Precious metal-free solar-to-fuel generation: SSM-DSCs powering water splitting with NanoCOT and NiMoZn electrocatalysts

Cheema, Hammad; Watson, Jonathon; Shinde, Pravin S.; Rodrigues, Roberta R.; Pan, Shanlin; Delcamp, Jared H.

doi:10.1039/C9CC09209A

Title: Precious metal-free solar-to-fuel generation: SSM-DSCs powering water splitting with NanoCOT and NiMoZn electrocatalysts

Abstract

A precious metal-free sequential series multijunction dye-sensitized solar cell (SSM-DSC)-powered water electrolysis system is shown using NanoCOT and NiMoZn electrodes. Furthermore, a stable 3.9% solar-to-hydrogen (STH) efficiency is achieved using a recently reported black organic dye and graphene electrodes for DSCs.

Authors:

^[1];

^[2];

^[1];

^[2];

^[1]

Univ. of Mississippi, Oxford, MS (United States)
Univ. of Alabama, Tuscaloosa, AL (United States)

Publication Date:: 2019-12-20

Research Org.:: Univ. of Mississippi, Oxford, MS (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)

OSTI Identifier:: 1596581

Alternate Identifier(s):: OSTI ID: 1582483

Grant/Contract Number:: SC0019131

Resource Type:: Accepted Manuscript

Journal Name:: ChemComm

Additional Journal Information:: Journal Volume: 56; Journal Issue: 10; Related Information: This document is an accepted manuscript version of a published article that appeared in final form in Chemical Communications, copyright © Royal Society of Chemistry after peer review and technical editing by the publisher. To access the final edited and published work see https://pubs.rsc.org/en/content/articlelanding/2020/cc/c9cc09209a/unauth#!divAbstract.; Journal ID: ISSN 1359-7345

Publisher:: Royal Society of Chemistry

Country of Publication:: United States

Language:: English

Subject:: 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY

Citation Formats


                    Cheema, Hammad, Watson, Jonathon, Shinde, Pravin S., Rodrigues, Roberta R., Pan, Shanlin, and Delcamp, Jared H. Precious metal-free solar-to-fuel generation: SSM-DSCs powering water splitting with NanoCOT and NiMoZn electrocatalysts.  United States: N. p., 2019. 
Web.  doi:10.1039/C9CC09209A.

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                    Cheema, Hammad, Watson, Jonathon, Shinde, Pravin S., Rodrigues, Roberta R., Pan, Shanlin, & Delcamp, Jared H. Precious metal-free solar-to-fuel generation: SSM-DSCs powering water splitting with NanoCOT and NiMoZn electrocatalysts.  United States.  https://doi.org/10.1039/C9CC09209A

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                    Cheema, Hammad, Watson, Jonathon, Shinde, Pravin S., Rodrigues, Roberta R., Pan, Shanlin, and Delcamp, Jared H. Fri .  
"Precious metal-free solar-to-fuel generation: SSM-DSCs powering water splitting with NanoCOT and NiMoZn electrocatalysts".  United States.  https://doi.org/10.1039/C9CC09209A.  https://www.osti.gov/servlets/purl/1596581.

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@article{osti_1596581,

  title        = {Precious metal-free solar-to-fuel generation: SSM-DSCs powering water splitting with NanoCOT and NiMoZn electrocatalysts},

  author       = {Cheema, Hammad and Watson, Jonathon and Shinde, Pravin S. and Rodrigues, Roberta R. and Pan, Shanlin and Delcamp, Jared H.},

  abstractNote = {A precious metal-free sequential series multijunction dye-sensitized solar cell (SSM-DSC)-powered water electrolysis system is shown using NanoCOT and NiMoZn electrodes. Furthermore, a stable 3.9% solar-to-hydrogen (STH) efficiency is achieved using a recently reported black organic dye and graphene electrodes for DSCs.},

  doi          = {10.1039/C9CC09209A},

  journal      = {ChemComm},

  number       = 10,

  volume       = 56,

  place        = {United States},

  year         = {2019},

  month        = {12}

}

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Works referencing / citing this record:

A 25 mA/cm 2 Dye-Sensitized Solar Cell Based on a Near-Infrared-Absorbing Organic Dye and Application of the Device in SSM-DSCs
journal, January 2020

Cheema, Hammad; Watson, Jonathon; peddapuram, adithya
Chemical Communications
DOI: 10.1039/c9cc09372a

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Title: Precious metal-free solar-to-fuel generation: SSM-DSCs powering water splitting with NanoCOT and NiMoZn electrocatalysts

Abstract

Citation Formats

Chemical approaches to artificial photosynthesis journal, September 2012

A High-Voltage Molecular-Engineered Organic Sensitizer-Iron Redox Shuttle Pair: 1.4 V DSSC and 3.3 V SSM-DSSC Devices journal, April 2018

Hydrogen production, storage, transportation and key challenges with applications: A review journal, June 2018

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Design of Organic Dyes and Cobalt Polypyridine Redox Mediators for High-Efficiency Dye-Sensitized Solar Cells journal, November 2010

Symmetric and unsymmetric donor functionalization. comparing structural and spectral benefits of chromophores for dye-sensitized solar cells journal, January 2009

Sustainable Hydrogen Production journal, August 2004

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An overview of hydrogen production technologies journal, January 2009

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A perspective on the production of dye-sensitized solar modules journal, January 2014

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Wideband dye-sensitized solar cells employing a phosphine-coordinated ruthenium sensitizer journal, June 2013

Water photolysis at 12.3% efficiency via perovskite photovoltaics and Earth-abundant catalysts journal, September 2014

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A Stable Blue Photosensitizer for Color Palette of Dye-Sensitized Solar Cells Reaching 12.6% Efficiency journal, February 2018

