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Title: Mechanisms of Pressure-Induced Phase Transitions by Real-Time Laue Diffraction

Abstract

Synchrotron X-ray radiation Laue diffraction is a widely used diagnostic technique for characterizing the microstructure of materials. An exciting feature of this technique is that comparable numbers of reflections can be measured several orders of magnitude faster than using monochromatic methods. This makes polychromatic beam diffraction a powerful tool for time-resolved microstructural studies, critical for understanding pressure-induced phase transition mechanisms, by in situ and in operando measurements. The current status of this technique, including experimental routines and data analysis, is presented along with some case studies. The new experimental setup at the High-Pressure Collaborative Access Team (HPCAT) facility at the Advanced Photon Source, specifically dedicated for in situ and in operando microstructural studies by Laue diffraction under high pressure, is presented.

Authors:
 [1];  [2];  [1]
  1. Argonne National Lab. (ANL), Argonne, IL (United States)
  2. Argonne National Lab. (ANL), Argonne, IL (United States); Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Publication Date:
Research Org.:
Argonne National Lab. (ANL), Argonne, IL (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Scientific User Facilities Division
OSTI Identifier:
1581777
Grant/Contract Number:  
AC02-06CH11357; AC52-07NA27344
Resource Type:
Accepted Manuscript
Journal Name:
Crystals
Additional Journal Information:
Journal Volume: 9; Journal Issue: 12; Journal ID: ISSN 2073-4352
Publisher:
MDPI
Country of Publication:
United States
Language:
English
Subject:
36 MATERIALS SCIENCE; Laue diffraction; high pressure; mechanisms of phase transitions

Citation Formats

Popov, Dmitry, Velisavljevic, Nenad, and Somayazulu, Maddury. Mechanisms of Pressure-Induced Phase Transitions by Real-Time Laue Diffraction. United States: N. p., 2019. Web. doi:10.3390/cryst9120672.
Popov, Dmitry, Velisavljevic, Nenad, & Somayazulu, Maddury. Mechanisms of Pressure-Induced Phase Transitions by Real-Time Laue Diffraction. United States. doi:10.3390/cryst9120672.
Popov, Dmitry, Velisavljevic, Nenad, and Somayazulu, Maddury. Sat . "Mechanisms of Pressure-Induced Phase Transitions by Real-Time Laue Diffraction". United States. doi:10.3390/cryst9120672. https://www.osti.gov/servlets/purl/1581777.
@article{osti_1581777,
title = {Mechanisms of Pressure-Induced Phase Transitions by Real-Time Laue Diffraction},
author = {Popov, Dmitry and Velisavljevic, Nenad and Somayazulu, Maddury},
abstractNote = {Synchrotron X-ray radiation Laue diffraction is a widely used diagnostic technique for characterizing the microstructure of materials. An exciting feature of this technique is that comparable numbers of reflections can be measured several orders of magnitude faster than using monochromatic methods. This makes polychromatic beam diffraction a powerful tool for time-resolved microstructural studies, critical for understanding pressure-induced phase transition mechanisms, by in situ and in operando measurements. The current status of this technique, including experimental routines and data analysis, is presented along with some case studies. The new experimental setup at the High-Pressure Collaborative Access Team (HPCAT) facility at the Advanced Photon Source, specifically dedicated for in situ and in operando microstructural studies by Laue diffraction under high pressure, is presented.},
doi = {10.3390/cryst9120672},
journal = {Crystals},
number = 12,
volume = 9,
place = {United States},
year = {2019},
month = {12}
}

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