Electrostrictive Cavitation in Water Induced by a SnO 2 Nanoparticle
Abstract
Cavitation phenomenon in dielectric fluids has been a recent topic of interest in theory and experiment. We study a dielectric fluid–nanoparticle system subjected to an external electric field using molecular dynamics simulations. Electric fields ranging from 0.042 to 0.25 V/Å are applied to a water and tin dioxide system. Cavitation is observed in simulations with both SPC/E water and the hydrogen bonding polarizable model. The cavitation onset time displays a stretched exponential relaxation response with respect to the applied electric field with an exponent β = 0.423 ± 0.08. This is in accordance with the exact theoretical value for systems with long-ranged forces. Cavity growth rates are divided into two phases, a spherical growth phase and a cylindrical one. Both are reported as a function of the applied electric field. The structure of the electric field is analyzed both spatially and temporally.
- Publication Date:
- Research Org.:
- Univ. of Southern California, Los Angeles, CA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division; USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division
- OSTI Identifier:
- 1579968
- Alternate Identifier(s):
- OSTI ID: 1580691
- Grant/Contract Number:
- SC0018195; NA0003525
- Resource Type:
- Published Article
- Journal Name:
- ACS Omega
- Additional Journal Information:
- Journal Name: ACS Omega Journal Volume: 4 Journal Issue: 27; Journal ID: ISSN 2470-1343
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
Citation Formats
Jackson, Shane, Nakano, Aiichiro, Vashishta, Priya, and Kalia, Rajiv K. Electrostrictive Cavitation in Water Induced by a SnO 2 Nanoparticle. United States: N. p., 2019.
Web. doi:10.1021/acsomega.9b00979.
Jackson, Shane, Nakano, Aiichiro, Vashishta, Priya, & Kalia, Rajiv K. Electrostrictive Cavitation in Water Induced by a SnO 2 Nanoparticle. United States. https://doi.org/10.1021/acsomega.9b00979
Jackson, Shane, Nakano, Aiichiro, Vashishta, Priya, and Kalia, Rajiv K. Wed .
"Electrostrictive Cavitation in Water Induced by a SnO 2 Nanoparticle". United States. https://doi.org/10.1021/acsomega.9b00979.
@article{osti_1579968,
title = {Electrostrictive Cavitation in Water Induced by a SnO 2 Nanoparticle},
author = {Jackson, Shane and Nakano, Aiichiro and Vashishta, Priya and Kalia, Rajiv K.},
abstractNote = {Cavitation phenomenon in dielectric fluids has been a recent topic of interest in theory and experiment. We study a dielectric fluid–nanoparticle system subjected to an external electric field using molecular dynamics simulations. Electric fields ranging from 0.042 to 0.25 V/Å are applied to a water and tin dioxide system. Cavitation is observed in simulations with both SPC/E water and the hydrogen bonding polarizable model. The cavitation onset time displays a stretched exponential relaxation response with respect to the applied electric field with an exponent β = 0.423 ± 0.08. This is in accordance with the exact theoretical value for systems with long-ranged forces. Cavity growth rates are divided into two phases, a spherical growth phase and a cylindrical one. Both are reported as a function of the applied electric field. The structure of the electric field is analyzed both spatially and temporally.},
doi = {10.1021/acsomega.9b00979},
journal = {ACS Omega},
number = 27,
volume = 4,
place = {United States},
year = {Wed Dec 18 00:00:00 EST 2019},
month = {Wed Dec 18 00:00:00 EST 2019}
}
Free Publicly Available Full Text
Publisher's Version of Record
https://doi.org/10.1021/acsomega.9b00979
https://doi.org/10.1021/acsomega.9b00979
Other availability
Search WorldCat to find libraries that may hold this journal
Cited by: 2 works
Citation information provided by
Web of Science
Web of Science
Save to My Library
You must Sign In or Create an Account in order to save documents to your library.
Works referenced in this record:
Observation of bubble dynamics within luminescent cavitation clouds: Sonoluminescence at the nano-scale
journal, December 2000
- Weninger, K. R.; Camara, C. G.; Putterman, S. J.
- Physical Review E, Vol. 63, Issue 1
Liquids at Large Negative Pressures: Water at the Homogeneous Nucleation Limit
journal, November 1991
- Zheng, Q.; Durben, D. J.; Wolf, G. H.
- Science, Vol. 254, Issue 5033
Recent advances with liposomes as pharmaceutical carriers
journal, February 2005
- Torchilin, Vladimir P.
- Nature Reviews Drug Discovery, Vol. 4, Issue 2
Characteristics of thermal conductivity in classical water models
journal, February 2013
- Sirk, Timothy W.; Moore, Stan; Brown, Eugene F.
