Gapless Surface Dirac Cone in Antiferromagnetic Topological Insulator
Abstract
The recently discovered antiferromagnetic topological insulators in the Mn-Bi-Te family with intrinsic magnetic ordering have rapidly drawn broad interest since its cleaved surface state is believed to be gapped, hosting the unprecedented axion states with a half-integer quantum Hall effect. Here, however, we show unambiguously by using high-resolution angle resolved photoemission spectroscopy that a gapless Dirac cone at the (0001) surface of MnBi2Te4 exists inside the bulk band gap. Such an unexpected surface state remains unchanged across the bulk N´eel temperature, and is even robust against severe surface degradation, indicating additional topological protection. Through symmetry analysis and ab initio calculations we consider different types of surface reconstruction of the magnetic moments as possible origins giving rise to such linear dispersion. Our results unveil the experimental topological properties of MnBi2Te4, revealing that the intrinsic magnetic topological insulator hosts a rich platform to realize various topological phases by tuning the magnetic or structural configurations, and thus push forward the comprehensive understanding of magnetic topological materials.
- Authors:
- more »
- Publication Date:
- Research Org.:
- Univ. of California, Los Angeles, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1595174
- Alternate Identifier(s):
- OSTI ID: 1802300
- Grant/Contract Number:
- SC0011978; 19AG014; 19AG004; 2019B030301001; ZDSYS20170303165926217; JCYJ20150630145302240; KYTDPT20181011104202253
- Resource Type:
- Published Article
- Journal Name:
- Physical Review. X
- Additional Journal Information:
- Journal Name: Physical Review. X Journal Volume: 9 Journal Issue: 4; Journal ID: ISSN 2160-3308
- Publisher:
- American Physical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; Physics
Citation Formats
Hao, Yu-Jie, Liu, Pengfei, Feng, Yue, Ma, Xiao-Ming, Schwier, Eike F., Arita, Masashi, Kumar, Shiv, Hu, Chaowei, Lu, Rui’e, Zeng, Meng, Wang, Yuan, Hao, Zhanyang, Sun, Hong-Yi, Zhang, Ke, Mei, Jiawei, Ni, Ni, Wu, Liusuo, Shimada, Kenya, Chen, Chaoyu, Liu, Qihang, and Liu, Chang. Gapless Surface Dirac Cone in Antiferromagnetic Topological Insulator MnBi 2 Te 4. United States: N. p., 2019.
Web. doi:10.1103/PhysRevX.9.041038.
Hao, Yu-Jie, Liu, Pengfei, Feng, Yue, Ma, Xiao-Ming, Schwier, Eike F., Arita, Masashi, Kumar, Shiv, Hu, Chaowei, Lu, Rui’e, Zeng, Meng, Wang, Yuan, Hao, Zhanyang, Sun, Hong-Yi, Zhang, Ke, Mei, Jiawei, Ni, Ni, Wu, Liusuo, Shimada, Kenya, Chen, Chaoyu, Liu, Qihang, & Liu, Chang. Gapless Surface Dirac Cone in Antiferromagnetic Topological Insulator MnBi 2 Te 4. United States. https://doi.org/10.1103/PhysRevX.9.041038
Hao, Yu-Jie, Liu, Pengfei, Feng, Yue, Ma, Xiao-Ming, Schwier, Eike F., Arita, Masashi, Kumar, Shiv, Hu, Chaowei, Lu, Rui’e, Zeng, Meng, Wang, Yuan, Hao, Zhanyang, Sun, Hong-Yi, Zhang, Ke, Mei, Jiawei, Ni, Ni, Wu, Liusuo, Shimada, Kenya, Chen, Chaoyu, Liu, Qihang, and Liu, Chang. Thu .
"Gapless Surface Dirac Cone in Antiferromagnetic Topological Insulator MnBi 2 Te 4". United States. https://doi.org/10.1103/PhysRevX.9.041038.
