Enhanced Surface Interactions Enable Fast Li + Conduction in Oxide/Polymer Composite Electrolyte

Wu, Nan; Chien, Po‐Hsiu; Qian, Yumin; Li, Yutao; Xu, Henghui; Grundish, Nicholas S.; Xu, Biyi; Jin, Haibo; Hu, Yan‐Yan; Yu, Guihua; Goodenough, John B.

doi:10.1002/ange.201914478

Title: Enhanced Surface Interactions Enable Fast Li ⁺ Conduction in Oxide/Polymer Composite Electrolyte

Authors:

^[1]; Chien, Po‐Hsiu ^[2]; Qian, Yumin ^[3];

^[3];

^[3]; Grundish, Nicholas S. ^[3];

^[3]; Jin, Haibo ^[4]; Hu, Yan‐Yan ^[5]; Yu, Guihua ^[3];

^[3]

Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications School of Materials Science &, Engineering Beijing Institute of Technology Beijing 100081 P. R. China, Materials Science and Engineering Program and Texas Materials Institute The University of Texas at Austin Austin TX 78712 USA
Center of Interdisciplinary Magnetic Resonance National High Magnetic Field Laboratory 1800 East Paul Dirac Drive Tallahassee FL 32310 USA
Materials Science and Engineering Program and Texas Materials Institute The University of Texas at Austin Austin TX 78712 USA
Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications School of Materials Science &, Engineering Beijing Institute of Technology Beijing 100081 P. R. China
Center of Interdisciplinary Magnetic Resonance National High Magnetic Field Laboratory 1800 East Paul Dirac Drive Tallahassee FL 32310 USA, Department of Chemistry and Biochemistry Florida State University Tallahassee FL 32306 USA

Publication Date:: 2020-01-23

Sponsoring Org.:: USDOE

OSTI Identifier:: 1593496

Grant/Contract Number:: EE0007762

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: Angewandte Chemie

Additional Journal Information:: Journal Name: Angewandte Chemie Journal Volume: 132 Journal Issue: 10; Journal ID: ISSN 0044-8249

Publisher:: Wiley Blackwell (John Wiley & Sons)

Country of Publication:: Germany

Language:: English

Citation Formats


                    Wu, Nan, Chien, Po‐Hsiu, Qian, Yumin, Li, Yutao, Xu, Henghui, Grundish, Nicholas S., Xu, Biyi, Jin, Haibo, Hu, Yan‐Yan, Yu, Guihua, and Goodenough, John B. Enhanced Surface Interactions Enable Fast Li + Conduction in Oxide/Polymer Composite Electrolyte.  Germany: N. p., 2020. 
Web.  doi:10.1002/ange.201914478.

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                    Wu, Nan, Chien, Po‐Hsiu, Qian, Yumin, Li, Yutao, Xu, Henghui, Grundish, Nicholas S., Xu, Biyi, Jin, Haibo, Hu, Yan‐Yan, Yu, Guihua, & Goodenough, John B. Enhanced Surface Interactions Enable Fast Li + Conduction in Oxide/Polymer Composite Electrolyte.  Germany.  https://doi.org/10.1002/ange.201914478

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                    Wu, Nan, Chien, Po‐Hsiu, Qian, Yumin, Li, Yutao, Xu, Henghui, Grundish, Nicholas S., Xu, Biyi, Jin, Haibo, Hu, Yan‐Yan, Yu, Guihua, and Goodenough, John B. Thu .  
"Enhanced Surface Interactions Enable Fast Li + Conduction in Oxide/Polymer Composite Electrolyte".  Germany.  https://doi.org/10.1002/ange.201914478.

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@article{osti_1593496,

  title        = {Enhanced Surface Interactions Enable Fast Li + Conduction in Oxide/Polymer Composite Electrolyte},

  author       = {Wu, Nan and Chien, Po‐Hsiu and Qian, Yumin and Li, Yutao and Xu, Henghui and Grundish, Nicholas S. and Xu, Biyi and Jin, Haibo and Hu, Yan‐Yan and Yu, Guihua and Goodenough, John B.},

  abstractNote = {},

  doi          = {10.1002/ange.201914478},

  journal      = {Angewandte Chemie},

  number       = 10,

  volume       = 132,

  place        = {Germany},

  year         = {2020},

  month        = {1}

}

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Title: Enhanced Surface Interactions Enable Fast Li + Conduction in Oxide/Polymer Composite Electrolyte

Citation Formats

The influence of phase segregation on properties of semicrystalline PEO:LiTFSI electrolytes journal, September 2008

A High-Energy-Density Potassium Battery with a Polymer-Gel Electrolyte and a Polyaniline Cathode journal, April 2018

Optimizing Li+ conductivity in a garnet framework journal, January 2012

Lithium-7 NMR studies of concentrated LiI/PEO-based solid electrolytes journal, February 1998

Lithium Ion Pathway within Li 7 La 3 Zr 2 O 12 -Polyethylene Oxide Composite Electrolytes journal, September 2016

Pathways for practical high-energy long-cycling lithium metal batteries journal, February 2019

