Click chemistry as a route to the synthesis of structurally new and magnetically interesting coordination clusters: a {NiII8} complex with a trapezoidal prismatic topology
Abstract
A {Ni 8 } cluster with trapezoidal prismatic topology was prepared via the click reaction between MeCN and N 3 − ions.
- Authors:
-
[2];
[3];
[1];
[1]
- Department of Chemistry, 1812 Sir Isaac Brock Way, Brock University, Canada
- Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, USA
- Department de Quimica Inorgànica i Orgànica, Secció Inorgànica and Institut de Nanociència i Nanotecnologia (IN2UB), Universitat de Barcelona, 08028 Barcelona, Spain
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1593493
- Alternate Identifier(s):
- OSTI ID: 1531184; OSTI ID: 1581603
- Grant/Contract Number:
- AC02-05CH11231
- Resource Type:
- Published Article
- Journal Name:
- Dalton Transactions
- Additional Journal Information:
- Journal Name: Dalton Transactions Journal Volume: 48 Journal Issue: 31; Journal ID: ISSN 1477-9226
- Publisher:
- Royal Society of Chemistry
- Country of Publication:
- United Kingdom
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
Citation Formats
Abbasi, Parisa, Athanasopoulou, Angeliki A., Mazarakioti, Eleni C., Gagnon, Kevin J., Teat, Simon J., Escuer, Albert, Pilkington, Melanie, and Stamatatos, Theocharis C. Click chemistry as a route to the synthesis of structurally new and magnetically interesting coordination clusters: a {NiII8} complex with a trapezoidal prismatic topology. United Kingdom: N. p., 2019.
Web. doi:10.1039/C9DT01998G.
Abbasi, Parisa, Athanasopoulou, Angeliki A., Mazarakioti, Eleni C., Gagnon, Kevin J., Teat, Simon J., Escuer, Albert, Pilkington, Melanie, & Stamatatos, Theocharis C. Click chemistry as a route to the synthesis of structurally new and magnetically interesting coordination clusters: a {NiII8} complex with a trapezoidal prismatic topology. United Kingdom. https://doi.org/10.1039/C9DT01998G
Abbasi, Parisa, Athanasopoulou, Angeliki A., Mazarakioti, Eleni C., Gagnon, Kevin J., Teat, Simon J., Escuer, Albert, Pilkington, Melanie, and Stamatatos, Theocharis C. Tue .
"Click chemistry as a route to the synthesis of structurally new and magnetically interesting coordination clusters: a {NiII8} complex with a trapezoidal prismatic topology". United Kingdom. https://doi.org/10.1039/C9DT01998G.
@article{osti_1593493,
title = {Click chemistry as a route to the synthesis of structurally new and magnetically interesting coordination clusters: a {NiII8} complex with a trapezoidal prismatic topology},
author = {Abbasi, Parisa and Athanasopoulou, Angeliki A. and Mazarakioti, Eleni C. and Gagnon, Kevin J. and Teat, Simon J. and Escuer, Albert and Pilkington, Melanie and Stamatatos, Theocharis C.},
abstractNote = {A {Ni 8 } cluster with trapezoidal prismatic topology was prepared via the click reaction between MeCN and N 3 − ions.},
doi = {10.1039/C9DT01998G},
journal = {Dalton Transactions},
number = 31,
volume = 48,
place = {United Kingdom},
year = {2019},
month = {8}
}
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https://doi.org/10.1039/C9DT01998G
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Works referenced in this record:
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Self-Assembled Dinuclear, Trinuclear, Tetranuclear, Pentanuclear, and Octanuclear Ni(II) Complexes of a Series of Polytopic Diazine Based Ligands: Structural and Magnetic Properties
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Effective dehydrogenation of 2-pyridylmethanol derivatives catalyzed by an iron complex
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Diol-type ligands as central ‘players’ in the chemistry of high-spin molecules and single-molecule magnets
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Bis-tris propane as a flexible ligand for high-nuclearity complexes
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Preparation of 5-Substituted 1 H -Tetrazoles from Nitriles in Water †
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Cu-Catalyzed Azide−Alkyne Cycloaddition
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Using tripodal alcohols to build high-spin molecules and single-molecule magnets
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Polyhedral Metal-Imidazolate Cages: Control of Self-Assembly and Cage to Cage Transformation
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Tripodal Tetraamine Ligands Containing Three Pyridine Units: Theother Polypyridyl Ligands