@article{osti_1595174,
title = {Gapless Surface Dirac Cone in Antiferromagnetic Topological Insulator MnBi 2 Te 4},
author = {Hao, Yu-Jie and Liu, Pengfei and Feng, Yue and Ma, Xiao-Ming and Schwier, Eike F. and Arita, Masashi and Kumar, Shiv and Hu, Chaowei and Lu, Rui’e and Zeng, Meng and Wang, Yuan and Hao, Zhanyang and Sun, Hong-Yi and Zhang, Ke and Mei, Jiawei and Ni, Ni and Wu, Liusuo and Shimada, Kenya and Chen, Chaoyu and Liu, Qihang and Liu, Chang},
abstractNote = {The recently discovered antiferromagnetic topological insulators in the Mn-Bi-Te family with intrinsic magnetic ordering have rapidly drawn broad interest since its cleaved surface state is believed to be gapped, hosting the unprecedented axion states with a half-integer quantum Hall effect. Here, however, we show unambiguously by using high-resolution angle resolved photoemission spectroscopy that a gapless Dirac cone at the (0001) surface of MnBi2Te4 exists inside the bulk band gap. Such an unexpected surface state remains unchanged across the bulk N´eel temperature, and is even robust against severe surface degradation, indicating additional topological protection. Through symmetry analysis and ab initio calculations we consider different types of surface reconstruction of the magnetic moments as possible origins giving rise to such linear dispersion. Our results unveil the experimental topological properties of MnBi2Te4, revealing that the intrinsic magnetic topological insulator hosts a rich platform to realize various topological phases by tuning the magnetic or structural configurations, and thus push forward the comprehensive understanding of magnetic topological materials.},
doi = {10.1103/PhysRevX.9.041038},
journal = {Physical Review. X},
number = 4,
volume = 9,
place = {United States},
year = {Thu Nov 21 00:00:00 EST 2019},
month = {Thu Nov 21 00:00:00 EST 2019}
}
https://doi.org/10.1103/PhysRevX.9.041038
Web of Science
Works referenced in this record:
Generalized Gradient Approximation Made Simple
journal, October 1996
- Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
- Physical Review Letters, Vol. 77, Issue 18, p. 3865-3868
One-Dimensional Edge States with Giant Spin Splitting in a Bismuth Thin Film
journal, February 2015
- Takayama, A.; Sato, T.; Souma, S.
- Physical Review Letters, Vol. 114, Issue 6
Dirac Surface States in Intrinsic Magnetic Topological Insulators EuSn 2 As 2 and MnBi 2 n Te 3 n + 1
journal, November 2019
- Li, Hang; Gao, Shun-Ye; Duan, Shao-Feng
- Physical Review X, Vol. 9, Issue 4
An updated version of wannier90: A tool for obtaining maximally-localised Wannier functions
journal, August 2014
- Mostofi, Arash A.; Yates, Jonathan R.; Pizzi, Giovanni
- Computer Physics Communications, Vol. 185, Issue 8
Electrically Controllable Surface Magnetism on the Surface of Topological Insulators
journal, February 2011
- Zhu, Jia-Ji; Yao, Dao-Xin; Zhang, Shou-Cheng
- Physical Review Letters, Vol. 106, Issue 9
Development of laser-based scanning µ-ARPES system with ultimate energy and momentum resolutions
journal, November 2017
- Iwasawa, Hideaki; Schwier, Eike F.; Arita, Masashi
- Ultramicroscopy, Vol. 182
Quasiparticle dynamics in reshaped helical Dirac cone of topological insulators
journal, February 2013
- Miao, L.; Wang, Z. F.; Ming, W.
