Valence bond phases of herbertsmithite and related copper kagome materials
Abstract
Recent evidence from magnetic torque, electron spin resonance, and second harmonic generation indicate that the prototypical quantum spin liquid candidate, herbertsmithite, has a symmetry lower than its x-ray refined trigonal space group. Here we consider known and possible distortions of this mineral class, along with related copper kagome oxides and fluorides, relate these to possible valence bond patterns, and comment on their relevance to the physics of these interesting materials.
- Publication Date:
- Research Org.:
- Argonne National Lab. (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division
- OSTI Identifier:
- 1591970
- Alternate Identifier(s):
- OSTI ID: 1592408
- Grant/Contract Number:
- AC02-06CH11357; W911NF-17-1-0204
- Resource Type:
- Published Article
- Journal Name:
- Physical Review Research
- Additional Journal Information:
- Journal Name: Physical Review Research Journal Volume: 2 Journal Issue: 1; Journal ID: ISSN 2643-1564
- Publisher:
- American Physical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY
Citation Formats
Norman, M. R., Laurita, N. J., and Hsieh, D. Valence bond phases of herbertsmithite and related copper kagome materials. United States: N. p., 2020.
Web. doi:10.1103/PhysRevResearch.2.013055.
Norman, M. R., Laurita, N. J., & Hsieh, D. Valence bond phases of herbertsmithite and related copper kagome materials. United States. https://doi.org/10.1103/PhysRevResearch.2.013055
Norman, M. R., Laurita, N. J., and Hsieh, D. Thu .
"Valence bond phases of herbertsmithite and related copper kagome materials". United States. https://doi.org/10.1103/PhysRevResearch.2.013055.
@article{osti_1591970,
title = {Valence bond phases of herbertsmithite and related copper kagome materials},
author = {Norman, M. R. and Laurita, N. J. and Hsieh, D.},
abstractNote = {Recent evidence from magnetic torque, electron spin resonance, and second harmonic generation indicate that the prototypical quantum spin liquid candidate, herbertsmithite, has a symmetry lower than its x-ray refined trigonal space group. Here we consider known and possible distortions of this mineral class, along with related copper kagome oxides and fluorides, relate these to possible valence bond patterns, and comment on their relevance to the physics of these interesting materials.},
doi = {10.1103/PhysRevResearch.2.013055},
journal = {Physical Review Research},
number = 1,
volume = 2,
place = {United States},
year = {2020},
month = {1}
}
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