Balancing Ionic and Electronic Conduction for High‐Performance Organic Electrochemical Transistors

Savva, Achilleas; Hallani, Rawad; Cendra, Camila; Surgailis, Jokubas; Hidalgo, Tania C.; Wustoni, Shofarul; Sheelamanthula, Rajendar; Chen, Xingxing; Kirkus, Mindaugas; Giovannitti, Alexander; Salleo, Alberto; McCulloch, Iain; Inal, Sahika

doi:10.1002/adfm.201907657

Title: Balancing Ionic and Electronic Conduction for High‐Performance Organic Electrochemical Transistors

Authors:

^[1]; Hallani, Rawad ^[2]; Cendra, Camila ^[3]; Surgailis, Jokubas ^[1]; Hidalgo, Tania C. ^[1]; Wustoni, Shofarul ^[1]; Sheelamanthula, Rajendar ^[2]; Chen, Xingxing ^[2]; Kirkus, Mindaugas ^[2];

^[4];

^[3];

^[5];

^[1]

Organic Bioelectronics Laboratory Biological and Environmental Science and Engineering King Abdullah University of Science and Technology (KAUST) Thuwal 23955‐6900 Saudi Arabia
Division of Physical Sciences and Engineering KAUST Solar Center (KSC) King Abdullah University of Science and Technology (KAUST) Thuwal 23955‐6900 Saudi Arabia
Department of Materials Science and Engineering Stanford University Stanford CA 94305 USA
Department of Chemistry Imperial College London London SW72AZ UK
Division of Physical Sciences and Engineering KAUST Solar Center (KSC) King Abdullah University of Science and Technology (KAUST) Thuwal 23955‐6900 Saudi Arabia, Department of Chemistry Imperial College London London SW72AZ UK

Publication Date:: 2020-01-28

Sponsoring Org.:: USDOE

OSTI Identifier:: 1595531

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Advanced Functional Materials

Additional Journal Information:: Journal Name: Advanced Functional Materials Journal Volume: 30 Journal Issue: 11; Journal ID: ISSN 1616-301X

Publisher:: Wiley Blackwell (John Wiley & Sons)

Country of Publication:: Germany

Language:: English

Citation Formats


                    Savva, Achilleas, Hallani, Rawad, Cendra, Camila, Surgailis, Jokubas, Hidalgo, Tania C., Wustoni, Shofarul, Sheelamanthula, Rajendar, Chen, Xingxing, Kirkus, Mindaugas, Giovannitti, Alexander, Salleo, Alberto, McCulloch, Iain, and Inal, Sahika. Balancing Ionic and Electronic Conduction for High‐Performance Organic Electrochemical Transistors.  Germany: N. p., 2020. 
Web.  doi:10.1002/adfm.201907657.

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                    Savva, Achilleas, Hallani, Rawad, Cendra, Camila, Surgailis, Jokubas, Hidalgo, Tania C., Wustoni, Shofarul, Sheelamanthula, Rajendar, Chen, Xingxing, Kirkus, Mindaugas, Giovannitti, Alexander, Salleo, Alberto, McCulloch, Iain, & Inal, Sahika. Balancing Ionic and Electronic Conduction for High‐Performance Organic Electrochemical Transistors.  Germany.  https://doi.org/10.1002/adfm.201907657

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                    Savva, Achilleas, Hallani, Rawad, Cendra, Camila, Surgailis, Jokubas, Hidalgo, Tania C., Wustoni, Shofarul, Sheelamanthula, Rajendar, Chen, Xingxing, Kirkus, Mindaugas, Giovannitti, Alexander, Salleo, Alberto, McCulloch, Iain, and Inal, Sahika. Tue .  
"Balancing Ionic and Electronic Conduction for High‐Performance Organic Electrochemical Transistors".  Germany.  https://doi.org/10.1002/adfm.201907657.