Boosting Solid-State Diffusivity and Conductivity in Lithium Superionic Argyrodites by Halide Substitution journal, May 2019

IONIC CONDUCTIVITY AND LITHIUM TRANSFERENCE NUMBER OF POLY(ETHYLENE OXIDE):LiTFSI SYSTEM journal, February 2017

Li 0.33 La 0.557 TiO 3 ceramic nanofiber-enhanced polyethylene oxide-based composite polymer electrolytes for all-solid-state lithium batteries journal, January 2018

Enhancing ionic conductivity in composite polymer electrolytes with well-aligned ceramic nanowires journal, April 2017

Synthesis of and densification of oxygen-conducting La0.8Sr0.2Ga0.8Mg0.2O2.8 nano powder prepared from a low temperature hydrothermal urea precipitation process journal, January 2008

New Insights into the Compositional Dependence of Li-Ion Transport in Polymer–Ceramic Composite Electrolytes journal, January 2018

Structural, morphological and electrical properties of Gd0.1Ce0.9O1.95 prepared by a citrate complexation method journal, January 2009

Study on ionic transport mechanism and interactions between salt and polymer chain in PAN based solid polymer electrolytes containing LiCF3SO3 journal, November 2004

Poly(ethylene oxide)-based electrolytes for lithium-ion batteries journal, January 2015

Recent advances in all-solid-state rechargeable lithium batteries journal, March 2017

Nanocomposite polymer electrolytes for lithium batteries journal, July 1998

Lithium Ion Pathway within Li 7 La 3 Zr 2 O 12 -Polyethylene Oxide Composite Electrolytes journal, September 2016

PEO/garnet composite electrolytes for solid-state lithium batteries: From “ceramic-in-polymer” to “polymer-in-ceramic” journal, April 2018

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Schnelle Lithiumionenleitung in granatartigem Li7La3Zr2O12 journal, October 2007

Solid Halide Electrolytes with High Lithium-Ion Conductivity for Application in 4 V Class Bulk-Type All-Solid-State Batteries journal, September 2018

Nanotechnology for environmentally sustainable electromobility journal, December 2016

Mastering the interface for advanced all-solid-state lithium rechargeable batteries journal, November 2016

Li-ion transport in a representative ceramic–polymer–plasticizer composite electrolyte: Li 7 La 3 Zr 2 O 12 –polyethylene oxide–tetraethylene glycol dimethyl ether journal, January 2017

Lithium coordination and mobility in gel electrolytes based on an acrylate polymer with ethylene oxide side chains journal, February 2003

Dendrite-Free Li-Metal Battery Enabled by a Thin Asymmetric Solid Electrolyte with Engineered Layers journal, December 2017

A High-Energy-Density Potassium Battery with a Polymer-Gel Electrolyte and a Polyaniline Cathode journal, April 2018

Ionic Conductivity Enhancement of Polymer Electrolytes with Ceramic Nanowire Fillers journal, March 2015

Li6PS5X: A Class of Crystalline Li-Rich Solids With an Unusually High Li+ Mobility journal, January 2008

Garnet Electrolyte with an Ultralow Interfacial Resistance for Li-Metal Batteries journal, April 2018

Flexible, solid-state, ion-conducting membrane with 3D garnet nanofiber networks for lithium batteries journal, June 2016

All solid-state polymer electrolytes for high-performance lithium ion batteries journal, October 2016

Ultrathin, flexible, solid polymer composite electrolyte enabled with aligned nanoporous host for lithium batteries journal, May 2019

Crystalline phases, morphology and conductivity of PEO:LiTFSI electrolytes in the eutectic region journal, September 2006

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Mixed phase solid electrolytes journal, September 1988

Boosting Solid‐State Diffusivity and Conductivity in Lithium Superionic Argyrodites by Halide Substitution journal, May 2019

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The Li-Ion Rechargeable Battery: A Perspective journal, January 2013

High-performance all-solid-state batteries enabled by salt bonding to perovskite in poly(ethylene oxide) journal, August 2019

Contact ion pair formation and ether oxygen coordination in the polymer electrolytes M[N(CF3SO2)2]2PEOn for M = Mg, Ca, Sr and Ba journal, January 1995

Li6PS5X: A Class of Crystalline Li-Rich Solids With an Unusually High Li+ Mobility journal, January 2008

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Title: Enhanced Surface Interactions Enable Fast Li ⁺ Conduction in Oxide/Polymer Composite Electrolyte

The influence of phase segregation on properties of semicrystalline PEO:LiTFSI electrolytes
journal, September 2008

A High-Energy-Density Potassium Battery with a Polymer-Gel Electrolyte and a Polyaniline Cathode
journal, April 2018

Optimizing Li+ conductivity in a garnet framework
journal, January 2012

Lithium-7 NMR studies of concentrated LiI/PEO-based solid electrolytes
journal, February 1998

Lithium Ion Pathway within Li ₇ La ₃ Zr ₂ O ₁₂ -Polyethylene Oxide Composite Electrolytes
journal, September 2016

Pathways for practical high-energy long-cycling lithium metal batteries
journal, February 2019