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An Improved Synthesis of 5-Substituted Tetrazoles
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Unprecedented cationic copper(i)–iodide aggregates trapped in “click” formation of anionic-tetrazolate-based coordination polymers
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- Chemical Communications, Issue 29
In situ synthesized 3D heterometallic metal–organic framework (MOF) as a high-energy-density material shows high heat of detonation, good thermostability and insensitivity
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- Feng, Yaya; Liu, Xiangyu; Duan, Linqiang
- Dalton Transactions, Vol. 44, Issue 5
Unprecedented chemical transformation: crystallographic evidence for 1,1,2,2-tetrahydroxyethane captured within an Fe6Dy3 single molecule magnet
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A Polyoxometalate Containing the{Ni2N3} Fragment: Ferromagnetic Coupling in a NiIIμ-1,1 Azido Complex with a Large Bridging Angle
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A novel high-spin tridecanuclear Ni II cluster with an azido-bridged core exhibiting disk-like topology
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- Chem. Commun., Vol. 48, Issue 9
Rational linkage of magnetic molecules using click chemistry
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Organic chelate-free and azido-rich metal clusters and coordination polymers from the use of Me 3 SiN 3 : a new synthetic route to complexes with beautiful structures and diverse magnetic properties
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- Chemical Communications, Vol. 55, Issue 1
Adventures in the Coordination Chemistry of Di-2-pyridyl Ketone and Related Ligands: From High-Spin Molecules and Single-Molecule Magnets to Coordination Polymers, and from Structural Aesthetics to an Exciting New Reactivity Chemistry of Coordinated Ligands
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Directed assembly of metal–organic cubes from deliberately predesigned molecular building blocks
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- Liu, Yunling; Kravtsov, Victor; Walsh, Rosa D.
- Chem. Commun., Issue 24
Targeted construction of azido-bridged Ni 4 complexes with decisive effect of µ-1,3-azide torsion on the spin ground state
journal, January 2006
- Demeshko, Serhiy; Leibeling, Guido; Dechert, Sebastian
- Dalton Trans., Issue 28
Nucleophilic Addition of Water and Alcohols to Dicyanonitrosomethanide: Ligands with Diverse Bonding Modes in Magnetically Coupled d-Block Complexes
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A Mn 6 Cluster inside a Mn 10 Wheel: Characterization of a Mn 16 -Oximate Complex Resulting from a Tetrazole-2-pyridylketoneoximate Ligand : A Mn
journal, January 2015
- Alcazar, Laura; Font-Bardia, Mercè; Escuer, Albert
- European Journal of Inorganic Chemistry, Vol. 2015, Issue 8
Ground state spin-switching via targeted structural distortion: twisted single-molecule magnets from derivatised salicylaldoximes
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- Milios, Constantinos J.; Piligkos, Stergios; Brechin, Euan K.
- Dalton Trans., Issue 14
Synthesis, spectroscopic characterization, and magnetic properties of unusual 3,5-dialkyl-1,2,4-triazole compounds containing N-bridging isothiocyanato ligands. X-ray structure of trinuclear bis[(.mu.-thiocyanato-N)bis(.mu.-3,5-diethyl-1,2,4-triazole-N1,N2)bis(thiocyanato-N)(3,5-diethyl-1,2,4-triazole-N1)nickel(II)-N,N1,N1']nickel(II) dihydrate
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Mechanisms of Tetrazole Formation by Addition of Azide to Nitriles
journal, October 2002
- Himo, Fahmi; Demko, Zachary P.; Noodleman, Louis
- Journal of the American Chemical Society, Vol. 124, Issue 41
Versatility of Azide in Serendipitous Assembly of Copper(II) Magnetic Polyclusters
journal, June 2013
- Mukherjee, Sandip; Mukherjee, Partha Sarathi
- Accounts of Chemical Research, Vol. 46, Issue 11
Magnetic Coupling in End-On Azido-Bridged Transition Metal Complexes: A Density Functional Study
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- Journal of the American Chemical Society, Vol. 120, Issue 43
The bridging azido ligand as a central “player” in high-nuclearity 3d-metal cluster chemistry
journal, September 2014
- Escuer, Albert; Esteban, Jordi; Perlepes, Spyros P.
