) Tsukuba 305–8565 Japan
Department of Mechanical Engineering and Materials Science and Institute of Materials Science and Engineering Washington University in St. Louis St. Louis MO 63130 USA
School of Electronic Electrical and Communication Engineering University of Chinese Academy of Science Beijing 100049 China, CAS Center for Excellence in Topological Quantum Computation University of Chinese Academy of Sciences Beijing 100049 China
School of Materials Science and Engineering Nanyang Technological University Singapore 639798 Singapore, Centre for Micro‐/Nano‐electronics (NOVITAS) School of Electrical &, Electronic Engineering Nanyang Technological University 50 Nanyang Avenue Singapore 639798 Singapore, CINTRA CNRS/NTU/THALES UMI 3288 Research Techno Plaza 50 Nanyang Drive, Border X Block, Level 6 Singapore 637553 Singapore
CAS Center for Excellence in Topological Quantum Computation University of Chinese Academy of Sciences Beijing 100049 China, School of Physical Sciences and CAS Key Laboratory of Vacuum Sciences University of Chinese Academy of Sciences Beijing 100049 China

Publication Date:: 2020-02-06

Sponsoring Org.:: USDOE

OSTI Identifier:: 1598076

Grant/Contract Number:: DE‐FG02‐09ER46554; DE‐AC02‐05CH11231

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Advanced Materials

Additional Journal Information:: Journal Name: Advanced Materials Journal Volume: 32 Journal Issue: 11; Journal ID: ISSN 0935-9648

Publisher:: Wiley Blackwell (John Wiley & Sons)

Country of Publication:: Germany

Language:: English

Citation Formats


                    Zhou, Jiadong, Lin, Junhao, Sims, Hunter, Jiang, Chongyun, Cong, Chunxiao, Brehm, John A., Zhang, Zhaowei, Niu, Lin, Chen, Yu, Zhou, Yao, Wang, Yanlong, Liu, Fucai, Zhu, Chao, Yu, Ting, Suenaga, Kazu, Mishra, Rohan, Pantelides, Sokrates T., Zhu, Zhen‐Gang, Gao, Weibo, Liu, Zheng, and Zhou, Wu. Synthesis of Co‐Doped MoS 2 Monolayers with Enhanced Valley Splitting.  Germany: N. p., 2020. 
Web.  doi:10.1002/adma.201906536.

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                    Zhou, Jiadong, Lin, Junhao, Sims, Hunter, Jiang, Chongyun, Cong, Chunxiao, Brehm, John A., Zhang, Zhaowei, Niu, Lin, Chen, Yu, Zhou, Yao, Wang, Yanlong, Liu, Fucai, Zhu, Chao, Yu, Ting, Suenaga, Kazu, Mishra, Rohan, Pantelides, Sokrates T., Zhu, Zhen‐Gang, Gao, Weibo, Liu, Zheng, & Zhou, Wu. Synthesis of Co‐Doped MoS 2 Monolayers with Enhanced Valley Splitting.  Germany.  https://doi.org/10.1002/adma.201906536

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                    Zhou, Jiadong, Lin, Junhao, Sims, Hunter, Jiang, Chongyun, Cong, Chunxiao, Brehm, John A., Zhang, Zhaowei, Niu, Lin, Chen, Yu, Zhou, Yao, Wang, Yanlong, Liu, Fucai, Zhu, Chao, Yu, Ting, Suenaga, Kazu, Mishra, Rohan, Pantelides, Sokrates T., Zhu, Zhen‐Gang, Gao, Weibo, Liu, Zheng, and Zhou, Wu. Thu .  
"Synthesis of Co‐Doped MoS 2 Monolayers with Enhanced Valley Splitting".  Germany.  https://doi.org/10.1002/adma.201906536.

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@article{osti_1598076,

  title        = {Synthesis of Co‐Doped MoS 2 Monolayers with Enhanced Valley Splitting},

  author       = {Zhou, Jiadong and Lin, Junhao and Sims, Hunter and Jiang, Chongyun and Cong, Chunxiao and Brehm, John A. and Zhang, Zhaowei and Niu, Lin and Chen, Yu and Zhou, Yao and Wang, Yanlong and Liu, Fucai and Zhu, Chao and Yu, Ting and Suenaga, Kazu and Mishra, Rohan and Pantelides, Sokrates T. and Zhu, Zhen‐Gang and Gao, Weibo and Liu, Zheng and Zhou, Wu},

  abstractNote = {},

  doi          = {10.1002/adma.201906536},

  journal      = {Advanced Materials},

  number       = 11,

  volume       = 32,

  place        = {Germany},

  year         = {2020},

  month        = {2}

}

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Title: Synthesis of Co‐Doped MoS 2 Monolayers with Enhanced Valley Splitting

Citation Formats

Generalized Gradient Approximation Made Simple journal, October 1996

Breaking of Valley Degeneracy by Magnetic Field in Monolayer MoSe 2 journal, January 2015