Boosting Solid-State Diffusivity and Conductivity in Lithium Superionic Argyrodites by Halide Substitution
journal, May 2019

IONIC CONDUCTIVITY AND LITHIUM TRANSFERENCE NUMBER OF POLY(ETHYLENE OXIDE):LiTFSI SYSTEM
journal, February 2017

Li _0.33 La _0.557 TiO ₃ ceramic nanofiber-enhanced polyethylene oxide-based composite polymer electrolytes for all-solid-state lithium batteries
journal, January 2018

Enhancing ionic conductivity in composite polymer electrolytes with well-aligned ceramic nanowires
journal, April 2017

Synthesis of and densification of oxygen-conducting La0.8Sr0.2Ga0.8Mg0.2O2.8 nano powder prepared from a low temperature hydrothermal urea precipitation process
journal, January 2008

New Insights into the Compositional Dependence of Li-Ion Transport in Polymer–Ceramic Composite Electrolytes
journal, January 2018

Structural, morphological and electrical properties of Gd0.1Ce0.9O1.95 prepared by a citrate complexation method
journal, January 2009

Study on ionic transport mechanism and interactions between salt and polymer chain in PAN based solid polymer electrolytes containing LiCF3SO3
journal, November 2004

Poly(ethylene oxide)-based electrolytes for lithium-ion batteries
journal, January 2015

Recent advances in all-solid-state rechargeable lithium batteries
journal, March 2017

Nanocomposite polymer electrolytes for lithium batteries
journal, July 1998

Lithium Ion Pathway within Li 7 La 3 Zr 2 O 12 -Polyethylene Oxide Composite Electrolytes
journal, September 2016

PEO/garnet composite electrolytes for solid-state lithium batteries: From “ceramic-in-polymer” to “polymer-in-ceramic”
journal, April 2018

Solid polymer electrolytes incorporating cubic Li7La3Zr2O12 for all-solid-state lithium rechargeable batteries
journal, December 2017

Schnelle Lithiumionenleitung in granatartigem Li7La3Zr2O12
journal, October 2007

Solid Halide Electrolytes with High Lithium-Ion Conductivity for Application in 4 V Class Bulk-Type All-Solid-State Batteries
journal, September 2018

Nanotechnology for environmentally sustainable electromobility
journal, December 2016

Mastering the interface for advanced all-solid-state lithium rechargeable batteries
journal, November 2016

Li-ion transport in a representative ceramic–polymer–plasticizer composite electrolyte: Li ₇ La ₃ Zr ₂ O ₁₂ –polyethylene oxide–tetraethylene glycol dimethyl ether
journal, January 2017

Lithium coordination and mobility in gel electrolytes based on an acrylate polymer with ethylene oxide side chains
journal, February 2003

Dendrite-Free Li-Metal Battery Enabled by a Thin Asymmetric Solid Electrolyte with Engineered Layers
journal, December 2017

A High-Energy-Density Potassium Battery with a Polymer-Gel Electrolyte and a Polyaniline Cathode
journal, April 2018

Ionic Conductivity Enhancement of Polymer Electrolytes with Ceramic Nanowire Fillers
journal, March 2015

Li6PS5X: A Class of Crystalline Li-Rich Solids With an Unusually High Li+ Mobility
journal, January 2008

Garnet Electrolyte with an Ultralow Interfacial Resistance for Li-Metal Batteries
journal, April 2018

Flexible, solid-state, ion-conducting membrane with 3D garnet nanofiber networks for lithium batteries
journal, June 2016

All solid-state polymer electrolytes for high-performance lithium ion batteries
journal, October 2016

Ultrathin, flexible, solid polymer composite electrolyte enabled with aligned nanoporous host for lithium batteries
journal, May 2019

Crystalline phases, morphology and conductivity of PEO:LiTFSI electrolytes in the eutectic region
journal, September 2006

Polymer Electrolytes for Lithium-Ion Batteries
journal, April 1998

Vertically Aligned and Continuous Nanoscale Ceramic–Polymer Interfaces in Composite Solid Polymer Electrolytes for Enhanced Ionic Conductivity
journal, May 2018

Mixed phase solid electrolytes
journal, September 1988

Boosting Solid‐State Diffusivity and Conductivity in Lithium Superionic Argyrodites by Halide Substitution
journal, May 2019

Polymer Electrolytes
journal, August 1986

The Li-Ion Rechargeable Battery: A Perspective
journal, January 2013

High-performance all-solid-state batteries enabled by salt bonding to perovskite in poly(ethylene oxide)
journal, August 2019

Contact ion pair formation and ether oxygen coordination in the polymer electrolytes M[N(CF3SO2)2]2PEOn for M = Mg, Ca, Sr and Ba
journal, January 1995

Li6PS5X: A Class of Crystalline Li-Rich Solids With an Unusually High Li+ Mobility
journal, January 2008

Lithium battery chemistries enabled by solid-state electrolytes
journal, February 2017

Fast Lithium Ion Conduction in Garnet-Type Li₇La₃Zr₂O₁₂
journal, October 2007