In Situ Transmission Electron Microscopy on Energy-Related Catalysis
Abstract
Energy-related catalytic reactions have been extensively investigated in past years in order to efficiently utilize clean and environmentally benign energy sources. In these systems, the catalysts and the catalyst/active medium interfaces play a crucial role in determining their performance. Thus, understanding the physical and chemical properties of catalysts during reactions is of importance to provide fundamental insights for designing the devices. Transmission electron microscopy can provide tremendous information of materials' morphology, microstructure, and chemical properties at nanoscales. With in situ electron microscopy, dynamic processes of catalytic reactions in both gas and liquid environments have been investigated in real-time. In this review, the recent research progresses of in situ and operando electron microscopy techniques are introduced with the representative works in energy-related reactions, including electrochemical catalysis in liquid media and heterogeneous catalysis in gas media. The uniqueness of the specific electron microscopy methods and scientific merits of each work are highlighted. Lastly, outlooks on emerging research opportunities are discussed.
- Authors:
-
[3]
- Brookhaven National Lab. (BNL), Upton, NY (United States)
- State Univ. of New York, Binghamton, NY (United States)
- Brookhaven National Lab. (BNL), Upton, NY (United States); Chinese Academy of Sciences (CAS), Beijing (China)
- Publication Date:
- Research Org.:
- Brookhaven National Lab. (BNL), Upton, NY (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1580236
- Alternate Identifier(s):
- OSTI ID: 1577003
- Report Number(s):
- BNL-212464-2019-JAAM
Journal ID: ISSN 1614-6832
- Grant/Contract Number:
- SC0012704; SC0001135
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Energy Materials
- Additional Journal Information:
- Journal Volume: 10; Journal Issue: 11; Journal ID: ISSN 1614-6832
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE; energy‐related catalysts; ETEM; gas cell; in situ TEM; liquid cell
Citation Formats
Hwang, Sooyeon, Chen, Xiaobo, Zhou, Guangwen, and Su, Dong. In Situ Transmission Electron Microscopy on Energy-Related Catalysis. United States: N. p., 2019.
Web. doi:10.1002/aenm.201902105.
Hwang, Sooyeon, Chen, Xiaobo, Zhou, Guangwen, & Su, Dong. In Situ Transmission Electron Microscopy on Energy-Related Catalysis. United States. https://doi.org/10.1002/aenm.201902105
Hwang, Sooyeon, Chen, Xiaobo, Zhou, Guangwen, and Su, Dong. Tue .
"In Situ Transmission Electron Microscopy on Energy-Related Catalysis". United States. https://doi.org/10.1002/aenm.201902105. https://www.osti.gov/servlets/purl/1580236.
@article{osti_1580236,
title = {In Situ Transmission Electron Microscopy on Energy-Related Catalysis},
author = {Hwang, Sooyeon and Chen, Xiaobo and Zhou, Guangwen and Su, Dong},
abstractNote = {Energy-related catalytic reactions have been extensively investigated in past years in order to efficiently utilize clean and environmentally benign energy sources. In these systems, the catalysts and the catalyst/active medium interfaces play a crucial role in determining their performance. Thus, understanding the physical and chemical properties of catalysts during reactions is of importance to provide fundamental insights for designing the devices. Transmission electron microscopy can provide tremendous information of materials' morphology, microstructure, and chemical properties at nanoscales. With in situ electron microscopy, dynamic processes of catalytic reactions in both gas and liquid environments have been investigated in real-time. In this review, the recent research progresses of in situ and operando electron microscopy techniques are introduced with the representative works in energy-related reactions, including electrochemical catalysis in liquid media and heterogeneous catalysis in gas media. The uniqueness of the specific electron microscopy methods and scientific merits of each work are highlighted. Lastly, outlooks on emerging research opportunities are discussed.},
doi = {10.1002/aenm.201902105},
journal = {Advanced Energy Materials},
number = 11,
volume = 10,
place = {United States},
year = {2019},
month = {12}
}
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