- Coordination Chemistry Reviews, Vol. 275
Octanuclear Ni( ii ) cubes based on halogen-substituted pyrazolates: synthesis, structure, electrochemistry and magnetism
journal, January 2016
- Wang, Zhi; Jagličić, Zvonko; Han, Lu-Lu
- CrystEngComm, Vol. 18, Issue 19
Synthesis, crystal and molecular structure and magnetic properties of [Ni3(L1)4(NCS)4(OH)2(OH2)2](L1= 2,5-diamino-1,3,4-thiadiazole)
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- Journal of the Chemical Society, Dalton Transactions, Issue 9
Reversible shrinkage and expansion of a blue photofluorescent cadmium coordination polymer and in situ tetrazole ligand synthesis
journal, January 2008
- Deng, Hong; Qiu, Yong-Cai; Li, Ying-Hua
- Chemical Communications, Issue 19
In situ tetrazole templated chair-like decanuclear azido-cobalt( ii ) SMM containing both tetra- and octa-hedral Co( ii ) ions
journal, January 2015
- Zhang, Yuan-Zhu; Gao, Song; Sato, Osamu
- Dalton Transactions, Vol. 44, Issue 2
Transition Metal Single-Molecule Magnets: A {Mn 31 } Nanosized Cluster with a Large Energy Barrier of ∼60 K and Magnetic Hysteresis at ∼5 K
journal, October 2017
- Abbasi, Parisa; Quinn, Kevan; Alexandropoulos, Dimitris I.
- Journal of the American Chemical Society, Vol. 139, Issue 44
Two Novel Nanoporous Supramolecular Architectures Based on Copper(I) Coordination Polymers with Uniform (8, 3) and (8 2 10) Nets: In Situ Formation of Tetrazolate Ligands
journal, June 2005
- Wu, Tao; Yi, Bi-Hua; Li, Dan
- Inorganic Chemistry, Vol. 44, Issue 12
The growing applications of click chemistry
journal, January 2007
- Moses, John E.; Moorhouse, Adam D.
- Chem. Soc. Rev., Vol. 36, Issue 8
Filling the gap between the quantum and classical worlds of nanoscale magnetism: giant molecular aggregates based on paramagnetic 3d metal ions
journal, January 2016
- Papatriantafyllopoulou, Constantina; Moushi, Eleni E.; Christou, George
- Chemical Society Reviews, Vol. 45, Issue 6
Decorating Diruthenium Compounds with Fréchet Dendrons via the Click Reaction
journal, October 2011
- Forrest, William P.; Cao, Zhi; Chen, Wei-Zhong
- Inorganic Chemistry, Vol. 50, Issue 19
In situhydrothermal synthesis of tetrazole coordination polymers with interesting physical properties
journal, January 2008
- Zhao, Hong; Qu, Zhi-Rong; Ye, Heng-Yun
- Chem. Soc. Rev., Vol. 37, Issue 1
A Polyoxometalate Containing the{Ni2N3} Fragment: Ferromagnetic Coupling in a NiIIμ-1,1 Azido Complex with a Large Bridging Angle
journal, April 2004
- Mialane, Pierre; Dolbecq, Anne; Rivière, Eric
- Angewandte Chemie, Vol. 116, Issue 17
Adventures in the Coordination Chemistry of Di-2-pyridyl Ketone and Related Ligands: From High-Spin Molecules and Single-Molecule Magnets to Coordination Polymers, and from Structural Aesthetics to an Exciting New Reactivity Chemistry of Coordinated Ligands (Eur. J. Inorg. Chem. 23/2009)
journal, August 2009
- Stamatatos, Theocharis C.; Efthymiou, Constantinos G.; Stoumpos, Constantinos C.
