Key drivers of cloud response to surface-active organics

Lowe, S. J.; Partridge, D. G.; Davies, J. F.; Wilson, K. R.; Topping, D.; Riipinen, I.

doi:10.1038/s41467-019-12982-0

Title: Key drivers of cloud response to surface-active organics

Journal Article · 17 November 2019 · Nature Communications

DOI: https://doi.org/10.1038/s41467-019-12982-0 · OSTI ID:1580985

Lowe, S. J. ^[1];

^[2]; Davies, J. F. ^[3]; Wilson, K. R. ^[4]; Topping, D. ^[5]; Riipinen, I. ^[6]

Stockholm Univ. (Sweden)
Univ. of Exeter, Exeter (United Kingdom)
Univ. of California, Riverside, CA (United States)
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Univ. of Manchester (United Kingdom)
Stockholm Univ. (Sweden); Tampere Univ. of Technology, Tampere (Finland)

Aerosol-cloud interactions constitute the largest source of uncertainty in global radiative forcing estimates, hampering our understanding of climate evolution. Recent empirical evidence suggests surface tension depression by organic aerosol to significantly influence the formation of cloud droplets, and hence cloud optical properties. In climate models, however, surface tension of water is generally assumed when predicting cloud droplet concentrations. Here we show that the sensitivity of cloud microphysics, optical properties and shortwave radiative effects to the surface phase are dictated by an interplay between the aerosol particle size distribution, composition, water availability and atmospheric dynamics. We demonstrate that accounting for the surface phase becomes essential in clean environments in which ultrafine particle sources are present. Through detailed sensitivity analysis, quantitative constraints on the key drivers – aerosol particle number concentrations, organic fraction and fixed updraft velocity – are derived for instances of significant cloud microphysical susceptibilities to the surface phase.

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Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Chemical Sciences, Geosciences & Biosciences Division; Knut and Alice Wallenberg foundation

Grant/Contract Number:: AC02-05CH11231

OSTI ID:: 1580985

Journal Information:: Nature Communications, Journal Name: Nature Communications Journal Issue: 1 Vol. 10; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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