Pyrene‐Based Noncovalent Immobilization of Nitrogenase on Carbon Surfaces

doi:10.1002/cbic.201900697

This content will become publicly available on January 19, 2021

Title: Pyrene‐Based Noncovalent Immobilization of Nitrogenase on Carbon Surfaces

Authors:

Patel, Janki ^[1]; Cai, Rong ^[1]; Milton, Ross ^[2]; Chen, Hui ^[1];

^[1]

Department of ChemistryUniversity of Utah 315 S 1400 E Salt Lake City UT 84112 USA
Department of Inorganic and Analytical ChemistryUniversity of Geneva, Sciences II Quai Ernest-Ansermet 30 1211 Geneva 4 Switzerland

Publication Date:: 2020-01-20

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

OSTI Identifier:: 1592522

Grant/Contract Number:: 134124-G003970

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: ChemBioChem: a European journal of chemical biology

Additional Journal Information:: Journal Name: ChemBioChem: a European journal of chemical biology; Journal ID: ISSN 1439-4227

Publisher:: Wiley Blackwell (John Wiley & Sons)

Country of Publication:: France

Language:: English

Citation Formats


                    Patel, Janki, Cai, Rong, Milton, Ross, Chen, Hui, and Minteer, Shelley D. Pyrene‐Based Noncovalent Immobilization of Nitrogenase on Carbon Surfaces.  France: N. p., 2020. 
        Web.  doi:10.1002/cbic.201900697.

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                    Patel, Janki, Cai, Rong, Milton, Ross, Chen, Hui, & Minteer, Shelley D. Pyrene‐Based Noncovalent Immobilization of Nitrogenase on Carbon Surfaces.  France.  doi:10.1002/cbic.201900697.

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                    Patel, Janki, Cai, Rong, Milton, Ross, Chen, Hui, and Minteer, Shelley D. Mon .  
        "Pyrene‐Based Noncovalent Immobilization of Nitrogenase on Carbon Surfaces".  France.  doi:10.1002/cbic.201900697.

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@article{osti_1592522,

  title        = {Pyrene‐Based Noncovalent Immobilization of Nitrogenase on Carbon Surfaces},

  author       = {Patel, Janki and Cai, Rong and Milton, Ross and Chen, Hui and Minteer, Shelley D.},

  abstractNote = {},

  doi          = {10.1002/cbic.201900697},

  journal      = {ChemBioChem: a European journal of chemical biology},

  number       = ,

  volume       = ,

  place        = {France},

  year         = {2020},

  month        = {1}

}

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DOI: 10.1002/cbic.201900697

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Similar Records

This content will become publicly available on January 19, 2021

Title: Pyrene‐Based Noncovalent Immobilization of Nitrogenase on Carbon Surfaces

Citation Formats

A Pyrene-Substituted Tris(bipyridine)osmium(II) Complex as a Versatile Redox Probe for Characterizing and Functionalizing Carbon Nanotube- and Graphene-Based Electrodes journal, June 2013

X-ray Magnetic Circular Dichroism Spectroscopy Applied to Nitrogenase and Related Models: Experimental Evidence for a Spin-Coupled Molybdenum(III) Center journal, June 2019

The In Vivo Potential-Regulated Protective Protein of Nitrogenase in Azotobacter vinelandii Supports Aerobic Bioelectrochemical Dinitrogen Reduction In Vitro journal, June 2017

A Voltammetric Study of Nitrogenase Catalysis Using Electron Transfer Mediators journal, January 2019

Wiring of pyranose dehydrogenase with osmium polymers of different redox potentials journal, November 2010

Infrared spectroscopy of the nitrogenase MoFe protein under electrochemical control: potential-triggered CO binding journal, January 2017

Trapping H - Bound to the Nitrogenase FeMo-Cofactor Active Site during H 2 Evolution: Characterization by ENDOR Spectroscopy journal, May 2005

Establishing a Thermodynamic Landscape for the Active Site of Mo-Dependent Nitrogenase journal, October 2019

Peptide-tags for site-specific protein labelling in vitro and in vivo journal, January 2016

X‐ray Magnetic Circular Dichroism Spectroscopy Applied to Nitrogenase and Related Models: Experimental Evidence for a Spin‐Coupled Molybdenum(III) Center journal, June 2019

Noncovalent Immobilization of Molecular Electrocatalysts for Chemical Synthesis: Efficient Electrochemical Alcohol Oxidation with a Pyrene-TEMPO Conjugate journal, June 2017

Targetting redox polymers as mediators for laccase oxygen reduction in a membrane-less biofuel cell journal, March 2004

Multiple functionalization of single-walled carbon nanotubes by dip coating journal, January 2011

