Magnetic and transport behaviors of non-centrosymmetric Nd7Ni2Pd

Pathak, Arjun K.; Mudryk, Y.; Provino, A.; Manfrinetti, P.; Pecharsky, V. K.

doi:10.1063/1.5129907

Title: Magnetic and transport behaviors of non-centrosymmetric Nd₇Ni₂Pd

Abstract

Crystallographic, magnetic, electrical transport and thermodynamic properties of pseudo-binary Nd₇Ni₂Pd compound have been studied using temperature-dependent x-ray powder diffraction and physical property measurements. Compared to the ferromagnetic parent Nd₇Pd₃, the ground state of Nd₇Ni₂Pd is antiferromagnetic, and it exhibits strong metamagnetism. The measurements indicate two antiferromagnetic transitions in fields less than 8 kOe: a second-order paramagnetic to antiferromagnetic at T_N2 = 29 K and a weak first-order antiferromagnetic to antiferromagnetic transition at T_N1 = 24.5 K. Here, the compound becomes ferromagnetic in fields of 8 kOe and higher with T_C = 30 K. Temperature dependence of lattice parameters is anomalous, most prominently in the basal plane at ~30 K; however, there is no detectable structural distortion or clear volume discontinuity around 25 K, suggesting a significant weakening of the first-order transition when compared to the binary Nd₇Pd₃.

Authors:

^[1];

^[2]; Provino, A. ^[3]; Manfrinetti, P. ^[3]; Pecharsky, V. K. ^[2]

SUNY Buffalo State, Buffalo, NY (United States)
Ames Lab., and Iowa State Univ., Ames, IA (United States)
Univ. of Genova (Italy); Inst. SPIN-CNR, Genova (Italy)

Publication Date:: Thu Jan 02 00:00:00 EST 2020

Research Org.:: Ames Lab., Ames, IA (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division

OSTI Identifier:: 1581590

Alternate Identifier(s):: OSTI ID: 1580792

Report Number(s):: IS-J-10130
Journal ID: ISSN 2158-3226; TRN: US2100761

Grant/Contract Number:: AC02-07CH11358; 734303

Resource Type:: Accepted Manuscript

Journal Name:: AIP Advances

Additional Journal Information:: Journal Volume: 10; Journal Issue: 1; Journal ID: ISSN 2158-3226

Publisher:: American Institute of Physics (AIP)

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE

Citation Formats


                    Pathak, Arjun K., Mudryk, Y., Provino, A., Manfrinetti, P., and Pecharsky, V. K. Magnetic and transport behaviors of non-centrosymmetric Nd7Ni2Pd.  United States: N. p., 2020. 
Web.  doi:10.1063/1.5129907.

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                    Pathak, Arjun K., Mudryk, Y., Provino, A., Manfrinetti, P., & Pecharsky, V. K. Magnetic and transport behaviors of non-centrosymmetric Nd7Ni2Pd.  United States.  https://doi.org/10.1063/1.5129907

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                    Pathak, Arjun K., Mudryk, Y., Provino, A., Manfrinetti, P., and Pecharsky, V. K. Thu .  
"Magnetic and transport behaviors of non-centrosymmetric Nd7Ni2Pd".  United States.  https://doi.org/10.1063/1.5129907.  https://www.osti.gov/servlets/purl/1581590.

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@article{osti_1581590,

  title        = {Magnetic and transport behaviors of non-centrosymmetric Nd7Ni2Pd},

  author       = {Pathak, Arjun K. and Mudryk, Y. and Provino, A. and Manfrinetti, P. and Pecharsky, V. K.},

  abstractNote = {Crystallographic, magnetic, electrical transport and thermodynamic properties of pseudo-binary Nd7Ni2Pd compound have been studied using temperature-dependent x-ray powder diffraction and physical property measurements. Compared to the ferromagnetic parent Nd7Pd3, the ground state of Nd7Ni2Pd is antiferromagnetic, and it exhibits strong metamagnetism. The measurements indicate two antiferromagnetic transitions in fields less than 8 kOe: a second-order paramagnetic to antiferromagnetic at TN2 = 29 K and a weak first-order antiferromagnetic to antiferromagnetic transition at TN1 = 24.5 K. Here, the compound becomes ferromagnetic in fields of 8 kOe and higher with TC = 30 K. Temperature dependence of lattice parameters is anomalous, most prominently in the basal plane at ~30 K; however, there is no detectable structural distortion or clear volume discontinuity around 25 K, suggesting a significant weakening of the first-order transition when compared to the binary Nd7Pd3.},

  doi          = {10.1063/1.5129907},

  journal      = {AIP Advances},

  number       = 1,

  volume       = 10,

  place        = {United States},

  year         = {Thu Jan 02 00:00:00 EST 2020},

  month        = {Thu Jan 02 00:00:00 EST 2020}

}

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Title: Magnetic and transport behaviors of non-centrosymmetric Nd7Ni2Pd

Abstract

Citation Formats

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