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@article{osti_1595531,

  title        = {Balancing Ionic and Electronic Conduction for High‐Performance Organic Electrochemical Transistors},

  author       = {Savva, Achilleas and Hallani, Rawad and Cendra, Camila and Surgailis, Jokubas and Hidalgo, Tania C. and Wustoni, Shofarul and Sheelamanthula, Rajendar and Chen, Xingxing and Kirkus, Mindaugas and Giovannitti, Alexander and Salleo, Alberto and McCulloch, Iain and Inal, Sahika},

  abstractNote = {},

  doi          = {10.1002/adfm.201907657},

  journal      = {Advanced Functional Materials},

  number       = 11,

  volume       = 30,

  place        = {Germany},

  year         = {2020},

  month        = {1}

}

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https://doi.org/10.1002/adfm.201907657

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Title: Balancing Ionic and Electronic Conduction for High‐Performance Organic Electrochemical Transistors

Citation Formats

Influence of PEDOT:PSS crystallinity and composition on electrochemical transistor performance and long-term stability journal, September 2018

Organic transistor platform with integrated microfluidics for in-line multi-parametric in vitro cell monitoring journal, August 2017

Ionic-to-electronic coupling efficiency in PEDOT:PSS films operated in aqueous electrolytes journal, January 2018

Organic electrochemical transistors based on PEDOT with different anionic polyelectrolyte dopants journal, October 2015

Role of the Anion on the Transport and Structure of Organic Mixed Conductors journal, December 2018

Perylene Polyimide-Polyether Anodes for Aqueous All-Organic Polymer Batteries journal, October 2018

Organic electrochemical transistors journal, January 2018

Direct Measurement of Ion Mobility in a Conducting Polymer journal, June 2013

Influence of Side-Chain Chemistry on Structure and Ionic Conduction Characteristics of Polythiophene Derivatives: A Computational and Experimental Study journal, February 2019

Structural control of mixed ionic and electronic transport in conducting polymers journal, April 2016

Morphological effects on polymeric mixed ionic/electronic conductors journal, January 2019

A Microfluidic Ion Pump for In Vivo Drug Delivery journal, May 2017

The Role of the Side Chain on the Performance of N-type Conjugated Polymers in Aqueous Electrolytes journal, April 2018

Solvent Engineering for High‐Performance n‐Type Organic Electrochemical Transistors journal, June 2019

Recent Progress in High-Mobility Organic Transistors: A Reality Check journal, July 2018

Polymer-Fullerene Bulk-Heterojunction Solar Cells journal, April 2009

Chemical Oxidation of Polymer Electrodes for Redox Active Devices: Stabilization through Interfacial Interactions journal, December 2017

High-Performance Organic Electrochemical Transistors Based on Conjugated Polyelectrolyte Copolymers journal, June 2019

Effects of environmental factors on the electrooptical properties of conjugated polymers containing oligo(oxyethylene) substituents journal, October 1991

Improving the Compatibility of Diketopyrrolopyrrole Semiconducting Polymers for Biological Interfacing by Lysine Attachment journal, August 2018

Conducting Polymers for Pseudocapacitive Energy Storage journal, July 2016

Light-emitting diodes based on conjugated polymers journal, October 1990

Controlling the mode of operation of organic transistors through side-chain engineering journal, October 2016

Direct metabolite detection with an n-type accumulation mode organic electrochemical transistor journal, June 2018

Steady-State and Transient Behavior of Organic Electrochemical Transistors journal, October 2007

Design and evaluation of conjugated polymers with polar side chains as electrode materials for electrochemical energy storage in aqueous electrolytes journal, January 2019

Electrochemical strain microscopy probes morphology-induced variations in ion uptake and performance in organic electrochemical transistors journal, June 2017

In Vitro and In Vivo Evaluation of PEDOT Microelectrodes for Neural Stimulation and Recording journal, June 2011

Label-free electrochemical DNA sensor based on functionalised conducting copolymer journal, March 2005

High-performance transistors for bioelectronics through tuning of channel thickness journal, May 2015

Influence of Water on the Performance of Organic Electrochemical Transistors journal, January 2019

Organic electronics for neuromorphic computing journal, July 2018

Conjugated Polymer Actuators for Biomedical Applications journal, March 2003

Benchmarking organic mixed conductors for transistors journal, November 2017

Polymer Crystallinity Controls Water Uptake in Glycol Side-Chain Polymer Organic Electrochemical Transistors journal, February 2019

In vivo recordings of brain activity using organic transistors journal, March 2013