- European Journal of Inorganic Chemistry, Vol. 2009, Issue 23
Works referencing / citing this record:
Click Chemistry: Diverse Chemical Function from a Few Good Reactions
journal, June 2001
- Kolb, Hartmuth C.; Finn, M. G.; Sharpless, K. Barry
- Angewandte Chemie International Edition, Vol. 40, Issue 11, p. 2004-2021
A Polyoxometalate Containing the{Ni2N3} Fragment: Ferromagnetic Coupling in a NiIIμ-1,1 Azido Complex with a Large Bridging Angle
journal, April 2004
- Mialane, Pierre; Dolbecq, Anne; Rivière, Eric
- Angewandte Chemie International Edition, Vol. 43, Issue 17
Tripodal Tetraamine Ligands Containing Three Pyridine Units: Theother Polypyridyl Ligands
journal, June 2008
- Blackman, Allan G.
- European Journal of Inorganic Chemistry, Vol. 2008, Issue 17
Adventures in the Coordination Chemistry of Di-2-pyridyl Ketone and Related Ligands: From High-Spin Molecules and Single-Molecule Magnets to Coordination Polymers, and from Structural Aesthetics to an Exciting New Reactivity Chemistry of Coordinated Ligands
journal, August 2009
- Stamatatos, Theocharis C.; Efthymiou, Constantinos G.; Stoumpos, Constantinos C.
- European Journal of Inorganic Chemistry, Vol. 2009, Issue 23
Nucleophilic Addition of Water and Alcohols to Dicyanonitrosomethanide: Ligands with Diverse Bonding Modes in Magnetically Coupled d-Block Complexes
journal, November 2009
- Chesman, Anthony S. R.; Turner, David R.; Moubaraki, Boujemaa
- European Journal of Inorganic Chemistry, Vol. 2010, Issue 1
A Mn 6 Cluster inside a Mn 10 Wheel: Characterization of a Mn 16 -Oximate Complex Resulting from a Tetrazole-2-pyridylketoneoximate Ligand : A Mn
journal, January 2015
- Alcazar, Laura; Font-Bardia, Mercè; Escuer, Albert
- European Journal of Inorganic Chemistry, Vol. 2015, Issue 8
The bridging azido ligand as a central “player” in high-nuclearity 3d-metal cluster chemistry
journal, September 2014
- Escuer, Albert; Esteban, Jordi; Perlepes, Spyros P.
- Coordination Chemistry Reviews, Vol. 275
Bis-tris propane as a flexible ligand for high-nuclearity complexes
journal, August 2018
- Murrie, Mark
- Polyhedron, Vol. 150
Versatility of Azide in Serendipitous Assembly of Copper(II) Magnetic Polyclusters
journal, June 2013
- Mukherjee, Sandip; Mukherjee, Partha Sarathi
- Accounts of Chemical Research, Vol. 46, Issue 11
Self-Assembly of Thiacalix[4]arene-Supported Nickel(II)/Cobalt(II) Complexes Sustained by in Situ Generated 5-Methyltetrazolate Ligand
journal, May 2012
- Xiong, Kecai; Jiang, Feilong; Gai, Yanli
- Crystal Growth & Design, Vol. 12, Issue 6
Cu-Catalyzed Azide−Alkyne Cycloaddition
journal, August 2008
- Meldal, Morten; Tornøe, Christian Wenzel
- Chemical Reviews, Vol. 108, Issue 8
Synthesis, spectroscopic characterization, and magnetic properties of unusual 3,5-dialkyl-1,2,4-triazole compounds containing N-bridging isothiocyanato ligands. X-ray structure of trinuclear bis[(.mu.-thiocyanato-N)bis(.mu.-3,5-diethyl-1,2,4-triazole-N1,N2)bis(thiocyanato-N)(3,5-diethyl-1,2,4-triazole-N1)nickel(II)-N,N1,N1']nickel(II) dihydrate
journal, May 1984
- Van Albada, Gerard A.; De Graaff, Rudolf A. G.; Haasnoot, Jaap G.