- Proceedings of the National Academy of Sciences, Vol. 110, Issue 8
Scale-Invariant Quantum Anomalous Hall Effect in Magnetic Topological Insulators beyond the Two-Dimensional Limit
journal, September 2014
- Kou, Xufeng; Guo, Shih-Ting; Fan, Yabin
- Physical Review Letters, Vol. 113, Issue 13
Crystal structure, properties and nanostructuring of a new layered chalcogenide semiconductor, Bi2MnTe4
journal, January 2013
- Lee, Dong Sun; Kim, Tae-Hoon; Park, Cheol-Hee
- CrystEngComm, Vol. 15, Issue 27
From ultrasoft pseudopotentials to the projector augmented-wave method
journal, January 1999
- Kresse, G.; Joubert, D.
- Physical Review B, Vol. 59, Issue 3, p. 1758-1775
Rational Design Principles of the Quantum Anomalous Hall Effect in Superlatticelike Magnetic Topological Insulators
journal, August 2019
- Sun, Hongyi; Xia, Bowen; Chen, Zhongjia
- Physical Review Letters, Vol. 123, Issue 9
Topological magnetic crystalline insulators and corepresentation theory
journal, March 2015
- Zhang, Rui-Xing; Liu, Chao-Xing
- Physical Review B, Vol. 91, Issue 11
Spin scattering and noncollinear spin structure-induced intrinsic anomalous Hall effect in antiferromagnetic topological insulator
journal, August 2019
- Lee, Seng Huat; Zhu, Yanglin; Wang, Yu
- Physical Review Research, Vol. 1, Issue 1
Electron-energy-loss spectra and the structural stability of nickel oxide: An LSDA+U study
journal, January 1998
- Dudarev, S. L.; Botton, G. A.; Savrasov, S. Y.
- Physical Review B, Vol. 57, Issue 3, p. 1505-1509
Maximally localized generalized Wannier functions for composite energy bands
journal, November 1997
- Marzari, Nicola; Vanderbilt, David
- Physical Review B, Vol. 56, Issue 20
Topological Axion States in the Magnetic Insulator with the Quantized Magnetoelectric Effect
journal, May 2019
- Zhang, Dongqin; Shi, Minji; Zhu, Tongshuai
- Physical Review Letters, Vol. 122, Issue 20
Topological Electronic Structure and Its Temperature Evolution in Antiferromagnetic Topological Insulator MnBi 2 Te 4
journal, November 2019
- Chen, Y. J.; Xu, L. X.; Li, J. H.
- Physical Review X, Vol. 9, Issue 4
Erratum: Scale-Invariant Quantum Anomalous Hall Effect in Magnetic Topological Insulators beyond the Two-Dimensional Limit [Phys. Rev. Lett. 113 , 137201 (2014)]
journal, November 2014
- Kou, Xufeng; Guo, Shih-Ting; Fan, Yabin
- Physical Review Letters, Vol. 113, Issue 19
Hexagonal Warping Effects in the Surface States of the Topological Insulator
journal, December 2009
- Fu, Liang
- Physical Review Letters, Vol. 103, Issue 26
Topological field theory of time-reversal invariant insulators
journal, November 2008
- Qi, Xiao-Liang; Hughes, Taylor L.; Zhang, Shou-Cheng
- Physical Review B, Vol. 78, Issue 19, Article No. 195424
A topological insulator surface under strong Coulomb, magnetic and disorder perturbations
journal, December 2010
- Wray, L. Andrew; Xu, Su-Yang; Xia, Yuqi
- Nature Physics, Vol. 7, Issue 1
Fractional Chern Insulator
journal, December 2011
- Regnault, N.; Bernevig, B. Andrei
- Physical Review X, Vol. 1, Issue 2
Intrinsic magnetic topological insulators in van der Waals layered MnBi 2 Te 4 -family materials
journal, June 2019
- Li, Jiaheng; Li, Yang; Du, Shiqiao
- Science Advances, Vol. 5, Issue 6
Unique Thickness-Dependent Properties of the van der Waals Interlayer Antiferromagnet Films
journal, March 2019
- Otrokov, M. M.; Rusinov, I. P.; Blanco-Rey, M.
