DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Design of additively manufactured methanol conversion reactor for high throughput production

Abstract

Additively manufactured methanol conversion reactor was designed and fabricated for high throughput fuel production while capturing carbon dioxide. Here, the reactor designed is part of large effort in integrating electrolyzer and catalytic reactor system. Processing in fabricating the steel, titanium, and nickel alloy reactors were optimized to improve the catalyst deposition process and reaction efficiency. Microstructure of the additively manufactured reactors were characterized. General design is utilized to improve the performance of the reactor while exploring the benefit of freeform in additive manufacturing.

Authors:
ORCiD logo [1];  [2];  [2];  [3]
  1. Advanced Manufacturing LLC, East Hartford, CT (United States)
  2. Connecticut Center for Advanced Technology, East Hartford, CT (United States)
  3. Western New England University, Springfield, MA (United States)
Publication Date:
Research Org.:
Advanced Manufacturing LLC, East Hartford, CT (United States); Connecticut Center for Advanced Technology, East Hartford, CT (United States)
Sponsoring Org.:
USDOE Office of Energy Efficiency and Renewable Energy (EERE), Office of Sustainable Transportation. Hydrogen Fuel Cell Technologies Office (HFTO); USDOE
OSTI Identifier:
2332939
Alternate Identifier(s):
OSTI ID: 1595846
Grant/Contract Number:  
EE0008423; DE‐0008423
Resource Type:
Accepted Manuscript
Journal Name:
Material Design & Processing Communications
Additional Journal Information:
Journal Volume: 3; Journal Issue: 1; Journal ID: ISSN 2577-6576
Publisher:
Hindawi
Country of Publication:
United States
Language:
English
Subject:
10 SYNTHETIC FUELS; 08 HYDROGEN; 36 MATERIALS SCIENCE; Additive Manufacturing; methanol; hydrogen; synthetic fuels; microstructure; carbon dioxide hydrogenation

Citation Formats

Li, Dongsheng, Maloney, Tom, Mannan, Nasir, and Niknam, Seyed. Design of additively manufactured methanol conversion reactor for high throughput production. United States: N. p., 2020. Web. doi:10.1002/mdp2.143.
Li, Dongsheng, Maloney, Tom, Mannan, Nasir, & Niknam, Seyed. Design of additively manufactured methanol conversion reactor for high throughput production. United States. https://doi.org/10.1002/mdp2.143
Li, Dongsheng, Maloney, Tom, Mannan, Nasir, and Niknam, Seyed. Thu . "Design of additively manufactured methanol conversion reactor for high throughput production". United States. https://doi.org/10.1002/mdp2.143. https://www.osti.gov/servlets/purl/2332939.
@article{osti_2332939,
title = {Design of additively manufactured methanol conversion reactor for high throughput production},
author = {Li, Dongsheng and Maloney, Tom and Mannan, Nasir and Niknam, Seyed},
abstractNote = {Additively manufactured methanol conversion reactor was designed and fabricated for high throughput fuel production while capturing carbon dioxide. Here, the reactor designed is part of large effort in integrating electrolyzer and catalytic reactor system. Processing in fabricating the steel, titanium, and nickel alloy reactors were optimized to improve the catalyst deposition process and reaction efficiency. Microstructure of the additively manufactured reactors were characterized. General design is utilized to improve the performance of the reactor while exploring the benefit of freeform in additive manufacturing.},
doi = {10.1002/mdp2.143},
journal = {Material Design & Processing Communications},
number = 1,
volume = 3,
place = {United States},
year = {Thu Jan 23 00:00:00 EST 2020},
month = {Thu Jan 23 00:00:00 EST 2020}
}

Works referenced in this record:

Combining additive manufacturing and catalysis: a review
journal, January 2017

  • Hurt, C.; Brandt, M.; Priya, S. S.
  • Catalysis Science & Technology, Vol. 7, Issue 16
  • DOI: 10.1039/C7CY00615B

Design and additive manufacture for flow chemistry
journal, January 2013

  • Capel, Andrew J.; Edmondson, Steve; Christie, Steven D. R.
  • Lab on a Chip, Vol. 13, Issue 23
  • DOI: 10.1039/c3lc50844g

3D printing in chemical engineering and catalytic technology: structured catalysts, mixers and reactors
journal, January 2018

  • Parra-Cabrera, Cesar; Achille, Clement; Kuhn, Simon
  • Chemical Society Reviews, Vol. 47, Issue 1
  • DOI: 10.1039/C7CS00631D

Simple design of monolith reactor for selective catalytic reduction of nitric oxide for power plant emission control
journal, October 1990

  • Buzanowski, Marek A.; Yang, Ralph T.
  • Industrial & Engineering Chemistry Research, Vol. 29, Issue 10
  • DOI: 10.1021/ie00106a015

Monolithic Honeycombs in Loop Reactor Configuration for Intensification of Multiphase Processes
journal, September 2015

  • Güttel, Robert; Eisenbeis, Christian; Knochen, Jens
  • Chemical Engineering & Technology, Vol. 38, Issue 10
  • DOI: 10.1002/ceat.201400727

Cu-Decorated ZnO Nanorod Array Integrated Structured Catalysts for Low-Pressure CO 2 Hydrogenation to Methanol
journal, December 2017

  • Du, Shoucheng; Tang, Wenxiang; Lu, Xingxu
  • Advanced Materials Interfaces, Vol. 5, Issue 3
  • DOI: 10.1002/admi.201700730

Methanol Synthesis: Optimal Solution for a Better Efficiency of the Process
journal, February 2018