- The Journal of Chemical Physics, Vol. 138, Issue 6
General formulation of pressure and stress tensor for arbitrary many-body interaction potentials under periodic boundary conditions
journal, October 2009
- Thompson, Aidan P.; Plimpton, Steven J.; Mattson, William
- The Journal of Chemical Physics, Vol. 131, Issue 15
Hydrogen-Bonding Polarizable Intermolecular Potential Model for Water
journal, November 2016
- Jiang, Hao; Moultos, Othonas A.; Economou, Ioannis G.
- The Journal of Physical Chemistry B, Vol. 120, Issue 48
Water and Solutions at Negative Pressure: Raman Spectroscopic Study to -80 Megapascals
journal, August 1990
- Green, J. L.; Durben, D. J.; Wolf, G. H.
- Science, Vol. 249, Issue 4969
Derivation of Force Field Parameters for SnO 2 −H 2 O Surface Systems from Plane-Wave Density Functional Theory Calculations
journal, April 2006
- Bandura, A. V.; Sofo, J. O.; Kubicki, J. D.
- The Journal of Physical Chemistry B, Vol. 110, Issue 16
Fast Parallel Algorithms for Short-Range Molecular Dynamics
journal, March 1995
- Plimpton, Steve
- Journal of Computational Physics, Vol. 117, Issue 1
Anode initiated impulse breakdown in water: the dependence on pulse rise time for nanosecond and sub-nanosecond pulses and initiation mechanism based on electrostriction
journal, September 2015
- Seepersad, Yohan; Fridman, Alexander; Dobrynin, Danil
- Journal of Physics D: Applied Physics, Vol. 48, Issue 42
Topological origin of stretched exponential relaxation in glass
journal, December 2011
- Potuzak, Marcel; Welch, Roger C.; Mauro, John C.
- The Journal of Chemical Physics, Vol. 135, Issue 21
Phase transitions in vapor-deposited water under the influence of high surface electric fields
journal, June 2000
- Scovell, D. L.; Pinkerton, T. D.; Medvedev, V. K.
- Surface Science, Vol. 457, Issue 3
Topological derivation of shape exponents for stretched exponential relaxation
journal, February 2005
- Macdonald, J. R.; Phillips, J. C.
- The Journal of Chemical Physics, Vol. 122, Issue 7
Cavitation in dielectric fluid in inhomogeneous pulsed electric field
journal, December 2013
- Shneider, M. N.; Pekker, M.
- Journal of Applied Physics, Vol. 114, Issue 21
Rayleigh scattering on the cavitation region emerging in liquids
journal, January 2016
- Shneider, M. N.; Pekker, M.
- Optics Letters, Vol. 41, Issue 6
Hydrogen bonding and molecular mobility in liquid water in external electromagnetic fields
journal, December 2003
- English, Niall J.; MacElroy, J. M. D.
- The Journal of Chemical Physics, Vol. 119, Issue 22
Simultaneous Femtosecond X-ray Spectroscopy and Diffraction of Photosystem II at Room Temperature
journal, February 2013
- Kern, J.; Alonso-Mori, R.; Tran, R.
- Science, Vol. 340, Issue 6131
Mechanochemistry of shock-induced nanobubble collapse near silica in water
journal, August 2012
- Nomura, K.; Kalia, R. K.; Nakano, A.
- Applied Physics Letters, Vol. 101, Issue 7
Stretched exponential relaxation in molecular and electronic glasses
journal, September 1996
- Phillips, J. C.
- Reports on Progress in Physics, Vol. 59, Issue 9
Axiomatic theories of ideal stretched exponential relaxation (SER)
journal, November 2006
- Phillips, J. C.
- Journal of Non-Crystalline Solids, Vol. 352, Issue 42-49
A coherent picture of water at extreme negative pressure
journal, November 2012
- Azouzi, Mouna El Mekki; Ramboz, Claire; Lenain, Jean-François
- Nature Physics, Vol. 9, Issue 1
Picosecond Melting of Ice by an Infrared Laser Pulse: A Simulation Study
journal, February 2008
- Caleman, Carl; van der Spoel, David
- Angewandte Chemie International Edition, Vol. 47, Issue 8
Principle and applications of microbubble and nanobubble technology for water treatment
journal, August 2011
- Agarwal, Ashutosh; Ng, Wun Jern; Liu, Yu
- Chemosphere, Vol. 84, Issue 9
Cavitation in water: a review
journal, November 2006
- Caupin, Frédéric; Herbert, Eric
- Comptes Rendus Physique, Vol. 7, Issue 9-10
Pre-breakdown processes in a dielectric fluid in inhomogeneous pulsed electric fields
journal, June 2015
- Shneider, Mikhail N.; Pekker, Mikhail
- Journal of Applied Physics, Vol. 117, Issue 22
Nanoflow electrospinning serial femtosecond crystallography
journal, October 2012
- Sierra, Raymond G.; Laksmono, Hartawan; Kern, Jan
- Acta Crystallographica Section D Biological Crystallography, Vol. 68, Issue 11, p. 1584-1587