- Inorganic Chemistry, Vol. 23, Issue 10
Self-Assembled Dinuclear, Trinuclear, Tetranuclear, Pentanuclear, and Octanuclear Ni(II) Complexes of a Series of Polytopic Diazine Based Ligands: Structural and Magnetic Properties
journal, May 2003
- Xu, Zhiqiang; Thompson, Laurence K.; Milway, Victoria A.
- Inorganic Chemistry, Vol. 42, Issue 9
Two Novel Nanoporous Supramolecular Architectures Based on Copper(I) Coordination Polymers with Uniform (8, 3) and (8 2 10) Nets: In Situ Formation of Tetrazolate Ligands
journal, June 2005
- Wu, Tao; Yi, Bi-Hua; Li, Dan
- Inorganic Chemistry, Vol. 44, Issue 12
Decorating Diruthenium Compounds with Fréchet Dendrons via the Click Reaction
journal, October 2011
- Forrest, William P.; Cao, Zhi; Chen, Wei-Zhong
- Inorganic Chemistry, Vol. 50, Issue 19
An Improved Synthesis of 5-Substituted Tetrazoles
journal, August 1958
- Finnegan, William G.; Henry, Ronald A.; Lofquist, Robert
- Journal of the American Chemical Society, Vol. 80, Issue 15
Mechanisms of Tetrazole Formation by Addition of Azide to Nitriles
journal, October 2002
- Himo, Fahmi; Demko, Zachary P.; Noodleman, Louis
- Journal of the American Chemical Society, Vol. 124, Issue 41
Polyhedral Metal-Imidazolate Cages: Control of Self-Assembly and Cage to Cage Transformation
journal, October 2013
- Zhou, Xiao-Ping; Wu, Yuan; Li, Dan
- Journal of the American Chemical Society, Vol. 135, Issue 43
Magnetic Coupling in End-On Azido-Bridged Transition Metal Complexes: A Density Functional Study
journal, November 1998
- Ruiz, Eliseo; Cano, Joan; Alvarez, Santiago
- Journal of the American Chemical Society, Vol. 120, Issue 43
Transition Metal Single-Molecule Magnets: A {Mn 31 } Nanosized Cluster with a Large Energy Barrier of ∼60 K and Magnetic Hysteresis at ∼5 K
journal, October 2017
- Abbasi, Parisa; Quinn, Kevan; Alexandropoulos, Dimitris I.
- Journal of the American Chemical Society, Vol. 139, Issue 44
Preparation of 5-Substituted 1 H -Tetrazoles from Nitriles in Water †
journal, November 2001
- Demko, Zachary P.; Sharpless, K. Barry
- The Journal of Organic Chemistry, Vol. 66, Issue 24
Directed assembly of metal–organic cubes from deliberately predesigned molecular building blocks
journal, January 2004
- Liu, Yunling; Kravtsov, Victor; Walsh, Rosa D.
- Chem. Commun., Issue 24
Using tripodal alcohols to build high-spin molecules and single-molecule magnets
journal, January 2005
- Brechin, Euan K.
- Chemical Communications, Issue 41
Targeted construction of azido-bridged Ni 4 complexes with decisive effect of µ-1,3-azide torsion on the spin ground state
journal, January 2006
- Demeshko, Serhiy; Leibeling, Guido; Dechert, Sebastian
- Dalton Trans., Issue 28
The growing applications of click chemistry
journal, January 2007
- Moses, John E.; Moorhouse, Adam D.
- Chem. Soc. Rev., Vol. 36, Issue 8
In situhydrothermal synthesis of tetrazole coordination polymers with interesting physical properties
journal, January 2008
- Zhao, Hong; Qu, Zhi-Rong; Ye, Heng-Yun
- Chem. Soc. Rev., Vol. 37, Issue 1
Ground state spin-switching via targeted structural distortion: twisted single-molecule magnets from derivatised salicylaldoximes
journal, January 2008
- Milios, Constantinos J.; Piligkos, Stergios; Brechin, Euan K.
