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Title: A Perspective on Studying Electronic Structure of Batteries through Soft X-ray Spectroscopy

Abstract

Understanding electronic structure is vital to enhance the battery performance. Soft X-ray spectroscopy (SXS) is one of most effective methods to provide direct probe of electronic states. Here, spectroscopic measurements of transition metal 3d and oxygen 2p states are simply reviewed. Then, we mainly focus on the perspective of the development direction of modern SXS techniques. While the true power of recently developed high efficiency mapping of resonant inelastic x-ray scattering (mRIXS) has been apparent for materials and chemistry studies. Great challenges remain for mRIXS spectroscopic interpretation, and the understanding of the battery materials on novel redox activities remains elusive.

Authors:
 [1];  [1];  [2]
  1. Peking Univ., Shenzhen (China). School of Advanced Materials
  2. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)
Publication Date:
Research Org.:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division
OSTI Identifier:
1594941
Grant/Contract Number:  
AC02-05CH11231
Resource Type:
Accepted Manuscript
Journal Name:
Chinese Journal of Structural Chemistry
Additional Journal Information:
Journal Volume: 38; Journal Issue: 12; Journal ID: ISSN 0254-5861
Publisher:
CNKI - China Academic Journals Electronic Publishing House Co., Ltd.
Country of Publication:
United States
Language:
English
Subject:
25 ENERGY STORAGE; electronic structure; soft x-ray spectroscopy; oxygen redox; O-K mRIXS

Citation Formats

Zeng-Qing, Zhuo, Feng, Pan, and Wan-Li, Yang. A Perspective on Studying Electronic Structure of Batteries through Soft X-ray Spectroscopy. United States: N. p., 2019. Web. https://doi.org/10.14102/j.cnki.0254-5861.2011-2677.
Zeng-Qing, Zhuo, Feng, Pan, & Wan-Li, Yang. A Perspective on Studying Electronic Structure of Batteries through Soft X-ray Spectroscopy. United States. https://doi.org/10.14102/j.cnki.0254-5861.2011-2677
Zeng-Qing, Zhuo, Feng, Pan, and Wan-Li, Yang. Sun . "A Perspective on Studying Electronic Structure of Batteries through Soft X-ray Spectroscopy". United States. https://doi.org/10.14102/j.cnki.0254-5861.2011-2677. https://www.osti.gov/servlets/purl/1594941.
@article{osti_1594941,
title = {A Perspective on Studying Electronic Structure of Batteries through Soft X-ray Spectroscopy},
author = {Zeng-Qing, Zhuo and Feng, Pan and Wan-Li, Yang},
abstractNote = {Understanding electronic structure is vital to enhance the battery performance. Soft X-ray spectroscopy (SXS) is one of most effective methods to provide direct probe of electronic states. Here, spectroscopic measurements of transition metal 3d and oxygen 2p states are simply reviewed. Then, we mainly focus on the perspective of the development direction of modern SXS techniques. While the true power of recently developed high efficiency mapping of resonant inelastic x-ray scattering (mRIXS) has been apparent for materials and chemistry studies. Great challenges remain for mRIXS spectroscopic interpretation, and the understanding of the battery materials on novel redox activities remains elusive.},
doi = {10.14102/j.cnki.0254-5861.2011-2677},
journal = {Chinese Journal of Structural Chemistry},
number = 12,
volume = 38,
place = {United States},
year = {2019},
month = {12}
}

Journal Article:
Free Publicly Available Full Text
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