- Physical Review Letters, Vol. 122, Issue 10
Massive Dirac Fermion on the Surface of a Magnetically Doped Topological Insulator
journal, August 2010
- Chen, Y. L.; Chu, J. - H.; Analytis, J. G.
- Science, Vol. 329, Issue 5992
Magnetic Impurities on the Surface of a Topological Insulator
journal, April 2009
- Liu, Qin; Liu, Chao-Xing; Xu, Cenke
- Physical Review Letters, Vol. 102, Issue 15
Surface states and Rashba-type spin polarization in antiferromagnetic MnBi 2 Te 4 (0001)
journal, September 2019
- Vidal, R. C.; Bentmann, H.; Peixoto, T. R. F.
- Physical Review B, Vol. 100, Issue 12
Magnetically controllable topological quantum phase transitions in the antiferromagnetic topological insulator
journal, September 2019
- Li, Jiaheng; Wang, Chong; Zhang, Zetao
- Physical Review B, Vol. 100, Issue 12
Magnetic topological insulators
journal, January 2019
- Tokura, Yoshinori; Yasuda, Kenji; Tsukazaki, Atsushi
- Nature Reviews Physics, Vol. 1, Issue 2
High-precision realization of robust quantum anomalous Hall state in a hard ferromagnetic topological insulator
journal, March 2015
- Chang, Cui-Zu; Zhao, Weiwei; Kim, Duk Y.
- Nature Materials, Vol. 14, Issue 5
Generalized Gradient Approximation Made Simple [Phys. Rev. Lett. 77, 3865 (1996)]
journal, February 1997
- Perdew, John P.; Burke, Kieron; Ernzerhof, Matthias
- Physical Review Letters, Vol. 78, Issue 7
Efficiency of ab-initio total energy calculations for metals and semiconductors using a plane-wave basis set
journal, July 1996
- Kresse, G.; Furthmüller, J.
- Computational Materials Science, Vol. 6, Issue 1, p. 15-50
Evolution of structural, magnetic, and transport properties in
journal, September 2019
- Yan, J. -Q.; Okamoto, S.; McGuire, M. A.
- Physical Review B, Vol. 100, Issue 10
Chemical Aspects of the Candidate Antiferromagnetic Topological Insulator MnBi 2 Te 4
journal, March 2019
- Zeugner, Alexander; Nietschke, Frederik; Wolter, Anja U. B.
- Chemistry of Materials, Vol. 31, Issue 8
Experimental Observation of the Quantum Anomalous Hall Effect in a Magnetic Topological Insulator
journal, March 2013
- Chang, C. -Z.; Zhang, J.; Feng, X.
- Science, Vol. 340, Issue 6129
Higher-order topology in bismuth
journal, July 2018
- Schindler, Frank; Wang, Zhijun; Vergniory, Maia G.
- Nature Physics, Vol. 14, Issue 9
Experimental Realization of an Intrinsic Magnetic Topological Insulator *
journal, June 2019
- Gong, Yan; Guo, Jingwen; Li, Jiaheng
- Chinese Physics Letters, Vol. 36, Issue 7
Bulk topological invariants in noninteracting point group symmetric insulators
journal, September 2012
- Fang, Chen; Gilbert, Matthew J.; Bernevig, B. Andrei
- Physical Review B, Vol. 86, Issue 11
Surface magnetic ordering in topological insulators with bulk magnetic dopants
journal, May 2012
- Rosenberg, G.; Franz, M.
- Physical Review B, Vol. 85, Issue 19
Dual Topological Character of Chalcogenides: Theory for
journal, January 2014
- Rauch, Tomáš; Flieger, Markus; Henk, Jürgen
- Physical Review Letters, Vol. 112, Issue 1
Crystal growth and magnetic structure of
journal, June 2019
- Yan, J. -Q.; Zhang, Q.; Heitmann, T.