- Dalton Trans., Issue 14
Reversible shrinkage and expansion of a blue photofluorescent cadmium coordination polymer and in situ tetrazole ligand synthesis
journal, January 2008
- Deng, Hong; Qiu, Yong-Cai; Li, Ying-Hua
- Chemical Communications, Issue 19
Unprecedented cationic copper(i)–iodide aggregates trapped in “click” formation of anionic-tetrazolate-based coordination polymers
journal, January 2008
- Li, Mian; Li, Zhen; Li, Dan
- Chemical Communications, Issue 29
Diol-type ligands as central ‘players’ in the chemistry of high-spin molecules and single-molecule magnets
journal, January 2008
- Tasiopoulos, Anastasios J.; Perlepes, Spyros P.
- Dalton Transactions, Issue 41
A novel high-spin tridecanuclear Ni II cluster with an azido-bridged core exhibiting disk-like topology
journal, January 2012
- Brunet, Gabriel; Habib, Fatemah; Cook, Cyril
- Chem. Commun., Vol. 48, Issue 9
Unprecedented chemical transformation: crystallographic evidence for 1,1,2,2-tetrahydroxyethane captured within an Fe6Dy3 single molecule magnet
journal, January 2013
- Schmidt, Sebastian; Prodius, Denis; Mereacre, Valeriu
- Chemical Communications, Vol. 49, Issue 17
Effective dehydrogenation of 2-pyridylmethanol derivatives catalyzed by an iron complex
journal, January 2014
- Kamitani, Masahiro; Ito, Masaki; Itazaki, Masumi
- Chem. Commun., Vol. 50, Issue 59
In situ synthesized 3D heterometallic metal–organic framework (MOF) as a high-energy-density material shows high heat of detonation, good thermostability and insensitivity
journal, January 2015
- Feng, Yaya; Liu, Xiangyu; Duan, Linqiang
- Dalton Transactions, Vol. 44, Issue 5
In situ tetrazole templated chair-like decanuclear azido-cobalt( ii ) SMM containing both tetra- and octa-hedral Co( ii ) ions
journal, January 2015
- Zhang, Yuan-Zhu; Gao, Song; Sato, Osamu
- Dalton Transactions, Vol. 44, Issue 2
Rational linkage of magnetic molecules using click chemistry
journal, January 2015
- Plenk, Christian; Krause, Jasmin; Beck, Martin
- Chemical Communications, Vol. 51, Issue 30
Filling the gap between the quantum and classical worlds of nanoscale magnetism: giant molecular aggregates based on paramagnetic 3d metal ions
journal, January 2016
- Papatriantafyllopoulou, Constantina; Moushi, Eleni E.; Christou, George
- Chemical Society Reviews, Vol. 45, Issue 6
Octanuclear Ni( ii ) cubes based on halogen-substituted pyrazolates: synthesis, structure, electrochemistry and magnetism
journal, January 2016
- Wang, Zhi; Jagličić, Zvonko; Han, Lu-Lu
- CrystEngComm, Vol. 18, Issue 19
Organic chelate-free and azido-rich metal clusters and coordination polymers from the use of Me 3 SiN 3 : a new synthetic route to complexes with beautiful structures and diverse magnetic properties
journal, January 2019
- Stamatatos, Theocharis C.; Rentschler, Eva
- Chemical Communications, Vol. 55, Issue 1
Waterproof architectures through subcomponent self-assembly
journal, January 2019
- Percástegui, Edmundo G.; Mosquera, Jesús; Ronson, Tanya K.
- Chemical Science, Vol. 10, Issue 7
Synthesis, crystal and molecular structure and magnetic properties of [Ni3(L1)4(NCS)4(OH)2(OH2)2](L1= 2,5-diamino-1,3,4-thiadiazole)
journal, January 1991
- Fabretti, Antonio C.; Malavasi, Wanda; Gatteschi, Dante
- Journal of the Chemical Society, Dalton Transactions, Issue 9