Semitransparent Sb2S3 thin film solar cells by ultrasonic spray pyrolysis for use in solar windows

Eensalu, Jako S.; Katerski, Atanas; Kärber, Erki; Weinhardt, Lothar; Blum, Monika; Heske, Clemens; Yang, Wanli; Oja Acik, Ilona; Krunks, Malle

doi:10.3762/bjnano.10.230

Title: Semitransparent Sb₂S₃ thin film solar cells by ultrasonic spray pyrolysis for use in solar windows

Journal Article · 06 December 2019 · Beilstein Journal of Nanotechnology

DOI: https://doi.org/10.3762/bjnano.10.230 · OSTI ID:1591802

^[1];

^[1]; Kärber, Erki ^[2]; Weinhardt, Lothar ^[3]; Blum, Monika ^[4]; Heske, Clemens ^[3];

^[4]; Oja Acik, Ilona ^[1]; Krunks, Malle ^[1]

Tallinn Univ. of Technology, Ehitajate (Estonia)
Tallinn Univ. of Technology, Ehitajate (Estonia); Univ. of Nevada, Las Vegas, NV (United States)
Univ. of Nevada, Las Vegas, NV (United States); Karlsruhe Inst. of Technology (KIT), Eggenstein-Leopoldshafen (Germany)
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Advanced Light Source (ALS)

The integration of photovoltaic (PV) solar energy in zero-energy buildings requires durable and efficient solar windows composed of lightweight and semitransparent thin film solar cells. Inorganic materials with a high optical absorption coefficient, such as Sb₂S₃(>10⁵cm^-1 at 450 nm), offer semitransparency, appreciable efficiency, and long-term durability at low cost. Oxide-free throughout the Sb₂S₃ layer thickness, as confirmed by combined studies of energy dispersive X-ray spectroscopy and synchrotron soft X-ray emission spectroscopy, semitransparent Sb₂S₃ thin films can be rapidly grown in air by the area-scalable ultrasonic spray pyrolysis method. Integrated into a ITO/TiO ₂/Sb₂S₃/P3HT/Au solar cell, a power conversion efficiency (PCE) of 5.5% at air mass 1.5 global (AM1.5G) is achieved, which is a record among spray-deposited Sb₂S₃ solar cells. An average visible transparency (AVT) of 26% of the back-contact-less ITO/TiO₂/Sb₂S₃solar cell stack in the wavelength range of 380–740 nm is attained by tuning the Sb₂S₃ absorber thickness to 100 nm. In scale-up from mm²to cm²areas, the Sb₂S₃hybrid solar cells show a decrease in efficiency of only 3.2% for an 88 mm²Sb₂S₃ solar cell, which retains 70% relative efficiency after one year of non-encapsulated storage. A cell with a PCE of 3.9% at 1 sun shows a PCE of 7.4% at 0.1 sun, attesting to the applicability of these solar cells for light harvesting under cloud cover.

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Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC02-05CH11231

OSTI ID:: 1591802

Journal Information:: Beilstein Journal of Nanotechnology, Journal Name: Beilstein Journal of Nanotechnology Vol. 10; ISSN BJNEAH; ISSN 2190-4286

Publisher:: Beilstein InstituteCopyright Statement

Country of Publication:: United States

Language:: English

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Related Subjects

36 MATERIALS SCIENCE
antimony sulfide
semitransparent solar cells
solar windows
thin films
ultrasonic spray pyrolysis

Title: Semitransparent Sb2S3 thin film solar cells by ultrasonic spray pyrolysis for use in solar windows

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Title: Semitransparent Sb₂S₃ thin film solar cells by ultrasonic spray pyrolysis for use in solar windows