Pyrene‐Based Noncovalent Immobilization of Nitrogenase on Carbon Surfaces

Patel, Janki; Cai, Rong; Milton, Ross; Chen, Hui; Minteer, Shelley D.

doi:10.1002/cbic.201900697

Title: Pyrene‐Based Noncovalent Immobilization of Nitrogenase on Carbon Surfaces

Authors:

Patel, Janki ^[1]; Cai, Rong ^[1]; Milton, Ross ^[2]; Chen, Hui ^[1];

^[1]

Department of Chemistry University of Utah 315 S 1400 E Salt Lake City UT 84112 USA
Department of Inorganic and Analytical Chemistry University of Geneva, Sciences II Quai Ernest-Ansermet 30 1211 Geneva 4 Switzerland

Publication Date:: 2020-01-20

Sponsoring Org.:: USDOE

OSTI Identifier:: 1592522

Resource Type:: Publisher's Accepted Manuscript

Journal Name:: ChemBioChem: a European journal of chemical biology

Additional Journal Information:: Journal Name: ChemBioChem: a European journal of chemical biology Journal Volume: 21 Journal Issue: 12; Journal ID: ISSN 1439-4227

Publisher:: Wiley Blackwell (John Wiley & Sons)

Country of Publication:: France

Language:: English

Citation Formats


                    Patel, Janki, Cai, Rong, Milton, Ross, Chen, Hui, and Minteer, Shelley D. Pyrene‐Based Noncovalent Immobilization of Nitrogenase on Carbon Surfaces.  France: N. p., 2020. 
Web.  doi:10.1002/cbic.201900697.

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                    Patel, Janki, Cai, Rong, Milton, Ross, Chen, Hui, & Minteer, Shelley D. Pyrene‐Based Noncovalent Immobilization of Nitrogenase on Carbon Surfaces.  France.  https://doi.org/10.1002/cbic.201900697

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                    Patel, Janki, Cai, Rong, Milton, Ross, Chen, Hui, and Minteer, Shelley D. Mon .  
"Pyrene‐Based Noncovalent Immobilization of Nitrogenase on Carbon Surfaces".  France.  https://doi.org/10.1002/cbic.201900697.

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@article{osti_1592522,

  title        = {Pyrene‐Based Noncovalent Immobilization of Nitrogenase on Carbon Surfaces},

  author       = {Patel, Janki and Cai, Rong and Milton, Ross and Chen, Hui and Minteer, Shelley D.},

  abstractNote = {},

  doi          = {10.1002/cbic.201900697},

  journal      = {ChemBioChem: a European journal of chemical biology},

  number       = 12,

  volume       = 21,

  place        = {France},

  year         = {2020},

  month        = {1}

}

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https://doi.org/10.1002/cbic.201900697

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Works referenced in this record:

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Title: Pyrene‐Based Noncovalent Immobilization of Nitrogenase on Carbon Surfaces

Citation Formats

A Pyrene-Substituted Tris(bipyridine)osmium(II) Complex as a Versatile Redox Probe for Characterizing and Functionalizing Carbon Nanotube- and Graphene-Based Electrodes journal, June 2013

X-ray Magnetic Circular Dichroism Spectroscopy Applied to Nitrogenase and Related Models: Experimental Evidence for a Spin-Coupled Molybdenum(III) Center journal, June 2019

The In Vivo Potential-Regulated Protective Protein of Nitrogenase in Azotobacter vinelandii Supports Aerobic Bioelectrochemical Dinitrogen Reduction In Vitro journal, June 2017

A Voltammetric Study of Nitrogenase Catalysis Using Electron Transfer Mediators journal, January 2019

Wiring of pyranose dehydrogenase with osmium polymers of different redox potentials journal, November 2010

Infrared spectroscopy of the nitrogenase MoFe protein under electrochemical control: potential-triggered CO binding journal, January 2017

Trapping H - Bound to the Nitrogenase FeMo-Cofactor Active Site during H 2 Evolution: Characterization by ENDOR Spectroscopy journal, May 2005

Establishing a Thermodynamic Landscape for the Active Site of Mo-Dependent Nitrogenase journal, October 2019

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X‐ray Magnetic Circular Dichroism Spectroscopy Applied to Nitrogenase and Related Models: Experimental Evidence for a Spin‐Coupled Molybdenum(III) Center journal, June 2019

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Spectroscopic Description of the E 1 State of Mo Nitrogenase Based on Mo and Fe X-ray Absorption and Mössbauer Studies journal, August 2019

A VTVH MCD and EPR Spectroscopic Study of the Maturation of the “Second” Nitrogenase P-Cluster journal, March 2018

Direct Raman Spectroscopic Measurements of Biological Nitrogen Fixation under Natural Conditions: An Analytical Approach for Studying Nitrogenase Activity journal, December 2016

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Wiring of Photosystem I and Hydrogenase on an Electrode for Photoelectrochemical H 2 Production by using Redox Polymers for Relatively Positive Onset Potential journal, September 2016

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Infrared spectroscopy of the nitrogenase MoFe protein under electrochemical control: potential-triggered CO binding
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Peptide-tags for site-specific protein labelling in vitro and in vivo
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X‐ray Magnetic Circular Dichroism Spectroscopy Applied to Nitrogenase and Related Models: Experimental Evidence for a Spin‐Coupled Molybdenum(III) Center
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Noncovalent Immobilization of Molecular Electrocatalysts for Chemical Synthesis: Efficient Electrochemical Alcohol Oxidation with a Pyrene-TEMPO Conjugate
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Targetting redox polymers as mediators for laccase oxygen reduction in a membrane-less biofuel cell
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journal, January 2013

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Mechanism of Nitrogenase Inhibition in Soybean Nodules: Pulse-Modulated Spectroscopy Indicates that Nitrogenase Activity Is Limited by O
journal, April 1990

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A VTVH MCD and EPR Spectroscopic Study of the Maturation of the “Second” Nitrogenase P-Cluster
journal, March 2018

Direct Raman Spectroscopic Measurements of Biological Nitrogen Fixation under Natural Conditions: An Analytical Approach for Studying Nitrogenase Activity
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Mechanism of Nitrogenase H ₂ Formation by Metal-Hydride Protonation Probed by Mediated Electrocatalysis and H/D Isotope Effects
journal, September 2017

Design of a bioelectrocatalytic electrode interface for oxygen reduction in biofuel cells based on a specifically adapted Os-complex containing redox polymer with entrapped Trametes hirsuta laccase
journal, May 2010

Wiring of Photosystem I and Hydrogenase on an Electrode for Photoelectrochemical H 2 Production by using Redox Polymers for Relatively Positive Onset Potential
journal, September 2016

Redox polymers in electrochemical systems: From methods of mediation to energy storage
journal, June 2019

Bioelectrochemical Haber-Bosch Process: An Ammonia-Producing H ₂ /N ₂ Fuel Cell
journal, February 2017

Noncovalent Functionalization of Single-Walled Carbon Nanotubes
journal, August 2009

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journal, January 2016

Nitrogenase FeMoco investigated by spatially resolved anomalous dispersion refinement
journal, March 2016

Pyrene hydrogel for promoting direct bioelectrochemistry: ATP-independent electroenzymatic reduction of N ₂
journal, January 2018