The chemistry of pristine graphene journal, January 2013

Bioelectrochemical Haber-Bosch Process: An Ammonia-Producing H 2 /N 2 Fuel Cell journal, February 2017

Molybdenum-Dependent Formate Dehydrogenase for Formate Bioelectrocatalysis in a Formate/O 2 Enzymatic Fuel Cell journal, January 2018

Mechanism of Nitrogenase Inhibition in Soybean Nodules: Pulse-Modulated Spectroscopy Indicates that Nitrogenase Activity Is Limited by O journal, April 1990

Spectroscopic Description of the E 1 State of Mo Nitrogenase Based on Mo and Fe X-ray Absorption and Mössbauer Studies journal, August 2019

A VTVH MCD and EPR Spectroscopic Study of the Maturation of the “Second” Nitrogenase P-Cluster journal, March 2018

Direct Raman Spectroscopic Measurements of Biological Nitrogen Fixation under Natural Conditions: An Analytical Approach for Studying Nitrogenase Activity journal, December 2016

Noncovalent Immobilization of Molecular Electrocatalysts for Chemical Synthesis: Efficient Electrochemical Alcohol Oxidation with a Pyrene-TEMPO Conjugate journal, June 2017

Mechanism of Nitrogenase H 2 Formation by Metal-Hydride Protonation Probed by Mediated Electrocatalysis and H/D Isotope Effects journal, September 2017

Design of a bioelectrocatalytic electrode interface for oxygen reduction in biofuel cells based on a specifically adapted Os-complex containing redox polymer with entrapped Trametes hirsuta laccase journal, May 2010

Wiring of Photosystem I and Hydrogenase on an Electrode for Photoelectrochemical H 2 Production by using Redox Polymers for Relatively Positive Onset Potential journal, September 2016

Redox polymers in electrochemical systems: From methods of mediation to energy storage journal, June 2019

Bioelectrochemical Haber-Bosch Process: An Ammonia-Producing H 2 /N 2 Fuel Cell journal, February 2017

Noncovalent Functionalization of Single-Walled Carbon Nanotubes journal, August 2009

Nitrogenase bioelectrocatalysis: heterogeneous ammonia and hydrogen production by MoFe protein journal, January 2016

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A Pyrene-Substituted Tris(bipyridine)osmium(II) Complex as a Versatile Redox Probe for Characterizing and Functionalizing Carbon Nanotube- and Graphene-Based Electrodes
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X-ray Magnetic Circular Dichroism Spectroscopy Applied to Nitrogenase and Related Models: Experimental Evidence for a Spin-Coupled Molybdenum(III) Center
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A Voltammetric Study of Nitrogenase Catalysis Using Electron Transfer Mediators
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Wiring of pyranose dehydrogenase with osmium polymers of different redox potentials
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Infrared spectroscopy of the nitrogenase MoFe protein under electrochemical control: potential-triggered CO binding
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Establishing a Thermodynamic Landscape for the Active Site of Mo-Dependent Nitrogenase
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Peptide-tags for site-specific protein labelling in vitro and in vivo
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journal, June 2019

Noncovalent Immobilization of Molecular Electrocatalysts for Chemical Synthesis: Efficient Electrochemical Alcohol Oxidation with a Pyrene-TEMPO Conjugate
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Targetting redox polymers as mediators for laccase oxygen reduction in a membrane-less biofuel cell
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journal, January 2011

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journal, January 2013

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journal, January 2018

Mechanism of Nitrogenase Inhibition in Soybean Nodules: Pulse-Modulated Spectroscopy Indicates that Nitrogenase Activity Is Limited by O
journal, April 1990

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journal, August 2019

A VTVH MCD and EPR Spectroscopic Study of the Maturation of the “Second” Nitrogenase P-Cluster
journal, March 2018

Direct Raman Spectroscopic Measurements of Biological Nitrogen Fixation under Natural Conditions: An Analytical Approach for Studying Nitrogenase Activity
journal, December 2016

Noncovalent Immobilization of Molecular Electrocatalysts for Chemical Synthesis: Efficient Electrochemical Alcohol Oxidation with a Pyrene-TEMPO Conjugate
journal, June 2017

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journal, September 2017

Design of a bioelectrocatalytic electrode interface for oxygen reduction in biofuel cells based on a specifically adapted Os-complex containing redox polymer with entrapped Trametes hirsuta laccase
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journal, September 2016

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journal, June 2019

Bioelectrochemical Haber-Bosch Process: An Ammonia-Producing H ₂ /N ₂ Fuel Cell
journal, February 2017

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journal, August 2009

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journal, January 2016

Nitrogenase FeMoco investigated by spatially resolved anomalous dispersion refinement
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