- Physical Review Materials, Vol. 3, Issue 6
Realization of the Axion Insulator State in Quantum Anomalous Hall Sandwich Heterostructures
journal, January 2018
- Xiao, Di; Jiang, Jue; Shin, Jae-Ho
- Physical Review Letters, Vol. 120, Issue 5
Trajectory of the anomalous Hall effect towards the quantized state in a ferromagnetic topological insulator
journal, August 2014
- Checkelsky, J. G.; Yoshimi, R.; Tsukazaki, A.
- Nature Physics, Vol. 10, Issue 10
Intrinsic magnetic topological insulator phases in the Sb doped MnBi2Te4 bulks and thin flakes
journal, October 2019
- Chen, Bo; Fei, Fucong; Zhang, Dongqin
- Nature Communications, Vol. 10, Issue 1
Band theory and Mott insulators: Hubbard U instead of Stoner I
journal, July 1991
- Anisimov, Vladimir I.; Zaanen, Jan; Andersen, Ole K.
- Physical Review B, Vol. 44, Issue 3, p. 943-954
Erratum: Topological field theory of time-reversal invariant insulators [Phys. Rev. B 78 , 195424 (2008)]
journal, April 2010
- Qi, Xiao-Liang; Hughes, Taylor L.; Zhang, Shou-Cheng
- Physical Review B, Vol. 81, Issue 15
Antiferromagnetic topological insulators
journal, June 2010
- Mong, Roger S. K.; Essin, Andrew M.; Moore, Joel E.
- Physical Review B, Vol. 81, Issue 24
Layer-dependent ferromagnetism in a van der Waals crystal down to the monolayer limit
journal, June 2017
- Huang, Bevin; Clark, Genevieve; Navarro-Moratalla, Efrén
- Nature, Vol. 546, Issue 7657
Special quasirandom structures
journal, July 1990
- Zunger, Alex; Wei, S.-H.; Ferreira, L. G.
- Physical Review Letters, Vol. 65, Issue 3, p. 353-356
WannierTools: An open-source software package for novel topological materials
journal, March 2018
- Wu, QuanSheng; Zhang, ShengNan; Song, Hai-Feng
- Computer Physics Communications, Vol. 224
Robustness of topological order and formation of quantum well states in topological insulators exposed to ambient environment
journal, February 2012
- Chen, C.; He, S.; Weng, H.
- Proceedings of the National Academy of Sciences, Vol. 109, Issue 10
Hedgehog spin texture and Berry’s phase tuning in a magnetic topological insulator
journal, June 2012
- Xu, Su-Yang; Neupane, Madhab; Liu, Chang
- Nature Physics, Vol. 8, Issue 8
Quantized Anomalous Hall Effect in Magnetic Topological Insulators
journal, June 2010
- Yu, R.; Zhang, W.; Zhang, H. -J.
- Science, Vol. 329, Issue 5987
Highly-ordered wide bandgap materials for quantized anomalous Hall and magnetoelectric effects
journal, April 2017
- Otrokov, M. M.; Menshchikova, T. V.; Vergniory, M. G.
- 2D Materials, Vol. 4, Issue 2
On the matter of topological insulators as magnetoelectrics
journal, January 2019
- Armitage, N. Peter; Wu, Liang
- SciPost Physics, Vol. 6, Issue 4
Novel ternary layered manganese bismuth tellurides of the MnTe-Bi2Te3 system: Synthesis and crystal structure
journal, June 2019
- Aliev, Ziya S.; Amiraslanov, Imamaddin R.; Nasonova, Daria I.
- Journal of Alloys and Compounds, Vol. 789
Transport properties of thin flakes of the antiferromagnetic topological insulator
journal, April 2019
- Cui, Jianhua; Shi, Mengzhu; Wang, Honghui
- Physical Review B, Vol. 99, Issue 15