Materials for solar fuels and chemicals journal, December 2016

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Toward Cost-Effective Solar Energy Use journal, February 2007

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Precious-metal free photoelectrochemical water splitting with immobilised molecular Ni and Fe redox catalysts journal, January 2016

Application of transparent dye-sensitized solar cells to building integrated photovoltaic systems journal, October 2011

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Cyclopentadithiophene Bridged Donor-Acceptor Dyes Achieve High Power Conversion Efficiencies in Dye-Sensitized Solar Cells Based on the tris-Cobalt Bipyridine Redox Couple journal, May 2011

Efficient solar-to-fuels production from a hybrid microbial–water-splitting catalyst system journal, February 2015

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Ultrafast Fabrication of Flexible Dye-Sensitized Solar Cells by Ultrasonic Spray-Coating Technology journal, September 2015

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A High-Voltage Molecular-Engineered Organic Sensitizer-Iron Redox Shuttle Pair: 1.4 V DSSC and 3.3 V SSM-DSSC Devices journal, April 2018

A 25 mA/cm 2 Dye-Sensitized Solar Cell Based on a Near-Infrared-Absorbing Organic Dye and Application of the Device in SSM-DSCs journal, January 2020

Chemical approaches to artificial photosynthesis
journal, September 2012

A High-Voltage Molecular-Engineered Organic Sensitizer-Iron Redox Shuttle Pair: 1.4 V DSSC and 3.3 V SSM-DSSC Devices
journal, April 2018

Hydrogen production, storage, transportation and key challenges with applications: A review
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Sequential series multijunction dye-sensitized solar cells (SSM-DSCs): 4.7 volts from a single illuminated area
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Porphyrin Sensitizers with Donor Structural Engineering for Superior Performance Dye-Sensitized Solar Cells and Tandem Solar Cells for Water Splitting Applications
journal, December 2016

Design of Organic Dyes and Cobalt Polypyridine Redox Mediators for High-Efficiency Dye-Sensitized Solar Cells
journal, November 2010

Symmetric and unsymmetric donor functionalization. comparing structural and spectral benefits of chromophores for dye-sensitized solar cells
journal, January 2009

Sustainable Hydrogen Production
journal, August 2004

Low-Recombination Thieno[3,4-b]thiophene-Based Photosensitizers for Dye-Sensitized Solar Cells with Panchromatic Photoresponses
journal, August 2017

An overview of hydrogen production technologies
journal, January 2009

Solar-hydrogen: Environmentally safe fuel for the future
journal, April 2005

A low-cost, high-efficiency solar cell based on dye-sensitized colloidal TiO₂ films
journal, October 1991

A perspective on the production of dye-sensitized solar modules
journal, January 2014

A cobalt complex redox shuttle for dye-sensitized solar cells with high open-circuit potentials
journal, January 2012

Photo-electrochemical hydrogen generation from water using solar energy. Materials-related aspects
journal, October 2002

Dye-Sensitized Solar Cells
journal, November 2010

Wideband dye-sensitized solar cells employing a phosphine-coordinated ruthenium sensitizer
journal, June 2013

Water photolysis at 12.3% efficiency via perovskite photovoltaics and Earth-abundant catalysts
journal, September 2014

Series-connected tandem dye-sensitized solar cell for improving efficiency to more than 10%
journal, June 2009

PEDOT counter electrodes for dye-sensitized solar cells prepared by aqueous micellar electrodeposition
journal, September 2013

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journal, January 2013

A 25 mA/cm 2 Dye-Sensitized Solar Cell Based on a Near-Infrared-Absorbing Organic Dye and Application of the Device in SSM-DSCs
journal, January 2020

NanoCOT: Low-Cost Nanostructured Electrode Containing Carbon, Oxygen, and Titanium for Efficient Oxygen Evolution Reaction
journal, September 2015

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journal, February 2018

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journal, January 2017

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journal, February 2007

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journal, January 2008

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journal, December 2017

Precious-metal free photoelectrochemical water splitting with immobilised molecular Ni and Fe redox catalysts
journal, January 2016

Application of transparent dye-sensitized solar cells to building integrated photovoltaic systems
journal, October 2011

Solar water splitting by photovoltaic-electrolysis with a solar-to-hydrogen efficiency over 30%
journal, October 2016

Cyclopentadithiophene Bridged Donor-Acceptor Dyes Achieve High Power Conversion Efficiencies in Dye-Sensitized Solar Cells Based on the tris-Cobalt Bipyridine Redox Couple
journal, May 2011

Efficient solar-to-fuels production from a hybrid microbial–water-splitting catalyst system
journal, February 2015

The Role of Antireflective Coating CYTOP, Immersion Oil, and Sensitizer Selection in Fabricating a 2.3 V, 10% Power Conversion Efficiency SSM‐DSC Device
journal, February 2019

Ultrafast Fabrication of Flexible Dye-Sensitized Solar Cells by Ultrasonic Spray-Coating Technology
journal, September 2015

Toward practical solar hydrogen production – an artificial photosynthetic leaf-to-farm challenge
journal, January 2019

Artificial photosynthesis: opportunities and challenges of molecular catalysts
journal, January 2019

Graphene Nanoplatelets Outperforming Platinum as the Electrocatalyst in Co-Bipyridine-Mediated Dye-Sensitized Solar Cells
journal, December 2011

A High-Voltage Molecular-Engineered Organic Sensitizer-Iron Redox Shuttle Pair: 1.4 V DSSC and 3.3 V SSM-DSSC Devices
journal, April 2018

A 25 mA/cm 2 Dye-Sensitized Solar Cell Based on a Near-Infrared-Absorbing Organic Dye and Application of the Device in SSM-DSCs
journal, January 2020