Electrical control of the valley Hall effect in bilayer MoS2 transistors journal, January 2016

Long-range ferromagnetic ordering in manganese-doped two-dimensional dichalcogenides journal, October 2013

Projector augmented-wave method journal, December 1994

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Valley Zeeman Splitting and Valley Polarization of Neutral and Charged Excitons in Monolayer MoTe 2 at High Magnetic Fields journal, May 2016

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Synthesis and Transport Properties of Large-Scale Alloy Co 0.16 Mo 0.84 S 2 Bilayer Nanosheets journal, January 2015

Large Spin-Valley Polarization in Monolayer MoTe 2 on Top of EuO(111) journal, December 2015

Special points for Brillouin-zone integrations journal, June 1976

Strain tuning of magnetism in Mn doped MoS 2 monolayer journal, June 2014

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Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set journal, October 1996

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Mn-doped monolayer MoS 2 : An atomically thin dilute magnetic semiconductor journal, May 2013

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Atomic Structure and Spectroscopy of Single Metal (Cr, V) Substitutional Dopants in Monolayer MoS 2 journal, November 2016

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Title: Synthesis of Co‐Doped MoS ₂ Monolayers with Enhanced Valley Splitting

Generalized Gradient Approximation Made Simple
journal, October 1996

Breaking of Valley Degeneracy by Magnetic Field in Monolayer ${MoSe}_{2}$
journal, January 2015

Electrical control of the valley Hall effect in bilayer MoS2 transistors
journal, January 2016

Long-range ferromagnetic ordering in manganese-doped two-dimensional dichalcogenides
journal, October 2013

Projector augmented-wave method
journal, December 1994

Tunable magnetic properties of transition metal doped ${MoS}_{2}$
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Valley Zeeman Splitting and Valley Polarization of Neutral and Charged Excitons in Monolayer MoTe ₂ at High Magnetic Fields
journal, May 2016

MAGNETO-TRANSPORT AND MAGNETO-OPTICAL PROPERTIES OF FERROMAGNETIC (III,Mn)V SEMICONDUCTORS: A REVIEW
journal, March 2004

Synthesis and Transport Properties of Large-Scale Alloy Co _0.16 Mo _0.84 S ₂ Bilayer Nanosheets
journal, January 2015

Large Spin-Valley Polarization in Monolayer MoTe ₂ on Top of EuO(111)
journal, December 2015

Special points for Brillouin-zone integrations
journal, June 1976

Strain tuning of magnetism in Mn doped MoS ₂ monolayer
journal, June 2014

Electrical generation and control of the valley carriers in a monolayer transition metal dichalcogenide
journal, April 2016

Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set
journal, October 1996

Chemical potential dependence of defect formation energies in GaAs: Application to Ga self-diffusion
journal, October 1991

Single quantum emitters in monolayer semiconductors
journal, May 2015

Optical Investigation of Monolayer and Bulk Tungsten Diselenide (WSe ₂ ) in High Magnetic Fields
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Commentary: The Materials Project: A materials genome approach to accelerating materials innovation
journal, July 2013

Mn-doped monolayer MoS $_{2}$ : An atomically thin dilute magnetic semiconductor
journal, May 2013

Magnetoexcitons in large area CVD-grown monolayer ${MoS}_{2}$ and ${MoSe}_{2}$ on sapphire
journal, April 2016

Ab initiomolecular dynamics for liquid metals
journal, January 1993

Magneto-optics in transition metal diselenide monolayers
journal, June 2015

Ferromagnetism in Transitional Metal-Doped MoS2 Monolayer
journal, March 2016

Exciton diamagnetic shifts and valley Zeeman effects in monolayer WS2 and MoS2 to 65 Tesla
journal, February 2016

Atomic Structure and Spectroscopy of Single Metal (Cr, V) Substitutional Dopants in Monolayer MoS ₂
journal, November 2016

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journal, January 2015

Intrinsic Structural Defects in Monolayer Molybdenum Disulfide
journal, May 2013

Van der Waals engineering of ferromagnetic semiconductor heterostructures for spin and valleytronics
journal, May 2017

Diluted magnetic semiconductors
journal, August 1988

Magnetic control of valley pseudospin in monolayer WSe2
journal, January 2015

Enhanced valley splitting in monolayer WSe2 due to magnetic exchange field
journal, May 2017

Manganese Doping of Monolayer MoS ₂ : The Substrate Is Critical
journal, September 2015

Optically active quantum dots in monolayer WSe2
journal, May 2015

Zeeman-type spin splitting controlled by an electric field
journal, July 2013

Probing the Influence of Dielectric Environment on Excitons in Monolayer WSe ₂ : Insight from High Magnetic Fields
journal, October 2016

A novel optical property induced by MO, S vacancy and V-doped in monolayer MoS2
journal, September 2015

Defect-induced magnetism: Codoping and a prescription for enhanced magnetism
journal, April 2013