Understanding volumetric capacitance in conducting polymers journal, March 2016

Hydrophilic Oligo(oxyethylene)-Derivatized Poly(3,4-ethylenedioxythiophenes): Cation-Responsive Optoelectroelectrochemical Properties and Solid-State Chromism journal, January 2002

Influence of PEDOT:PSS crystallinity and composition on electrochemical transistor performance and long-term stability
journal, September 2018

Organic transistor platform with integrated microfluidics for in-line multi-parametric in vitro cell monitoring
journal, August 2017

Ionic-to-electronic coupling efficiency in PEDOT:PSS films operated in aqueous electrolytes
journal, January 2018

Organic electrochemical transistors based on PEDOT with different anionic polyelectrolyte dopants
journal, October 2015

Role of the Anion on the Transport and Structure of Organic Mixed Conductors
journal, December 2018

Perylene Polyimide-Polyether Anodes for Aqueous All-Organic Polymer Batteries
journal, October 2018

Organic electrochemical transistors
journal, January 2018

Direct Measurement of Ion Mobility in a Conducting Polymer
journal, June 2013

Influence of Side-Chain Chemistry on Structure and Ionic Conduction Characteristics of Polythiophene Derivatives: A Computational and Experimental Study
journal, February 2019

Structural control of mixed ionic and electronic transport in conducting polymers
journal, April 2016

Morphological effects on polymeric mixed ionic/electronic conductors
journal, January 2019

A Microfluidic Ion Pump for In Vivo Drug Delivery
journal, May 2017

The Role of the Side Chain on the Performance of N-type Conjugated Polymers in Aqueous Electrolytes
journal, April 2018

Solvent Engineering for High‐Performance n‐Type Organic Electrochemical Transistors
journal, June 2019

Recent Progress in High-Mobility Organic Transistors: A Reality Check
journal, July 2018

Polymer-Fullerene Bulk-Heterojunction Solar Cells
journal, April 2009

Chemical Oxidation of Polymer Electrodes for Redox Active Devices: Stabilization through Interfacial Interactions
journal, December 2017

High-Performance Organic Electrochemical Transistors Based on Conjugated Polyelectrolyte Copolymers
journal, June 2019

Effects of environmental factors on the electrooptical properties of conjugated polymers containing oligo(oxyethylene) substituents
journal, October 1991

Improving the Compatibility of Diketopyrrolopyrrole Semiconducting Polymers for Biological Interfacing by Lysine Attachment
journal, August 2018

Conducting Polymers for Pseudocapacitive Energy Storage
journal, July 2016

Light-emitting diodes based on conjugated polymers
journal, October 1990

Controlling the mode of operation of organic transistors through side-chain engineering
journal, October 2016

Direct metabolite detection with an n-type accumulation mode organic electrochemical transistor
journal, June 2018

Steady-State and Transient Behavior of Organic Electrochemical Transistors
journal, October 2007

Design and evaluation of conjugated polymers with polar side chains as electrode materials for electrochemical energy storage in aqueous electrolytes
journal, January 2019

Electrochemical strain microscopy probes morphology-induced variations in ion uptake and performance in organic electrochemical transistors
journal, June 2017

In Vitro and In Vivo Evaluation of PEDOT Microelectrodes for Neural Stimulation and Recording
journal, June 2011

Label-free electrochemical DNA sensor based on functionalised conducting copolymer
journal, March 2005

High-performance transistors for bioelectronics through tuning of channel thickness
journal, May 2015

Influence of Water on the Performance of Organic Electrochemical Transistors
journal, January 2019

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journal, July 2018

Conjugated Polymer Actuators for Biomedical Applications
journal, March 2003

Benchmarking organic mixed conductors for transistors
journal, November 2017

Polymer Crystallinity Controls Water Uptake in Glycol Side-Chain Polymer Organic Electrochemical Transistors
journal, February 2019

In vivo recordings of brain activity using organic transistors
journal, March 2013

Understanding volumetric capacitance in conducting polymers
journal, March 2016

Hydrophilic Oligo(oxyethylene)-Derivatized Poly(3,4-ethylenedioxythiophenes): Cation-Responsive Optoelectroelectrochemical Properties and Solid-State Chromism
journal, January 2002